Shen, Huijia, Yin, Zhenping, He, Yun, Ansmann, Albert, Zhan, Yifan, Wang, Longlong, and Jing, Dongzhe
Cirrus clouds are of great importance to the global climate, with their net radiative forcing strongly dependent on the microphysical properties that are related to the ice‐nucleating regime. However, the influence of long‐range transport of dust on primary ice formation in cirrus clouds is limitedly understood, specifically over the clean remote ocean regions. Here, two case studies show that transpacific Asian dust can impact the ice formation of cirrus clouds over the central Pacific based on Cloud‐Aerosol Lidar with Orthogonal Polarization and Cloud Profiling Radar (CPR, CloudSat) observations. One case shows a well‐developed horizontally extended cirrus embedded in a pure dust layer, with an average dust‐related ice‐nucleating particle concentration (INPC) of 7 L−1 and 96 L−1 for an ice saturation ratio Si of 1.15 and 1.25, respectively; ice crystal number concentration (ICNC) with diameters >25 and 100 μm (denoted as nice,25 μm and nice,100 μm) are 64 L−1 and 7 L−1, respectively. Another case shows that cirrus clouds with a much smaller horizontal extent appeared in the vicinity of polluted dust, with an average INPC of 42–310 L−1 for the typical higher Si of 1.25–1.35 by considering a tenfold reduction of the ice nucleation efficiency of ice crystals; nice,25 μm and nice,100 μm are 168 L−1 and 20 L−1, respectively. The estimated INPC and ICNC values suggest the dominance of ice formation by dust‐induced heterogeneous nucleation, proving that the long‐range transport of dust toward the upper troposphere and the potential influence on cirrus formation over the central Pacific should be well considered in atmospheric models. Plain Language Summary: Cirrus clouds are vital to the global radiative balance. Their net radiation effect is very uncertain, depending on the microphysical properties that are mainly determined by the ice nucleation mechanism, that is, heterogeneous and homogeneous ice nucleation. In this work, two dust‐cirrus interaction cases are studied with the combinational observations of space‐borne lidar and radar. Over the remote central Pacific, where is generally very clean, we show that the long‐range transported Asian dust can significantly influence the ice nucleation at cirrus height by acting as efficient ice‐nucleating particles (INPs). The estimated number concentrations of INPs and ice crystals reveal that dust‐induced heterogeneous nucleation is dominant in ice formation, which should thus be better considered in atmospheric and climate models. Key Points: Cloud‐Aerosol Lidar with Orthogonal Polarization (CALIOP)‐CloudSat observations corroborate that dust in the outflow regime of Asia can influence cirrus formation over the central PacificCALIOP observations indicate the strongest dust occurrence in the upper troposphere over the Pacific during the spring seasonDust transport toward the upper troposphere and the potential impact on cirrus formation should be well considered in atmospheric models [ABSTRACT FROM AUTHOR]