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1. New synthetic routes toward enantiopure nitrogen donor ligands

Author

Sala, Xavier, Rodriquez, Anna M., Rodriguez, Montserrat, Romero, Isabel, Parella, Teodor, von Zelewsky, Alexander, Llobet, Antoni, and Benet-Buchholz, Jordi

Subjects
Chemical synthesis -- Analysis, Chirality -- Research, Styrene -- Structure, Styrene -- Chemical properties, X-ray crystallography -- Observations, Biological sciences, Chemistry
Abstract

The preparation of new polypyridylic chiral ligands having either [C.sub.3] or lower symmetry via a de novo construction of the pyridine nucleus by means of Krohnke methodology is presented. The preliminary catalytic results performed with the Ru complex (-)-21 show moderate enantioselectivities in styrene epoxidation with PhI[(AcO).sub.2].

Published
2006

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