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Ionising radiation interactions in matter can trigger a cascade of processes that underpin long-lived damage in the medium. To date, however, a lack of suitable methodologies has precluded our ability to understand the role that material nanostructure plays in this cascade. Here, we use transient photoabsorption to track the lifetime of free electrons (t_c) in bulk and nanostructured SiO2 (aerogel) irradiated by picosecond-scale (10^-12 s) bursts of X-rays and protons from a laser-driven accelerator. Optical streaking reveals a sharp increase in t_c from < 1 ps to > 50 ps over a narrow average density (p_av) range spanning the expected phonon-fracton crossover in aerogels. Numerical modelling suggests that this discontinuity can be understood by a quenching of rapid, phonon-assisted recovery in irradiated nanostructured SiO_2. This is shown to lead to an extended period of enhanced energy density in the excited electron population. Overall, these results open a direct route to tracking how low-level processes in complex systems can underpin macroscopically observed phenomena and, importantly, the conditions that permit them to emerge.

Understanding the interaction of kilojoule, picosecond laser pulse with long-scale length preplasma or homogeneous near critical density (NCD) plasma is crucial for guiding experiments at national short-pulse laser facilities. Using full three-dimensional particle-in-cell simulations, we demonstrate that in this regime, cross-filament stochastic acceleration is an important mechanism that contributes to the production of superponderomotive, high-flux electron beams. Since the laser power significantly exceeds the threshold of the relativistic self-focusing, multiple filaments are generated and can propagate independently over a long distance. Electrons jump across the filaments during the acceleration, and their motion becomes stochastic. We find that the effective temperature of electrons increases with the total interaction time following a scaling like $T_{\rm eff}\propto\tau_{i}^{0.65}$. By irradiating a submillimeter thick NCD target, the space charge of electrons with energy above 2.5 MeV reaches tens of $\mu$C. Such high-flux electrons with superponderomotive energies significantly facilitate applications in high-energy-density science, nuclear science, secondary sources and diagnostic techniques.

Direct laser acceleration (DLA) of electrons in a plasma of near critical electron density (NCD) and associated synchrotron-like radiation are discussed for moderate relativistic laser intensity (the normalized laser amplitude $a_0$ $\leq$ 4.3) and ps-long pulse. This regime is typical for kJ PW-class laser facilities designed for high energy density research. Currently, in experiments at the PHELX laser it was demonstrated that interaction of 10$^{19}$ W/cm$^{2}$ sub-ps laser pulse with sub-mm long NCD plasma results in generation of high-current well-directed super-ponderomotive electrons with effective temperature that is 10$\times$ higher than the ponderomotive potential [O. Rosmej et al., PPCF 62, 115024 (2020)]. Three-dimensional Particle-In-Cell simulations provided a good agreement with the measured electron energy distribution and were used in the current work to study synchrotron radiation of the DLA accelerated electrons. The resulting x-ray spectrum with a critical energy of 5 keV reveals an ultra-high photon number of 7$\times$10$^{11}$ in the 1-30 keV photon energy range at the focused laser energy of 20 J. Numerical simulations of a betatron x-ray phasecontrast imaging based on the DLA process for the parameters of a PHELIX laser is presented. The results are of interest for applications in high energy density (HED) experiments, which require a picosecond x-ray pulse and a high photon flux., Comment: under review at Matter and Radiation at Extremes

Ultra-intense MeV photon and neutron beams are indispensable tools in many research fields such as nuclear, atomic and material science as well as in medical and biophysical applications. For astrophysical applications aimed for laboratory investigations, neutron fluxes in excess of 10$^{21}$ n/(cm$^2$ s) are required. Such ultra-high fluxes are unattainable with existing conventional reactor- and accelerator-based facilities. Currently discussed concepts for generating high-flux neutron beams are based on ultra-high-power multi-petawatt lasers operating at >10$^{23}$ W/cm$^2$ intensities. Here, we present a novel efficient concept for generating $\gamma$ and neutron beams based on enhanced generation of direct laser accelerated electrons in relativistic laser interactions with a long-scale near critical density plasma at 10$^{19}$ W/cm$^{2}$ intensity. New experimental insights in the laser-driven generation of ultra-intense well-directed multi-MeV beams of photons with >10$^{12}$ ph/sr and a ultra-high intense neutron source with >6$\times$10$^{10}$ neutrons per shot are presented. More than 1.4\% laser-to-gamma conversion efficiency above 10 MeV and 0.05\% laser-to-neutron conversion efficiency were recorded, already at moderate relativistic laser intensities and ps pulse duration. This approach promises a strong boost of the diagnostic potential of existing kJ PW laser systems used for ICF research.

We report on new findings in a laser driven enhanced electron beam generation in the multi MeV energy range at moderate relativistic laser intensities and their applications. In our experiment, an intense sub-picosecond laser pulse propagates through a plasma of a near critical electron density (NCD) and direct laser acceleration (DLA) of electrons takes place. The breakthrough toward high current relativistic electron beams became possible due to application of low density polymer foams of sub-mm thickness. In foams, the NCD-plasma was produced by a mechanism of super-sonic ionization. Compared to NCD-plasmas generated by laser irradiation of conventional foils, the DLA acceleration path in foams was strongly enhanced. Measurements resulted into 11{\div}13 MeV of the effective electron temperature and up to 100 MeV maximum of the electron energy measured in the laser pulse propagation direction. The growth of the electron energy was accompanied by a strong increase of the number of super-ponderomotive electrons and a well-defined directionality of the electron beam that propagates in a divergence cone with a half angle of 12{\deg}. For the energy range above 7.5 MeV that is relevant for gamma-driven nuclear reactions, we estimate a charge carried by these well-directed electron beams as high as 50 nC and a corresponding efficiency of the laser energy conversion into electrons of 6%. The electron spectra generated by the DLA-mechanism in NCD-plasma at 1019 Wcm-2 laser intensity were compared with those measured in shots onto conventional metallic foils at ultra-relativistic laser intensities of 1021 Wcm-2 . In the last case, the twice lower effective electron temperature and the twice lower maximum of the electron energy were registered. The substantial difference in the electron spectra for these two cases presented itself in the isotope production yield.

Experiments were performed to study electron acceleration by intense sub-picosecond laser pulses propagating in sub-mm long plasmas of near critical electron density (NCD). Low density foam layers of 300-500 um thickness were used as targets. The NCD-plasma was produced by a mechanism of a super-sonic ionization when a well-defined separate ns-pulse was sent onto the foam-target forerunning the relativistic main pulse. The effect of the relativistic laser pulse channeling and creation of quasi-static azimuthal magnetic and radial electric fields that keeps electrons in the channel ensured effective coupling of the laser energy into energetic electrons. Application of sub-mm thick low density foam layers provided substantial increase of the electron acceleration path in a NCD-plasma compared to the case of freely expanding plasmas created in the interaction of the ns-laser pulse with solid foils. Performed experiments on the electron heating by a 100J, 750 fs short laser pulse of (2-5)x1019 W/cm2 intensity demonstrated that the effective temperature of supra-thermal electrons increased from 1.5-2 MeV, in the case of the relativistic laser interaction with a metallic foil at high laser contrast, up to 13 MeV for the laser shots onto the pre-ionized foam. The observed tendency towards the strong increase of the mean electron energy and the number of ultra-relativistic laser-accelerated electrons is reinforced by the results of gamma-yield measurements that showed a 1000-fold increase of the measured doses. The experiment was supported by the 3D-PIC and FLUKA simulations made for used laser parameters and geometry of the experimental set-up. Both measurements and simulations show high directionality of the acceleration process close to the direction of the laser pulse propagation. The charge of super-ponderomotive electrons with E > 30 MeV reaches a high value of 78nC., Comment: 17 pages, 10 figures

We present experimental evidence of ultra-high energy density plasma states with the keV bulk electron temperatures and near-solid electron densities generated during the interaction of high contrast, relativistically intense laser pulses with planar metallic foils. The bulk electron temperature and density have been measured using x-ray spectroscopy tools; the temperature of supra-thermal electrons traversing the target was determined from measured bremsstrahlung spectra; run-away electrons were detected using magnet spectrometers. The measured electron energy distribution was in a good agreement with results of Particle-in-Cell (PIC) simulations. Analysis of the bremsstrahlung spectra and results on measurements of the run-away electrons showed a suppression of the hot electrons production in the case of the high laser contrast. By application of Ti-foils covered with nm-thin Fe-layers we demonstrated that the thickness of the created keV hot dense plasma does not exceed 150 nm. Results of the pilot hydro-dynamic simulations that are based on a wide-range two-temperature EOS, wide-range description of all transport and optical properties, ionization, electron and radiative heating, plasma expansion, and Maxwell equations (with a wide-range permittivity) for description of the laser absorption are in excellent agreement with experimental results. According to these simulations, the generation of keV-hot bulk electrons is caused by the collisional mechanism of the laser pulse absorption in plasmas with a near solid step-like electron density profile. The laser energy firstly deposited into the nm-thin skin-layer is then transported into the target depth by the electron heat conductivity. This scenario is opposite to the volumetric character of the energy deposition produced by supra-thermal electrons., Comment: 15 pages, 10 figures