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Quantum sensors based on Nitrogen Vacancy (NV) centers in diamond are highly capable of sensing multiple physical quantities. In this study, we use amplitude-modulated lock-in detection of optically detected magnetic resonance of NV nanodiamonds (NVND) to investigate the link between temperature (T) and the zero-field splitting parameter (D) and also the relationship between magnetic field values and the difference of resonance frequencies. We also present NVNDs' capacity to simultaneously sense both thermal and magnetic fields in real time. This dual-sensing approach is beneficial for studying magnetic materials whose magnetization depends on temperature and the applied magnetic field, such as certain ferromagnetic and ferrimagnetic materials. Integrating real-time thermal and magnetic field measurements provides unique opportunities for failure analysis in the integrated circuit (IC) industry and for studying thermodynamic processes in cell physiology. The ability to concurrently monitor temperature and magnetic field variations offers a powerful toolset for advancing precision diagnostics and monitoring in these fields.

With the second quantum revolution underway, quantum-enhanced sensors are moving from laboratory demonstrations to field deployments, providing enhanced and even new capabilities. Signal processing and operational software is becoming integral parts of these emerging sensing systems to reap the benefits of this progress. This paper looks into widefield Nitrogen Vacancy Center-based magnetometry and focuses on estimating the magnetic field from the Optically Detected Magnetic Resonances (ODMR) signal, a crucial output for various applications. Mapping the shifts of ODMR signals to phase estimation, a computationally efficient approaches are proposed. Involving Fourier Transform and Filtering as pre-processing steps, the suggested approaches involve linear curve fit or complex frequency estimation based on well-known super-resolution technique Estimation of Signal Parameters via Rotational Invariant Techniques (ESPRIT). The existing methods in the quantum sensing literature take different routes based on Lorentzian fitting for determining magnetic field maps. To showcase the functionality and effectiveness of the suggested techniques, relevant results, based on experimental data are provided, which shows a significant reduction in computational time with the proposed method over existing methods, Comment: 4 pages, 3 figures, typos corrected

Phase transitions in many-body systems are often associated with the emergence of spatial inhomogeneities. Such features may develop at microscopic lengthscales and are not necessarily evident in measurements of macroscopic quantities. In this work, we address the topic of distribution of current paths in superconducting films. Typical lengthscales associated with superconductivity are in the range of nanometres. Accordingly, measurements of electrical resistance over much larger distances are supposed to be insensitive to details of spatial inhomogeneities of electronic properties. We observe that, contrary to expectations, current paths adopt a highly non-uniform distribution at the onset of the superconducting transition which is manifested in the development of a finite transverse resistance. The anisotropic distribution of current density is unrelated to the structural properties of the superconducting films, and indicates the emergence of electronic inhomogeneities perceivable over macroscopic distances. Our experiments reveal the ubiquitous nature of this phenomenon in conventional superconductors.

AC susceptometry, unlike static susceptometry, offers a deeper insight into magnetic materials. By employing AC susceptibility measurements, one can glean into crucial details regarding magnetic dynamics. Nevertheless, traditional AC susceptometers are constrained to measuring changes in magnetic moments within the range of a few nano-joules per tesla. Additionally, their spatial resolution is severely limited, confining their application to bulk samples only. In this study, we introduce the utilization of a Nitrogen Vacancy (NV) center-based quantum diamond microscope for mapping the AC susceptibility of micron-scale ferromagnetic specimens. By employing coherent pulse sequences, we extract both magnitude and the phase of the field from samples within a field of view spanning 70 micro-meters while achieving a resolution of 1 micro-meter. Furthermore, we quantify changes in dipole moment on the order of a femto-joules per tesla induced by excitations at frequencies reaching several hundred kilohertz.

Nitrogen vacancy (NV) centers in diamonds have been explored for realizing a wide range of sensing applications in the last decade due to their unique quantum properties. Here we realize a compact and portable magnetometer with an ensemble of NV centers which we call the Quantum MagPI (Quantum Magnetometer with Proportional Integral control). Including the sensor head and associated electronics, our sensor assembly can fit inside 10 cm x 10 cm x 7 cm box and control electronics in 30 cm x 25 cm x 5 cm box. We achieve a bandwidth normalized sensitivity of ~ 10 nT/sqrt(Hz). Using closed-loop feedback for locking to the resonance frequency, we extend the linear dynamic range to 200 microT (20x improvement compared to the intrinsic dynamic range) without compromising the sensitivity. We report a detailed performance analysis of the magnetometer through measurements of noise spectra, Allan deviation, and tracking of nT-level magnetic fields in real-time. Additionally, we demonstrate the utility of such a magnetometer by real-time tracking the movement of the elevator car and door opening by measuring the projection of the magnetic field along one of the NV-axes under ambient temperature and humidity., Comment: 6 pages and 5 figures

Quantum Diamond Microscopy using Nitrogen-Vacancy (NV) defects in diamond crystals has enabled the magnetic field imaging of a wide variety of nanoscale current profiles. Intimately linked with the imaging process is the problem of reconstructing the current density, which provides critical insight into the structure under study. This manifests as a non-trivial inverse problem of current reconstruction from noisy data, typically conducted via Fourier-based approaches. Learning algorithms and Bayesian methods have been proposed as novel alternatives for inference-based reconstructions. We study the applicability of Fourier-based and Bayesian methods for reconstructing two-dimensional current density maps from magnetic field images obtained from NV imaging. We discuss extensive numerical simulations to elucidate the performance of the reconstruction algorithms in various parameter regimes, and further validate our analysis via performing reconstructions on experimental data. Finally, we examine parameter regimes that favor specific reconstruction algorithms and provide an empirical approach for selecting regularization in Bayesian methods., Comment: 12 Pages main paper with 7 Figures. 6 pages and 2 figures in supplementary material

Deterministic optical manipulation of fluorescent nanodiamonds (FNDs) in fluids has emerged as an experimental challenge in multimodal biological imaging. Designing and developing nano-optical trapping strategies to serve this purpose is an important task. In this letter, we show how chemically-prepared gold nanoparticles and silver nanowires can facilitate Opto-thermoelectric force to trap individual entities of FNDs using a long working distance lens, low power-density illumination (532 nm laser, 12 ${\mu}W/{\mu}m^2$). Our trapping configuration combines the thermoplasmonic fields generated by individual plasmonic nanoparticles and the opto-thermoelectric effect facilitated by the surfactant to realise a nano-optical trap down to a single FND 120 nm in diameter. We utilise the same trapping excitation source to capture the spectral signatures of single FNDs and track their position. By tracking the FND, we observe the differences in the dynamics of FND around different plasmonic structures. We envisage that our drop-casting platform can be extrapolated to perform targeted, low-power trapping, manipulation, and multimodal imaging of FNDs inside biological systems such as cells., Comment: 11 pages, 12 figures, 3 tables. Supplementary videos may be found at: https://drive.google.com/drive/folders/1gkW9g5Z7Fhl4i3ZQUOBQYuUYAPrHykzY?usp=sharing

We present a novel technique for determining the microscale AC susceptibility of magnetic materials. We use magnetic field sensing properties of nitrogen-vacancy (\ce{NV-}) centers in diamond to gather quantitative data about the magnetic state of the magnetic material under investigation. In order to achieve the requisite speed in imaging, a lock-in camera is used to perform pixel-by-pixel lock-in detection of \ce{NV-} photo-luminescence. In addition, a secondary sensor is employed to isolate the effect of the excitation field from fields arising from magnetic structures on \ce{NV-} centers. We demonstrate our experimental technique by measuring the AC susceptibility of soft permalloy micro-magnets at excitation frequencies of up to \SI{20}{\hertz} with a spatial resolution of \SI{1.2}{\micro \meter} and a field of view of \SI{100}{\um}. Our work paves the way for microscopic measurement of AC susceptibilities of magnetic materials relevant to physical, biological, and material sciences.

Nitrogen-Vacancy (NV) centers in diamonds provide a room-temperature platform for various emerging quantum technologies, e.g. the long nuclear spin coherence times as potential quantum memory registers. We demonstrate a freezing protocol for an NV center to isolate its intrinsic nuclear spin from a noisy electromagnetic environment. Any initial state of the nuclear spin can be frozen when the hyperfine-coupled electron and nuclear spins are simultaneously driven with unequal Rabi frequencies. Through numerical simulations, we show that our protocol can effectively shield the nuclear spin from strong drive or noise fields. We also observe a clear suppression of quantum correlations in the frozen nuclear spin regime by measuring the quantum discord of the electron-nuclear spin system. These features can be instrumental in extending the storage times of NV nuclear-spin based quantum memories in hybrid quantum systems.

Wide field-of-view magnetic field microscopy has been realised by probing shifts in optically detected magnetic resonance (ODMR) spectrum of Nitrogen Vacancy (NV) defect centers in diamond. However, these widefield diamond NV magnetometers require few to several minutes of acquisition to get a single magnetic field image, rendering the technique temporally static in it's current form. This limitation prevents application of diamond NV magnetometers to novel imaging of dynamically varying microscale magnetic field processes. Here, we show that the magnetic field imaging frame rate can be significantly enhanced by performing lock-in detection of NV photo-luminescence (PL), simultaneously over multiple pixels of a lock-in camera. A detailed protocol for synchronization of frequency modulated PL of NV centers with fast camera frame demodulation, at few kilohertz frequencies, has been experimentally demonstrated. This experimental technique allows magnetic field imaging of sub-second varying microscale currents in planar microcoils with imaging frame rates in the range of 50 to 200 frames per second (fps). Our work demonstrates that widefield per-pixel lock-in detection of frequency modulated NV ODMR enables dynamic magnetic field microscopy., Comment: 19 pages, 12 figures

We study the Hall effect in square, planar type-II superconductors using numerical simulations of time dependent Ginzburg-Landau (TDGL) equations. The Hall field in some type-II superconductors displays sign-change behavior at some magnetic fields due to the induced field of vortex flow, when its contribution is strong enough to reverse the field direction. In this work, we use modified TDGL equations which couple an externally applied current, and also incorporate normal-state and flux-flow Hall effects. We obtain the profile of Hall angle as a function of applied magnetic field for four different sizes (l\times l) of the superconductor: l/ \xi belongs to {3, 5, 15, 20}. We obtain vastly different profiles for each size, proving that size is an important parameter that determines Hall behavior. We find that electric field dynamics provides an insight into several anomalous features including signchange of Hall angle, and leads us to the precise transient behavior of order parameter responsible for them., Comment: 8 Pages, 8 Figures

Magnetic field sensing, with its recent advances, is emerging as a viable alternative to measure functional activity of single neurons in the brain by sensing action potential associated magnetic fields (APMFs). Measurement of APMFs of large axons of worms have been possible due to their size. In the mammalian brain, axon sizes, their numbers and routes, restricts using such functional imaging methods. With segmented model of mammalian pyramidal neurons, we show that the APMF of intra-axonal currents in the axon hillock are two orders of magnitude larger than other neuronal locations. Expected 2-dimensional vector magnetic field maps of naturalistic spiking activity of a volume of neurons via widefield diamond-nitrogen-vacancy-center-magnetometry (DNVM) were simulated. A dictionary based matching pursuit type algorithm applied to the data using the axon-hillock's APMF signature allowed spatiotemporal reconstruction of APs in the volume of brain tissue at single cell resolution. Enhancement of APMF signals coupled with NVMM advances thus can potentially replace current functional brain mapping techniques.

We report the fabrication and characterization results of a simple and low-cost pH sensor fabricated using a graphite pencil to define a working electrode and silver paste to define a reference electrode on scotch tape. The sensor operation is based on potentiometric measurement and thereby insensitive to fabrication variations in shape of the electrode unlike amperometric and chemiresistive measurement techniques. The substrate of the disposable sensor is prepared by pasting scotch tape atop a piece of chart paper, and two types of sensors fabricated with 6B and 2B graphite pencils are tested with three solutions with different pH values. The sensor functions as a passive sensing tag without requiring any external power or stimulus, and the measured sensitivities of the pH sensors fabricated using 2B and 6B pencil carbon electrodes (PCEs) are $-4.54mV/pH$ and $-4.09mV/pH$ respectively.

Generic mesoscopic quantum systems that interact with their environment tend to display appreciable correlations with environment that often play an important role in the physical properties of the system. However, the experimental methods needed to characterize such systems either ignore the role of initial correlations or scale unfavourably with system dimensions. Here, we present a technique that is agnostic to system-environment correlations and can be potentially implemented experimentally. Under a specific set of constraints, we demonstrate the ability to detect and measure specific correlations. We apply the technique on a hybrid quantum system of Nitrogen Vacancy Centers (NV) coupled to an optical cavity with initial correlations. We extract the interaction strength and effective number of interacting NVs from the initial correlations using our technique., Comment: 15 pages, comments welcome

Quantum sensors, such as the Nitrogen Vacancy (NV) color center in diamond, are known for their exquisite sensitivity, but their performance over time are subject to degradation by environmental noise. To improve the long-term robustness of a quantum sensor, here we realize an integrated combinatorial spin sensor in the same micrometer-scale footprint, which exploits two different spin sensitivities to distinct physical quantities to stabilize one spin sensor with local information collected in realtime via the second sensor. We show that we can use the electronic spins of a large ensemble of NV centers as sensors of the local magnetic field fluctuations, affecting both spin sensors, in order to stabilize the output signal of interleaved Ramsey sequences performed on the 14N nuclear spin. An envisioned application of such a device is to sense rotation rates with a stability of several days, allowing navigation with limited or no requirement of geo-localization. Our results would enable stable rotation sensing for over several hours, which already reflects better performance than MEMS gyroscopes of comparable sensitivity and size.

Quantum memories are critical for solid-state quantum computing devices and a good quantum memory requires both long storage time and fast read/write operations. A promising system is the Nitrogen-Vacancy (NV) center in diamond, where the NV electronic spin serves as the computing qubit and a nearby nuclear spin as the memory qubit. Previous works used remote, weakly coupled $^{13}$C nuclear spins, trading read/write speed for long storage time. Here we focus instead on the intrinsic strongly coupled $^{14}$N nuclear spin. We first quantitatively understand its decoherence mechanism, identifying as its source the electronic spin that acts as a quantum fluctuator. We then propose a scheme to protect the quantum memory from the fluctuating noise by applying dynamical decoupling on the environment itself. We demonstrate a factor of $3$ enhancement of the storage time in a proof-of-principle experiment, showing the potential for a quantum memory that combines fast operation with long coherence time., Comment: 21 pages, 10 figures

Theoretical studies indicating the presence of long-lived coherence in the radical pair system have engendered questions about the utilitarian role of sustained coherence in the avian compass. In this manuscript, we investigate this for a realistic multi-nuclear radical pair system, along with the related question of its sensitivity to the geomagnetic field. Firstly, we find that sustenance of long-lived coherence is unlikely in a realistic hyperfine environment. Secondly, probing the role of the hyperfine interactions on the compass sensitivity, we establish the hyperfine anisotropy as an essential parameter for the sensitivity. Thereby, we are able to identify a parameter regime where the compass would exhibit sensitivity even without sustained coherence., Comment: Submitted version

Development of ultrashort pulse sources has had an immense impact on condensed-matter physics, biomedical imaging, high-field physics, frequency metrology, telecommunications, nonlinear optics, and molecular spectroscopy. Although numerous advancements of such sources have been made, it remains a challenge to create a highly compact, robust platform capable of producing femtosecond pulses over a wide range of wavelengths, durations, and repetition rates. Recent observations of frequency comb generation via cascaded parametric oscillation in microresonators11 suggest a path for achieving this goal. Here we investigate the temporal and spectral properties of parametric combs generated in silicon-nitride microresonators and observe a transition to passive modelocking of the comb consistent with soliton-pulse formation, resulting in the generation of 160-fs pulses at a 99-GHz repetition rate. This platform offers the prospect of producing pulses from 10 fs to a few ps at repetition rates from 10 GHz to > 1 THz and over a wavelength range of 0.8 - 6 \mu m.

We demonstrate a frequency comb spanning an octave via the parametric process of cascaded four-wave mixing in a monolithic, high-Q silicon nitride microring resonator. The comb is generated from a single-frequency pump laser at 1562 nm and spans 128 THz with a spacing of 226 GHz, which can be tuned slightly with the pump power. In addition, we investigate the RF-noise characteristics of the parametric comb and find that the comb can operate in a low-noise state with a 30-dB reduction in noise as the pump frequency is tuned into the cavity resonance.

We demonstrate a stable CMOS-compatible on-chip multiple-wavelength source by filtering and modulating individual lines from a frequency comb generated by a microring resonator optical parametric oscillator.. We show comb operation in a low-noise state that is stable and usable for many hours. Bit-error rate measurements demonstrate negligible power penalty from six independent frequencies when compared to a tunable diode laser baseline. Open eye diagrams confirm the fidelity of the 10 Gb/s data transmitted at the comb frequencies and the suitability of this device for use as a fully integrated silicon-based WDM source., Comment: 3 pages, 3 figures

Recently developed techniques for generating precisely equidistant optical frequencies over broad wavelength ranges are revolutionizing precision physical measurement [1-3]. These frequency "combs" are produced primarily using relatively large, ultrafast laser systems. However, recent research has shown that broad-bandwidth combs can be produced using highly-nonlinear interactions in microresonator optical parametric oscillators [4-11]. Such devices not only offer the potential for developing extremely compact optical atomic clocks but are also promising for astronomical spectroscopy [12-14], ultrashort pulse shaping [15], and ultrahigh-speed communications systems. Here we demonstrate the generation of broad-bandwidth optical frequency combs from a CMOS-compatible integrated microresonator [16,17], which is a fully-monolithic and sealed chip-scale device making it insensitive to the surrounding environment. We characterize the comb quality using a novel self-referencing method and verify that the comb line frequencies are equidistant over a bandwidth that is nearly an order of magnitude larger than previous measurements. In addition, we investigate the ultrafast temporal properties of the comb and demonstrate its potential to serve as a chip-scale source of ultrafast (sub-ps) pulses.

We show that two-photon absorption (TPA) in Rubidium atoms can be greatly enhanced by the use of a hollow-core photonic bandgap fiber. We investigate off-resonant, degenerate Doppler-free TPA on the 5S1/2 - 5D5/2 transition and observe 1% absorption of a pump beam with a total power of only 1 mW in the fiber. These results are verified by measuring the amount of emitted blue fluorescence and are consistent with the theoretical predictions which indicate that transit time effects play an important role in determining the two-photon absorption cross-section in a confined geometry., Comment: 5 pages, 6 figures