Search

Spectrum shape measurements in nuclear $\beta$ decay can be used to test physics beyond the Standard Model with results being complementary to high-energy collider experiments. In particular, Beyond Standard Model sensitivity of the weak interaction is expressed through the so-called Fierz interference term. Additionally, the $\beta$ spectrum shape is a useful tool to probe Standard Model effects, among which the most prominent is \textit{weak magnetism}, a higher-order recoil correction induced by nuclear pion exchange. To study effects in the $\beta$ spectrum shape at a precision level competitive with the LHC, a new spectrometer was designed and built. It consists of a 3D low-pressure gas electron tracker and a plastic scintillator used for triggering the data acquisition and recording the $\beta$ particle energy. In this Letter, the results from $\beta$ spectrum shape measurements on the allowed Gamow-Teller transition $^{114}\text{In} \rightarrow ^{114}\text{Sn}$ are presented, including a first extraction of the weak magnetism form factor in the high nuclear mass range and a new estimate of the $90\%$ confidence interval for the Fierz interference term., Comment: 6 pages, 2 figures

High-precision searches for an electric dipole moment of the neutron (nEDM) require stable and uniform magnetic field environments. We present the recent achievements of degaussing and equilibrating the magnetically shielded room (MSR) for the n2EDM experiment at the Paul Scherrer Institute. We present the final degaussing configuration that will be used for n2EDM after numerous studies. The optimized procedure results in a residual magnetic field that has been reduced by a factor of two. The ultra-low field is achieved with the full magnetic-field-coil system, and a large vacuum vessel installed, both in the MSR. In the inner volume of ~1.4 m^3, the field is now more uniform and below 300 pT. In addition, the procedure is faster and dissipates less heat into the magnetic environment, which in turn, reduces its thermal relaxation time from 12 h down to ~1.5 h.

We present a novel Active Magnetic Shield (AMS), designed and implemented for the n2EDM experiment at the Paul Scherrer Institute. The experiment will perform a high-sensitivity search for the electric dipole moment of the neutron. Magnetic-field stability and control is of key importance for n2EDM. A large, cubic, 5m side length, magnetically shielded room (MSR) provides a passive, quasi-static shielding-factor of about 10^5 for its inner sensitive volume. The AMS consists of a system of eight complex, feedback-controlled compensation coils constructed on an irregular grid spanned on a volume of less than 1000m^3 around the MSR. The AMS is designed to provide a stable and uniform magnetic-field environment around the MSR, while being reasonably compact. The system can compensate static and variable magnetic fields up to +-50muT (homogeneous components) and +-5muT (first-order gradients), suppressing them to a few muT in the sub-Hertz frequency range. The presented design concept and implementation of the AMS fulfills the requirements of the n2EDM experiment and can be useful for other applications, where magnetically silent environments are important and spatial constraints inhibit simpler geometrical solutions.

We report on a search for a new, short-range, spin-dependent interaction using a modified version of the experimental apparatus used to measure the permanent neutron electric dipole moment at the Paul Scherrer Institute. This interaction, which could be mediated by axion-like particles, concerned the unpolarized nucleons (protons and neutrons) near the material surfaces of the apparatus and polarized ultracold neutrons stored in vacuum. The dominant systematic uncertainty resulting from magnetic-field gradients was controlled to an unprecedented level of approximately 4 pT/cm using an array of optically-pumped cesium vapor magnetometers and magnetic-field maps independently recorded using a dedicated measurement device. No signature of a theoretically predicted new interaction was found, and we set a new limit on the product of the scalar and the pseudoscalar couplings $g_sg_p\lambda^2 < 8.3 \times 10^{-28}\,\text{m}^2$ (95% C.L.) in a range of $5\,\mu\text{m} < \lambda < 25\,\text{mm}$ for the monopole-dipole interaction. This new result confirms and improves our previous limit by a factor of 2.7 and provides the current tightest limit obtained with free neutrons.

Ultra-low-mass axions are a viable dark matter candidate and may form a coherently oscillating classical field. Nuclear spins in experiments on Earth might couple to this oscillating axion dark-matter field, when propagating on Earth's trajectory through our Galaxy. This spin coupling resembles an oscillating pseudo-magnetic field which modulates the spin precession of nuclear spins. Here we report on the null result of a demonstration experiment searching for a frequency modulation of the free spin-precession signal of \magHg in a \SI{1}{\micro\tesla} magnetic field. Our search covers the axion mass range $10^{-16}~\textrm{eV} \lesssim m_a \lesssim 10^{-13}~\textrm{eV}$ and achieves a peak sensitivity to the axion-nucleon coupling of $g_{aNN} \approx 3.5 \times 10^{-6}~\textrm{GeV}^{-1}$., Comment: 18 pages, 4 images, submitted to SciPost Physics

Muonic atom spectroscopy -- the measurement of the x rays emitted during the formation process of a muonic atom -- has a long standing history in probing the shape and size of nuclei. In fact, almost all stable elements have been subject to muonic atom spectroscopy measurements and the absolute charge radii extracted from these measurements typically offer the highest accuracy available. However, so far only targets of at least a few hundred milligram could be used as it required to stop a muon beam directly in the target to form the muonic atom. We have developed a new method relying on repeated transfer reactions taking place inside a 100-bar hydrogen gas cell with an admixture of 0.25% deuterium that allows us to drastically reduce the amount of target material needed while still offering an adequate efficiency. Detailed simulations of the transfer reactions match the measured data, suggesting good understanding of the processes taking place inside the gas mixture. As a proof of principle we demonstrate the method with a measurement of the 2p-1s muonic x rays from a 5-{\mu}g gold target., Comment: 16 pages, 14 figures

For identification and 3D-tracking of low-energy electrons a new type of gas-based detector was designed that minimizes scattering and energy loss. The current version of the detector is a combination of a plastic scintillator, serving as a trigger source and energy detector, and a hexagonally structured multi-wire drift chamber (MWDC), filled with a mixture of helium and isobutane gas. The drift time information is used to track particles in the plane perpendicular to the wires, while a charge division technique provides spatial information along the wires. The gas tracker was successfully used in the miniBETA project as a beta spectrometer for a measurement of the weak magnetism form factor in nuclear beta decay. The precision of the three-dimensional electron tracking, in combination with low-mass, low-Z materials and identification of backscattering from scintillator, facilitated a reduction of the main systematics effects. At certain conditions, a spatial resolution better than 0.5 mm was obtained in the plane perpendicular to the wires, while resolutions of about 6 mm were achieved along wires. Thanks to precise tracking information, it is possible to eliminate electrons and other particles not originating from the desired decay with high efficiency. Additionally, using the coincidence between MWDC and scintillator, background from gamma emission typically accompanying radioactive decays, was highly suppressed. An overview of different event topologies is presented together with the tracker's ability to correctly recognize them. The analysis is supported by Monte Carlo simulations using Geant4 and Garfield++ packages. Finally, the preliminary results from the 114In spectrum study are presented., Comment: 5 pages, 3 figures, accepted for publication in JINST - PSD12(2021)

We present the magnetically shielded room (MSR) for the n2EDM experiment at the Paul Scherrer Institute which features an interior cubic volume with each side of length 2.92m, thus providing an accessible space of 25m3. The MSR has 87 openings up to 220mm diameter to operate the experimental apparatus inside, and an intermediate space between the layers for sensitive signal processing electronics. The characterization measurements show a remanent magnetic field in the central 1m3 below 100pT, and a field below 600pT in the entire inner volume, up to 4\,cm to the walls. The quasi-static shielding factor at 0.01\,Hz measured with a sinusoidal 2muT peak-to-peak signal is about 100,000 in all three spatial directions and rises fast with frequency to reach 10^8 above 1Hz., Comment: 10 pages, 15 Figures, submitted to Review of Scientific Instruments

Measurements of the beta decay correlation coefficients in nuclear decay aim for a precision below $1\%$ and theoretical predictions should follow this trend. In this work, the influence of the two dominant Standard Model correction terms, i.e. the recoil-order and the radiative correction, are studied for the most commonly measured beta correlations, i.e. the $\beta$-asymmetry parameter ($A_{\beta}$) and the $\beta-\nu$ angular correlation ($a_{\beta \nu}$). The recoil-order correction is calculated with the well-known Holstein formalism using the impulse approximation to evaluate experimentally inaccessible form factors. For the $\beta-\nu$ angular correlation previously unpublished, semi-analytical radiative correction values are tabulated. Results are presented for the mirror beta decays up to $A=45$. We examine the effect of both corrections and provide a comparison between different isotopes. This comparison will help planning, analysing, and comparing future experimental efforts., Comment: 16 pages, 10 figures

In recent years a number of correlation measurements in nuclear $\beta$ decay have been performed reaching a precision of the order of 1\% and below and it is expected that even higher precision will be reached in the near future. At these levels of precision higher-order corrections due to e.g. recoil terms induced by the strong interaction and radiative corrections cannot necessarily be neglected anymore when interpreting these results in terms of new physics or extracting a value for the $V_{ud}$ quark-mixing matrix element. We provide here an update of the $\mathcal{F} t$ values of the $T=1/2$ mirror $\beta$ decays as well as an overview of current experimental and theoretical knowledge of the most important recoil term, weak magnetism, for both the $T=1/2$ mirror $\beta$ transitions and a large set of $\beta$ decays in higher isospin multiplets. The matrix elements determining weak magnetism were calculated in the nuclear shell model and cross-checked against experimental data, showing overall good agreement. Additionally, we show that further insight can be obtained from properly deformed nuclear potentials, in particular for mirror $T=1/2$ decays.. The results provide new insights in the size of weak magnetism, extending the available information to $\beta$ transitions of nuclei with masses up to $A =$ 75. This provides important guidance for the planning and interpretation of ongoing and new precise correlation measurements in nuclear $\beta$ decay searching for new physics or to extract the $V_{ud}$ quark-mixing matrix element in mirror $\beta$ decays. This more detailed knowledge of weak magnetism can also be of interest for further theoretical work related to the reactor neutrino problem., Comment: 64 pages, 21 figures

Experiments dedicated to the measurement of the electric dipole moment of the neutron require outstanding control of the magnetic field uniformity. The neutron electric dipole moment (nEDM) experiment at the Paul Scherrer Institute uses a 199Hg co-magnetometer to precisely monitor magnetic field variations. This co-magnetometer, in the presence of field non-uniformity, is responsible for the largest systematic effect of this measurement. To evaluate and correct that effect, offline measurements of the field non-uniformity were performed during mapping campaigns in 2013, 2014 and 2017. We present the results of these campaigns, and the improvement the correction of this effect brings to the neutron electric dipole moment measurement.

Magnetic Johnson-Nyquist noise (JNN) originating from metal electrodes, used to create a static electric field in neutron electric-dipole-moment (nEDM) experiments, may limit the sensitivity of measurements. We present here the first dedicated study on JNN applied to a large-scale long-measurement-time experiment with the implementation of a co-magnetometry. In this study, we derive surface- and volume-averaged root-mean-square normal noise amplitudes at a certain frequency bandwidth for a cylindrical geometry. In addition, we model the source of noise as a finite number of current dipoles and demonstrate a method to simulate temporal and three-dimensional spatial dependencies of JNN. The calculations are applied to estimate the impact of JNN on measurements with the new apparatus, n2EDM, at the Paul Scherrer Institute. We demonstrate that the performances of the optically pumped $^{133}$Cs magnetometers and $^{199}$Hg co-magnetometers, which will be used in the apparatus, are not limited by JNN. Further, we find that in measurements deploying a co-magnetometer system, the impact of JNN is negligible for nEDM searches down to a sensitivity of $4\,\times\,10^{-28}\,e\cdot{\rm cm}$ in a single measurement; therefore, the use of economically and mechanically favored solid aluminum electrodes is possible.

We present the design of a next-generation experiment, n2EDM, currently under construction at the ultracold neutron source at the Paul Scherrer Institute (PSI) with the aim of carrying out a high-precision search for an electric dipole moment of the neutron. The project builds on experience gained with the previous apparatus operated at PSI until 2017, and is expected to deliver an order of magnitude better sensitivity with provision for further substantial improvements. An overview is given of the experimental method and setup, the sensitivity requirements for the apparatus are derived, and its technical design is described.

It has been proposed that there could be a mirror copy of the standard model particles, restoring the parity symmetry in the weak interaction on the global level. Oscillations between a neutral standard model particle, such as the neutron, and its mirror counterpart could potentially answer various standing issues in physics today. Astrophysical studies and terrestrial experiments led by ultracold neutron storage measurements have investigated neutron to mirror-neutron oscillations and imposed constraints on the theoretical parameters. Recently, further analysis of these ultracold neutron storage experiments has yielded statistically significant anomalous signals that may be interpreted as neutron to mirror-neutron oscillations, assuming nonzero mirror magnetic fields. The neutron electric dipole moment collaboration performed a dedicated search at the Paul Scherrer Institute and found no evidence of neutron to mirror-neutron oscillations. Thereby, the following new lower limits on the oscillation time were obtained: $\tau_{nn'} > 352~$s at $B'=0$ (95% C.L.), $\tau_{nn'} > 6~\text{s}$ for all $0.4~\mu\text{T}9~\text{s}$ for all $5.0~\mu\text{T}

The hyperfine splitting of the 5g -> 4f transitions in muonic 185,187-Re has been measured using high resolution HPGe detectors and compared to state-of-the-art atomic theoretical predictions. The spectroscopic quadrupole moment has been extracted using modern fitting procedures and compared to the values available in literature obtained from muonic X rays of natural rhenium. The extracted values of the nuclear spectroscopic quadrupole moment are 2.07(5) barn and 1.94(5) barn, respectively for 185-Re and 187-Re. This work is part of a larger effort at the Paul Scherrer Institut towards the measurement of the nuclear charge radii of radioactive elements., Comment: 15 pages, 8 figures, 8 tables; accepted for publication in Phys. Rev. C

We present the result of an experiment to measure the electric dipole moment (EDM) of the neutron at the Paul Scherrer Institute using Ramsey's method of separated oscillating magnetic fields with ultracold neutrons (UCN). Our measurement stands in the long history of EDM experiments probing physics violating time reversal invariance. The salient features of this experiment were the use of a Hg-199 co-magnetometer and an array of optically pumped cesium vapor magnetometers to cancel and correct for magnetic field changes. The statistical analysis was performed on blinded datasets by two separate groups while the estimation of systematic effects profited from an unprecedented knowledge of the magnetic field. The measured value of the neutron EDM is $d_{\rm n} = (0.0\pm1.1_{\rm stat}\pm0.2_{\rm sys})\times10^{-26}e\,{\rm cm}$., Comment: 5 pages, 4 figures, submitted to PRL on 18.12.2019

An array of sixteen laser-pumped scalar Cs magnetometers was part of the neutron electric dipole moment (nEDM) experiment taking data at the Paul Scherrer Institute in 2015 and 2016. It was deployed to measure the gradients of the experiment's magnetic field and to monitor their temporal evolution. The originality of the array lies in its compact design, in which a single near-infrared diode laser drives all magnetometers that are located in a high-vacuum chamber, with a selection of the sensors mounted on a high-voltage electrode. We describe details of the Cs sensors' construction and modes of operation, emphasizing the accuracy and sensitivity of the magnetic field readout. We present two applications of the magnetometer array directly beneficial to the nEDM experiment: (i) the implementation of a strategy to correct for the drift of the vertical magnetic field gradient and (ii) a procedure to homogenize the magnetic field. The first reduces the uncertainty of the new nEDM result. The second enables transverse neutron spin relaxation times exceeding 1500 s, improving the statistical sensitivity of the nEDM experiment by about 35% and effectively increasing the rate of nEDM data taking by a factor of 1.8.

We report first time measurements of the beta-neutrino angular correlation based on the kinetic energy shift of protons emitted in parallel or anti-parallel directions with respect to the positron in the beta decay of $^{32}$Ar. This proof of principle experiment provided simultaneous measurements for the superallowed 0$^+$~$\rightarrow$~0$^+$ transition followed by a 3356~keV proton emission and for a Gamow-Teller transition followed by a 2123~keV proton emission. The results, respectively ${\tilde a_{\beta\nu}}=1.01(3)_{(stat)}(2)_{(syst)}$ and ${\tilde a_{\beta\nu}}=-0.22(9)_{(stat)}(2)_{(syst)}$, are found in agreement with the Standard Model. A careful analysis of the data shows that future measurements can reach a precision level of 10$^{-3}$ for both pure Fermi and pure Gamow-Teller decay channels, providing new constraints on both scalar and tensor weak interactions., Comment: 5 pages, 5 figures

The Nab experiment will measure the ratio of the weak axial-vector and vector coupling constants $\lambda=g_A/g_V$ with precision $\delta\lambda/\lambda\sim3\times10^{-4}$ and search for a Fierz term $b_F$ at a level $\Delta b_F<10^{-3}$. The Nab detection system uses thick, large area, segmented silicon detectors to very precisely determine the decay proton's time of flight and the decay electron's energy in coincidence and reconstruct the correlation between the antineutrino and electron momenta. Excellent understanding of systematic effects affecting timing and energy reconstruction using this detection system are required. To explore these effects, a series of ex situ studies have been undertaken, including a search for a Fierz term at a less sensitive level of $\Delta b_F<10^{-2}$ in the beta decay of $^{45}$Ca using the UCNA spectrometer., Comment: Proceedings of the 7th International Syposium on Symmetries in Subatomic Physics SSP2018, Aachen (Germany), 10 - 15 Jun 2018. This is a pre-print of an article published in Hyperfine Interactions. The final authenticated version is available online at: https://doi.org/10.1007/s10751-018-1538-7

The MORA (Matter's Origin from the RadioActivity of trapped and oriented ions) project aims at measuring with unprecedented precision the D correlation in the nuclear beta decay of trapped and oriented ions. The D correlation offers the possibility to search for new CP-violating interactions, complementary to searches done at the LHC and with Electric Dipole Moments. Technically, MORA uses an innovative in-trap orientation method which combines the high trapping efficiency of a transparent Paul trap with laser orientation techniques. The trapping, detection, and laser setups are under development, for first tests at the Accelerator laboratory, JYFL, in the coming years., Comment: 16 pages, 6 figures, proceedings of the TCP 2018 conference, to appear in Hyp. Int

Magnetic field uniformity is of the utmost importance in experiments to measure the electric dipole moment of the neutron. A general parametrization of the magnetic field in terms of harmonic polynomial modes is proposed, going beyond the linear-gradients approximation. We review the main undesirable effects of non-uniformities: depolarization of ultracold neutrons, and Larmor frequency shifts of neutrons and mercury atoms. The theoretical predictions for these effects were verified by dedicated measurements with the single-chamber nEDM apparatus installed at the Paul Scherrer Institute.

We report on the strategy used to optimize the sensitivity of our search for a neutron electric dipole moment at the Paul Scherrer Institute. Measurements were made upon ultracold neutrons stored within a single chamber at the heart of our apparatus. A mercury cohabiting magnetometer together with an array of cesium magnetometers were used to monitor the magnetic field, which was controlled and shaped by a series of precision field coils. In addition to details of the setup itself, we describe the chosen path to realize an appropriate balance between achieving the highest statistical sensitivity alongside the necessary control on systematic effects. The resulting irreducible sensitivity is better than 1*10-26 ecm. This contribution summarizes in a single coherent picture the results of the most recent publications of the collaboration., Comment: Submitted as a web of conference proceedings paper for PPNS2018

We present the new spectrometer for the neutron electric dipole moment (nEDM) search at the Paul Scherrer Institute (PSI), called n2EDM. The setup is at room temperature in vacuum using ultracold neutrons. n2EDM features a large UCN double storage chamber design with neutron transport adapted to the PSI UCN source. The design builds on experience gained from the previous apparatus operated at PSI until 2017. An order of magnitude increase in sensitivity is calculated for the new baseline setup based on scalable results from the previous apparatus, and the UCN source performance achieved in 2016., Comment: Submitted as a web of conference proceedings paper

The neutron and its hypothetical mirror counterpart, a sterile state degenerate in mass, could spontaneously mix in a process much faster than the neutron $\beta$-decay. Two groups have performed a series of experiments in search of neutron - mirror-neutron ($n-n'$) oscillations. They reported no evidence, thereby setting stringent limits on the oscillation time $\tau_{nn'}$. Later, these data sets have been further analyzed by Berezhiani et al.(2009-2017), and signals, compatible with $n-n'$ oscillations in the presence of mirror magnetic fields, have been reported. The Neutron Electric Dipole Moment Collaboration based at the Paul Scherrer Institute performed a new series of experiments to further test these signals. In this paper, we describe and motivate our choice of run configurations with an optimal filling time of $29~$s, storage times of $180~$s and $380~$s, and applied magnetic fields of $10~\mu$T and $20~\mu$T. The choice of these run configurations ensures a reliable overlap in settings with the previous efforts and also improves the sensitivity to test the signals. We also elaborate on the technique of normalizing the neutron counts, making such a counting experiment at the ultra-cold neutron source at the Paul Scherrer Institute possible. Furthermore, the magnetic field characterization to meet the requirements of this $n-n'$ oscillation search is demonstrated. Finally, we show that this effort has a statistical sensitivity comparable to the current leading constraints for $n-n'$ oscillations., Comment: Proceedings of International Workshop on Particle Physics at Neutron Sources, PPNS-2018; May 24-26, 2018, LPSC, Grenoble, France; Abs. ID: 28 and 60. 10 Pages, 9 Figures

Searches of new physics beyond the Standard Model (SM) performed at low energy frontiers are complementary to experiments carried out at high energy colliders. Among the methods for testing the SM and beyond at low energies are the precision spectrum shape and correlation coefficient measurements in nuclear and neutron beta decay. In order to study tiny effects in beta spectrum shape, a special spectrometer was built. It consists of a 3D low pressure gas tracker (drift chamber with hexagonal cells, signal readout at both wire ends) and plastic scintillators for triggering data acquisition and registration of the beta particle energy. The results of the characterization process indicate the possibility of using such a gas tracker in a range of experiments with low energy electrons where beta particle tracking with minimal kinematics deterioration is beneficial. Application of this technique is also planned for neutron decay correlation experiments. In the paper, the first application of this tracker in a high-precision beta spectrum shape study is discussed. The measurement technique, commissioning results, and the future outlook are presented., Comment: Talk presented at CIPANP2018. 10 pages, 6 figures

A beamline dedicated to the production of laser-polarized radioactive beams has been constructed at ISOLDE, CERN. We present here different simulations leading to the design and construction of the setup, as well as technical details of the full setup and examples of the achieved polarizations for several radioisotopes. Beamline simulations show a good transmission through the entire line, in agreement with observations. Simulations of the induced nuclear spin-polarization as a function of atom-laser interaction length are presented for $^{26,28}$Na, [1] and for $^{35}$Ar, which is studied in this work. Adiabatic spin rotation of the spin-polarized ensemble of atoms, and how this influences the observed nuclear ensemble polarization, are also performed for the same nuclei. For $^{35}$Ar, we show that multiple-frequency pumping enhances the ensemble polarization by a factor 1.85, in agreement with predictions from a rate equations model. [1] J. Phys. G: Nucl. Part. Phys./1744084005

We study the dominant forbidden transitions in the antineutrino spectra of the fission actinides from 4 MeV onward using the nuclear shell model. Through explicit calculation of the shape factor, taking into account Coulomb corrections, we show the expected changes on cumulative electron and antineutrino spectra. Compared to the usual allowed approximation this results in a minor decrease of electron spectra from 4 MeV and onward, whereas an increase of several percent is observed in antineutrino spectra. We show that, despite their limited number, forbidden transitions dominate the spectral flux for most of the experimentally accessible range. Based on the shell model calculations we attempt a parametrization of forbidden transitions and propose a spectral correction for all forbidden transitions. We enforce correspondence with the ILL dataset using a summation+conversion approach. When compared against modern reactor neutrino experiments, the resultant spectral change is observed to be of comparable magnitude and shape as the reported spectral shoulder, drastically decreasing the statistical significance of the latter., Comment: Additional information regarding uncertainty estimation, extension of the final analysis to a summation+conversion approach

We report on a laser based $^{199}$Hg co-magnetometer deployed in an experiment searching for a permanent electric dipole moment of the neutron. We demonstrate a more than five times increased signal to-noise-ratio in a direct comparison measurement with its $^{204}$Hg discharge bulb-based predecessor. An improved data model for the extraction of important system parameters such as the degrees of absorption and polarization is derived. Laser- and lamp-based data-sets can be consistently described by the improved model which permits to compare measurements using the two different light sources and to explain the increase in magnetometer performance. The laser-based magnetometer satisfies the magnetic field sensitivity requirements for the next generation nEDM experiments.

The electron shakeoff of 19F and 35Cl atoms resulting from the \b{eta}+ decay of 19Ne+ and 35Ar+ ions has been investigated using a Paul trap coupled to a time of flight recoil-ion spectrometer. The charge-state distributions of the recoiling daughter nuclei were compared to theoretical calculations based on the sudden approximation and accounting for subsequent Auger processes. The excellent agreement obtained for 35Cl is not reproduced in 19F. The shortcoming is attributed to the inaccuracy of the independent particle model employed to calculate the primary shakeoff probabilities in systems with rather low atomic numbers. This calls for more elaborate calculations, including explicitly the electron-electron correlations., Comment: published in Phys. Rev. A (2018)

We report on a search for ultra-low-mass axion-like dark matter by analysing the ratio of the spin-precession frequencies of stored ultracold neutrons and $^{199}$Hg atoms for an axion-induced oscillating electric dipole moment of the neutron and an axion-wind spin-precession effect. No signal consistent with dark matter is observed for the axion mass range $10^{-24}~\textrm{eV} \le m_a \le 10^{-17}~\textrm{eV}$. Our null result sets the first laboratory constraints on the coupling of axion dark matter to gluons, which improve on astrophysical limits by up to 3 orders of magnitude, and also improves on previous laboratory constraints on the axion coupling to nucleons by up to a factor of 40.

This paper summarizes the results from measurements aiming to characterize ultracold neutron detection with 6Li-doped glass scintillators. Single GS10 or GS20 scintillators, with a thickness of 100-200 micrometer, fulfill the ultracold neutron detection requirements with an acceptable neutron-gamma discrimination. This discrimination is clearly improved with a stack of two scintillators: a 6Li-depleted glass bonded to a 6Li-enriched glass. The optical contact bonding is used between the scintillators in order to obtain a perfect optical contact. The scintillator's detection efficiency is similar to that of a 3He Strelkov gas detector. Coupled to a digital data acquisition system, counting rates up to a few 10^5 counts/s can be handled. A detector based on such a scintillator stack arrangement was built and has been used in the neutron electric dipole moment experiment at the Paul Scherrer Institute since 2010. Its response for the regular runs of the neutron electric dipole moment experiment is presented., Comment: 14 pages, 12 figures, regular article submitted for publication

This paper presents the design and implementation of the front-end electronics and the data acquisition (DAQ) system for readout of multi-wire drift chambers (MWDC). Apart of the conventional drift time measurement the system delivers the hit position along the wire utilizing the charge division technique. The system consists of preamplifiers, and analog and digital boards sending data to a back-end computer via an Ethernet interface. The data logging software formats the received data and enables an easy access to the data analysis software. The use of specially designed preamplifiers and peak detectors allows the charge-division readout of the low resistance signal wire. The implication of the charge-division circuitry onto the drift time measurement was studied and the overall performance of the electronic system was evaluated in dedicated off-line tests., Comment: 9 pages, 20 figures

We present for the first time a detailed and comprehensive analysis of the experimental results that set the current world sensitivity limit on the magnitude of the electric dipole moment (EDM) of the neutron. We have extended and enhanced our earlier analysis to include recent developments in the understanding of the effects of gravity in depolarizing ultracold neutrons (UCN); an improved calculation of the spectrum of the neutrons; and conservative estimates of other possible systematic errors, which are also shown to be consistent with more recent measurements undertaken with the apparatus. We obtain a net result of $d_\mathrm{n} = -0.21 \pm 1.82 \times10^{-26}$ $e$cm, which may be interpreted as a slightly revised upper limit on the magnitude of the EDM of $3.0 \times10^{-26}$ $e$cm (90% CL) or $ 3.6 \times10^{-26}$ $e$cm (95% CL). This paper is dedicated by the remaining authors to the memory of Prof. J. Michael Pendlebury., Comment: 23 pages, 19 figures. Authorship list changed to put J.M. Pendlebury first. Other very minor edits

The experimental achievements and the results obtained so far with the LPCTrap device installed at GANIL are presented. The apparatus is dedicated to the study of the weak interaction at low energy by means of precise measurements of the BETA-NU angular correlation parameter in nuclear BETA decays. So far, the data collected with three isotopes have enabled to determine, for the first time, the charge state distributions of the recoiling ions, induced by shakeoff process. The analysis is presently refined to deduce the correlation parameters, with the potential of improving both the constraint deduced at low energy on exotic tensor currents (6He1+) and the precision on the V u d element of the quark-mixing matrix (35Ar1+ and 19Ne1+) deduced from the mirror transitions dataset., Comment: 6th International Conference on Trapped Charged Particles and Fundamental Physics (TCP 2014), Takamatsu, Japan, December 2014, to be published in Hyperfine Interactions

We compare the expected effects of so-called gravitationally enhanced depolarization of ultracold neutrons to measurements carried out in a spin-precession chamber exposed to a variety of vertical magnetic-field gradients. In particular, we have investigated the dependence upon these field gradients of spin depolarization rates and also of shifts in the measured neutron Larmor precession frequency. We find excellent qualitative agreement, with gravitationally enhanced depolarization accounting for several previously unexplained features in the data., Comment: 10 pages, 6 figures. Updated: section added about implications for current nEDM limit

We describe a spin-echo method for ultracold neutrons (UCNs) confined in a precession chamber and exposed to a $|B_0|=1~\text{\mu T}$ magnetic field. We have demonstrated that the analysis of UCN spin-echo resonance signals in combination with knowledge of the ambient magnetic field provides an excellent method by which to reconstruct the energy spectrum of a confined ensemble of neutrons. The method takes advantage of the relative dephasing of spins arising from a gravitationally induced striation of stored UCN of different energies, and also permits an improved determination of the vertical magnetic-field gradient with an exceptional accuracy of $1.1~\text{pT/cm}$. This novel combination of a well-known nuclear resonance method and gravitationally induced vertical striation is unique in the realm of nuclear and particle physics and should prove to be invaluable for the assessment of systematic effects in precision experiments such as searches for an electric dipole moment of the neutron or the measurement of the neutron lifetime., Comment: 7 pages 5 figures, accepted by PRL, September, 08 2015

We report on the measurement of a Larmor frequency shift proportional to the electric-field strength for $^{199}{\rm Hg}$ atoms contained in a volume permeated with aligned magnetic and electric fields. This shift arises from the interplay between the inevitable magnetic field gradients and the motional magnetic field. The proportionality to electric-field strength makes it apparently similar to an electric dipole moment (EDM) signal, although unlike an EDM this effect is P- and T-conserving. We have used a neutron magnetic resonance EDM spectrometer, featuring a mercury co-magnetometer and an array of external cesium magnetometers, to measure the shift as a function of the applied magnetic field gradient. Our results are in good agreement with theoretical expectations.

We report on the design and first tests of a device allowing for measurement of ultracold neutrons polarisation by means of the simultaneous analysis of the two spin components. The device was developed in the framework of the neutron electric dipole moment experiment at the Paul Scherrer Institute. Individual parts and the entire newly built system have been characterised with ultracold neutrons. The gain in statistical sensitivity obtained with the simultaneous spin analyser is $(18.2\pm6.1)\%$ relative to the former sequential analyser under nominal running conditions.

We report a new limit on a possible short range spin-dependent interaction from the precise measurement of the ratio of Larmor precession frequencies of stored ultracold neutrons and $^{199}$Hg atoms confined in the same volume. The measurement was performed in a $\sim$1$\mu$ T vertical magnetic holding field with the apparatus searching for a permanent electric dipole moment of the neutron at the Paul Scherrer Institute. A possible coupling between freely precessing polarized neutron spins and unpolarized nucleons of the wall material can be investigated by searching for a tiny change of the precession frequencies of neutron and mercury spins. Such a frequency change can be interpreted as a consequence of a short range spin-dependent interaction that could possibly be mediated by axions or axion-like particles. The interaction strength is proportional to the CP violating product of scalar and pseudoscalar coupling constants $g_Sg_P$. Our result confirms limits from complementary experiments with spin-polarized nuclei in a model-independent way. Limits from other neutron experiments are improved by up to two orders of magnitude in the interaction range of $10^{-6}<\lambda<10^{-4}$ m.

The neutron gyromagnetic ratio has been measured relative to that of the 199Hg atom with an uncertainty of 0.8 ppm. We employed an apparatus where ultracold neutrons and mercury atoms are stored in the same volume and report the result $\gamma_{\rm n}/\gamma_{\rm Hg} = 3.8424574(30)$.

Precision measurements at low energy search for physics beyond the Standard Model in a way complementary to searches for new particles at colliders. In the weak sector the most general $\beta$ decay Hamiltonian contains, besides vector and axial-vector terms, also scalar, tensor and pseudoscalar terms. Current limits on the scalar and tensor coupling constants from neutron and nuclear $\beta$ decay are on the level of several percent. The goal of this paper is extracting new information on tensor coupling constants by measuring the $\beta$-asymmetry parameter in the pure Gamow-Teller decay of $^{67}$Cu, thereby testing the V-A structure of the weak interaction. An iron sample foil into which the radioactive nuclei were implanted was cooled down to milliKelvin temperatures in a $^3$He-$^4$He dilution refrigerator. An external magnetic field of 0.1 T, in combination with the internal hyperfine magnetic field, oriented the nuclei. The anisotropic $\beta$ radiation was observed with planar high purity germanium detectors operating at a temperature of about 10\,K. An on-line measurement of the $\beta$ asymmetry of $^{68}$Cu was performed as well for normalization purposes. Systematic effects were investigated using Geant4 simulations. The experimental value, $\tilde{A}$ = 0.587(14), is in agreement with the Standard Model value of 0.5991(2) and is interpreted in terms of physics beyond the Standard Model. The limits obtained on possible tensor type charged currents in the weak interaction hamiltonian are -0.045 $< (C_T+C'_T)/C_A <$ 0.159 (90\% C.L.). The obtained limits are comparable to limits from other correlation measurements in nuclear $\beta$ decay and contribute to further constraining tensor coupling constants.

The Surrounding Field Compensation (SFC) system described in this work is installed around the four-layer Mu-metal magnetic shield of the neutron electric dipole moment spectrometer located at the Paul Scherrer Institute. The SFC system reduces the DC component of the external magnetic field by a factor of about 20. Within a control volume of approximately 2.5m x 2.5m x 3m disturbances of the magnetic field are attenuated by factors of 5 to 50 at a bandwidth from $10^{-3}$ Hz up to 0.5 Hz, which corresponds to integration times longer than several hundreds of seconds and represent the important timescale for the nEDM measurement. These shielding factors apply to random environmental noise from arbitrary sources. This is achieved via a proportional-integral feedback stabilization system that includes a regularized pseudoinverse matrix of proportionality factors which correlates magnetic field changes at all sensor positions to current changes in the SFC coils., Comment: 33 pages, 18 figures

The electron shakeoff of $^{35}$Cl atoms resulting from the $\beta$$^+$ decay of $^{35}$Ar$^+$ ions has been investigated using a Paul trap coupled to a recoil-ion spectrometer. The charge-state distribution of the recoiling daughter nuclei is compared to theoretical calculations accounting for shakeoff and Auger processes. The calculations are in excellent agreement with the experimental results and enable to identify the ionization reaction routes leading to the formation of all charge states., Comment: Physical Review A In press (2013)