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Pulse self-compression is a simple and economical method for improving the peak power of ultra-intense laser pulses. By solving a modified nonlinear Schrodinger equation considering the fifth-order susceptibility, we found that self-compression appeared even in normally dispersive medium owing to the negative fifth-order susceptibility inducing a mass of negative frequency chirp. Furthermore, negatively pre-chirped pulses allow for self-compression at lower intensity, avoiding medium damage. We numerically analyze the optimal choice of pre-chirp, input intensity, and medium length. A proof-of-principle experiment successfully proves the above theoretical findings. It is expected that petawatt or even exawatt laser pulses with 25 fs/15 fs transform limited pulse duration can be self-compressed to about 9.9 fs/7.6 fs in normally dispersive medium, such as fused silica glass plate., Comment: 24 pages, 8 figures, 1 table

Spatiotemporal optical vortex (STOV) is a unique optical vortex with phase singularity in the space-time domain and the photons in a STOV can carry transverse orbital angular momentum (OAM). The STOV shows many fantastic properties which are worth exploring. Here, we theoretically and experimentally study the diffraction property of STOV, which is a fundamental wave phenomenon. The diffraction behaviors of STOVs are obviously affected by the transverse OAM. The diffraction patterns of STOV pulses diffracted by a grating show multi-lobe structure with each gap corresponding to 1 topological charge. The diffraction properties of lights with transverse OAM are demonstrated clearly and help us understanding the physical properties of STOV, which will be of special applications, such as the realization of fast detection of STOVs with different topological charges, which may pay the way for STOV based optical communication., Comment: 12 pages, 8 figures

A multistage smoothing multistep pulse compressor (MPC) based on a single-pass single-grating-pair (SSGP) main compressor is proposed to simplify the entire petawatt (PW) compressor. Only one grating pair with relatively long distance is used to generate the same amount of spectral dispersion in the main compressor compared with a four-grating main compressor. As the SSGP induces the largest spatial dispersion, it can introduce the best beam-smoothing effect to the laser beam on the last grating. When considering the diffraction loss of only two gratings, the total compression efficiency of the SSGP main compressor is even larger than that of a four-grating main compressor. Furthermore, the spatiotemporal aberration induced by single-grating-pair can be compensated effectively by using deformable mirrors, however it is difficult or complicated to be well compensated in a four-grating compressor. Approximately 50-100 PW laser pulses can be obtained using this SSGP-based multistage smoothing MPC with a single laser beam, Comment: 12 pages, 8 figures

Ultrahigh peak power lasers are important scientific tools for frontier laser-physics researches, in which both the peak power improvement and operating safety are very important meanwhile limited by the damage threshold and size of compression gratings currently. Based on a recent reported method "multistep pulse compressor (MPC)", a multistage smoothing based MPC (MS-MPC) is proposed here to further improve the running safety, operating convenience, and simplify the whole setup of the MPC. In this optimized design, the beam smoothing is not simply executed in the pre-compressor or main-compressor, but separated into multistage. Then, it can protect important optics in every stage directly and reduce the executing difficult of typical MPC at the same time. The prism pair based pre-compressor will induce suitable spatial dispersion which is easier to be achieved and enough to protect the first grating directly. At the same time, the asymmetric four-grating compressor (AFGC) will also induce spatial dispersion to further smooth the laser beam which helps to protect the last grating directly. In this way, 10s-100s PW lasers can be compressed by using current available optics with improved operating safety owing to remove random spatial intensity modulations. Furthermore, an additional beam smoothing stage can be added before the main amplifier to protect the biggest amplification crystal away from damage. This MS-MPC optical design can be easily extended to be used in all exist PW laser facilities to improve their potential compressed pulse energy and running safety., Comment: 15pages, 7 figures

Ultra-short ultra-intense laser provides unprecedented experimental tools and extreme physical conditions to explore frontier secrets of nature. Recently, multistep pulse compressor (MPC) was proposed to break through the limitation of the size and damage threshold of the grating in the compressor during the realization of higher peak power laser. In the MPC methods, beam smoothing in the pre-compressor is a very important process. Here, beam smoothing based on prism pair were studied technically, in which both the spatial profiles and the spectral dispersive properties were analyzed in detail. The simulation results show clearly that the prism pair can effectively smooth the laser beam. Furthermore, the beam smoothing is much more efficiency with shorter separated distance if two prism pairs are arranged to induce spatial dispersion at one direction or two directions. The results of beam smoothing here will help the optimized optical designs in all PW laser systems to improve their output and running safety., Comment: 12pages,7figures

Increasing any degree of freedom of light beam may open a wide application area of this special light beam. Vortex beam with a dimension of orbital angular momentum (OAM) as a useful light source has been widely applied in many fields. Here, unique multicolor concentric ultrafast vortex beams (MUCU-VBs), which are also named ultrafast photonic rainbow, with controllable orbital angular momentum are firstly generated using cascaded four-wave mixing (CFWM) in an yttrium aluminum garnet (YAG) plate. Up to 9 multicolor concentric annular ultrafast vortex sidebands are generated simultaneously. The topological charges of the sidebands, which are controllable by changing the topological charges of the two input pump beams, are measured and in according with the theoretical analysis very well. The novel MUCU-VBs can be manipulated simultaneously in temporal, spatial, spectral domains and OAM state, which open more than one new degree of freedoms of vortex light beam and will be of wide and special applications, such as multicolor pump-probe experiments, simultaneous microparticle manipulation and exploring, and optical communication. Moreover, the special focusing properties of the multicolor ultrafast sidebands, such as multi-focus of different wavelengths, may further extend their application area., Comment: 11 pages, 7 figures

The peak power improvement and running safety of petawatt (PW) lasers are limited by laser-induced damage of optical components with limited sizes and damage thresholds. Diffraction gratings in pulse compressors have been the shortest stave of PW lasers up to now, as to manufacture a high quality meter-sized grating remains particularly challenging. Here, the asymmetric four-grating compressor (AFGC) with asymmetric configuration is proposed for PW lasers to increase the maximum bearable output pulse energy and running safety without neither additional optical component nor extra control in comparison to a traditional Treacy four-grating compressor (TFGC) with symmetric configuration. In AFGC, suitable spatial dispersion can be introduced in the output laser beam which is able to decrease the laser spatial intensity modulation (LSIM) of the output beam on the final grating. The introduced spatial dispersion can be automatically compensated at the focal plane by using the spatiotemporal focusing technique. Based on this simple AFGC design, not only the damage risk of the final grating can be reduced, but also the maximum output pulse energy can be improved by about 1.8 times theoretically. As an example, 100 PW output power can be achieved theoretically by using the AFGC with an input beam size of 550*700 mm2., Comment: 11pages,4 figures

High-energy tens (10s) to hundreds (100s) petawatt (PW) lasers are key tools for exploring frontier fundamental researches such as strong-field quantum electrodynamics (QED), and the generation of positron-electron pair from vacuum. Recently, pulse compressor became the main obstacle on achieving higher peak power due to the limitation of damage threshold and size of diffraction gratings. Here, we propose a feasible multistep pulse compressor (MPC) to increase the maximum bearable input and output pulse energies through modifying their spatiotemporal properties. Typically, the new MPC including a prism pair for pre-compression, a four-grating compressor (FGC) for main compression, and a spatiotemporal focusing based self-compressor for post-compression. The prism pair can induce spatial dispersion to smooth and enlarge the laser beam, which increase the maximum input and output pulse energies. As a result, as high as 100 PW laser with single beam or more than 150 PW through combining two beams can be obtained by using MPC and current available optics. This new optical design will simplify the compressor, improve the stability, and save expensive gratings/optics simultaneously. Together with the multi-beam tiled-aperture combining method, the tiled-grating method, larger gratings, or negative chirp pulse based self-compression method, several 100s PW laser beam is expected to be obtained by using this MPC method in the future, which will further extend the ultra-intense laser physics research fields., Comment: 18 pages, 10 figures

One of the most serious bottleneck on achieving kilojoule-level high-energy petawatt (PW) to hundreds-petawatt (100PW) lasers with ps to fs pulse duration is the requirement of as large as meter-sized gratings in the compressor so as to avoid the laser-induced damage to the gratings. However, this kind of meter-sized grating with high quality is hard to manufacture so far. Here, we propose a new in-house beam-splitting compressor based on the property that the damage threshold of gratings depend on the pulse duration. The new scheme will simultaneously improve the stability, save expensive gratings, and simplify the size of compressor because the split beams share the first two parallel gratings. Furthermore, based on the fact that the transmitted wavefront of a glass plate can be much better and more precisely controlled than that of the diffraction wavefront of a large grating, then glass plates with designed transmitted wavefront are proposed to compensate the wavefront distortion introduced by the second, the third gratings, and other optics in-house such as the beam splitter. This simple and economical method can compensate the space-time distortion in the compressor and then improve the focal intensity, which otherwise cannot be compensated by the deformable mirror outside the compressor due to angular chirp. Together with multi-beams tiled-aperture combining scheme, the novel compressor provides a new scheme to achieve high-energy PW-100PW lasers or even exawatt lasers with relatively small gratings in the future., Comment: 6 figures

The temporal contrast is one of the most important parameters of an ultra-high intense laser pulse. Third-order auto-correlator or cross-correlator have been widely used to characterize the temporal contrast of an ultra-intense laser pulse in the past decades. Here, a novel and simple single-shot fourth-order auto-correlator to characterize the temporal contrast with higher time resolution and better pulse contrast fidelity in comparison to third-order correlators is proposed. The single-shot fourth-order autocorrelation consists of a frequency degenerate four-wave mixing process and a sum-frequency mixing process. The proof-of-principle experiments show that a dynamic range of approximately 10^11 compared with the noise level, a time resolution of approximately 160 fs, and a time window of 65 ps can be successfully obtained using the novel single-shot fourth-order auto-correlator, which is the highest dynamic range with simultaneous high time resolution for single-shot temporal contrast measurement so far. Furthermore, the temporal contrast of laser pulse from a PW laser system is successfully measured in single-shot with a dynamic range of about 2*10^10 and simultaneous a time resolution of 160 fs., Comment: 29 pages 9 figures

A single-shot characterization of the temporal contrast of a petawatt laser pulse with a high dynamic-range, is important not only for improving conditions of the petawatt laser facility itself, but also for various high-intensity laser physics experiments, which is still a difficult problem. In this study, a new idea for improving the dynamic-range of a single-shot temporal contrast measurement using novel temporal contrast reduction techniques is proposed. The proof-of-principle experiments applying single stage of pulse stretching, anti-saturated absorption, or optical Kerr effect successfully reduce the temporal contrast by approximately one order of magnitude. Combining with the SRSI-ETE method, its dynamic-range characterization capability is improved by approximately one order of magnitude to approximately 109. It is expected that a higher dynamic-range temporal contrast can be characterized using cascaded temporal contrast reduction processes., Comment: 29 pages, 7 figures

We demonstrate the generation of 100-{\mu}J-level multicolored femtosecond pulses based on a single-stage cascaded four-wave mixing (CFWM) process in a thin glass plate. The generated high-energy CFWM signals can shift the central wavelength and have well-enhanced temporal contrast because of the third-order nonlinear process. They are innovatively used as clean sampling pulses of a cross-correlator for single-shot temporal contrast measurement. With a simple home-made setup, the proof-of-principle experimental results demonstrate the single-shot cross-correlator with dynamic range of 1010, temporal resolution of about 160 fs and temporal window of 50 ps. To the best of our knowledge, this is the first demonstration in which both the dynamic range and the temporal resolution of a single-shot temporal contrast measurement are comparable to those of a commercial delay-scanning cross-correlator., Comment: 20 pages, 8 figures

The self-referenced spectral interferometry (SRSI) technique, which is usually used for microjoule-level femtosecond pulses characterization, is improved to characterize weak femtosecond pulses with nanojoule based on the transient-grating effect. Both femtosecond pulses from an amplifier with 3 nJ per pulse at 1 kHz repetition rates and femtosecond pulses from an oscillator with less than 0.5 nJ per pulse at 84 MHz repetition rates are successfully characterized. Furthermore, through a special design, the optical setup of the device is even smaller than a palm which will makes it simple and convenient during the application. These improvements extend the application of SRSI technique to the characterization of femtosecond pulses in a broad range. Not only pulses from an amplifier but also pulses from an oscillator or weak pulses used in ultrafast spectroscopy can be monitored with this SRSI method right now., Comment: 8 pages 3 figures