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Spin-orbit coupled honeycomb magnets with the Kitaev interaction have received a lot of attention due to their potential of hosting exotic quantum states including quantum spin liquids. Thus far, the most studied Kitaev systems are 4d/5d-based honeycomb magnets. Recent theoretical studies predicted that 3d-based honeycomb magnets, including Na2Co2TeO6 (NCTO), could also be a potential Kitaev system. Here, we have used a combination of heat capacity, magnetization, electron spin resonance measurements alongside inelastic neutron scattering (INS) to study NCTO's quantum magnetism, and we have found a field-induced spin disordered state in an applied magnetic field range of 7.5 T < B (vertical to b-axis) < 10.5 T. The INS spectra were also simulated to tentatively extract the exchange interactions. As a 3d-magnet with a field-induced disordered state on an effective spin-1/2 honeycomb lattice, NCTO expands the Kitaev model to 3d compounds, promoting further interests on the spin-orbital effect in quantum magnets., 19 pages and 5 figures for main text. 16 pages and 6 figures for Supplemental Material more...

Observation of a quantum spin liquid (QSL) state is one of the most important goals in condensed-matter physics, as well as the development of new spintronic devices that support next-generation industries. The QSL in two dimensional quantum spin systems is expected to be due to geometrical magnetic frustration, and thus a kagome-based lattice is the most probable playground for QSL. Here, we report the first experimental results of the QSL state on a square-kagome quantum antiferromagnet, KCu6AlBiO4(SO4)5Cl. Comprehensive experimental studies via magnetic susceptibility, magnetisation, heat capacity, muon spin relaxation (μSR), and inelastic neutron scattering (INS) measurements reveal the formation of a gapless QSL at very low temperatures close to the ground state. The QSL behavior cannot be explained fully by a frustrated Heisenberg model with nearest-neighbor exchange interactions, providing a theoretical challenge to unveil the nature of the QSL state., There exist many theoretical models of frustrated quantum magnetism, most of which lack convincing experimental realisations. Here the authors combine several experimental methods to argue that KCu6AlBiO4(SO4)5Cl behaves as a square-kagome-lattice quantum Heisenberg antiferromagnet. more...

The kagome lattice is a fertile platform to explore topological excitations with both Fermi-Dirac and Bose-Einstein statistics. While relativistic Dirac Fermions and flat-bands have been discovered in the electronic structure of kagome metals, the spin excitations have received less attention. Here we report inelastic neutron scattering studies of the prototypical kagome magnetic metal FeSn. The spectra display well-defined spin waves extending up to 120 meV. Above this energy, the spin waves become progressively broadened, reflecting interactions with the Stoner continuum. Using linear spin wave theory, we determine an effective spin Hamiltonian that reproduces the measured dispersion. This analysis indicates that the Dirac magnon at the K-point remarkably occurs on the brink of a region where well-defined spin waves become unobservable. Our results emphasize the influential role of itinerant carriers on the topological spin excitations of metallic kagome magnets., 6 pages, 4 figures more...

The High Resolution Chopper Spectrometer (HRC) is installed at the Japan Proton Accelerator Research Complex (J-PARC) and is utilized for a wide range of dynamical studies of materials over a wide energy-momentum space with high resolution. Neutron Brillouin scattering (NBS), i.e., inelastic neutron scattering close to the forward direction, can be performed with the HRC, because this instrument utilizes low angle detectors and high-energy neutrons which facilitates a high resolution. Since the solid angle of the detection area for NBS experiments is limited to very low scattering angles, improvements of the HRC are required to increase the neutron flux with reducing the background. Given the success of the HRC for NBS studies, the neutron intensities for NBS experiments have been improved by changing the detector layout, reducing deformation of the slit package during rotation of the Fermi chopper, and fabricating a longer collimator. At present, we have made further improvements. At around the incident neutron energy Ei = 100 meV, the neutron flux was significantly increased for an energy resolution of ΔE∕Ei = 2%, and the best energy resolution achieved was nearly 1% resolution with an acceptable neutron flux. more...

Seven time-of-flight quasielastic/inelastic neutron scattering instruments are installed on six beamlines in the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (J-PARC). Four of these instruments are chopper-type direct-geometry spectrometers, one is a near-backscattering indirect-geometry spectrometer, and the other two are spin-echo-type spectrometers. This paper reviews the characteristic features, recent scientific outcomes, and progress in development of MLF spectrometers. more...

Finding new materials with antiferromagnetic (AFM) Kitaev interaction is an urgent issue for quantum magnetism research. We conclude that Na

The magnetic excitations in $\mathrm{CoP}{\mathrm{S}}_{3}$, a two-dimensional van der Waals (vdW) antiferromagnet with ${\mathrm{Co}}^{2+}$ ion on a honeycomb lattice, have been measured using powder inelastic neutron scattering. The absence of spin-orbit exciton around 30 meV indicates that ${\mathrm{Co}}^{2+}$ ions in $\mathrm{CoP}{\mathrm{S}}_{3}$ have an $S=3/2$ state rather than a spin-orbital entangled ${J}_{\mathrm{eff}}=1/2$ ground state. And, clear dispersive spin waves are observed with a large spin gap of \ensuremath{\sim}13 meV. The magnon spectra were fitted using an XXZ-type ${J}_{1}\text{\ensuremath{-}}{J}_{2}\text{\ensuremath{-}}{J}_{3}$ Heisenberg Hamiltonian with single-ion anisotropy assuming no magnetic exchange interaction between the honeycomb layers. The best-fit parameters show ferromagnetic exchange interactions ${J}_{1}=\ensuremath{-}2.08\phantom{\rule{0.16em}{0ex}}\mathrm{meV}$ and ${J}_{2}=\ensuremath{-}0.26\phantom{\rule{0.16em}{0ex}}\mathrm{meV}$ for the nearest- and second-nearest neighbors and a sizable antiferromagnetic exchange interaction ${J}_{3}=4.21\phantom{\rule{0.16em}{0ex}}\mathrm{meV}$ for the third-nearest neighbor with the strong easy-axis anisotropy $K=\ensuremath{-}2.06\phantom{\rule{0.16em}{0ex}}\mathrm{meV}$. The anisotropic XXZ-type Hamiltonian could only achieve a suitable fitting. The exchange interaction for the out-of-plane spin component is smaller than that for the in-plane one by a ratio $\ensuremath{\alpha}={J}_{z}/{J}_{x}=0.6$. Our result directly shows that $\mathrm{CoP}{\mathrm{S}}_{3}$ is an experimental realization of the XXZ model with a honeycomb lattice in two-dimensional vdW magnets. more...

Magnetic correlation in ${\mathrm{YBaCo}}_{4}{\mathrm{O}}_{7}$ with kagome and triangular lattices was studied through inelastic-neutron-scattering measurements on a single crystal sample. The broad magnetic excitation was observed below 45 meV and showed dispersions both within the $c$ plane and along the $c$ axis. The wave vector with the minimum energy of the magnetic excitation was totally different from the magnetic Bragg point. Our analysis with the first-moment-sum rule suggests that Co ions in ${\mathrm{YBaCo}}_{4}{\mathrm{O}}_{7}$ form a unique three-dimensional network with the geometrically frustration. more...

Neutron scattering experiments have been performed to elucidate magnetic properties of the quasicrystal approximant Au

We performed neutron diffraction experiments on a single crystal of an $S=\frac{1}{2}$ frustrated ferromagnetic chain compound ${\mathrm{NaCuMoO}}_{4}$(OH) at zero and finite magnetic fields. Three magnetic Bragg peaks with the propagation vector of $\mathbit{q}=(0,\ensuremath{\delta},0)$ $[\ensuremath{\delta}=0.481(1)]$ were observed at the zero field, which means that an incommensurate helical magnetic order was realized. Using the ratio of the intensities between these magnetic peaks, a proper-screw structure was suggested, where the spiral plane is the crystallographic $ac$ plane. While the $\ensuremath{\delta}$ is unchanged at lower fields, it decreases linearly with the field where ${\ensuremath{\mu}}_{0}H\ensuremath{\ge}2.5\phantom{\rule{0.16em}{0ex}}\mathrm{T}$. The field dependence is consistent with that of the field-induced spin density wave state that originated from the formation of the bound state of two magnons in the $S=\frac{1}{2}$ frustrated ferromagnetic chain. more...

We report magnetic studies on the charge and spin ordering in La2− xSrxCoO4 for x = 1 / 3 , 0.60, and 0.75. The magnetic susceptibility displays a clear cusp which we attribute to a spin glass freezing transition in all three compositions stduied. The behaviors of the evaluated effective magnetic moment and Curie-Weiss temperature indicate that the antiferromagnetic (AFM) interaction among Co 2 + ions surrounded by the non-magnetic Co 3 + weakens with increasing the doping concentration x. In addition, we have found that the incommensurate AFM short range order is frozen at T g which is further below the onset temperature T IC of the neutron intensity of the incommensurate AFM correlation. more...

One of the consequences of antisymmetric spin–orbit interactions due to a lack of inversion symmetry are unusually large upper critical fields observed in heavy-electron superconductors. The upper ... more...

Magnetic excitations in the metallic antiferromagnet F e 0.5 M n 0.5 were investigated using the inelastic neutron scattering technique at low temperatures well below the antiferromagnetic transition temperatures ( T N ). The observed peak positions in low energies well sit on the antiferromagnetic dispersion relation reported in the early study. However, the peak positions in higher energies shift to higher energies than that of the antiferromagnetic spin wave dispersion relation. This behavior is the same as one of the behaviors suggesting that the spin waves merge with the continuum of the individual particle-hole excitations at higher energies in F e 0.7 M n 0.3 . more...

The crystalline electric field (CEF) excitations in CePtSi3 with the non-centrosymmetric structure were investigated by inelastic neutron scattering (INS) experiment. CEF excitations were observed at 5.3 and 17.5 meV. We discuss the CEF parameters and wave function of CePtSi3 by comparing those of other CeTX3(T: transition metal, X: Si, Ge) systems. more...

Inelastic X-ray scattering (IXS) experiments were performed on polycrystalline Mg97Zn1Y2 and Mg85Zn6Y9 alloys with synchronized long-period stacking ordered (LPSO) phase of about 24% and 100%, respectively, together with the reference pure Mg at room temperature for investigating the impurity effects in the microscopic elastic properties of the LPSO alloys. Inelastic neutron scattering (INS) measurements were also carried out on a polycrystalline Mg97Zn1Y2 alloy. The IXS measurements were carried out for the momentum transfers Q between 1.6 and 15.9 nm−1 including the whole first- and partially second Brillouin zones, and for the energy transfers ω below 40 meV. Peaks arising from longitudinal acoustic (LA) modes were clearly observed in the IXS spectra of both the LPSO alloys and pure Mg, while transverse acoustic (TA) modes can mainly be detected in the second Brillouin zone. The dispersion relations in pure polycrystalline Mg are in good agreement with those of previous INS data on single crystal Mg. Broader inelastic signals and larger quasielastic peaks are characteristic for the LPSO alloys due to the phonon scattering by the Zn/Y impurities. Only the TA excitation energies increase by adding the impurities, which indicate a harder stiffness of the bond angles relating to the existence of the L12-type clusters in the LPSO alloys. Besides, new impurity-derived dispersion-less excitation modes are observed at about 10 meV by adding the Zn/Y impurities. By comparing with the INS data on the polycrystalline LPSO alloy, the contributions of the impurities to these excitation modes are discussed using the differences in the scattering cross-sections between neutrons and X-rays. more...

J-PARC, Japan Proton Accelerator Research Complex provides short pulse proton beam at a repetition rate 25Hz and the maximum power is expected to be 1MW. Materials and Life Science Experimental Facility (MLF) has 23 neutron beam ports and 21 instruments have already been operated or under construction/commissioning. There are 6 inelastic/quasi-elastic neutron scattering spectrometers and the complementary use of these spectrometers will open new insight for life science.This article is part of a Special Issue entitled “Science for Life” Guest Editor: Dr. Austen Angell, Dr. Salvatore Magazù and Dr. Federica Migliardo. more...

Weyl fermions that emerge at band crossings in momentum space caused by the spin–orbit interaction act as magnetic monopoles of the Berry curvature and contribute to a variety of novel transport phenomena such as anomalous Hall effect and magnetoresistance. However, their roles in other physical properties remain mostly unexplored. Here, we provide evidence by neutron Brillouin scattering that the spin dynamics of the metallic ferromagnet SrRuO3 in the very low energy range of milli-electron volts is closely relevant to Weyl fermions near Fermi energy. Although the observed spin wave dispersion is well described by the quadratic momentum dependence, the temperature dependence of the spin wave gap shows a nonmonotonous behaviour, which can be related to that of the anomalous Hall conductivity. This shows that the spin dynamics directly reflects the crucial role of Weyl fermions in the metallic ferromagnet., Whilst Weyl fermions have characteristic effects in magnetotransport measurements in condensed matter systems, their effects on other properties remain unexplored. Here, the authors use neutron Brillouin scattering to evidence the interaction of Weyl fermions with the spin wave dynamics in SrRuO3. more...

We report on a wide angle neutron spin analyzer for neutron energies up to 40 meV ( λ = 1.4 A) that was recently realized in collaboration with Tohoku University and KEK, Japan (Ohoyama et al., 2014; Yokoo et al., 2014). Curved polarizing Fe/Si supermirrors with m = 5.5/1.5 (Schanzer et al., 2016) are arranged radially around the sample covering an angular range of 40° if all channels are equipped with supermirrors. The mirrors are saturated by a vertical permanent magnetic field B ≃ 40 mT generated by NdFeB magnets. It was optimized using finite element analysis. The polarization and transmission of the spin filter have been determined at the beamline BOA at the Swiss spallation neutron source (SINQ) to be P = ( 0 . 975 ± 0 . 01 ) and T u p = T = ( 0 . 55 ± 0 . 017 ) for spin-up neutrons at λ = 3 A ( E = 9 meV), respectively. The transmission is excellent considering that approximately one third of the neutrons hit the front faces of the polarizing blades. The experimental results are in good agreement with Monte Carlo simulations using the software package McStas. more...

Neutron scattering experiments have been performed to elucidate magnetic properties of the quasicrystal approximant Au$_{70}$Si$_{17}$Tb$_{13}$, consisting of icosahedral spin clusters in a body-centered-cubic lattice. Bulk magnetic measurements performed on the single crystalline sample unambiguously confirm long-range ordering at $T_{\rm C} = 11.6 \pm 1$ K. In contrast to the simple ferromagnetic response in the bulk measurements, single crystal neutron diffraction confirms a formation of intriguing non-collinear and non-coplanar magnetic order. The magnetic moment direction was found to be nearly tangential to the icosahedral cluster surface in the local mirror plane, which is quite similar to that recently found in the antiferromagnetic quasicrystal approximant Au$_{72}$Al$_{14}$Tb$_{14}$. Inelastic neutron scattering on the powdered sample exhibits a very broad peak centered at $\hbar \omega \simeq 4$ meV. The observed inelastic spectrum was explained by the crystalline-electric-field model taking account of the chemical disorder at the fractional Au/Si sites. The resulting averaged anisotropy axis for the crystalline-electric-field ground state is consistent with the ordered moment direction determined in the magnetic structure analysis, confirming that the non-coplanar magnetic order is stabilized by the local uniaxial anisotropy., Comment: 14 pages, 10 figures, 3 tables more...

We have studied the pressure-induced quantum phase transition in the singlet-ground-state antiferromagnet ${\mathrm{CsFeCl}}_{3}$. Neutron diffraction experiments under pressure evidence the magnetic long-range order at low temperatures. Magnetic structure analysis reveals a ${120}^{\ensuremath{\circ}}$ structure with a propagation vector of ${\mathbit{k}}_{\mathrm{mag}}=(1/3,1/3,0)$. The estimated critical exponent of the order parameter suggests that ${\mathrm{CsFeCl}}_{3}$ belongs to the universality class of $U(1)\ifmmode\times\else\texttimes\fi{}{Z}_{2}$ symmetry which is expected to realize the chiral liquid state. more...

Collective dynamics of liquid deuterated methanol was studied at room temperature using neutron scattering. The inelastic excitation energy of coherent scattering from liquid deuterated methanol was proportional to the momentum transfer Q in the range of 0.2 to 0.9 A − 1 ; the high-frequency sound velocity of liquid deuterated methanol obtained from the dispersion relation was 1770 ± 30 m s − 1 . The positive dispersion for liquid deuterated methanol was ~ 60%, about half that of liquid heavy water (~ 100%) previously reported. This could be reflective of the different number of hydrogen bonds. At Q positions below the first peak in S ( Q ), the dispersion relation of liquid deuterated methanol derived from neutron scattering was almost identical to that obtained from X-ray scattering. However, the excitation energy obtained from neutron scattering at Q positions above the first peak in S ( Q ) is larger than that from X-ray scattering, which could be ascribed to intramolecular methanol vibrations. more...

POLANO is a newly constructed chopper spectrometer for polarization analysis in J-PARC. Its construction is almost complete, even though a few upgrades, the tuning, and R&D of some devices and the beam line are still pending. After radiation assessments, POLANO has been approved as a proper neutron beam line and the beam commissioning process will commence soon. Our primary objective is to achieve higher-energy polarization analysis of inelastic scattering beyond a reactor-based neutron source up to 100 meV, with medium (reasonable) resolution. The other devices, such as spin filter polarizer and magnetic system are currently under development. more...

The High Resolution Chopper Spectrometer (HRC) installed at MLF, J-PARC provides opportunities for dynamical studies of materials over a wide energy-momentum space with high resolution. Three types of inelastic neutron scattering experiments can be performed with the HRC: high-resolution experiments in a conventional energy-momentum space, eV neutron spectroscopy, and neutron Brillouin scattering (NBS). Some results have been obtained using these techniques. The NBS option makes the HRC different from other chopper spectrometers. Coherent excitations in non-single-crystal samples can be observed with NBS. On the HRC, NBS experiments were made feasible by reducing the background noise at low scattering angles, and some results were obtained. more...

We studied the effect of magnetic Nd-ion substitution on the metal-nonmetal transition at a transition temperature of 63 K of PrRu4P12, which is characterized by antiferro-type electric multipole ordering of Pr-ion 4f electrons. The transition temperature of Pr1-xNdxRu4P12 depends weakly on the Nd concentration x as compared to Laand Ce-substituted compounds. Inelastic neutron-scattering measurements revealed that the energies and widths of crystalline field excitation peaks of Pr 4f 2 in Pr0.85Nd0.15Ru4P12 are very similar to those of PrRu4P12. These experimental results indicate that the ordered state is robust against the substitution of magnetic Nd ions as compared to the La and Ce substitutions. Magnetic interactions between the Pr ions and the Nd ions in Pr1-xNdxRu4P12 help stabilize the magnetic triplet ground state of the Pr ions that appears in the antiferro-type multipole ordered phase. Therefore, the nonmagnetic multipole ordered phase of PrRu4P12 is compatible with the magnetic perturbation., Conference : 20th International Conference on Magnetism, ICM 2015, Location : Barcelona, SPAIN, Date : JUL 05-10, 2015 more...

AIM Angiotensin Ⅱ(Ang Ⅱ) produces reactive oxygen species (ROS), thus contributing to the development of cardiac hypertrophy and subsequent heart failure, and stimulates the expression of monocyte chemoattractant protein-1 (MCP-1). In addition, Toll-like receptor 4 (TLR4) is involved in the upregulation of MCP-1. In order to clarify whether TLR4 is involved in the onset of cardiac dysfunction caused by Ang Ⅱ stimulation, we investigated the effects of TLR4 on oxidative stress, the MCP-1 expression and cardiac dysfunction in mice with Ang Ⅱ-induced hypertension. METHODS TLR4-deficient (Tlr4(lps-d)) and wild-type (WT) mice were randomized into groups treated with Ang Ⅱ, norepinephrine (NE) or a subdepressor dose of the Ang Ⅱreceptor blocker irbesartan (IRB) and Ang Ⅱ for two weeks. RESULTS Ang Ⅱ and NE similarly increased systolic blood pressure in all drug-treated groups compared to that observed in the control group among both WT and Tlr4(lps-d) mice (p＜0.05). In the WT mice, Ang Ⅱ induced cardiac hypertrophy as well as vascular remodeling and perivascular fibrosis of the intramyocardial arteries and monocyte/macrophage infiltration in the heart (p＜0.05). Furthermore, Ang Ⅱ treatment decreased the left ventricular diastolic function and resulted in a greater left ventricular end-systolic dimension (p＜0.05) in addition to producing a five-fold increase in the NADPH oxidase activity, ROS content and MCP-1 expression (p＜0.05). In contrast, the Tlr4(lps-d) mice showed little effects of Ang Ⅱ on these indices. In the WT mice, IRB treatment reversed these changes compared to that seen in the mice treated with Ang Ⅱ alone. NE produced little effect on any of the indices in either the WT or Tlr4(lps-d) mice. CONCLUSIONS TLR4 may be involved in the processes underlying the increased oxidative stress, selectively activated MCP-1 expression and cardiac hypertrophy and dysfunction seen in cases of Ang Ⅱ- induced hypertension. more...

We use inelastic neutron scattering to study the low-energy spin excitations of 112-type iron pnictide Ca$_{0.82}$La$_{0.18}$Fe$_{0.96}$Ni$_{0.04}$As$_{2}$ with bulk superconductivity below $T_c=22$ K. A two-dimensional spin resonance mode is found around $E=$ 11 meV, where the resonance energy is almost temperature independent and linearly scales with $T_c$ along with other iron-based superconductors. Polarized neutron analysis reveals the resonance is nearly isotropic in spin space without any $L$ modulations. Due to the unique monoclinic structure with additional zigzag arsenic chains, the As $4p$ orbitals contribute to a three-dimensional hole pocket around $\Gamma$ point and an extra electron pocket at $X$ point. Our results suggest that the energy and momentum distribution of spin resonance does not directly response to the $k_z$ dependence of fermiology, and the spin resonance intrinsically is a spin-1 mode from singlet-triplet excitations of the Cooper pairs in the case of weak spin-orbital coupling., Comment: 9 pages, 8 figures, with supplementary materials more...

K3Cu3AlO2(SO4)4 is a highly one-dimensional spin-1/2 inequilateral diamond-chain antiferromagnet. Spinon continuum and spin-singlet dimer excitations are observed in the inelastic neutron scattering spectra, which is in excellent agreement with a theoretical prediction: a dimer-monomer composite structure, where the dimer is caused by strong antiferromagnetic (AFM) coupling and the monomer forms an almost isolated quantum AFM chain controlling low-energy excitations. Moreover, muon spin rotation/relaxation spectroscopy shows no long-range ordering down to 90 mK, which is roughly three orders of magnitude lower than the exchange interaction of the quantum AFM chain. K3Cu3AlO2(SO4)4 is, thus, regarded as a compound that exhibits a Tomonaga-Luttinger spin liquid behavior at low temperatures close to the ground state. more...

A spin-1/2 triangular-lattice Heisenberg antiferromagnet (TLHAF) is a prototypical frustrated quantum magnet, which exhibits remarkable quantum many-body effects that arise from the synergy between spin frustration and quantum fluctuation. The ground-state properties of a spin-1/2 TLHAF are theoretically well understood. However, the theoretical consensus regarding the magnetic excitations is limited. The experimental study of the magnetic excitations in spin-1/2 TLHAFs has also been limited. Here we show the structure of magnetic excitations in the spin-1/2 TLHAF Ba3CoSb2O9 investigated by inelastic neutron scattering. Significantly different from theoretical expectations, the excitation spectrum has a three-stage energy structure. The lowest-energy first stage is composed of dispersion branches of single-magnon excitations. The second and third stages are dispersive continua accompanied by a columnar continuum extending above 10 meV, which is six times larger than the exchange interaction J = 1.67 meV. Our results indicate the shortcomings of the current theoretical framework. Two-dimensional frustrated magnets are heavily studied because theories predict that quantum effects may lead to the emergence of fractionalized excitations. Ito et al. use inelastic neutron scattering to show that the excitation spectrum of Ba3CoSb2O9 disagrees with current theoretical expectations. more...

Neutron devices such as neutron detectors, optical devices including supermirror devices and 3He neutron spin filters, and choppers are successfully developed and installed at the Materials Life Science Facility (MLF) of the Japan Proton Accelerator Research Complex (J-PARC), Tokai, Japan. Four software components of MLF computational environment, instrument control, data acquisition, data analysis, and a database, have been developed and equipped at MLF. MLF also provides a wide variety of sample environment options including high and low temperatures, high magnetic fields, and high pressures. This paper describes the current status of neutron devices, computational and sample environments at MLF. more...

The collective spin-wave excitations in the antiferromagnetic state of $\gamma$-Fe$_{0.7}$Mn$_{0.3}$ were investigated using the inelastic neutron scattering technique. The spin excitations remain isotropic up to the high excitation energy, ${\hbar\omega}= 78$ meV. The excitations gradually become broad and damped above 40 meV. The damping parameter ${\gamma}$ reaches 110(16) meV at ${\hbar\omega} = 78$ meV, which is much larger than that for other metallic compounds, e.g., CaFe$_2$As$_2$ (24 meV), La$_{2-2x}$Sr$_{1+2x}$Mn$_2$O$_7$ ($52-72$ meV), and Mn$_{90}$Cu$_{10}$ (88 meV). In addition, the spin-wave dispersion shows a deviation from the relation $({\hbar\omega})^2 = c^2q^2 + {\Delta}^2$ above 40 meV. The group velocity above this energy increases to 470(40) meVA, which is higher than that at the low energies, $c = 226(5)$ meVA. These results could suggest that the spin-wave excitations merge with the continuum of the individual particle-hole excitations at 40 meV. more...

Neutron Brillouin scattering (NBS) is an inelastic neutron scattering near the forward direction. This technique is effective for observing coherent excitations in non-single-crystal samples, such ... more...