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3 results on '"Secrist, Carlee"'

1. Homogeneous versus MOF-supported catalysis: a direct comparison of catalytic hydroboration with Ni tripodal P3E (E = Si, Ge) complexes

Author

Barrios-Vargas, Luz J., primary, Abeynayake, Niroshani S., additional, Secrist, Carlee, additional, Le, Nghia, additional, Webster, Charles Edwin, additional, Donnadieu, Bruno, additional, Kaphan, David M., additional, Roy, Amitava D., additional, Ibarra, Ilich A., additional, and Montiel-Palma, Virginia, additional

Published
2023
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2. Homogeneous versus MOF-supported catalysis: a direct comparison of catalytic hydroboration with Ni tripodal P3E (E = Si, Ge) complexes.

Author

Barrios-Vargas, Luz J., Abeynayake, Niroshani S., Secrist, Carlee, Le, Nghia, Webster, Charles Edwin, Donnadieu, Bruno, Kaphan, David M., Roy, Amitava D., Ibarra, Ilich A., and Montiel-Palma, Virginia

Subjects
HYDROBORATION, NICKEL catalysts, CATALYSIS, INHOMOGENEOUS materials, WASTE recycling, HETEROGENEOUS catalysts, KETONES
Abstract

The MOF material NU-1000 was employed to host Ni tripodal complexes prepared from new organometallic precursors [HNi(κ4(E,P,P,P)-E(o-C6H4CH2PPh2)3], E = Si (Ni-1), Ge (Ni-2). The new heterogeneous catalytic materials, Ni-1@NU-1000 and Ni-2@NU-1000, show the advantages of both homogeneous and heterogeneous catalysts. They catalyze the hydroboration of aldehydes and ketones more efficiently than the homogeneous Ni-1 and Ni-2, under aerobic conditions and show recyclability. [ABSTRACT FROM AUTHOR]

Published
2023
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3. Homogeneous versus MOF-supported catalysis: a direct comparison of catalytic hydroboration with Ni tripodal P 3 E (E = Si, Ge) complexes.

Author

Barrios-Vargas LJ, Abeynayake NS, Secrist C, Le N, Webster CE, Donnadieu B, Kaphan DM, Roy AD, Ibarra IA, and Montiel-Palma V

Abstract

The MOF material NU-1000 was employed to host Ni tripodal complexes prepared from new organometallic precursors [HNi( κ 4 ( E , P , P , P )-E( o -C 6 H 4 CH 2 PPh 2 ) 3 ], E = Si (Ni-1), Ge (Ni-2). The new heterogeneous catalytic materials, Ni-1@NU-1000 and Ni-2@NU-1000, show the advantages of both homogeneous and heterogeneous catalysts. They catalyze the hydroboration of aldehydes and ketones more efficiently than the homogeneous Ni-1 and Ni-2, under aerobic conditions and show recyclability.

Published
2023
Full Text
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