Search

Continuous quantum phase transitions are widely assumed and frequently observed in various systems of quantum particles or spins. Their characteristic trait involves scaling laws governing a second-order, gradual suppression of the order parameter as the quantum critical point is approached. The localization of Cooper pairs in disordered superconductors and the resulting breakdown of superconductivity have long stood as a prototypical example. Here, we show a departure from this paradigm, showcasing that amorphous superconducting films of indium oxide undergo a distinctive, discontinuous first-order quantum phase transition tuned by disorder. Through systematic measurements of the plasmon spectrum in superconducting microwave resonators, we provide evidence for a marked jump of both the zero-temperature superfluid stiffness and the transition temperature at the critical disorder. This discontinuous transition sheds light on the previously overlooked role of repulsive interactions between Cooper pairs and the subsequent competition between superconductivity and insulating Cooper-pair glass. Furthermore, our investigation shows that the critical temperature of the films no longer relates to the pairing amplitude but aligns with the superfluid stiffness, consistent with the pseudogap regime of preformed Cooper pairs. Our findings raise fundamental new questions into the role of disorder in quantum phase transitions and carry implications for superinductances in quantum circuits., Comment: Updated text

In the last decade, graphene has become an exciting platform for electron optical experiments, in many aspects superior to conventional two-dimensional electron gases (2DEGs). A major advantage, besides the ultra-large mobilities, is the fine control over the electrostatics, which gives the possibility of realising gap-less and compact p-n interfaces with high precision. The latter host non-trivial states, \eg, snake states in moderate magnetic fields, and serve as building blocks of complex electron interferometers. Thanks to the Dirac spectrum and its non-trivial Berry phase, the internal (valley and sublattice) degrees of freedom, and the possibility to tailor the band structure using proximity effects, such interferometers open up a completely new playground based on novel device architectures. In this review, we introduce the theoretical background of graphene electron optics, fabrication methods used to realise electron-optical devices, and techniques for corresponding numerical simulations. Based on this, we give a comprehensive review of ballistic transport experiments and simple building blocks of electron optical devices both in single and bilayer graphene, highlighting the novel physics that is brought in compared to conventional 2DEGs. After describing the different magnetic field regimes in graphene p-n junctions and nanostructures, we conclude by discussing the state of the art in graphene-based Mach-Zender and Fabry-Perot interferometers., Comment: The authors welcome any comments regarding the content of the review

Pairing of electrons is ubiquitous in electronic systems featuring attractive inter-electron interactions, as exemplified in superconductors. Counter-intuitively, it can also be mediated in certain circumstances by the repulsive Coulomb interaction alone. Quantum Hall (QH) Fabry-P\'erot interferometers (FPIs) tailored in two-dimensional electron gas under a perpendicular magnetic field has been argued to exhibit such unusual electron pairing seemingly without attractive interaction. Here, we show evidence in graphene QH FPIs revealing not only a similar electron pairing at bulk filling factor nu=2 but also an unforeseen emergence of electron tripling characterized by a fractional Aharonov-Bohm flux period h/3e (h is the Planck constant and e the electron charge) at nu=3. Leveraging a novel plunger-gate spectroscopy, we demonstrate that electron pairing (tripling) involves correlated charge transport on two (three) entangled QH edge channels. This spectroscopy indicates a quantum interference flux-periodicity determined by the sum of the phases acquired by the distinct QH edge channels having slightly different interfering areas. While recent theory invokes the dynamical exchange of neutral magnetoplasmons -- dubbed neutralons -- as mediator for electron pairing, our discovery of three entangled QH edge channels with apparent electron tripling defies understanding and introduces a new three-body problem for interacting fermions.

In BCS superconductors, the superfluid stiffness is virtually constant at low temperature and only slightly affected by the exponentially low density of thermal quasiparticles. Here, we present an experimental and theoretical study on the temperature dependence of superfluid stiffness $\Theta\left(T\right)$ in a strongly disordered pseudo-gaped superconductor, amorphous $\text{InO}_{x}$, which exhibits non-BCS behavior. Experimentally, we report an unusual power-law suppression of the superfluid stiffness $\delta\Theta\left(T\right)\propto T^{b}$ at $T\ll T_{c}$, with $b\sim1.6$, which we measured via the frequency shift of microwave resonators. Theoretically, by combining analytical and numerical methods to a model of a disordered superconductor with pseudogap and spatial inhomogeneities of the superconducting order parameter, we found a qualitatively similar low-temperature power-law behavior with exponent $b\sim1.6-3$ being disorder-dependent. This power-law suppression of the superfluid density occurs mainly due to the broad distribution of the superconducting order parameter that is known to exist in such superconductors [arXiv:1012.3630], even moderately far from the superconductor-insulator transition. The presence of the power-law dependence $\delta\Theta\left(T\right)\propto T^{b}$ at low $T\ll T_{c}$ demonstrates the existence of low-energy collective excitations; in turn, it implies the presence of a new channel of dissipation in inhomogeneous superconductors caused by sub-gap excitations that are not quasiparticles. Our findings have implications for the use of strongly disordered superconductors as superinductance in quantum circuits., Comment: 27 pages, 15 figures; Several small typos fixed

Semiconducting transition-metal dichalcogenides (TMDs) exhibit high mobility, strong spin-orbit coupling, and large effective masses, which simultaneously leads to a rich wealth of Landau quantizations and inherently strong electronic interactions. However, in spite of their extensively explored Landau levels (LL) structure, probing electron correlations in the fractionally filled LL regime has not been possible due to the difficulty of reaching the quantum limit. Here, we report evidence for fractional quantum Hall (FQH) states at filling fractions 4/5 and 2/5 in the lowest LL of bilayer MoS$_{2}$, manifested in fractionally quantized transverse conductance plateaus accompanied by longitudinal resistance minima. We further show that the observed FQH states sensitively depend on the dielectric and gate screening of the Coulomb interactions. Our findings establish a new FQH experimental platform which are a scarce resource: an intrinsic semiconducting high mobility electron gas, whose electronic interactions in the FQH regime are in principle tunable by Coulomb-screening engineering, and as such, could be the missing link between atomically thin graphene and semiconducting quantum wells., Comment: 10 pages, 4 figures

Hybridizing superconductivity with the quantum Hall (QH) effects has major potential for designing novel circuits capable of inducing and manipulating non-Abelian states for topological quantum computation. However, despite recent experimental progress towards this hybridization, concrete evidence for a chiral QH Josephson junction -- the elemental building block for coherent superconducting-QH circuits -- is still lacking. Its expected signature is an unusual chiral supercurrent flowing in QH edge channels, which oscillates with a specific $2\phi_0$ magnetic flux periodicity ($\phi_0=h/2e$ is the superconducting flux quantum, $h$ the Planck constant and $e$ the electron charge). Here, we show that ultra-narrow Josephson junctions defined in encapsulated graphene nanoribbons exhibit such a chiral supercurrent, visible up to 8 teslas, and carried by the spin-degenerate edge channel of the QH plateau of resistance $h/2e^2\simeq 12.9$ k$\Omega$. We observe reproducible $2\phi_0$-periodic oscillation of the supercurrent, which emerges at constant filling factor when the area of the loop formed by the QH edge channel is constant, within a magnetic-length correction that we resolve in the data. Furthermore, by varying the junction geometry, we show that reducing the superconductor/normal interface length is pivotal to obtain a measurable supercurrent on QH plateaus, in agreement with theories predicting dephasing along the superconducting interface. Our findings mark a critical milestone along the path to explore correlated and fractional QH-based superconducting devices that should host non-Abelian Majorana and parafermion zero modes., Comment: Maintext and SI

Electronic edge states in topological insulators have become a major paradigm in physics. The oldest and primary example is that of quantum Hall (QH) edge channels that propagate along the periphery of two-dimensional electron gases (2DEGs) under perpendicular magnetic field. Yet, despite 40 years of intensive studies using a variety of transport and scanning probe techniques, imaging the real-space structure of QH edge channels has proven difficult, mainly due to the buried nature of most 2DEGs in semiconductors. Here, we show that QH edge states in graphene are confined to a few magnetic lengths at the crystal edges by performing scanning tunneling spectroscopy up to the edge of a graphene flake on hexagonal boron nitride. These findings indicate that QH edge states are defined by boundary conditions of vanishing electronic wavefunctions at the crystal edges, resulting in ideal one-dimensional chiral channels, free of electrostatic reconstruction. We further evidence a uniform charge carrier density at the edges, contrasting with conjectures on the existence of non-topological upstream modes. The absence of electrostatic reconstruction of quantum Hall edge states has profound implications for the universality of electron and heat transport experiments in graphene-based systems and other 2D crystalline materials., Comment: New theoretical simulations of the tunneling DOS added

When electrons populate a flat band their kinetic energy becomes negligible, forcing them to organize in exotic many-body states to minimize their Coulomb energy. The zeroth Landau level of graphene under magnetic field is a particularly interesting strongly interacting flat band because inter-electron interactions are predicted to induce a rich variety of broken-symmetry states with distinct topological and lattice-scale orders. Evidence for these stems mostly from indirect transport experiments that suggest that broken-symmetry states are tunable by boosting the Zeeman energy or by dielectric screening of the Coulomb interaction. However, confirming the existence of these ground states requires a direct visualization of their lattice-scale orders. Here, we image three distinct broken-symmetry phases in graphene using scanning tunneling spectroscopy. We explore the phase diagram by tuning the screening of the Coulomb interaction by a low or high dielectric constant environment, and with a magnetic field. In the unscreened case, we unveil a Kekul\'e bond order, consistent with observations of an insulating state undergoing a magnetic-field driven Kosterlitz-Thouless transition. Under dielectric screening, a sublattice-unpolarized ground state emerges at low magnetic fields, and transits to a charge-density-wave order with partial sublattice polarization at higher magnetic fields. The Kekul\'e and charge-density-wave orders furthermore coexist with additional, secondary lattice-scale orders that enrich the phase diagram beyond current theory predictions. This screening-induced tunability of broken-symmetry orders may prove valuable to uncover correlated phases of matter in other quantum materials., Comment: Main text + SI

Electron interferometry with quantum Hall edge channels holds promise for probing and harnessing exotic exchange statistics of non-Abelian anyons. In semiconductor heterostructures, however, quantum Hall interferometry has proven challenging and often obscured by charging effects. Here we show that high-mobility monolayer graphene equipped with a series of gate-tunable quantum point contacts that act as electron beam-splitters provides a model system to perform Fabry-P\'{e}rot quantum Hall interferometry. We observe high-visibility Aharonov-Bohm interference free of charging effects and widely tunable through electrostatic gating or magnetic field, in remarkable agreement with theory. A coherence length of $\mathbf{10 \,\mu m}$ at a temperature of $0.02$ K allows us to further achieve coherently-coupled double Fabry-P\'{e}rot interferometry. Our results open a new avenue for quantum Hall interferometry and the exploitation of topological excitations for quantum computation., Comment: Revised main text

In order to understand the emergence of superconductivity it is useful to study and identify the various pathways leading to the destruction of superconductivity. One way is to use the increase in Coulomb-repulsion due to the increase in disorder, which overpowers the attractive interaction responsible for Cooper-pair formation. A second pathway, applicable to uniformly disordered materials, is the competition between superconductivity and Anderson localization, which leads to electronic granularity in which phase and amplitude fluctuations of the superconducting order parameter play a role. Finally, a third pathway is an array of superconducting islands coupled by some form of proximity-effect, due to Andreev-reflections, and which leads from a superconducting state to a state with finite resistivity, which appears like a metallic groundstate. This review summarizes recent progress in understanding of these different pathways, including experiments in low dimensional materials and application in superconducting quantum devices., Comment: Review Article

Finite-size scaling analysis is a well-accepted method for identification and characterization of quantum phase transitions (QPTs) in superconducting, magnetic and insulating systems. We formally apply this analysis in the form suitable for QPTs in 2-dimensional superconducting films to magnetic-field driven superconductor-metal transition in 1-dimensional MoGe nanowires. Despite being obviously inapplicable to nanowires, the 2d scaling equation leads to a high-quality scaling collapse of the nanowire resistance in the temperature and resistance ranges comparable or better to what is accepted in the analysis of the films. Our results suggest that the appearance and the quality of the scaling collapse by itself is not a reliable indicator of a QPT. We have also observed a sign-change of the zero-bias anomaly (ZBA) in the non-linear resistance, occurring exactly at the critical field of the accidental QPT. This behavior is often taken as an additional confirmation of the transition. We argue that in nanowires, the non-linearity is caused by electron heating and has no relation to the critical fluctuations. Our observation suggests that similar to the scaling collapse, the sign-change of ZBA can be a misleading indicator of QPT., Comment: 9 pages, 5 figures

The ground state of charge neutral graphene under perpendicular magnetic field was predicted to be a quantum Hall topological insulator with a ferromagnetic order and spin-filtered, helical edge channels. In most experiments, however, an otherwise insulating state is observed and is accounted for by lattice-scale interactions that promote a broken-symmetry state with gapped bulk and edge excitations. We tuned the ground state of the graphene zeroth Landau level to the topological phase via a suitable screening of the Coulomb interaction with a SrTiO$_3$ high-$k$ dielectric substrate. We observed robust helical edge transport emerging at a magnetic field as low as 1 tesla and withstanding temperatures up to 110 kelvins over micron-long distances. This new and versatile graphene platform opens new avenues for spintronics and topological quantum computation., Comment: Main text + SI

We report the operation of a field-effect transistor based on a single InAs nanowire gated by an ionic liquid. Liquid gating yields very efficient carrier modulation with a transconductance value thirty time larger than standard back gating with the SiO2 /Si++ substrate. Thanks to this wide modulation we show the controlled evolution from semiconductor to metallic-like behavior in the nanowire. This work provides the first systematic study of ionic-liquid gating in electronic devices based on individual III-V semiconductor nanowires: we argue this architecture opens the way to a wide range of fundamental and applied studies from the phase-transitions to bioelectronics., Comment: 11 pages (abstract and bibliography included), 5 Figures

We report on the evolution of the coherent electronic transport through a gate-defined constriction in a high-mobility graphene device from ballistic transport to quantum Hall regime upon increasing the magnetic field. At low field, the conductance exhibits Fabry-P\'erot resonances resulting from the npn cavities formed beneath the top-gated regions. Above a critical field $B^*$ corresponding to the cyclotron radius equal to the npn cavity length, Fabry-P\'erot resonances vanish and snake trajectories are guided through the constriction with a characteristic set of conductance oscillations. Increasing further the magnetic field allows us to probe the Landau level spectrum in the constriction, with distortions due to the combination of confinement and de-confinement of Landau levels in a saddle potential. These observations are confirmed by numerical calculations.

In most superconductors the transition to the superconducting state is driven by the binding of electrons into Cooper-pairs. The condensation of these pairs into a single, phase coherent, quantum state takes place concomitantly with their formation at the transition temperature, $T_c$. A different scenario occurs in some disordered, amorphous, superconductors: Instead of a pairing-driven transition, incoherent Cooper pairs first pre-form above $T_c$, causing the opening of a pseudogap, and then, at $T_c$, condense into the phase coherent superconducting state. Such a two-step scenario implies the existence of a new energy scale, $\Delta_{c}$, driving the collective superconducting transition of the preformed pairs. Here we unveil this energy scale by means of Andreev spectroscopy in superconducting thin films of amorphous indium oxide. We observe two Andreev conductance peaks at $\pm \Delta_{c}$ that develop only below $T_c$ and for highly disordered films on the verge of the transition to insulator. Our findings demonstrate that amorphous superconducting films provide prototypical disordered quantum systems to explore the collective superfluid transition of preformed Cooper-pairs pairs., Comment: Main text + SI

A quantum phase transition (QPT) between distinct ground states of matter is a wide-spread phenomenon in nature, yet there are only a few experimentally accessible systems where the microscopic mechanism of the transition can be tested and understood. These cases are unique and form the experimentally established foundation for our understanding of quantum critical phenomena. Here we report the discovery that a magnetic-field-driven QPT in superconducting nanowires - a prototypical 1d-system - can be fully explained by the critical theory of pair-breaking transitions characterized by a correlation length exponent $\nu \approx 1$ and dynamic critical exponent $z \approx 2$. We find that in the quantum critical regime, the electrical conductivity is in agreement with a theoretically predicted scaling function and, moreover, that the theory quantitatively describes the dependence of conductivity on the critical temperature, field magnitude and orientation, nanowire cross sectional area, and microscopic parameters of the nanowire material. At the critical field, the conductivity follows a $T^{(d-2)/z}$ dependence predicted by phenomenological scaling theories and more recently obtained within a holographic framework. Our work uncovers the microscopic processes governing the transition: The pair-breaking effect of the magnetic field on interacting Cooper pairs overdamped by their coupling to electronic degrees of freedom. It also reveals the universal character of continuous quantum phase transitions., Comment: 22 pages, 5 figures

Thin films of Amorphous indium oxide undergo a magnetic field driven superconducting to insulator quantum phase transition. In the insulating phase, the current-voltage characteristics show large current discontinuities due to overheating of electrons. We show that the onset voltage for the discontinuities vanishes as we approach the quantum critical point. As a result the insulating phase becomes unstable with respect to any applied voltage making it, at least experimentally, immeasurable. We emphasize that unlike previous reports of the absence of linear response near quantum phase transitions, in our system, the departure from equilibrium is discontinuous. Because the conditions for these discontinuities are satisfied in most insulators at low temperatures, and due to the decay of all characteristic energy scales near quantum phase transitions, we believe that this instability is general and should occur in various systems while approaching their quantum critical point. Accounting for this instability is crucial for determining the critical behavior of systems near the transition.

Charge carriers in the quantum Hall regime propagate via one-dimensional conducting channels that form along the edges of a two-dimensional electron gas. Controlling their transmission through a gate-tunable constriction, also called quantum point contact (QPC), is fundamental for many coherent transport experiments. However, in graphene, tailoring a QPC with electrostatic gates remains challenging due to the formation of p-n junctions below gate electrodes along which electron and hole edge channels co-propagate and mix, short-circuiting the constriction. Here we show that this electron-hole mixing is drastically reduced in high mobility boron-nitride/graphene/boron-nitride van-der-Waals heterostructures thanks to the full degeneracy lifting of the Landau levels, enabling QPC operation with full channel pinch-off. We demonstrate gate-tunable selective transmission of quantum Hall edge channels through the QPC, both in the integer and the fractional quantum Hall regimes. This gate-control of edge channel propagation in graphene van-der-Waals heterostructures opens the door to quantum Hall interferometry and electron quantum optics experiments in the integer and fractional quantum Hall regimes of graphene., Comment: New data in the fractional quantum Hall regime added

We study the response of high-critical current proximity Josephson junctions to a microwave excitation. Electron over-heating in such devices is known to create hysteretic dc voltage-current characteristics. Here we demonstrate that it also strongly influences the ac response. The interplay of electron over-heating and ac Josephson dynamics is revealed by the evolution of the Shapiro steps with the microwave drive amplitude. Extending the resistively shunted Josephson junction model by including a thermal balance for the electronic bath coupled to phonons, a strong electron over-heating is obtained.

When a Josephson junction array is built with hybrid superconductor/metal/superconductor junctions, a quantum phase transition from a superconducting to a two-dimensional (2D) metallic ground state is predicted to happen upon increasing the junction normal state resistance. Owing to its surface-exposed 2D electron gas and its gate-tunable charge carrier density, graphene coupled to superconductors is the ideal platform to study the above-mentioned transition between ground states. Here we show that decorating graphene with a sparse and regular array of superconducting nanodisks enables to continuously gate-tune the quantum superconductor-to-metal transition of the Josephson junction array into a zero-temperature metallic state. The suppression of proximity-induced superconductivity is a direct consequence of the emergence of quantum fluctuations of the superconducting phase of the disks. Under perpendicular magnetic field, the competition between quantum fluctuations and disorder is responsible for the resilience at the lowest temperatures of a superconducting glassy state that persists above the upper critical field. Our results provide the entire phase diagram of the disorder and magnetic field-tuned transition and unveil the fundamental impact of quantum phase fluctuations in 2D superconducting systems., Comment: 25 pages, 6 figures

We investigate magneto-transport through graphene nano-ribbons as a function of gate and bias voltage, and temperature. We find that a magnetic field systematically leads to an increase of the conductance on a scale of a few tesla. This phenomenon is accompanied by a decrease in the energy scales associated to charging effects, and to hopping processes probed by temperature-dependent measurements. All the observations can be interpreted consistently in terms of strong-localization effects caused by the large disorder present, and exclude that the insulating state observed in nano-ribbons can be explained solely in terms of a true gap between valence and conduction band., Comment: 4 pages, 5 figures