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Three volcanic plumes were detected during the Tajogaite volcano eruptive activity (Canary Islands, Spain, September–December 2021) over the Iberian Peninsula. The spatiotemporal evolution of these events is characterised by combining passive satellite remote sensing and ground-based lidar and sun-photometer systems. The inversion algorithm GRASP is used with a suite of ground-based remote sensing instruments such as lidar/ceilometer and sun-photometer from eight sites at different locations throughout the Iberian Peninsula. Satellite observations showed that the volcanic ash plumes remained nearby the Canary Islands covering a mean area of 120 ± 202 km2 during the whole period of eruptive activity and that sulphur dioxide plumes reached the Iberian Peninsula. Remote sensing observations showed that the three events were mainly composed of sulphates, which were transported from the volcano into the free troposphere. The high backscatter-related Ångström exponents for wavelengths 532–1064 nm (1.17 ± 0.20 to 1.40 ± 0.24) and low particle depolarization ratios (0.08 ± 0.02 to 0.09 ± 0.02), measured by the multi-wavelength Raman lidar, hinted at the presence of spherical small particles. The layer aerosol optical depth at 532 nm (AODL532) obtained from lidar measurements contributed between 49% and 82% to the AERONET total column AOD at 532 nm in event II (11–13 October). According to the GRASP retrievals, the layer aerosol optical depth at 440 nm (AODL440) was higher in all sites during event II with values between 0.097 (Badajoz) and 0.233 (Guadiana-UGR) and lower in event III (19–21 October) varying between 0.003 (Granada) and 0.026 (Évora). Compared with the GRASP retrievals of total column AOD at 440 nm, the AODL440 had contributions between 21% and 52% during event II. In the event I (25–28 September), the mean volume concentrations (VC) varied between 5 ± 4 µm3cm-3 (El-Arenosillo/Huelva) and 17 ± 10 µm3cm-3 (Guadiana-UGR), while in event II this variation was from 11 ± 7 µm3cm-3 (Badajoz) to 27 ± 10 µm3cm-3 (Guadiana-UGR). Due to the impact of volcanic events on atmospheric and economic fields, such as radiative forcing and airspace security, a proper characterization is required. This work undertakes it using advanced instrumentation and methods. Évora team funded by national funds through FCT - Fundação para a Ciência e Tecnologia, I.P., in the framework of the ICT project with the references UIDB/04683/2020 and UIDP/04683/2020 and by TOMAQAPA (PTDC/CTAMET/29678/2017). The authors acknowledge the GRASP-ACE (Grant agreement ID: 778349), ACTRIS-IMP (Grant agreement ID:871115), ATMO-ACCESS (Grant Agreement ID: 101008004), PROBE (COST Action number: CA18235), HARMONIA (COST Action number: CA21119), EUMETNET through the E-PROFILE program and REALISTIC (Grant agreement ID:101086690) projects. The authors acknowledge the support through ACTRIS-2 under grant agreement no.654109. This work was partially supported by the Spanish national projects PID2019-103886RB-I00/AEI/10.13039/501100011033, INTEGRATYON3 (PID2020-117825GB-C21 and PID2020-117825GB-C22), ELPIS (PID2020-120015RB-I00), CLARIN (CGL2016-81092-R), ePOLAAR (RTI2018-097864-B-I00), CAMELIA (PID2019-104205GB-C21/AEI/10.13039/501100011033) and ACTRIS-España (CGL2017-90884REDT), by University of Granada Plan Propio through Singular Laboratory (LS2022-1) program, by the Andalusia Autonomous Government projects AEROPRE (P18-RT-3820) and ADAPNE (P20_00136), by the UGR-FEDER projects DEM3TRIOS (A-RNM-430-UGR20) and MOGATRACO (A-RNM-524-UGR20) and partially by the Scientific Units of Excellence Program (grant no. UCE-PP2017-02), and by the R+D+i grant RTI 2018-097332-B-C22 funded by MCIN/AEI/ 10.13039/501100011033/ and “ERDF A Way of Doing Europe”. M.-Á. López-Cayuela and C.V. Carvajal-Pérez are supported by the INTA predoctoral contract program.

This study explores the potential to retrieve aerosol properties with the GRASP algorithm (Generalized Retrieval of Atmosphere and Surface Properties) using as input measurements of zenith sky radiance (ZSR), which are sky radiances measured in the zenith direction, recorded at four wavelengths by a ZEN-R52 radiometer. To this end, the ZSR measured at 440, 500, 675 and 870 nm by a ZEN-R52 (ZSRZEN), installed in Valladolid (Spain), is employed. This instrument is calibrated intercomparing the signal of each channel with coincident ZSR values simulated (ZSRSIM) at the same wavelengths with a radiative transfer model (RTM). These simulations are carried out using the GRASP forward module as RTM and the aerosol information from a collocated CE318 photometer belonging to the AERONET network (Aerosol and Robotic Network) as input. Dark signal and the signal dependence on temperature are characterized and included in the calibration process. The uncertainties on each channel are quantified by an intercomparison with a collocated CE318 photometer, obtaining lower values for shorter wavelengths; between 3 % for 440 nm and 21 % for 870 nm. The proposed inversion strategy for the aerosol retrieval using the ZSRZEN measurements as input, so-called GRASP-ZEN, assumes the aerosol as an external mixture of five pre calculated aerosol types. A sensitivity analysis is conducted using synthetic ZSRZEN measurements, pointing out that these measurements are sensitive to aerosol load and type. It also assesses that the retrieved aerosol optical depth (AOD) values in general overestimates the reference ones by 0.03, 0.02, 0.02 and 0.01 for 440, 500, 675, 870 nm, respectively. The calibrated ZSRZEN measurements, recorded during two and half years at Valladolid, are inverted by GRASP-ZEN strategy to retrieve some aerosol properties like AOD. The retrieved AOD shows a high correlation with respect independent values obtained from the collocated AERONET CE318 photometer, with a determination coefficient (r2) about 0.86, 0.85, 0.79 and 0.72 for 440, 500, 675 and 870 nm, respectively, and finding uncertainties between 0.02 and 0.03 with respect to the AERONET values. Finally, it is studied the goodness of other retrieved aerosol properties like aerosol volume concentration for total, fine and coarse modes.

Durante la erupción del volcán de Cumbre Vieja, en la isla de La Palma en 2021, la Agencia Estatal de Meteorología (AEMET), en calidad de Servicio Nacional y Autoridad Meteorológica del Estado, prestó diferentes servicios de apoyo al Comité Científico y al Comité Asesor del Plan de Emergencias Volcánicas de Canarias (PEVOLCA). Parte de sus actividades abarcaron la vigilancia y predicción meteorológica, la monitorización y predicción del transporte del penacho volcánico, y la valoración del impacto de las emisiones de gases y cenizas de la erupción volcánica en la calidad del aire en la isla de La Palma y en la región de Canarias.