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We propose and numerically investigate a novel compact planar microcavity design based on a high-index dielectric slab waveguide with embedded monolayer semiconductor. In comparison to more traditional vertical Bragg microcavities, our design relies on the transmission of guided optical modes and achieves strong exciton-photon coupling in a chip-compatible and compact geometry with sub-100 nm thickness. We show that Rabi splitting values of more than 70 meV can be obtained in planar microcavities with the total length below 5 um. Further, we reveal the dependence of Rabi splitting on the dimensions of the structure and explain it with a simple theoretical model. Our results contribute towards the development of novel compact 2D semiconductor-based components for integrated photonic circuits.

Deeply subwavelength lasers (or nanolasers) are highly demanded for compact on-chip bioimaging and sensing at the nanoscale. One of the main obstacles for the development of single-particle nanolasers with all three dimensions shorter than the emitting wavelength in the visible range is the high lasing thresholds and the resulting overheating. Here we exploit exciton-polariton condensation and mirror-image Mie modes in a cuboid CsPbBr$_3$ nanoparticle to achieve coherent emission at the visible wavelength of around 0.53~$\mu $m from its ultra-small ($\approx$0.007$\mu$m$^3$ or $\approx\lambda^3$/20) semiconductor nanocavity. The polaritonic nature of the emission from the nanocavity localized in all three dimensions is proven by direct comparison with corresponding one-dimensional and two-dimensional waveguiding systems with similar material parameters. Such a deeply subwavelength nanolaser is enabled not only by the high values for exciton binding energy ($\approx$35 meV), refractive index ($>$2.5 at low temperature), and luminescence quantum yield of CsPbBr$_3$, but also by the optimization of polaritons condensation on the Mie resonances. Moreover, the key parameters for optimal lasing conditions are intermode free spectral range and phonons spectrum in CsPbBr$_3$, which govern polaritons condensation path. Such chemically synthesized colloidal CsPbBr$_3$ nanolasers can be easily deposited on arbitrary surfaces, which makes them a versatile tool for integration with various on-chip systems., Comment: 29 pages, 19 Figures

Guided 2D exciton-polaritons, resulting from the strong coupling of excitons in semiconductors with non-radiating waveguide modes, provide an attractive approach towards developing novel on-chip optical devices. These quasiparticles are characterized by long propagation distances and efficient nonlinear interaction but cannot be directly accessed from the free space. Here we demonstrate a powerful approach for probing and manipulating guided polaritons in a Ta2O5 slab integrated with a WS2 monolayer using evanescent coupling through a high-index solid immersion lens. Tuning the nanoscale lens-sample gap allows for extracting all the intrinsic parameters of the system. We also demonstrate the transition from weak to strong coupling accompanied by the onset of the motional narrowing effect: with the increase of exciton-photon coupling strength, the inhomogeneous contribution to polariton linewidth, inherited from the exciton resonance, becomes fully lifted. Our results enable the development of integrated optics employing room-temperature exciton-polaritons in 2D semiconductor-based structures.

Excitons in lead bromide perovskites exhibit high binding energy and high oscillator strength, allowing for a strong light-matter coupling regime in the perovskite-based cavities localizing photons at the nanoscale. This opens up the way for the realization of exciton-polariton Bose-Einstein condensation and polariton lasing at room temperature -- the inversion-free low-threshold stimulated emission. However, polariton lasing in perovskite planar photon cavities without Bragg mirrors has not yet been observed and proved experimentally. In this work, we employ perovskite metasurface, fabricated with nanoimprint lithography, supporting so-called exceptional points to demonstrate the room-temperature polariton lasing. The exceptional points in exciton-polariton dispersion of the metasurface appear upon optically pumping in the nonlinear regime in the spectral vicinity of a symmetry-protected bound state in the continuum providing high mode confinement with the enhanced local density of states beneficial for polariton condensation. The observed lasing emission possesses high directivity with a divergence angle of around 1$^\circ$ over one axis. The employed nanoimprinting approach for solution-processable large-scale polariton lasers is compatible with various planar photonic platforms suitable for on-chip integration., Comment: 12 pages, 3 figures

Systems supporting exciton-polaritons represent solid-state optical platforms with a strong built-in optical nonlinearity provided by exciton-exciton interactions. In conventional semiconductors with hydrogen-like excitons the nonlinearity rate demonstrates the inverse scaling with the binding energy. This makes excitons stable at room temperatures weakly interacting, which obviously limits the possibilities of practical applications of the corresponding materials for nonlinear photonics. We demonstrate experimentally and theoretically, that these limitations can be substantially softened in hybrid perovskites, such as MAPbBr3 due to the crucial role of the polaron effects mediating the inter-particle interactions. The resulting exciton-polaron-polaritons remain both stable and strongly interacting at room temperature, which is confirmed by large nonlinear blueshifts of lower polariton branch energy under resonant femtosecond laser pulse excitation. Our findings open novel perspectives for the management of the exciton-polariton nonlinearities in ambient conditions.

Exciton-polaritons offer a versatile platform for realization of all-optical integrated logic gates due to the strong effective optical nonlinearity resulting from the exciton-exciton interactions. In most of the current excitonic materials there exists a direct connection between the exciton robustness to thermal fluctuations and the strength of exciton-exciton interaction, making materials with highest levels of exciton nonlinearity applicable at cryogenic temperatures only. Here, we show that strong polaronic effects, characteristic for perovskite materials, allow to overcome this limitation. Namely, we demonstrate the record-high value of the nonlinear optical response in nanostructured organic-inorganic halide perovskite MAPbI$_3$, experimentally detected as 19.7 meV blueshift of the polariton branch under femtosecond laser irradiation. This is substantially higher than characteristic values for the samples based on conventional semiconductors and monolayers of transition metal dichalcogenides. The observed strong polaron-enhanced nonlinearity exists for both tetragonal and orthorombic phases of MAPbI$_3$, and remains stable at elevated temperatures.

Optical bound states in the continuum (BICs) provide a way to engineer very narrow resonances in photonic crystals. The extended interaction time in such systems is particularly promising for enhancement of nonlinear optical processes and development of the next generation of active optical devices. However, the achievable interaction strength is limited by the purely photonic character of optical BICs. Here, we mix optical BIC in a photonic crystal slab with excitons in atomically thin semiconductor MoSe$_2$ to form nonlinear exciton-polaritons with a Rabi splitting of 27~meV, exhibiting large interaction-induced spectral blueshifts. The asymptotic BIC-like suppression of polariton radiation into far-field towards the BIC wavevector, in combination with effective reduction of excitonic disorder through motional narrowing, results in small polariton linewidths below 3~meV. Together with strongly wavevector-dependent Q-factor, this provides for enhancement and control of polariton--polariton interactions and resulting nonlinear optical effects, paving the way towards tunable BIC-based polaritonic devices for sensing, lasing, and nonlinear optics.

Metasurfaces offer great potential to control near- and far-fields through engineering of optical properties of elementary cells or meta-atoms. Such perspective opens a route to efficient manipulation of the optical signals both at nanoscale and in photonics applications. In this paper we show that by using an effective surface conductivity tensor it is possible to unambigiously describe optical properties of an anisotropic metasurface in the far- and near-field regimes. We begin with retrieving the effective surface conductivity tensor from the comparative analysis of experimental and numerical reflectance spectra of a metasurface composed of elliptical gold nanoparticles. Afterwards restored conductivities are validated in the crosscheck versus semianalytic parameters obtained with the discrete dipole model with and without dipoles interaction contribution. The obtained effective parameters are further used for the dispersion analysis of surface plasmons localized at the metasurface. The effective medium model predicts existence of both TE- and TM-polarized plasmons in a wide range of optical frequencies and describes peculiarities of their dispersion, in particularly, topological transition from the elliptical to hyperbolic regime with eligible accuracy. The analysis in question offers a simple practical way to describe properties of metasurfaces including ones in the near-field zone by extracting effective parameters from the convenient far-field characterisation., Comment: 29 pages, 9 figures

Nanoantennas for highly efficient excitation and manipulation of surface waves at nanoscale are key elements of compact photonic circuits. However, previously implemented designs employ plasmonic nanoantennas with high Ohmic losses, relatively low spectral resolution, and complicated lithographically made architectures. Here we propose an ultracompact and simple dielectric nanoantenna (silicon nanosphere) allowing for both directional launching of surface plasmon polaritons on a thin gold film and their demultiplexing with a high spectral resolution. We show experimentally that mutual interference of magnetic and electric dipole moments supported by the dielectric nanoantenna results in opposite propagation of the excited surface waves whose wavelengths differ by less than 50 nm in the optical range. Broadband reconfigurability of the nanoantennas operational range is achieved simply by varying the diameter of the silicon sphere. Moreover, despite subwavelength size ($<\lambda/3$) of the proposed nanoantennas, they demonstrate highly efficient and directional launching of surface waves both in the forward and backward directions with the measured front-to-back ratio having a contrast of almost two orders of magnitude within a 50 nm spectral band. Our lithography-free design has great potential as highly efficient, low-cost, and ultracompact demultiplexer for advanced photonic circuits., Comment: added relevant references; fixed typos in Supplementary eq. 8,9,11

Photonic structures offer unique opportunities for controlling light-matter interaction, including the photonic spin Hall effect associated with the transverse spin-dependent displacement of light that propagates in specially designed optical media. However, due to small spin-orbit coupling, the photonic spin Hall effect is usually weak at the nanoscale. Here we suggest theoretically and demonstrate experimentally, in both optics and microwave experiments, the photonic spin Hall effect enhanced by topologically protected edge states in subwavelength arrays of resonant dielectric particles. Based on direct near-field measurements, we observe the selective excitation of the topological edge states controlled by the handedness of the incident light. Additionally, we reveal the main requirements to the symmetry of photonic structures to achieve a topology-enhanced spin Hall effect, and also analyse the robustness of the photonic edge states against the long-ranged coupling.

Enhancement of optical response with high-index dielectric nanoparticles is attributed to the excitation of their Mie-type magnetic and electric resonances. Here we study Raman scattering from crystalline silicon nanoparticles and reveal that magnetic dipole modes have much stronger effect on the scattering than electric modes of the same order. We demonstrate experimentally a 140-fold enhancement of Raman signal from individual silicon spherical nanoparticles at the magnetic dipole resonance. Our results confirm the importance of the optically-induced magnetic response of subwavelength dielectric nanoparticles for enhancing light-matter interactions.

Whispering gallery mode microdisk cavities fabricated by direct laser writing are studied using dark-field imaging and spectroscopy in the visible spectral range. {Dark-field imaging allows us to directly visualize the spatial intensity distribution of whispering gallery modes. We extract their azimuthal and radial mode indices from dark-field images, and find the axial mode number from the dispersion relation. The scattering spectrum obtained in the confocal arrangement provides information on the density of optical states in the resonator. The proposed technique is a simple non-invasive way to characterize the optical properties of microdisk cavities., Comment: 5 pages, 4 figures

The concept of high refractive index subwavelength dielectric nanoresonators, supporting electric and magnetic optical resonances, is a promising platform for waveguiding, sensing, and nonlinear nanophotonic devices. However, high concentration of defects in the nanoresonators diminishes their resonant properties, which are crucially dependent on their internal losses. Therefore, it seems to be inevitable to use initially crystalline materials for fabrication of the nanoresonators. Here, we show that the fabrication of crystalline (low-loss) resonant silicon nanoparticles by femtosecond laser ablation of amorphous (high-loss) silicon thin films is possible. We apply two conceptually different approaches: recently proposed laser-induced transfer and a novel laser writing technique for large-scale fabrication of the crystalline nanoparticles. The crystallinity of the fabricated nanoparticles is proven by Raman spectroscopy and electron transmission microscopy, whereas optical resonant properties of the nanoparticles are studied using dark-field optical spectroscopy and full-wave electromagnetic simulations., Comment: Published in Nanoscale