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On-demand spin orientation with long polarized lifetime and easily detectable signal is an ultimate goal for spintronics. However, there still exists a trade-off between controllability and stability of spin polarization, awaiting a significant breakthrough. Here, we demonstrate switchable optomagnet effects in (Fe$_{1-x}$Zn$_{x}$)$_{2}$Mo$_{3}$O$_{8}$, from which we can obtain tunable magnetization, spanning from -40$\%$ to 40$\%$ of a saturated magnetization that is created from zero magnetization in the antiferromagnetic state without magnetic fields. It is accomplishable via utilizing circularly-polarized laser pulses to excite spin-flip transitions in polar antiferromagnets that have no spin canting, traditionally hard to control without very strong magnetic fields. The spin controllability in (Fe$_{1-x}$Zn$_{x}$)$_{2}$Mo$_{3}$O$_{8}$ originates from its polar structure that breaks the crystal inversion symmetry, allowing distinct on-site $d$-$d$ transitions for selective spin flip. By chemical doping, we exploit the phase competition between antiferromagnetic and ferrimagnetic states to enhance and stabilize the optomagnet effects, which result in long-lived photoinduced Kerr rotations. The present study, creating switchable giant optomagnet effects in polar antiferromagnets, sketches a new blueprint for the function of antiferromagnetic spintronics.

Using previously described functional techniques for some non-perturbative, gauge invariant, renormalized QCD processes, a simplified version of the amplitudes - in which forms akin to Pomerons naturally appear - provides fits to ISR and LHC-TOTEM pp elastic scattering data. Those amplitudes rely on a specific function $\phi(b)$ which describes the fluctuations of the transverse position of quarks inside hadrons., Comment: 6 Pages, 8 figures. Presented at EDS Blois 2019 Conference, Quy Nhon, Vietnam, June 23--28, 2019

Using previously described functional techniques for some non--perturbative, gauge invariant, renormalized QCD processes, a simplified version of the amplitudes --- in which forms akin to Pomerons naturally appear --- provides fits to ISR and LHC--TOTEM $pp$ elastic scattering data. Those amplitudes rely on a specific function $\varphi (\vec b)$ which describes the fluctuations of the transverse position of quarks inside hadrons., Comment: 23 pages, 12 figures. arXiv admin note: text overlap with arXiv:1611.02691

We demonstrate that dynamics of the ab-spiral-spin order in a magnetoelectric multiferroic Eu0.55Y0.45MnO3 can be unambiguously probed through optical second harmonic signals, generated via the spin-induced ferroelectric polarization. In the case of relatively weak photoexcitation,the ferroelectric and the spiral-spin order remains interlocked, both relaxing through spin-lattice relaxation in the non-equilibrium state. When the additional optical pulse illuminating sample is intense enough to induced a local phase transition thermally, the system creates a metastable state of the bc-spiral-spin order (with the electric polarization P//c) via supercooling across the first-order phase transition between ab- and bc-spiral. The supercooled state of bc-spiral spin is formed in the thermodynamical ground state of ab-spiral (P//a), displaying a prolonged lifetime with strong dependence on the magnetic field along the a-axis. The observed photo-switching between the two distinct multiferroic states sheds light on novel photoinduced phenomena in spiral-spin multiferroics.

A new non-perturbative, gauge-invariant model QCD renormalization is applied to high energy elastic pp-scattering. The differential cross-section deduced from this model displays a diffraction dip that resembles those of experiments. Comparison with ISR and LHC data is currently underway., Comment: Conference proceedings for 4th International Conference on New Frontiers in Physics, ICNFP2015. Greece, 2015. subsequent work of Ann. Phys. 359, (2015); or arXiv:1412.2072, and arXiv:1502.04378

A new approach to all-optical detection and control of the coupling between electric and magnetic order on ultrafast timescales is achieved using time-resolved second harmonic generation (SHG) to study a ferroelectric (FE)/ferromagnet (FM) oxide heterostructure. We use femtosecond optical pulses to modify the spin alignment in a Ba$_{0.1}$Sr$_{0.9}$TiO$_{3}$(BSTO)/La$_{0.7}$Ca$_{0.3}$MnO$_{3}$ (LCMO) heterostructure and selectively probe the ferroelectric response using SHG. In this heterostructure, the pump pulses photoexcite non-equilibrium quasiparticles in LCMO, which rapidly interact with phonons before undergoing spin-lattice relaxation on a timescale of tens of picoseconds. This reduces the spin-spin interactions in LCMO, applying stress on BSTO through magnetostriction. This then modifies the FE polarization through the piezoelectric effect, on a timescale much faster than laser-induced heat diffusion from LCMO to BSTO. We have thus demonstrated an ultrafast indirect magnetoelectric effect in a FE/FM heterostructure mediated through elastic coupling, with a timescale primarily governed by spin-lattice relaxation in the FM layer.

A particular choice of renormalization, within the simplifications provided by the non-perturbative property of Effective Locality, leads to a completely finite, renormalized theory of QCD, in which all correlation functions can, in principle, be defined and calculated. In this Model of renormalization, only the Bundle chain-Graphs of the cluster expansion are non-zero. All Bundle graphs connecting to closed quark loops of whatever complexity, and attached to a single quark line, provided no 'self-energy' to that quark line, and hence no effective renormalization. However, the exchange of momentum between one quark line and another, involves only the cluster-expansion's chain graphs, and yields a set of contributions which can be summed and provide a finite color-charge renormalization that can be incorporated into all other QCD processes. An application to high energy elastic pp scattering is now underway., Comment: 30 pages, 8 figures,Minor revision in RevTeX 4.1, subsequent work of Eur. Phys. J. C65, 395-411 (2010), Ann. Phys. 327, 2666-2690 (2012), Ann. Phys. 338, 107-122 (2013), and Ann. Phys. 344, 78-96 (2014); or arXiv:0903.2644, arXiv:1003.2936, arXiv:1103.4179, arXiv:1104.4663, arXiv:1203.6137, arXiv:1204.2038, and arXiv:1207.5017

Using ultrafast optical spectroscopy, we show that polaronic behavior associated with interfacial antiferromagnetic order is likely the origin of tunable magnetotransport upon switching the ferroelectric polarity in a La$_{0.7}$Ca$_{0.3}$MnO$_{3}$/BiFeO$_{3}$ (LCMO/BFO) heterostructure. This is revealed through the difference in dynamic spectral weight transfer between LCMO and LCMO/BFO at low temperatures, which indicates that transport in LCMO/BFO is polaronic in nature. This polaronic feature in LCMO/BFO decreases in relatively high magnetic fields due to the increased spin alignment, while no discernible change is found in the LCMO film at low temperatures. These results thus shed new light on the intrinsic mechanisms governing magnetoelectric coupling in this heterostructure, potentially offering a new route to enhancing multiferroic functionality.

An emerging area in condensed matter physics is the use of multilayered heterostructures to enhance ferroelectricity in complex oxides. Here, we demonstrate that optically pumping carriers across the interface between thin films of a ferroelectric (FE) insulator and a ferromagnetic metal can significantly enhance the FE polarization. The photoinduced FE state remains stable at low temperatures for over one day. This occurs through screening of the internal electric field by the photoexcited carriers, leading to a larger, more stable polarization state that may be suitable for applications in areas such as data and energy storage.

We report ultrafast surface pump and interface probe experiments on photoexcited carrier transport across single crystal bismuth films on sapphire. The film thickness is sufficient to separate carrier dynamics from lattice heating and strain, allowing us to investigate the time-scales of momentum relaxation, heat transfer to the lattice and electron-hole recombination. The measured electron-hole ($e-h$) recombination time is 12--26 ps and ambipolar diffusivity is 18--40 cm$^{2}$/s for carrier excitation up to $\sim 10^{19} \text{cm}^{-3}$. By comparing the heating of the front and back sides of the film, we put lower limits on the rate of heat transfer to the lattice, and by observing the decay of the plasma at the back of the film, we estimate the timescale of electron-hole recombination. We interpret each of these timescales within a common framework of electron-phonon scattering and find qualitative agreement between the various relaxation times observed. We find that the carrier density is not determined by the $e-h$ plasma temperature after a few picoseconds. The diffusion and recombination become nonlinear with initial excitation $\gtrsim 10^{20} \text{cm}^{-3}$.

Even though approximated, strong coupling non-perturbative QCD amplitudes remain very difficult to obtain. In this article, in eikonal and quenched approximations, physical insights are presented that rely on the newly-discovered property of Effective Locality., Comment: Revised version (28 pages and 1 figure in REVTeX). Follow-up work of Eur. Phys. J. C65, pp. 395-411 (2010), (arXiv:1204.2038 [hep-ph]), and Ann. Phys. 327, pp. 2666-2690 (2012), (arXiv:1203.6137 [hep-ph])

Following a previous calculation of quark scattering in eikonal approximation, this paper presents a new, analytic and rigorous approach to the calculation of QCD phenomena. In this formulation a basic distinction between the conventional "idealistic" description of QCD and a more "realistic" description is brought into focus by a non-perturbative, gauge-invariant evaluation of the Schwinger solution for the QCD generating functional in terms of the exact Fradkin representations of the Green's functional and the vacuum functional. Because quarks exist asymptotically only in bound states, their transverse coordinates can never be measured with arbitrary precision; the non-perturbative neglect of this statement leads to obstructions that are easily corrected by invoking in the basic Lagrangian a probability amplitude which describes such transverse imprecision. The second result of this non-perturbative analysis is the appearance of a new and simplifying output called "Effective Locality", in which the interactions between quarks by the exchange of a "gluon bundle" - which "bundle" contains an infinite number of gluons, including cubic and quartic gluon interactions - display an exact locality property that reduces the several functional integrals of the formulation down to a set of ordinary integrals. It should be emphasized that "non-perturbative" here refers to the effective summation of all gluons between a pair of quark lines, but does not (yet) include a summation over all closed-quark loops which are tied by gluon-bundle exchange to the rest of the "Bundle Diagram". As an example of the power of these methods we offer as a first analytic calculation the quark-antiquark binding potential of a pion, and the corresponding three-quark binding potential of a nucleon, obtained in a simple way from relevant eikonal scattering approximations., Comment: 38 pages, 3 figures in REVTeX. Collections of follow-on work of Eur. Phys. J. C65, pp. 395-411 (2010). arXiv admin note: text overlap with arXiv:1103.4179, arXiv:1104.4663, arXiv:1003.2936

Removal of the quenched approximation in the mechanism which produced an analytic estimate of quark-binding potentials, along with a reasonable conjecture of the color structure of the nucleon formed by such a binding potential, is shown to generate an effective, nucleon scattering and binding potential. The mass-scale factor on the order of the pion mass, previously introduced to define transverse imprecision of quark coordinates, is again used, while the strength of the potential is proportional to the square of a renormalized QCD coupling constant. The potential so derived does not include corrections due to spin, angular momentum, nucleon structure, and electroweak interactions; rather, it is qualitative in nature, showing how Nuclear Physics can arise from fundamental QCD., Comment: 25 pages, 3 figures in REVTeX. The fifth of a series on Non-Perturbative QCD (Eur. Phys. J. C65, 395 (2010) or arXiv:0903.2644 [hep-th], arXiv:1003.2936 [hep-th], arXiv:1103.4179 [hep-th] and arXiv:1104.4663 [hep-th].)

We report a comprehensive study of ultrafast carrier dynamics in single crystals of multiferroic BiFeO$_{3}$. Using femtosecond optical pump-probe spectroscopy, we find that the photoexcited electrons relax to the conduction band minimum through electron-phonon coupling with a $\sim$1 picosecond time constant that does not significantly change across the antiferromagnetic transition. Photoexcited electrons subsequently leave the conduction band and primarily decay via radiative recombination, which is supported by photoluminescence measurements. We find that despite the coexisting ferroelectric and antiferromagnetic orders in BiFeO$_{3}$, the intrinsic nature of this charge-transfer insulator results in carrier relaxation similar to that observed in bulk semiconductors.

This paper applies the analytic forms of a recent non-perturbative, manifestly gauge- and Lorentz-invariant description (of the exchange of all possible virtual gluons between quarks ($Q$) and/or anti-quarks ($\bar{Q}$) in a quenched, eikonal approximation) to extract analytic forms for the binding potentials generating a model $Q$-$\bar{Q}$ "pion", and a model $QQQ$ "nucleon". Other, more complicated $Q$, $\bar{Q}$ contributions to such color-singlet states may also be identified analytically. An elementary minimization technique, relevant to the ground states of such bound systems, is adopted to approximate the solutions to a more proper, but far more complicated Schroedinger/Dirac equation; the existence of possible contributions to the pion and nucleon masses due to spin, angular momentum, and "deformation" degrees of freedom is noted but not pursued. Neglecting electromagnetic and weak interactions, this analysis illustrates how the one new parameter making its appearance in this exact, realistic formalism may be evaluated, along with a qualitative estimate of the lowest quark mass and the energy contributions to the ground states of the gluon fields, from a knowledge of the pion and (ground state) nucleon masses., Comment: 12 pages, no figures; The fourth piece of a series on Non-Perturbative QCD (Eur. Phys. J. C65, 395 (2010), arXiv:1003.2936 [hep-th] and arXiv:1103.4179 [hep-th])

A basic distinction, long overlooked, between the conventional, "idealistic" formulation of QCD, and a more "realistic" formulation is brought into focus by a rigorous, non-perturbative, gauge-invariant evaluation of the Schwinger solution for the QCD generating functional in terms of exact Fradkin representations for the Green's functional $\mathbf{G}_{c}(x,y|A)$ and the vacuum functional $\mathbf{L}[A]$. The quanta of all (Abelian) quantized fields may be expected to obey standard quantum-mechanical measurement properties, perfect position dependence at the cost of unknown momenta, and vice-versa, but this is impossible for quarks since they always appear asymptotically in bound states, and their transverse position or momenta can never, in principle, be exactly measured. Violation of this principle produces an absurdity in the exact evaluation of each and every QCD amplitude. We here suggest a phenomenological change in the basic QCD Lagrangian, such that a limitation of transverse precision is automatically contained in the now "realistic" theory, with the function essential to quark binding into hadrons appearing in the new Lagrangian. All absurdities in estimates of all "realistic" QCD amplitudes are then removed, and one obtains the possibility of hadron formation by appropriate quark binding potentials, and nucleon scattering and binding by effective, Yukawa-type potentials; the first of these potentials are constructed, in detail, in the following paper., Comment: 21 pages, 3 figures, the third piece of a series (Eur. Phys. J. C65, 395 (2010) and arXiv:1003.2936[hep-th]). Additional proof has been added along with 2 appendices for more details in the main text

For over a century, x-ray scattering has been the most powerful tool for determining the equilibrium structure of crystalline materials. Deviations from perfect periodicity, for example due to thermal motion of the atoms, reduces the intensity of the Bragg peaks as well as produces structure in the diffuse scattering background. Analysis of the thermal diffuse scattering (TDS) had been used to determine interatomic force constants and phonon dispersion in relatively simple cases before inelastic neutron scattering became the preferred technique to study lattice dynamics. With the advent of intense synchrotron x-ray sources, there was a renewed interest in TDS for measuring phonon dispersion. The relatively short x-ray pulses emanating from these sources also enables the measurement of phonon dynamics in the time domain. Prior experiments on nonequilibrium phonons were either limited by time-resolution and/or to relatively long wavelength excitations. Here we present the first images of nonequilibrium phonons throughout the Brillouin zone in photoexcited III-V semiconductors, indium-phosphide and indium-antimonide, using picosecond time-resolved diffuse scattering. In each case, we find that the lattice remain out of equilibrium for several hundred picoseconds up to nanoseconds after laser excitation. The non-equilibrium population is dominated by transverse acoustic phonons which in InP are directed along high-symmetry directions. The results have wide implications for the detailed study of electron-phonon and phonon-phonon coupling in solids., Comment: 10 pages, 3 figures

In a recent paper it was shown how quark scattering in a quenched, eikonal model led to a momentum-transfer dependent amplitude expressed in terms of Halpern's functional integral; and how the requirement of manifest gauge invariance converted that functional integral into a local integral, capable of being evaluated with precision by a finite set of numerical integrations. We here prove that this property of "effective locality" holds true for all quark processes, without approximation and without exception., Comment: Expanded and Revised in REVTeX 4.1, 14 pages, follow-on work of Eur. Phys. J. C65, pp.395-411 (2010) or arXiv:0903.2644v2 [hep-th]

The interpretation of virtual gluons as ghosts in the non-linear gluonic structure of QCD permits the formulation and realization of a manifestly gauge-invariant and Lorentz covariant theory of interacting quarks/anti-quarks, for all values of coupling. The simplest example of quark/anti-quark scattering in a high-energy, quenched, eikonal model at large coupling is shown to be expressible as a set of finite, local integrals which may be evaluated numerically; and before evaluation, it is clear that the result will be dependent only on, and is damped by increasing momentum transfer, while displaying physically-reasonable color dependence in a manner underlying the MIT Bag Model and an effective, asymptotic freedom. A similar but more complicated integral will result from all possible gluonic-radiative corrections to this simplest eikonal model. Our results are compatible with an earlier, field-strength analysis of Reinhardt et al., Comment: 35 pages, no figures

In anticipation of a subsequent application to QCD, we consider the case of QED at high temperature. We introduce a Fradkin representation into the exact, Schwingerian, functional expression of a fermion propagator, as well as a new and relevant version of the Bloch-Nordsieck (BN) model, which extracts the soft contributions of every perturbative graph, in contradistinction to the assumed separation of energy scales of previous semi-perturbative treatments. Our results are applicable to the absorption of a fast particle which enters a heat bath, as well as to the propagation of a symmetric pulse within the thermal medium due to the appearance of an instantaneous, shock-wave-like source acting in the medium. An exponentially-decreasing time dependence of the incident particle's initial momentum combines with a stronger decrease in the particle's energy, estimated by a sum over all Matsubara frequencies, to model an initial "fireball", which subsequently decays in a Gaussian fashion. When extended to QCD, qualitative applications could be made to RHIC scattering, in which a fireball appears, expands and is damped away., Comment: 22 pages, RevTeX with BibTeX