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We report on laser spectroscopic measurements on Li$^+$ ions in the experimental storage ring ESR at the GSI Helmholtz Centre for Heavy Ion Research. Driving the $2s\,^3\!{S}_1\;(F=\frac{3}{2}) \,\leftrightarrow\,2p\,^3\!P_2\;(F=\frac{5}{2}) \leftrightarrow 2s\,^3\!{S}_1\;(F=\frac{5}{2})$ $\Lambda$-transition in $^7$Li$^+$ with two superimposed laser beams it was found that the use of circularly polarized light leads to a disappearance of the resonance structure in the fluorescence signal. This can be explained by optical pumping into a dark state of polarized ions. We present a detailed theoretical analysis of this process that supports the interpretation of optical pumping and demonstrates that the polarization induced by the laser light must then be at least partially maintained during the round trip of the ions in the storage ring. Such polarized ion beams in storage rings will provide opportunities for new experiments, especially on parity violation., Comment: 14 pages, 8 figures, new version with small adjustments, closest to final publication in PRAB

We report on the first preliminary result of our 129Xe EDM measurement performed by the MIXed collaboration. The aim of this report is to demonstrate the feasibility of a new method to set limits on nuclear EDMs by investigating the EDM of the diamagnetic 129Xe atoms. In our setup, hyperpolarized 3He serves as a comagnetometer needed to suppress magnetic field fluctuations. The free induction decay of the two polarized spin species is directly measured by low noise DC SQUIDs, and the weighted phase difference extracted from these measurements is used to determine a preliminary upper limit on the 129Xe EDM.

The spin-lattice relaxation time T1 of hyperpolarized (HP)-(129)Xe was improved at typical storage conditions (i.e. low and homogeneous magnetic fields). Very long wall relaxation times T(1)(wall) of about 18 h were observed in uncoated, spherical GE180 glass cells of ∅=10 cm which were free of rubidium and not permanently sealed but attached to a standard glass stopcock. An "aging" process of the wall relaxation was identified by repeating measurements on the same cell. This effect could be easily removed by repeating the initial cleaning procedure. In this way, a constant wall relaxation was ensured. The Xe nuclear spin-relaxation rate 1/T1(Xe-Xe) due to van der Waals molecules was investigated too, by admixing three different buffer gases (N(2), SF(6) and CO(2)). Especially CO(2) exhibited an unexpected high efficiency (r) in shortening the lifetime of the Xe-Xe dimers and hence prolonging the total T1 relaxation even further. These measurements also yielded an improved accuracy for the van der Waals relaxation for pure Xe (with 85% (129)Xe) of T(1)(Xe-Xe)=(4.6±0.1)h. Repeating the measurements with HP (129)Xe in natural abundance in mixtures with SF6, a strong dependence of T(1)(Xe-Xe) and r on the isotopic enrichment was observed, uncovering a shorter T(1)(Xe-Xe) relaxation for the (129)Xe in natural composition as compared to the 85% isotopically enriched gas.

PURPOSE: To protect the patient with acute respiratory distress syndrome from ventilator associated lung injury (VALI) high-frequency oscillatory ventilation (HFOV) is used. Clinical experience has proven that HFOV is an efficient therapy when conventional artificial ventilation is insufficient. However, the optimal settings of HFOV parameters, eg, tidal volumes, pressure amplitudes and frequency for maximal lung protection, and efficient gas exchange are not established unambiguously. METHODS: In this work magnetic resonance imaging (MRI) with hyperpolarized (3)He was employed to visualize the redistribution of gas within the cadaver pig lung during HFOV. The saturated slice method was used to characterize fast gas kinetics. RESULTS: The strong differences in kinetics were observed for HFOV-driven gas exchange in comparison with diffusive gas transport (apnea). The significant regional and HFOV frequency dependence was detected for washout and gas exchange within the lungs. Gas redistribution was much faster in posterior than in anterior parts of the lungs during HFOV, in contrast to minor differences with an opposite trend observed in apnea. CONCLUSION: The method shows significant potential for visualization and quantification of gas redistribution under HFOV and may help in optimization of the parameters to improve the clinical effect of HFOV for patients.

We present novel types of permanently magnetized as well as current powered boxes built from soft-ferromagnetic materials. They provide shielded magnetic fields which are homogeneous within a large fraction of the enclosed volume, thus minimizing size, weight, and costs. For the permanently magnetized solutions, homogenization is achieved either by an optimized distribution of the permanent field sources or by jacketing the field with a soft-ferromagnetic cylindrical shell which is magnetized in parallel to the enclosed field. The latter principle may be applied up to fields of about 0.1 T. With fields of about 1 mT, such boxes are being used for shipping spin-polarized 3 He worldwide for MRI purposes. For current powered boxes, we present concepts and realizations of uniaxial and tri-axial shielded magnetic fields which are homogeneous on the level of 10 −4 within the entire shielded volume. This is achieved by inserting tightly fitting solenoids into a box from soft-magnetic material. The flexible tri-axial solution suits in particular laboratory applications, e.g. for establishing a spin quantization axis.

Time dilation is one of the most fascinating aspects of special relativity as it abolishes the notion of absolute time. It was first observed experimentally by Ives and Stilwell in 1938 using the Doppler effect. Here we report on a method, based on fast optical atomic clocks with large, but different Lorentz boosts, that tests relativistic time dilation with unprecedented precision. The approach combines ion storage and cooling with optical frequency counting using a frequency comb. 7Li+ ions are prepared at 6.4% and 3.0% of the speed of light in a storage ring, and their time is read with an accuracy of 2×10−10 using laser saturation spectroscopy. The comparison of the Doppler shifts yields a time dilation measurement represented by a Mansouri–Sexl parameter , consistent with special relativity. This constrains the existence of a preferred cosmological reference frame and CPT- and Lorentz-violating ‘new’ physics beyond the standard model.

We report frequency measurements at the rovibronic transition P(42)1-14 (772 nm) and R(114)2-11 (735 nm) from the electronic X 1 Σ g + → B 3 Π 0 u + transition of the iodine molecule 127I2 with the help of a frequency comb as a reference. By using Doppler-free saturation spectroscopy a frequency precision in the 7 × 10−10 region is reached and two iodine cells both operated at 550–600 °C are compared. To relate our results to other measurements, the absolute transition frequency of the hyperfine structure line P(148)1-14 a1 at 780 nm with an already known transition frequency was also determined.

The Doppler-free laser-spectroscopic frequency measurement of Doppler-shifted optical lines in forward and backward direction of a fast ion beam permits a sensitive test of the relativistic Doppler-formula and, hence, the relativistic time dilation factor γ SR=(1−ν 2/c 2)−1/2. An experiment on metastable 7Li+, stored at a velocity of ν=0.064c in the Heidelberg heavy-ion storage ring TSR, has confirmed time dilation with unprecedented accuracy. Latest tests at two different ion-velocities (ν=0.03c and ν=0.064c) will enhance these measurements. An improved version of this experiment will be carried out at the experimental storage ring (ESR) at the Gesellschaft fur Schwerionenforschung (GSI) in Darmstadt. The ESR permits 7Li+ to be stored at ν=0.33c which promises an improvement of the sensitivity to deviations from γ SRby an order of magnitude. A first test at the ESR has shown the feasibility for this kind of experiment.

The hyperfine structure splittings of the P(10)14-1, R(15)14-1, and R(99)15-1 transitions at 585 nm, P(62)17-1 at 576 nm, and P(80)21-1 at 565 nm in 127 I 2 are measured by heterodyne spectroscopy using two dye lasers. In addition, the absolute frequencies of the hyperfine components P(10)14-1 a 15 and P(80)21-1 a 10 are determined using a self-referenced frequency comb. These frequencies are used in an experiment testing relativistic time dilation by laser spectroscopy on a fast ion beam.

We report on the first laser cooling of a bunched beam of multiply charged C3+ ions performed at the ESR (GSI) at a beam energy of E = 1.47 GeV. Moderate bunching provided a force counteracting the decelerating laser force of one counterpropagating laser beam. This versatile type of laser cooling lead to longitudinally space-charge dominated beams with an unprecedented momentum spread of Δp/p ≈ 10−7. Concerning the beam energy and charge state of the ion, the experiment depicts an important intermediate step from the established field of laser cooling of ion beams at low energies toward the unique laser cooling scheme proposed for relativistic beams of highly charged heavy ions at SIS 300 (FAIR).

Spectroscopic and analytical properties of a trace analytical method using multi-step resonance ionization at high laser intensities (>kW/cm 2 ) have been investigated with gadolinium as a test element. Strongly saturated transitions are observed, which have been used for a temperature determination of the atoms in the laser ablated plume. Regimes of multi-step resonance ionization and multiphoton ionization could be distinguished. Analytical performances due to resonance enhancement and resulting discrimination against non-resonant background, precision in isotope ratio determination and overall detection efficiency are discussed.

We report morphologic changes of metallic surfaces at the onset of ablation, starting from gentle ablation to the emergence of ablation craters. The evolution of both observed melting zones and of ablation craters therein are investigated in dependence of the ablation laser fluence for nanosecond ultraviolet laser pulses. Further, consequences of crater formation for cluster synthesis within the released atomic vapor are pointed out.

The laser-spectroscopic frequency measurement of Doppler-shifted optical lines in the forward and backward directions of a fast ion beam permits a sensitive test of the relativistic Doppler formula and, hence, the relativistic time-dilation factor γSR = 1/[Formula: see text]. An experiment on 7Li+, stored at a velocity of v = 0.065c in the Heidelberg heavy-ion storage ring TSR, has confirmed time dilation with unprecedented accuracy limiting deviations to below 2.2 × 10–7. Ongoing improvements on the experimental setup will further tighten this limit.PACS Nos.: 03.30.+p, 06.30.Ft, and 42.62.Fi

A novel method for direct and spatially resolved elemental trace analysis with high sensitivity and elemental selectivity is presented. The concept is based on the combination of a commercial MALDI-TOF mass spectrometer with a pulsed laser system for resonant postionisation of neutrals. While the MALDI method is usually applied for investigations of large organic compounds and biomolecules, the technique discussed here concerns the low mass range around 1 ⩽ A ⩽ 300. The analytical performances of the setup with respect to mass analysis, spatial resolution and overall detection efficiency are discussed.

The frequency measurement of Doppler-shifted optical lines of ions circulating in a storage ring at high speed permits a sensitive test of the relativistic Doppler-formula and, hence, the time dilation factor γSR of special relativity. Previous measurements at the storage ring TSR with 7Li+ at v = 0.065c gave a new, improved limit, but were hampered by the large observed linewidth, exceeding the natural width 15-fold. Recently we have identified the broadening to be caused by velocity-changing processes in the storage ring. Saturation spectroscopy has proven to be largely immune against these effects and has yielded linewidths only a few MHz larger than the natural one. This is the major ingredient for an improved test of γSR, which is now under way.

We present the concluding result from an Ives-Stilwell-type time dilation experiment using 7Li+ ions confined at a velocity of β=v/c=0.338 in the storage ring ESR at Darmstadt. A Λ-type three-level system within the hyperfine structure of the 7Li+3S1 →3P2 line is driven by two laser beams aligned parallel and antiparallel relative to the ion beam. The lasers' Doppler shifted frequencies required for resonance are measured with an accuracy of

We give a brief overview of time dilation tests using high-resolution laser spectroscopy at heavy-ion storage rings. We reflect on the various methods used to eliminate the first-order Doppler effect and on the pitfalls encountered, and comment on possible extensions at future facilities providing relativistic heavy ion beams at $\gamma \gg 1$.

We describe a 3He magnetometer capable to measure high magnetic fields (B > 0.1 Tesla) with a relative accuracy of better than 10^-12. Our approach is based on the measurement of the free induction decay of gaseous, nuclear spin polarized 3He following a resonant radio frequency pulse excitation. The measurement sensitivity can be attributed to the long coherent spin precession time T2* being of order minutes which is achieved for spherical sample cells in the regime of motional narrowing where the disturbing influence of field inhomogeneities is strongly suppressed. The 3He gas is spin polarized in-situ using a new, non-standard variant of the metastability exchange optical pumping. We show that miniaturization helps to increase T2* further and that the measurement sensitivity is not significantly affected by temporal field fluctuations of order 10^-4., 27 pages, 7 figures

The schemes of light beam transformations by volume dynamic holograms in resonant media revealing the fifth- or higher-order nonlinearities have been theoretically analyzed. N-wave mixing has been realized by changing of the propagation direction or frequency of the read-out wave in the solution of Rhodamine 6G and polymethine 3274U dyes. It has been demonstrated that the experimental results are in good agreement with the theoretical data obtained for a three-level medium model with due regard to absorption from the excited singlet level.

A preparation scheme for a 7Li+ ion beam in a storage ring is presented which provides ions in the metastable triplet states with well controlled longitudinal phase space properties. For both state selective preparation and beam cooling, laser- and electron-cooler forces are applied. The spatial- and momentum distributions of the ions are directly detected by a time resolved measurement of the fluorescence light. At low beam intensities, the remaining heating rate of such a beam is completely determined by residual gas scattering.

We performed an experiment to search for a new spin-dependent P- and T-violating nucleon–nucleon interaction [Formula: see text] which is mediated by light pseudoscalar bosons such as axions or axionlike particles. This interaction causes a shift [Formula: see text] in the precession frequency of nuclear spin polarized gases in the presence of an unpolarized mass. In order to measure this frequency shift a 3He/[Formula: see text]Xe comagnetometer was used which is based on the detection of free precession of 3He and [Formula: see text]Xe nuclear spins using SQUIDs as detectors. For the upper limit of [Formula: see text] we obtained 7.1[Formula: see text]nHz. With this value, an upper limit of the scalar-pseudoscalar coupling of the axion to the spin of a bound neutron could be deduced within the axion mass window. For axion masses between 2 and 500[Formula: see text][Formula: see text]eV, the laboratory upper bounds were improved by up to 4 orders of magnitude.

We demonstrate sub-Doppler laser spectroscopy with a beam of ${^{7}\text{L}\text{i}}^{+}$ ions stored at 33.8% of the speed of light in the experimental storage ring at GSI. Using two lasers, the one copropagating and the other counterpropagating, with respect to the ion beam, a fluorescence line is observed via optical-optical double-resonance spectroscopy on a $\ensuremath{\Lambda}$-type level configuration. A linewidth of $\ensuremath{\approx}114\text{ }\text{MHz}$ is found, which is 12 times narrower than the Doppler broadening due to the momentum spread of the ion beam. Interpreted as a test of Lorentz invariance, we find $|{\stackrel{\ifmmode \hat{}\else \^{}\fi{}}{\ensuremath{\alpha}}}_{2}|l1.2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}5}$, a $25\ifmmode\times\else\texttimes\fi{}$ tighter limit on $O\mathbf{(}{(v/c)}^{4}\mathbf{)}$ deviations from time dilation than any other experiment.

A scheme for the formation and reconstruction, at the doubled frequency, of volume dynamic holograms is considered in the case of the fifth-order nonlinearity. The results are given of an experimental investigation of the diffraction of laser radiation by a transmission dynamic grating formed in a solution of polymethine dye No.3274U. A theoretical model is proposed for describing quadratic hologram formation and suitable for calculation of the energy efficiency of conversion of the radiation frequency.

We report on a type of surface structuring after short pulse laser ablation of a binary alloy. We observe the emergence of a concentric ring structure with changing elemental composition. The composition changes are interpreted by condensation of the ambient ablation vapor due to stress wave excitations in the ablation spot.

A precise, laser-spectroscopic test of time dilation in special relativity has been performed with fast ions stored in the heavy-ion storage ring TSR in Heidelberg. At a velocity of 6.4% of the speed of light, the Doppler-shifted frequencies of a transition in 7Li+ have been measured in forward and backward direction. First results confirm relativity and set an improved limit of 2.2 x for deviations from the Lorentz factor 7 s ~ = 1/J1 v2/c2. Ongoing improvements will tighten the limit further. Preliminary investigations indicate that Doppler-type experiments can have unique sensitivity for testing Lorentz/CPT-violating extensions of the Standard Model.

We have investigated the velocity distributions of atoms released from a metallic gadolinium surface by UV laser ablation. The fluences of the nanosecond laser pulses were chosen for a pure release of neutrals and at a higher fluence level for the release of both neutrals and ions. In both cases a thermal Maxwell-Boltzmann slope has been observed for the low velocities, whereas for high velocities strong deviations from a thermal distribution have been seen. The observed velocity distribution has been explained by a bimodal structure including a thermal phase and a shockwave driven ``blow-off'' phase.

An improved test of time dilation in special relativity has been performed using laser spectroscopy on fast ions at the heavy-ion storage-ring TSR in Heidelberg. The Doppler-shifted frequencies of a two-level transition in 7 Li + ions at v = 0.064c have been measured in the forward and backward direction to an accuracy of Δν/ν = 1 × 10 - 9 using collinear saturation spectroscopy. The result confirms the relativistic Doppler formula and sets a new limit of 2.2 × 10 - 7 for deviations from the time dilation factor γ S R = (1 - ν 2 /c 2 ) - 1 / 2 .

The possibility of phase conjugation with simultaneous doubling of the light-wave phase and frequency upon nondegenerate four-wave mixing has been suggested and substantiated theoretically. The dependence of the energy efficiency of double-phase conjugation on the spectroscopic characteristics of the multilevel resonant media has been analyzed.© (1996) COPYRIGHT SPIE--The International Society for Optical Engineering. Downloading of the abstract is permitted for personal use only.

In this paper we present concepts, developed to construct a compact 3He polarizing facility as well as first results of their realization. The apparatus, which is currently in the state of construction, is based on the method of metastability exchange optical pumping (MEOP). Contrary to the present apparatus at the university of Mainz, which serves as central polarizing facility, the compact polarizer is designed to serve as local polarizing facility in both basic research and medical application. With the new polarizer we aim to reach polarization degrees of P > 65% at a flux of several standard liters per hour.

We discuss the axial dynamics of laser-cooled relativistic C3+ ion beams at moderate bunching voltages. Schottky noise spectra measured at a beam energy of 122 MeV/u are compared to simulations of the axial beam dynamics. Ions confined in the bucket are addressed by the narrow-band force of a laser beam counter-propagating to the ion beam, while the laser frequency is detuned relatively to the cooling transition frequency in the rest frame of the bucket. At large detuning comparable to the momentum acceptance of the bucket, the axial dynamics can be well explained by the secular motion of individual non-interacting ions. At small detuning, corresponding to a small axial momentum spread Δpaxial/paxial < 10−6 of the ions, the measured Schottky noise spectra can no longer be explained using an approach which neglects the ion-ion interaction. Instead, the model fails when the ion bunch enters the space-charge dominatedregime, at which the mutual Coulomb-energy of the ions becomes comparable to the kinetic energy of the ions.