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Harmonic mode-locking, realized actively or passively, is an effective technique for increasing the repetition rate of lasers, with important applications in optical sampling, laser micro-machining and frequency metrology. It is critically important to understand how a harmonically mode-locked pulse train responds to external perturbations and noise, so as to make sure that it is stable and resistant to noise. Here, in a series of carefully designed experiments, we elucidate the retiming dynamics of laser pulses generated in a soliton fiber laser harmonically mode-locked at ~2 GHz to the acoustic resonance in a photonic crystal fiber (PCF) core. We characterize the self-driven optomechanical lattice along the PCF using a homodyne set-up, and reveal that each soliton undergoes damped oscillatory retiming within its trapping potential after an abrupt perturbation. In addition we show, through statistical analysis of the intra-cavity pulse spacing, how the trapping potentials are effective for suppressing timing jitter. The experimental results are well described using a dynamic model including dissipation, which provides valuable insight into the stability and noise performance of optomechanically mode-locked laser systems, and may also be useful for studying complex inter-soliton interactions.

We explore a magnetooptomechanical system consisting of a single magnetic microparticle optically levitated within the core of a helically twisted single-ring hollow-core photonic crystal fibre. We use newly-developed magnetic particles that have a core of antiferromagnetic yttrium-ortho-ferrite (YFeO3) and a shell of ferrimagnetic YIG (Y3Fe5O12) approximately 50 nm thick. Using a 632.8 nm probe beam, we observe optical-torque-induced rotation of the particle and rotation of the magnetization vector in presence of an external static magnetic field. This one-of-a-kind platform opens a path to novel investigations of optomagnetic physics with levitated magnetic particles.

The valley degree of freedom of electrons in materials promises routes toward energy-efficient information storage with enticing prospects towards quantum information processing. Current challenges in utilizing valley polarization are symmetry conditions that require monolayer structures or specific material engineering, non-resonant optical control to avoid energy dissipation, and the ability to switch valley polarization at optical speed. We demonstrate all-optical and non-resonant control over valley polarization using bulk MoS$_2$, a centrosymmetric material with zero Berry curvature at the valleys. Our universal method utilizes spin-angular momentum-shaped tri-foil optical control pulses to switch the material's electronic topology to induce valley polarization by transiently breaking time and space inversion symmetry through a simple phase rotation. The dependence of the generation of the second harmonic of an optical probe pulse on the phase rotation directly demonstrates the efficacy of valley polarization. It shows that direct optical control over the valley degree of freedom is not limited to monolayer structures. Instead, it is possible for systems with an arbitrary number of layers and bulk materials. Universal and non-resonant valley control at optical speeds unlocks the possibility of engineering efficient, multi-material valleytronic devices operating on quantum coherent timescales., Comment: 4 figures

We combine soliton dynamics in gas-filled hollow-core photonic crystal fibers with a state-of-the-art fiber laser to realize a turn-key system producing few-fs pulses at 8 MHz repetition rate at pump energies as low as 220 nJ. Furthermore, by exploiting the soliton self-frequency shift in a second hydrogen-filled hollow-core fiber, we efficiently generate pulses as short as 22 fs, continuously tunable from 1100 nm to 1474 nm.

We demonstrate generation of 7.6 fs near-UV pulses centered at 400 nm via 8-fold soliton-effect self-compression in an Ar-filled hollow-core kagom\'e-style photonic crystal fiber with ultrathin core walls. Analytical calculations of the effective compression length and soliton order permit adjustment of the experimental parameters, and numerical modelling of the nonlinear pulse dynamics in the fiber accurately predict the spectro-temporal profiles of the self-compressed pulses. After compensation of phase distortion introduced by the optical elements along the beam path from the fiber to the diagnostics, 71% of the pulse energy was in the main temporal lobe, with peak powers in excess of 0.2 GW. The convenient set-up opens up new opportunities for time-resolved studies in spectroscopy, chemistry and materials science., Comment: 7 pages, 5 figures

Optical vortices, which have been extensively studied over the last decades, offer an additional degree of freedom useful in many applications, such as optical tweezers and quantum control. Stimulated Brillouin scattering, providing a narrow linewidth and a strong nonlinear response, has been used to realise quasi-continuous wave (CW) lasers. Here, we report stable oscillation of optical vortices and acoustic modes in a Brillouin laser based on chiral photonic crystal fibre, which robustly supports helical Bloch modes (HBMs) that carry circularly-polarized optical vortex and display circular birefringence. We implement a narrow-linewidth Brillouin fibre laser that stably emits 1st- and 2nd-order vortex-carrying HBMs. Angular momentum conservation selection rules dictate that pump and backward Brillouin signals have opposite topological charge and spin. Additionally, we show that when the chiral PCF is placed within a laser ring cavity, the linewidth-narrowing associated with lasing permits the peak of the Brillouin gain that corresponds to acoustic mode to be measured with resolution of 10 kHz and accuracy of 520 kHz. The results pave the way to a new generation of vortex-carrying SBS systems with applications in quantum information processing, vortex-carrying nonreciprocal systems.

Optical non-reciprocity, which breaks the symmetry between forward and backward propagating optical waves, has become vital in photonic systems and enables many key devices, such as optical isolators, circulators and optical routers. Most conventional optical isolators involve magneto-optic materials, but devices based on optical nonlinearities, optomechanically induced transparency and stimulated Brillouin scattering (SBS) have also been demonstrated. So far, however, they have only been implemented for linearly or randomly polarized LP01-like fundamental modes. Here we report a light-driven nonreciprocal isolator for optical vortex modes, based on topology-selective SBS in chiral photonic crystal fibre. The device can be reconfigured as an amplifier or an isolator by adjusting the frequency of the control signal. The experimental results show vortex isolation of 22 dB, which is at the state-of-the-art in fundamental mode isolators using SBS. This unique device may find applications in optical communications, fibre lasers, quantum information processing and optical tweezers.

Stimulated Brillouin scattering (SBS) has many applications, for example, in sensing, microwave photonics and signal processing. Here we report the first experimental study of SBS in chiral photonic crystal fiber (PCF), which displays optical activity and robustly maintains circular polarization states against external perturbations. As a result, circularly polarized pump light is cleanly back-scattered into a Stokes signal with the orthogonal circular polarization state, as is required by angular momentum conservation. By comparison, untwisted PCF generates a Stokes signal with an unpredictable polarization state, owing to its high sensitivity to external perturbations. We use chiral PCF to realize a circularly polarized continuous-wave Brillouin laser. The results pave the way to a new generation of stable circularly polarized SBS systems with applications in quantum manipulation, optical tweezers, optical gyroscopes and fiber sensors.

We present the use of linearly down-tapered gas-filled hollow-core photonic crystal fiber in a single-stage, pumped with pulses from a compact infrared laser source, to generate a supercontinuum carrying significant spectral power in the deep ultraviolet (200 - 300 nm). The generated supercontinuum extends from the near infrared down to around 213 nm with up to 0.83 mW/nm in the deep ultraviolet., Comment: 4 pages (+1 page for full reference list), 3 figures

Flying particle sensors in hollow-core photonic crystal fibers require accurate localization of the optically trapped microparticles. We report position measurement to micrometer-resolution, using optical frequency domain reflectometry, of two 1.65-$\mu$m-diameter polystyrene particles., Comment: 4 pages, 3 figures, Accepted for presentation at the 27th International Conference on Optical Fibre Sensors (OFS) 2020, Alexandria, Virginia, USA

We report generation of ultrashort UV pulses by soliton self-compression in kagom\'e-style hollow-core photonic crystal fiber filled with ambient air. Pump pulses with energy 2.6 uJ and duration 54 fs at 400 nm were compressed temporally by a factor of 5, to a duration of ~11 fs. The experimental results are supported by numerical simulations, showing that both Raman and Kerr effects play a role in the compression dynamics. The convenience of using ambient air, and the absence of glass windows that would distort the compressed pulses, makes the setup highly attractive as the basis of an efficient table-top UV pulse compressor., Comment: 7 pages, 5 figures

The behavior of electromagnetic waves in chirally twisted structures is a topic of enduring interest, dating back at least to the invention in the 1940s of the microwave travelling wave tube amplifier and culminating in contemporary studies of chiral metamaterials, metasurfaces, and photonic crystal fibers (PCFs). Optical fibers with chiral microstructures, drawn from a spinning preform, have many useful properties, exhibiting for example circular birefringence and circular dichroism. It has recently been shown that chiral fibers with N fold rotationally symmetric (symmetry group CN) transverse microstructures support families of helical Bloch modes (HBMs), each of which consists of a superposition of azimuthal Bloch harmonics (or optical vortices). An example is a fiber with N coupled cores arranged in a ring around its central axis (N core single ring fiber). Although this type of fiber can be readily modelled using scalar coupled mode theory, a full description of its optical properties requires a vectorial analysis that takes account of the polarization state of the light particularly important in studies of circular and vortical birefringence. In this paper we develop, using an orthogonal two dimensional helicoidal coordinate system embedded in a cylindrical surface at constant radius, a rigorous vector coupled mode description of the fields using local Frenet Serret frames that rotate and twist with each of the N cores. The analysis places on a firm theoretical footing a previous HBM theory in which a heuristic approach was taken, based on physical intuition of the properties of Bloch waves. We believe this study provides clarity in what can sometimes be a rather difficult field, and will facilitate further exploration of real-world applications of these fascinating waveguiding systems., Comment: 20 pages, 10 figures

High-brightness sources of coherent and few-cycle-duration light waveforms with spectral coverage from the UV to the THz would offer unprecedented versatility and opportunities for a spectacular range of applications from bio-chemical sensing, to time-resolved and nonlinear spectroscopy, to attosecond light-wave electronics. Combinations of various sources with frequency conversion and supercontinuum generation can provide relatively large spectral coverage, but many applications require much broader spectral range and low-jitter synchronization for time-domain measurements. Here, we present a carrier-envelope-phase stable light source, seeded by a mid-IR frequency comb, with simultaneous spectral coverage across 7 optical octaves, from the UV (340 nm) into the THz (40,000 nm). Combining soliton self-compression and dispersive wave generation in an anti-resonant-reflection photonic crystal fibre with intra-pulse difference frequency generation in BaGa2GeSe6, the spectral brightness is 2-5 orders of magnitude above synchrotron sources. This enables high-dynamic-range spectroscopies and provides enticing prospects for attosecond physics and material sciences., Comment: 4 figures

We present a technique that uses noisy broadband pulse bursts generated by modulational instability to probe nonlinear processes, including infrared-inactive Raman transitions, in molecular gases. These processes imprint correlations between different regions of the noisy spectrum, which can be detected by acquiring single shot spectra and calculating the Pearson correlation coefficient between the different frequency components. Numerical simulations verify the experimental measurements and are used to further understand the system and discuss methods to improve the signal strength and the spectral resolution of the technique., Comment: 12 pages, 4 figures

The possibility of performing time-resolved spectroscopic studies in the molecular fingerprinting region or extending the cut-off wavelength of high-harmonic generation has recently boosted the development of efficient mid-infrared ultrafast lasers. In particular, fibre lasers based on active media such as thulium or holmium are a very active area of research since they are robust, compact and can operate at high repetition rates. These systems, however, are still complex, are unable to deliver pulses shorter than 100 fs and are not yet as mature as their near-infrared counterparts. Here we report generation of sub-40 fs pulses at 1.8 microns, with quantum efficiencies of 50% and without need for post-compression, in hydrogen-filled hollow-core photonic crystal fibre pumped by a commercial 300-fs fibre laser at 1030 nm. This is achieved by pressure-tuning the dispersion and avoiding Raman gain suppression by adjusting the chirp of the pump pulses and the proportion of higher order modes launched into the fibre. The system is optimized using a physical model that incorporates the main linear and nonlinear contributions to the optical response. The approach is average power-scalable, permits adjustment of the pulse shape and can potentially allow access to much longer wavelengths., Comment: 9 pages, 10 figures

We report the use of prism-assisted side-coupling to investigate the spatio-temporal dynamics of photoionization in an Ar-filled hollow-core photonic crystal fiber. By launching four different LP core modes we are able to probe temporal and spatial changes in the modal refractive index on timescales from a few hundred picoseconds to several hundred microseconds after the ionization event. We experimentally analyze the underlying gas density waves and find good agreement with quantitative and qualitative hydrodynamic predictions. Moreover, we observe periodic modulations in the MHz-range lasting for a few microseconds, indicating nanometer-scale vibrations of the fiber structure, driven by gas density waves., Comment: 8 pages, 4 figures, peer-reviewed and published

We present a pump-probe technique for monitoring ultrafast polarizability changes. In particular, we use it to measure the plasma density created at the temporal focus of a self-compressing higher-order pump soliton in gas-filled hollow-core photonic crystal fiber. This is done by monitoring the wavelength of the dispersive wave emission from a counter-propagating probe soliton. By varying the relative delay between pump and probe, the plasma density distribution along the fiber can be mapped out. Compared to the recently introduced interferometric side-probing for monitoring the plasma density, our new technique is relatively immune to instabilities caused by air turbulence and mechanical vibration. The results of two experiments on argon- and krypton-filled fiber are presented, and compared to numerical simulations. The technique provides an important new tool for probing photoionization in many different gases and gas mixtures as well as ultrafast changes in dispersion in many other contexts., Comment: 7 pages, 3 figures, peer-reviewed and published

Many fields such as bio-spectroscopy and photochemistry often require sources of vacuum ultraviolet (VUV) pulses featuring a narrow linewidth and tunable over a wide frequency range. However, the majority of available VUV light sources do not simultaneously fulfill those two requirements, and few if any are truly compact, cost-effective and easy to use by non-specialists. Here we introduce a novel approach that goes a long way to meeting this challenge. It is based on hydrogen-filled hollow-core photonic crystal fiber pumped simultaneously by two spectrally distant pulses. Stimulated Raman scattering enables the generation of coherence waves of collective molecular motion in the gas, which together with careful dispersion engineering and control over the modal content of the pump light, facilitates cooperation between the two separate Raman combs, resulting in a spectrum that reaches deep into the VUV. Using this system, we demonstrate the generation of a dual Raman comb of narrowband lines extending down to 141 nm using only 100 mW of input power delivered by a commercial solid-state laser. The approach may enable access to tunable VUV light to any laboratory and therefore boost progress in many research areas across multiple disciplines., Comment: 4 pages, 4 figures

Gas-filled hollow-core photonic crystal fiber (PCF) is used for efficient nonlinear temporal compression of femtosecond laser pulses, two main schemes being direct soliton-effect self-compression, and spectral broadening followed by phase compensation. To obtain stable compressed pulses, it is crucial to avoid decoherence through modulational instability (MI) during spectral broadening. Here we show that changes in dispersion due to spectral anti-crossings between the fundamental core mode and core wall resonances in anti-resonant-guiding hollow-core PCF can strongly alter the MI gain spectrum, enabling MI-free pulse compression for optimized fiber designs. In addition, higher-order dispersion can introduce MI even when the pump pulses lie in the normal dispersion region.

Mode-locked lasers have been widely used to explore interactions between optical solitons, including bound-soliton states that may be regarded as "photonic molecules". Conventional mode-locked lasers can however host at most only a few solitons, which means that stochastic behaviour involving large numbers of solitons cannot easily be studied under controlled experimental conditions. Here we report the use of an optoacoustically mode-locked fibre laser to create hundreds of temporal traps or "reactors" within which multiple solitons can be isolated and controlled both globally and individually. We achieve on-demand synthesis and dissociation of soliton molecules within these parallel reactors, in this way unfolding a novel panorama of diverse dynamics in which the statistics of multi-soliton interactions can be studied. The results are of potential importance in all-optical information processing and in the control of ultrafast pulsed lasers., Comment: 14 pages, 6 figures in main article, 28 pages, 21 figures in supplementary text

The unique ring-shaped intensity patterns and helical phase fronts of optical vortices make them useful in many applications. Here we report for the first time efficient Raman frequency conversion between vortex modes in twisted hydrogen-filled single-ring hollow core photonic crystal fiber (SR-PCF). High fidelity transmission of optical vortices in untwisted SR-PCF becomes more and more difficult as the orbital angular momentum (OAM) order increases, due to scattering at structural imperfections in the fiber microstructure. In helically twisted SR-PCF, however, the degeneracy between left- and right-handed versions of the same mode is lifted, with the result that they are topologically protected from such scattering. With launch efficiencies of ~75%, a high damage threshold and broadband guidance, these fibers are ideal for performing nonlinear experiments that require the polarization state and azimuthal order of the interacting modes to be preserved over long distances. Vortex coherence waves (VCW) of internal molecular motion, carrying angular momentum, are excited in the gas, permitting the polarization and orbital angular momentum of the Raman bands to be tailored, even in spectral regions where conventional solid-core waveguides are opaque or susceptible to optical damage.

Over the past years, ultrafast lasers with average powers in the 100 W range have become a mature technology, with a multitude of applications in science and technology. Nonlinear temporal compression of these lasers to few- or even single-cycle duration is often essential, yet still hard to achieve, in particular at high repetition rates. Here we report a two-stage system for compressing pulses from a 1030 nm ytterbium fiber laser to single-cycle durations with 5 ${\mu}$J output pulse energy at 9.6 MHz repetition rate. In the first stage, the laser pulses are compressed from 340 to 25 fs by spectral broadening in a krypton-filled single-ring photonic crystal fiber (SR-PCF), subsequent phase compensation being achieved with chirped mirrors. In the second stage, the pulses are further compressed to single-cycle duration by soliton-effect self-compression in a neon-filled SR-PCF. We estimate a pulse duration of ~3.4 fs at the fiber output by numerically back-propagating the measured pulses. Finally, we directly measured a pulse duration of 3.8 fs (1.25 optical cycles) after compensating (using chirped mirrors) the dispersion introduced by the optical elements after the fiber, more than 50% of the total pulse energy being in the main peak. The system can produce compressed pulses with peak powers >0.6 GW and a total transmission exceeding 70%.

We report on a highly-efficient experimental scheme for the generation of deep-ultraviolet ultrashort light pulses using four-wave mixing in gas-filled kagom\'e-style photonic crystal fiber. By pumping with ultrashort, few $\mu$J, pulses centered at 400 nm, we generate an idler pulse at 266 nm, and amplify a seeded signal at 800 nm. We achieve remarkably high pump-to-idler energy conversion efficiencies of up to 38%. Although the pump and seed pulse durations are ~100 fs, the generated ultraviolet spectral bandwidths support sub-15 fs pulses. These can be further extended to support few-cycle pulses. Four-wave mixing in gas-filled hollow-core fibres can be scaled to high average powers and different spectral regions such as the vacuum ultraviolet (100-200 nm)., Comment: 4 pages, 5 figures

Efficient monitoring of airborne particulate matter (PM), especially particles with aerodynamic diameter less than 2.5 um (PM2.5), is crucial for improving public health. Reliable information on the concentration, size distribution and chemical characteristics of PMs is key to evaluating air pollution and identifying its sources. Standard methods for PM2.5 characterization require sample collection from the atmosphere and post-analysis using sophisticated equipment in a laboratory environment, and are normally very time-consuming. Although optical methods based on analysis of scattering of free-space laser beams or evanescent fields are in principle suitable for real-time particle counting and sizing, lack of knowledge of the refractive index in these methods not only leads to inevitable sizing ambiguity but also prevents identification of the particle material. In the case of evanescent wave detection, the system lifetime is strongly limited by adhesion of particles to the surfaces. Here we report a novel technique for airborne particle metrology based on hollow-core photonic crystal fibre. It offers in situ particle counting, sizing and refractive index measurement with effectively unlimited device lifetime, and relies on optical forces that automatically capture airborne particles in front of the hollow core and propel them into the fibre. The resulting transmission drop, together with the time-of-flight of the particles passing through the fibre, provide unambiguous mapping of particle size and refractive index with high accuracy. The technique represents a considerable advance over currently available real-time particle metrology systems, and can be directly applied to monitoring air pollution in the open atmosphere as well as precise particle characterization in a local environment such as a closed room or a reaction vessel.

Broadband-tunable sources of circularly-polarized light are crucial in fields such as laser science, biomedicine and spectroscopy. Conventional sources rely on nonlinear wavelength conversion and polarization control using standard optical components, and are limited by the availability of suitably transparent crystals and glasses. Although gas-filled hollow-core photonic crystal fiber provides pressure-tunable dispersion, long well-controlled optical path-lengths, and high Raman conversion efficiency, it is unable to preserve circular polarization state, typically exhibiting weak linear birefringence. Here we report a revolutionary approach based on helically-twisted hollow-core photonic crystal fiber, which displays circular birefringence, thus robustly maintaining circular polarization state against external perturbations. This makes it possible to generate pure circularly-polarized Stokes and anti-Stokes signals by rotational Raman scattering in hydrogen. The polarization state of the frequency-shifted Raman bands can be continuously varied by tuning the gas pressure in the vicinity of the gain suppression point. The results pave the way to a new generation of compact and efficient fiber-based sources of broadband light with fully-controllable polarization state., Comment: 5 pages, 4 figures

Coherent ultraviolet (UV) light has many uses, for example in the study of molecular species relevant in biology and chemistry. Very few if any laser materials offer UV transparency along with damage-free operation at high photon energies and laser power. Here we report efficient generation of deep and vacuum UV light using hydrogen-filled hollow-core photonic crystal fiber (HC-PCF). Pumping above the stimulated Raman threshold at 532 nm, coherent molecular vibrations are excited in the gas, permitting highly efficient thresholdless wavelength conversion in the UV. The system is uniquely pressure-tunable, allows spatial structuring of the out-coupled radiation, and shows excellent performance in the vacuum UV. It can also in principle operate at the single-photon level, when all other approaches are extremely inefficient., Comment: 18 pages: 7 pages main paper, 11 pages supplementary material; 10 figures in total

Dispersive wave emission (DWE) in gas-filled hollow-core dielectric waveguides is a promising source of tuneable coherent and broadband radiation, but so far the generation of few-femtosecond pulses using this technique has not been demonstrated. Using in-vacuum frequency-resolved optical gating, we directly characterise tuneable 3fs pulses in the deep ultraviolet generated via DWE. Through numerical simulations, we identify that the use of a pressure gradient in the waveguide is critical for the generation of short pulses., Comment: 5 pages, 4 figures

Ultrafast broadband ultraviolet radiation is of importance in spectroscopy and photochemistry, since high photon energies enable single-photon excitations and ultrashort pulses allow time-resolved studies. Here we report the use of gas-filled hollow-core photonic crystal fibers (HC-PCFs) for efficient ultrafast nonlinear optics in the ultraviolet. Soliton self-compression of 400 nm pulses of (unprecedentedly low) ~500 nJ energies down to sub-6-fs durations is achieved, as well as resonant emission of tunable dispersive waves from these solitons. In addition, we discuss the generation of a flat supercontinuum extending from the deep ultraviolet to the visible in a hydrogen-filled HC-PCF. Comparisons with argon-filled fibers show that the enhanced Raman gain at high frequencies makes the hydrogen system more efficient. As HC-PCF technology develops, we expect these fiber-based ultraviolet sources to lead to new applications.

We investigate refractive index changes caused by femtosecond photoionization in a gas-filled hollow-core photonic crystal fiber. Using spatially-resolved interferometric side-probing, we find that these changes live for tens of microseconds after the photoionization event - eight orders of magnitude longer than the pulse duration. Oscillations in the megahertz frequency range are simultaneously observed, caused by mechanical vibrations of the thin-walled capillaries surrounding the hollow core. These two non-local effects can affect the propagation of a second pulse that arrives within their lifetime, which works out to repetition rates of tens of kilohertz. Filling the fiber with an atomically lighter gas significantly reduces ionization, lessening the strength of the refractive index changes. The results will be important for understanding the dynamics of gas-based fiber systems operating at high intensities and high repetition rates, when temporally non-local interactions between successive laser pulses become relevant., Comment: 5 pages with four figures and one table

We report a series of experimental, analytical and numerical studies demonstrating strong circular dichroism in helically twisted hollow-core single-ring photonic crystal fiber (SR-PCF), formed by spinning the preform during fiber drawing. In the SR-PCFs studied, the hollow core is surrounded by a single ring of non-touching capillaries. Coupling between these capillaries results in the formation of helical Bloch modes carrying orbital angular momentum. In the twisted fiber, strong circular birefringence appears in the ring, so that when a core mode with a certain circular polarization state (say LC) phase-matches to the ring, the other (RC) is strongly dephased. If in addition the orbital angular momentum is the same in core and ring, and the polarization states are non-orthogonal (e.g., slightly elliptical), the LC core mode will experience high loss while the RC mode is efficiently transmitted. The result is a single-circular-polarization SR-PCF that acts as a circular polarizer over a certain wavelength range. Such fibers have many potential applications, for example, for generating circularly polarized light in gas-filled SR-PCF and realizing polarizing elements in the deep and vacuum ultraviolet.

Binding of particles through weak (non-covalent) interactions plays a central role in multiple modern disciplines, from Cooper pairing of electrons in superconductivity to formation of supramolecules in biochemistry. Optical solitons, which are analogous in many ways to particles, arise from a balance between nonlinearity and dispersion and have only been known to be able to form molecule-like, localized structures through covalent interactions due to direct overlapping. Non-covalent binding of optical solitons that based on long-rang interactions have, however, so far escaped experimental observations. Long-range interactions between optical solitons have proven almost impossible to control, generally leading to disorder. In this paper, however we show that by tailoring weak, long-range soliton interactions, a large population of optical solitons in an optoacoustic mode-locking fiber laser can assemble into stable, highly-ordered structures that resemble biochemical supramolecules. We demonstrate here a theoretical model of the non-covalent binding mechanism, and provide some experimental results supporting this model., Comment: arXiv admin note: substantial text overlap with arXiv:1710.01034

Higher-order modes up to LP$_{33}$ are controllably excited in water-filled kagom\'{e}- and bandgap-style hollow-core photonic crystal fibers (HC-PCF). A spatial light modulator is used to create amplitude and phase distributions that closely match those of the fiber modes, resulting in typical launch efficiencies of 10-20% into the liquid-filled core. Modes, excited across the visible wavelength range, closely resemble those observed in air-filled kagom\'{e} HC-PCF and match numerical simulations. Mode indices are obtained by launching plane-waves at specific angles onto the fiber input-face and comparing the resulting intensity pattern to that of a particular mode. These results provide a framework for spatially-resolved sensing in HC-PCF microreactors and fiber-based optical manipulation.

Laser cooling of mechanical degrees of freedom is one of the most significant achievements in the field of opto-mechanics. Here, we report, for the first time to the best of our knowledge, efficient passive optomechanical cooling of the motion of a freestanding waveguide coupled to a whispering-gallery-mode (WGM) resonator. The waveguide is an 8 mm long glass-fiber nanospike, which has a fundamental flexural resonance at {\Omega}/2{\pi} = 2.5 kHz and a Q-factor of 1.2 10**5. Upon launching 250 {\mu}W laser power at an optical frequency close to the WGM resonant frequency, we observed cooling of the nanospike resonance from room temperature down to 1.8 K. Simultaneous cooling of the first higher-order mechanical mode is also observed. The strong suppression of the overall Brownian motion of the nanospike, observed as an 11.6 dB reduction in its mean square displacement, indicates strong optomechanical stabilization of linear coupling between the nanospike and the cavity mode. The cooling is caused predominantly by a combination of photothermal effects and optical forces between nanospike and WGM resonator. The results are of direct relevance in the many applications of WGM resonators, including atom physics, optomechanics, and sensing., Comment: 13 pages, 7 figures

Backward stimulated Raman scattering in gases provides a promising route to compression and amplification of a Stokes seed-pulse by counter-propagating against a pump-pulse, as has been already demonstrated in various platforms, mainly in free-space. However, the dynamics governing this process when seeded by noise has not yet been investigated in a fully controllable collinear environment. Here we report the first unambiguous observation of efficient noise-seeded backward stimulated Raman scattering in a hydrogen-filled hollow-core photonic crystal fiber. At high gas pressures, when the backward Raman gain is comparable with, but lower than, the forward gain, we report quantum conversion efficiencies exceeding 40% to the backward Stokes at 683 nm from a narrowband 532-nm-pump. The efficiency increases to 65% when the backward process is seeded by a small amount of back-reflected forward-generated Stokes light. At high pump powers the backward Stokes signal, emitted in a clean fundamental mode and spectrally pure, is unexpectedly always stronger than its forward-propagating counterpart. We attribute this striking observation to the unique temporal dynamics of the interacting fields, which cause the Raman coherence (which takes the form of a moving fine-period Bragg grating) to grow in strength towards the input end of the fiber. A good understanding of this process, together with the rapid development of novel anti-resonant-guiding hollow-core fibers, may lead to improved designs of efficient gas-based Raman lasers and amplifiers operating at wavelengths from the ultraviolet to the mid-infrared., Comment: 6 pages and 8 figures in the main section. 4 pages and 5 figures in the supplementary section

Whispering-gallery mode (WGM) resonators combine small optical mode volumes with narrow resonance linewidths, making them exciting platforms for a variety of applications. Here we report a flying WGM microlaser, realized by optically trapping a dye-doped microparticle within a liquid-filled hollow-core photonic crystal fiber (HC-PCF) using a CW laser and then pumping it with a pulsed excitation laser whose wavelength matches the absorption band of the dye. The laser emits into core-guided modes that can be detected at the endfaces of the HC-PCF. Using radiation forces, the microlaser can be freely propelled along the HC-PCF over multi-cm distances - orders of magnitude further than in previous experiments where tweezers and fiber traps were used. The system can be used to measure temperature with high spatial resolution, by exploiting the temperature-dependent frequency shift of the lasing modes, and also for precise delivery of light to remote locations.

Spectral anti-crossings between the fundamental guided mode and core wall resonances alter the dispersion in hollow-core anti-resonant-reflection photonic crystal fibers. Here we study the effect of this dispersion change on the nonlinear propagation and dynamics of ultrashort pulses. We find that it causes emission of narrow spectral peaks through a combination of four-wave mixing and dispersive wave emission. We further investigate the influence of the anti-crossings on nonlinear pulse propagation and show that their impact can be minimized by adjusting the core-wall thickness in such a way that the anti-crossings lie spectrally distant from the pump wavelength., Comment: 5 pages, 5 figures

A stream of optical pulses, transmitted over long distances in optical fiber, will be affected by a variety of noise sources, leading to degradation in the signal-to-noise ratio. This noise accumulation sets generic capacity limits of all fiber-based optical signal transmission systems and has long been regarded as unavoidable. We report that by tailoring long-range, non-covalent inter-pulse interactions, optical solitons in a fiber laser loop can robustly couple to each other and self-assemble into supramolecular structures that exhibit long-term stability, elementary diversity and the possibility of information encoding. We demonstrate error-free transmission of such self-assembled solitonic structures over many astronomical units without any active retiming, opening up the possibility of using bit-bit interactions to overcome noise accumulation in optical fiber telecommunications and bit-storage systems., Comment: 19 pages, 3 figures in main text, 7 figures in supplementary information

Optically levitated micro- and nanoparticles offer an ideal playground for investigating photon-phonon interactions over macroscopic distances. Here we report the observation of long-range optical binding of multiple microparticles, mediated by intermodal scattering and interference inside the evacuated core of a hollow-core photonic crystal fibre (HC-PCF). Three polystyrene particles with 1 {\mu}m diameter are stably bound together with an inter-particle distance of ~40 {\mu}m, or 50 times longer than the wavelength of the trapping laser. The bound-particle array can be translated to-and-fro over centimetre distances along the fibre. When evacuated to 6 mbar gas pressure, the collective mechanical modes of the bound-particle array could be observed. The measured inter-particle distance at equilibrium and mechanical eigen-frequencies are supported by a novel analytical formalism modelling the dynamics of the binding process. The HC-PCF system offers a unique platform for investigating the rich optomechanical dynamics of arrays of levitated particles in a well-isolated and protected environment.

We report a 21-W mid-IR OPCPA that generates 131-{\mu}J and 97 fs (sub-9-cycle) pulses at 160 kHz repetition rate and at a centre wavelength of 3.25 {\mu}m. Pulse-to-pulse stability of the CEP-stable output is excellent with 0.33% rms over 288 million pulses (30 min) and compression close to a single optical cycle was achieved through soliton self- compression inside a gas-filled mid-IR anti-resonant-guiding photonic crystal fibre. Without any additional compression device, stable generation of 14.5 fs (1.35-optical-cycle) pulses was achieved at an average power of 9.6 W. The resulting peak power of 3.9 GW in combination with the near-single-cycle duration and intrinsic CEP stability, make our OPCPA a key-enabling technology for the next generation of extreme photonics, strong-field attosecond research and coherent X-ray science.

Many reports on stimulated Raman scattering in mixtures of Raman-active and noble gases indicate that the addition of a dispersive buffer gas increases the phase-mismatch to higher-order Stokes and antiStokes sidebands, resulting in preferential conversion to the first few Stokes lines, accompanied by a significant reduction in Raman gain due to collisions with buffer gas molecules. Here we report that, provided the dispersion can be precisely controlled, the effective Raman gain in gas-filled hollow-core photonic crystal fiber (PCF) can actually be significantly enhanced when a buffer gas is added. This counterintuitive behavior occurs when the nonlinear coupling between the interacting fields is strong, and can result in a performance similar to that of a pure Raman-active gas, but at much lower total gas pressure, allowing competing effects such as Raman backscattering to be suppressed. We report high modal purity in all the emitted sidebands, along with anti-Stokes conversion efficiencies as high as 5% in the visible and 2% in the ultraviolet. The results point to a new class of gas-based waveguide device in which the pressure-tunable nonlinear optical response is beneficially adjusted by the addition of other gases., Comment: 8 pages, 10 figures, contains supplementary material

Coherent control of the resonant response in spatially extended optomechanical structures is complicated by the fact that the optical drive is affected by the back-action from the generated phonons. Here we report a new approach to coherent control based on stimulated Raman-like scattering, in which the optical pressure can remain unaffected by the induced vibrations even in the regime of strong optomechanical interactions. We demonstrate experimentally coherent control of flexural vibrations simultaneously along the whole length of a dual-nanoweb fiber, by imprinting steps in the relative phase between the components of a two-frequency pump signal,the beat frequency being chosen to match a flexural resonance. Furthermore, sequential switching of the relative phase at time intervals shorter than the lifetime of the vibrations reduces their amplitude to a constant value that is fully adjustable by tuning the phase-modulation depth and switching rate. The results may trigger new developments in silicon photonics, since such coherent control uniquely decouples the amplitude of optomechanical oscillations from power-dependent thermal effects and nonlinear optical loss., Comment: This 11 pages-long document includes the main text with 8 figures and an appendix with one figure

Although ultraviolet (UV) light is important in many areas of science and technology, there are very few if any lasers capable of delivering wavelength-tunable ultrashort UV pulses at MHz repetition rates. Here we report the generation of deep-UV laser pulses at MHz repetition rates and \mu J-energies by means of dispersive wave (DW) emission from self-compressed solitons in gas-filled single-ring hollow-core photonic crystal fiber (SR-PCF). Pulses from an ytterbium fiber laser (~300 fs) are first compressed to ~25 fs in a SR-PCF-based nonlinear compression stage, and subsequently used to pump a second SR-PCF stage for broadband DW generation in the deep UV. The UV wavelength is tunable by selecting the gas species and the pressure. At 100 kHz repetition rate, a pulse energy of 1.05 \mu J was obtained at 205 nm (average power 0.1 W), and at 1.92 MHz, a pulse energy of 0.54 \mu J was obtained at 275 nm (average power 1.03 W).

We report generation of high harmonics in a gas-jet pumped by pulses self-compressed in a He-filled hollow-core photonic crystal fiber through the soliton effect. The gas-jet is placed directly at the fiber output. As the energy increases the ionization-induced soliton blue-shift is transferred to the high harmonics, leading to a emission bands that are continuously tunable from 17 to 45 eV.

We present the results of an experimental and numerical investigation into temporally non-local coherent interactions between ultrashort pulses, mediated by Raman coherence, in gas-filled kagom\'{e}-style hollow-core photonic crystal fiber. A pump pulse first set up the Raman coherence, creating a refractive index grating in the gas that travels at the group velocity of the pump pulse. Varying the arrival time of a second probe pulse allows high degree of control over its evolution as it propagates along the fiber, in particular soliton self-compression and dispersive wave (DW) emission. In the experiments reported, a DW is emitted at ~300 nm, with a central frequency that oscillates with the pump-probe delay. The results demonstrate that strong Raman coherence created in broadband guiding gas-filled kagom\'e-PCF can be used to control the dynamics of ultrashort probe pulses, even in difficult-to-access spectral regions such as the deep and vacuum ultraviolet.

Optimum suppression of higher order modes in single-ring hollow-core photonic crystal fibers (SR-PCFs) occurs when the capillary-to-core diameter ratio d/D = 0.68. Here we report that, in SR-PCFs with sub-optimal values of d/D, higher-order mode suppression can be recovered by spinning the preform during fiber drawing, thus introducing a continuous helical twist. This geometrically increases the effective axial propagation constant (initially too low) of the LP01-like modes of the capillaries surrounding the core, enabling robust single-mode operation. The effect is explored by means of extensive numerical modeling, an analytical model and a series of experiments. Prism-assisted side-coupling is used to investigate the losses and near-field patterns of individual fiber modes in both the straight and twisted cases. More than 12 dB/m improvement in higher order mode suppression is achieved experimentally in a twisted PCF. The measurements also show that the higher order mode profiles change with twist rate, as predicted by numerical simulations. Helical twisting offers an additional tool for achieving effectively endlessly single-mode operation in hollow-core SR-PCFs.

We identify a novel regime of soliton-plasma interactions in which high-intensity ultrashort pulses of intermediate soliton order undergo coherent plasma-induced fission. Experimental results obtained in gas-filled hollow-core photonic crystal fibers are supported by rigorous numerical simulations. The cumulative blueshift of higher-order input solitons with ionizing intensities results in pulse splitting before the ultimate self-compression point, leading to the generation of robust pulse pairs with PHz bandwidths. The novel dynamics closes the gap between plasma-induced adiabatic soliton compression and modulational instability.

We report generation of an ultrafast supercontinuum extending into the mid- infrared in gas-filled single-ring hollow-core photonic crystal fiber (SR-PCF) pumped by 1.7 $\mu$m light from an optical parametric amplifier. The simple fiber structure offers shallow dispersion and flat transmission in the near and mid-infrared, enabling the generation of broadband spectra extending from 300 nm to 3.1 $\mu$m, with a total energy of a few $\mu$J. In addition, we report the emission of ultraviolet dispersive waves whose frequency can be tuned simply by adjusting the pump wavelength. SR-PCF also provides an effective means of compressing and delivering tunable ultrafast pulses in the near and mid-infrared spectral regions., Comment: 7 pages, 4 figures

Gas-filled hollow-core photonic crystal fibre (PCF) is being used to generate ever wider supercontinuum spectra, in particular via dispersive wave (DW) emission in the deep and vacuum ultraviolet, with a multitude of applications. DWs are the result of the resonant transfer of energy from a self-compressed soliton, a process which relies crucially on phase matching. It was recently predicted that, in the strong-field regime, the additional transient anomalous dispersion introduced by gas ionization would allow phase-matched DW generation in the mid-infrared (MIR)-something that is forbidden in the absence of free electrons. Here we report for the first time the experimental observation of such MIR DWs, embedded in a 4.7-octave-wide supercontinuum that uniquely reaches simultaneously to the vacuum ultraviolet, with up to 1.7 W of total average power.

We report a novel technique for launching broadband laser light into liquid-filled hollow-core photonic crystal fiber (HC-PCF). It uniquely offers self-alignment and self-stabilization via optomechanical trapping of a fused silica nanospike, fabricated by thermally tapering and chemically etching a single mode fiber into a tip diameter of 350 nm. We show that a trapping laser, delivering ~300 mW at 1064 nm, can be used to optically align and stably maintain the nanospike at the core center. Once this is done, a broadband supercontinuum beam (~575 to 1064 nm) can be efficiently and close to achromatically launched in the HC-PCF. The system is robust against liquid-flow in either direction inside the HC-PCF and the Fresnel back-reflections are reduced to negligible levels compared to free-space launching or butt-coupling. The results are of potential relevance for any application where the efficient delivery of broadband light into liquid-core waveguides is desired.