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The aim of the study was to determine air pollution over the sea surface (North Sea and Baltic Sea) comparing to concentration in the closest land areas to examine the impact of ships on the level of PM concentration. The analysis is based on the measurements made during the two weeks cruise of the tall ship Fryderyk Chopin from Edinburg to Kołobrzeg. The highest pollution levels were observed in locations distant from the coast, especially over Baltic Sea, with increasing concentrations when other ships approaching. The article attempts to assess the possibility of migration of pollutants to these areas from land-based sources, and thus indicate the degree of their participation in the level of pollution present at sea.

Shipping is one of the transport sectors less regulated, although more than 80% of world trade is transported by ships [1] and its share of total anthropogenic emissions is significant, with effects on climate, human health and air quality, especially in coastal areas. Recent studies [2] demonstrated the effectiveness of implementation of the 2005/33/EC European Directive in reducing the impact of ship traffic on aerosol concentrations at local scale, however, the effect on climate is more uncertain. Detailed information regarding the size distribution of the impacts to particles and their correlation with gaseous emissions is needed to investigate the complex air quality-climate interaction of this source. Much of the literature studies focus on NOX, SO2, and particulate matter (PM) emissions while there is a gap of knowledge about the size distribution of emitted particles, especially in coarse fraction. This study was done in the framework of POSEIDON (POllution monitoring of Ship Emission: an IntegrateD approach fOr harbour of the Adriatic basiN) project (MED 2007-2013). The aim was to estimate the contribution of in-port ship emissions to gaseous atmospheric pollutants and to PM of different sizes in a port-city in South-Eastern Italy (Adriatic Sea), after the enforcement of the low-sulphur fuel EU-Directive. Measurements were taken at high temporal resolution at the Passenger Terminal site in the harbour area of Brindisi (40° 38? 43.32? N-17° 57? 36.39? E). Data collected by a Mobile Laboratory, were gaseous pollutants (NO2, NO, O3, SO2; 5 min resolution), particle number concentrations (PNC; 1 min resolution), particle size distribution in the range 0.25-32 ?m (1 min resolution) and NO2 and SO2 flow-rate emissions with a DOAS (Differential Optical Absorption Spectroscopy) remote-sensing system, called GASCOD (Gas Absorption Spectrometer Correlating Optical Differences). The Port Authority provided data of ship traffic and a video camera was used to synchronize all measurements and visually estimate number of vehicles (cars, trucks) during loading/unloading of ships at berth. Characterization of ship plumes in aspect of particle size, gaseous concentrations, duration, ratio NO/NO2, was performed. The impact analysis [3] was applied separating manoeuvring (arrival/departure of ships) and hotelling (loading/unloading activities) phases. Results showed that the primary contribution to PM1 and PM2.5 was significantly lower with respect to those to PNC for both phases, confirming that the majority of the particles emitted were in the ultrafine size range. Manoeuvring phase was characterized by higher impacts to SO2, NO, and NO2 than those to PNC, PM1 and PM2.5. Hotelling phase represented a significant share of the impact for NO, NO2, PNC but gave a low contribution to SO2 impact (due to low-sulphur fuel). Ultrafine particles (Dp1) fraction while accumulation mode particles (0.25

Ship emissions are a growing concern, especially in coastal areas, for potential impacts on human health and climate. International mitigation strategies to curb these emission, based on low-sulphur content fuels, have proven useful to improve local air quality. However, the effect on climate forcing is less obvious. Detailed information on the influence of shipping to particles of different sizes is needed to investigate air quality and climate interaction. In this work, the contributions of maritime emissions to atmospheric concentrations of gaseous pollutants (NO, NO2, SO2, and O3) and of particles (sizes from 0.009 mm to 30 mm) were investigated considering manoeuvring (arrival and departure of ships) and hotelling phases (including loading/unloading activities). Results showed that the size distributions of shipping contributions were different for the two phases and could be efficiently described, using measured data, considering four size-ranges. The largest contribution to particles concentration was observed for Dp < 0.25 mm, however, a secondary maximum was observed at Dp ¼ 0.35 mm. The minimum contribution was observed at Dp around 0.8e0.9 mm with a negligible contribution from hotelling for size range 0.4e1 mm. The comparison of 2012 and 2014 datasets showed no significant changes of gaseous and particulate pollutant emissions and of the contribution to particle mass concentration. However, an increase of the contribution to particle number concentration (PNC) was observed. Results suggested that harbour logistic has a relevant role in determining the total impact of shipping on air quality of the nearby coastal areas. Additionally, future policies should focus on PNC that represents an important fraction of emissions also for low-sulphur fuels. DOAS remote sensing proved a useful tool to directly measure NO2 and SO2 ship emissions giving estimates comparable with those of emission inventory approach.

The aim of the study was to determine air pollution over the sea surface (North Sea and Baltic Sea) compared to the situation in ports, as well as to examine the impact of ships on the level of particulate matter (PM) concentration. The measurements, made during the two-week cruise of the tall ship Fryderyk Chopin, demonstrated that the principal source of PM emission over the sea surface are passing ships equipped with internal combustion engines, including quite numerous units powered by marine oil. The highest pollution levels were observed in locations distant from the coast, with increasing concentrations when other ships were approaching. During the cruise, at least two places were identified with increased PM concentration (18&ndash, 28 &mu, g/m3 for PM10 and 15&ndash, 25 &mu, g/m3 for PM2.5) caused by passing ships. The share of PM2.5 fraction in the general PM concentration in these places increased from 70&ndash, 72% to 82&ndash, 85%, which means that combustion emission dominated. In turn, measurements made in ports (Copenhagen and Kołobrzeg) showed lower levels of air pollution and indicated a typical variability of the PM concentrations characteristic for land areas. The results confirm the need for determining suitable solutions for sustainable sea transport.

It has been often claimed that the ships sail in open sea far away from the shoreline, leading to the assumption that emissions from the vessels do not contribute to the pollution of the land. The investigations does not support this approach .It is indicated that 74 - 83 % of the ships are sailing in world-wide trade within 200 nautical miles of the land. Thus most of the ships are actually relatively near the land and so the ships have a real impact on overrrall emission levels. The limitations of the NO and SO emission, international and local, are on the way. The engine speed dependent "IMO-curve" can be seen as a starting point for exhaust emission restrictions. Most of the modern engine types can meet the IMO -curve without any secondary means. The several proposals have been brought out following the general, relatively strict trend applied for landbased industry. Several ferry owners already invest today in Selective Catalytic Reduction (SCR) units or are at least prepared for later installation of SCR units for vessels operating on the Baltic Sea. Local restrictions will most obviously take place first through emission charges related to actual emissions in special areas.