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The number of intense wildfires may increase in the upcoming years as a consequence of climate change. Changing aerosol conditions may lead to changes in regional and global cloud and precipitation pattern. One key aspect of research is presently whether or not wildfire smoke particles can initiate ice nucleation. We found strong evidence that aged smoke particles (dominated by organic aerosol particles) originating from wildfires in North America triggered significant ice nucleation at temperatures from−47 to −53°C and caused the formation of extended cirrus layers. Our study is based on lidar observations over Limassol, Cyprus, from 27 October to 3 November 2020 when extended wildfire smoke fields crossed the Mediterranean Basin from Portugal to Cyprus. The observations suggest that the ice crystals were nucleated just below the tropopause in the presence of smoke particles serving as ice-nucleating particles (INPs). The main part of the 2-3 km thick smoke layer was,however, in the lower stratosphere just above the tropopause. With actual radiosonde observations of temperature and relative humidity and lidar-derived smoke particle surface area concentrations as starting values, gravity wave simulations show that lofting by 90-180 m is sufficient to initiate significant ice nucleation on the smoke particles, expressed in ice crystal number concentrations of 1-100 L−1 The authors acknowledge the ‘EXCELSIOR’: ERATOSTHENES: EXcellence reseacrh Centre for Earth Surveillance and Space-Based Monitoring of the Environment H2020 Widespread Teaming project (www.excelsior2020.eu). The ‘EXCELSIOR’ project has received funding from the European Union’s Horizon 2020 research and innovation programme under Grant Agreement No 857510, from the Government of the Republic of Cyprus through the Directorate General for the European Programmes, Coordination and Development and the Cyprus University of Technology. The authors acknowledge support through the European Research Infrastructure for the observation of Aerosol, Clouds and Trace Gases ACTRIS under grant agreement no. 654109 and 739530 from the European Union’s Horizon 2020 research and innovation programme. The PollyXT-CYP was funded by the German Federal Ministry of Education and Research (BMBF) via the PoLiCyTa project (grant no. 1LK1603A).The study is supported by “ACCEPT” project (Prot. No: LOCALDEV-0008) co-financed by the Financial Mechanism of Norway (85%) and the Republic of Cyprus (15%) in the framework of the programming period 2014 - 2021. The lidar analysis on smoke-cirrus interaction was further supported by BMBF funding of the SCiAMO project (MOSAIC-FKZ 03F0915A). DAK acknowledges support by U.S. Department of Energy’s (DOE) Atmospheric System Research (ASR) program, Office of Biological and Environmental Research (OBER) (grant no. DE-SC0021034).

Fires are a widespread ecological factor since ancient times. It has a negative impact not only on the environment but on the economy, society and people. A forest fire can lead to a change in land surface, the destruction of large areas of vegetation and soil erosion. As a result, the economy is negatively affected, the balance of ecosystems is disturbed, and the flora, fauna and natural beauty are destructed. Also, biomass burning smoke affects air quality due to the large quantities of trace gases and aerosol particles that are emitted, leading to global climate change and playing a significant role in troposphere chemistry. A fundamental tool for forest fire management is the science of remote sensing. Remote sensing is commonly used for mapping burnt areas as well as for studying the effects of fire incidents and this statement is very well supported by the literature at local, regional and global levels. This study is mainly focused on burned area mapping and damage assessment on land surface and atmosphere for the case of the Arakapas fire in Cyprus. For the purposes of this study, the satellite images acquired from Sentinel-2 were used for the burnt area mapping and the fire severity estimation based on the dNBR (difference Normalized Burn Ratio) spectral index, and the Corine land cover was used for the assessment of the vegetation type that was disturbed. This event considered one of the largest in recent years is explored using data from Sentinel-5P, where carbon monoxide product is studied in the region affected by the fires. Furthermore, on the morning of the 5th of July, due to the change of wind direction, the smoke travelled from the centre of the island to the southwest, and it was detected by the multiwavelength Raman lidar, installed in Limassol. Thus, the optical properties of the smoke plume retrieved from the lidar are presented. The PollyXT-CYP lidar system of the ECoE, observed multiple layers between 500m and 2.5km with depolarization ratio of 5-8% and lidar ratio of 75sr for the upper layers.For the purposes of this study, the image processing was performed using custom scripts in the GEE (Google Earth Engine) platform with the JavaScript programming interface. The area affected by the fire was calculated to be ~40Km2. The spatial distribution map of the dNBR was classified according to the USGS fire severity levels, where high dNBR values indicate a more severe fire and values near zero and negative values indicate unburned and/or decreased vegetation after the fire. AcknowledgementsThe authors acknowledge the 'EXCELSIOR': ERATOSTHENES: Excellence Research Centre for Earth Surveillance and Space-Based Monitoring of the Environment H2020 Widespread Teaming project (www.excelsior2020.eu). The 'EXCELSIOR' project has received funding from the European Union's Horizon 2020 research and innovation programme under Grant Agreement No 857510, from the Government of the Republic of Cyprus through the Directorate General for the European Programmes, Coordination and Development and the Cyprus University of Technology.

The presence of aerosol and clouds constitutes one of the highest uncertainties regarding the energy budget of the Earth. Therefore, their continuous observation can help reduce these uncertainties, by providing more information about aerosol-cloud interactions and how these atmospheric components contribute to climate change.To study the properties of aerosols and clouds, new infrastructure will soon be set up in Cyprus by the Eratosthenes Centre of Excellence, which was recently established through the ‘EXCELSIOR’ H2020 Widespread Teaming Project. Eratosthenes Centre of Excellence is a digital innovation hub for Earth Observation, Space Technology and Geospatial Information, aiming to become the reference centre in the East Mediterranean, north Africa and the Middle East (EMMENA region). The infrastructure will be installed in Limassol, on the south coast of the island. Apart from the fact that the site is less than 2 km from the island’s coastline, this location is extremely important in terms of the regional atmospheric composition, as the air masses affecting the site originate from the surrounding areas of EMMENA, as well as from south-eastern Europe.Infrastructure to sample aerosol is already represented by a state-of-the-art PollyXT lidar, with measurements being registered continuously since October 2020. By the end of 2023, a similar LACROS multi-instrument platform will be available for the continuous monitoring of clouds and aerosols. This new ground-based remote sensing platform consists of a 35GHz cloud radar, a ceilometer, a microwave radiometer, a Doppler lidar, and a disdrometer. The infrastructure will be integrated into the Cyprus Atmospheric Remote Sensing Observatory (CARO).An example of the value of the observations about cloud formation and the role of aerosol in the process of cloud formation that will be provided from the site in Limassol, can be reflected in the data collected during the CyCARE campaign, executed between October 2016 and March 2018, during which similar ground-based infrastructure was deployed. The authors acknowledge the ‘EXCELSIOR’: ERATOSTHENES: EΧcellence Research Centre for Earth Surveillance and Space-Based Monitoring of the Environment H2020 Widespread Teaming project (www.excelsior2020.eu). The ‘EXCELSIOR’ project has received funding from the European Union’s Horizon 2020 research and innovation programme under Grant Agreement No 857510, from the Government of the Republic of Cyprus through the Directorate General for the European Programmes, Coordination and Development and the Cyprus University of Technology.

In the summer of 2021, several wildfires were reported in the south of Turkey, fires that are considered one of the worst in the history of Turkey. Due to atmospheric conditions, the smoke plume travelled south between 27 July to 5 August 2021, and smoke layers arrived above Cyprus. In this work, the capabilities of the newly established ERATOSTHENES Centre of Excellence (CoE), to study large-scale atmospheric events is presented. The study is based on the synergistic use of different datasets of remote sensing techniques both from ground and space. The EARLINET multiwavelength-Raman-polarization lidar PollyXT-CYP hosted by the ERATOSTHENES CoE is continuously running since October 2020 in Limassol, and during summer 2021, the lidar observed smoke plumes from these extreme wildfires on the south coast of Turkey. The PollyXT-CYP is a key research infrastructure of the Cyprus Atmospheric Remote Sensing Observatory (CARO) of the ERATOSTHENES CoE established through the EXCELSIOR H2020 EU Teaming project coordinated by the Cyprus University of Technology. CARO will consist of two high-tech containers housing the PollyXT-CYP lidar and state-of-the art doppler lidar, cloud radar and radiometric equipment which will be used to measure the air quality, the dust transport, and the cloud properties over Cyprus. The CARO is a planning National Facility of the Republic of Cyprus for Aerosol and Cloud Remote Sensing Observations. Land cover information which shows the type of burned vegetation is used together with satellite products to capture additionally the burned area and to investigate the carbon monoxide of the smoke plume. The study is focusing on the optical characteristics of the plume, as it was detected by the PollyXT-CYP lidar at Limassol. An intense fresh smoke layer was detected on 28-29 July 2021, at an altitude between 2.5 to 4.0 km, having a volume depolarization ratio of ~15% at 355n and ~20% at 532nm, and lidar ratio of 75-80sr at 355nm and 65-70sr at 532nm. Acknowledgements The authors acknowledge the ‘EXCELSIOR’: ERATOSTHENES: EΧcellence Research Centre for Earth Surveillance and Space-Based Monitoring of the Environment H2020 Widespread Teaming project (www.excelsior2020.eu). The ‘EXCELSIOR’ project has received funding from the European Union’s Horizon 2020 research and innovation programme under Grant Agreement No 857510, from the Government of the Republic of Cyprus through the Directorate General for the European Programmes, Coordination and Development and the Cyprus University of Technology. The PollyXT-CYP was funded by the German Federal Ministry of Education and Research (BMBF) via the PoLiCyTa project (grant no. 01LK1603A). The study is supported by “ACCEPT” project (Prot. No: LOCALDEV-0008) co-financed by the Financial Mechanism of Norway (85%) and the Republic of Cyprus (15%) in the framework of the programming period 2014 - 2021.

This paper presents a collection of lidar-derived aerosol intensive optical properties for several aerosol types, namely the particle linear depolarization ratio, the extinction-to-backscatter ratio (lidar ratio) and the Ångström exponent. The data collection, named DeLiAn, is based on globally distributed, long-term, ground-based, multiwavelength, Raman and polarization lidar measurements, conducted mainly with lidars that have been developed at the Leibniz Institute for Tropospheric Research. The intensive optical properties are presented at two wavelengths, 355 and 532 nm, for 13 aerosol categories. The categories cover the basic aerosol types (i.e., marine, pollution, continental European background, volcanic ash, smoke, mineral dust), as well as the most frequently observed mixtures they form. This extensive collection also incorporates more peculiar aerosol categories, including dried marine aerosol that, compared to marine aerosol, exhibits a significantly enhanced depolarization ratio (up to 15 %). Besides Saharan dust, additional mineral dust types related to their source region were identified due to their lower lidar ratios (Central Asian and Middle Eastern dust). In addition, extreme wildfire events (such as in north America and Australia) emitted smoke into the stratosphere showing significantly different optical properties, i.e., high depolarization values (up to 25 %), compared to tropospheric smoke. The data collection reflects and underlines the variety of aerosol mixtures in the atmosphere and can be used for the development of aerosol-typing schemes. The paper contains the most up-to-date and comprehensive overview of optical properties from aerosol lidar measurements and, therefore, provides a solid basis for future aerosol retrievals in the frame of both spaceborne and ground-based lidars. Furthermore, DeLiAn can assist the efforts for the harmonization of satellite records of aerosol properties performed at different wavelengths.

Recent studies have shown that the Eastern Mediterranean and the Middle East are regions strongly affected by climate change, with a rate of warming two times faster than the global average. While climate change comes with major implications, including the fact that severe storms will become more virulent and more often, studies showed that the annual number of cyclones in the Mediterranean region tends to remain constant in the near future, with no visible trend. In this paper, we are studying the trends for convective indices in the region of Cyprus, with modelled, and also observational data. For the modelled data, we are using the CORDEX dataset for convective potential energy and convective inhibition with 3h temporal resolution, for the historical period (1971 - 2000), and for the near future (2021 - 2050), from which we extracted the daily maximum and mean values. Observational data is used from the ESWD database, reports on tornadoes, hail and heavy rain, together with radiosonde data from Athalassa station (radiosonde available in high-resolution mode from 2016, with two launches per day, at 05:00 and 11:00 UTC). Using the Python packages SHARPpy and MetPy we computed the convective indices from radiosounding data. It is estimated that two tornadoes and three waterspouts occur each year in Cyprus, and in a study from 2006 describing two tornadoes outbreaks from January 2003 and January 2004, these events had CAPE index 411 J/kg and 210 J/kg, and respectively lifted index of -2 and 0. The authors acknowledge the ‘EXCELSIOR’: ERATOSTHENES: EΧcellence Research Centre for Earth Surveillance and Space-Based Monitoring of the Environment H2020 Widespread Teaming project (www.excelsior2020.eu). The ‘EXCELSIOR’ project has received funding from the European Union’s Horizon 2020 research and innovation programme under Grant Agreement No 857510, from the Government of the Republic of Cyprus through the Directorate General for the European Programmes, Coordination and Development and the Cyprus University of Technology.

The purpose of this study is to investigate the ability of the Sentinel-5P TROPOspheric Monitoring Instrument (TROPOMI) to derive accurate geometrical features of lofted aerosol layers, selecting the Mediterranean Basin as the study area. Comparisons with ground-based correlative measurements constitute a key component in the validation of passive and active satellite aerosol products. For this purpose, we use ground-based observations from quality-controlled lidar stations reporting to the European Aerosol Research Lidar Network (EARLINET). An optimal methodology for validation purposes has been developed and applied using the EARLINET optical profiles and TROPOMI aerosol products, aiming at the in-depth evaluation of the TROPOMI aerosol layer height (ALH) product for the period 2018 to 2022 over the Mediterranean Basin. Seven EARLINET stations were chosen, taking into consideration their proximity to the sea, which provided 63 coincident aerosol cases for the satellite retrievals. In the following, we present the first validation results for the TROPOMI/S5P ALH using the optimized EARLINET lidar products employing the automated validation chain designed for this purpose. The quantitative validation at pixels over the selected EARLINET stations illustrates that the TROPOMI ALH product is consistent with the EARLINET lidar products, with a high correlation coefficient R = 0.82 (R = 0.51) and a mean bias of -0.51 +/- 0.77 km and -2.27 +/- 1.17 km over ocean and land, respectively. Overall, it appears that aerosol layer altitudes retrieved from TROPOMI are systematically lower than altitudes from the lidar retrievals. High-albedo scenes, as well as low-aerosol-load scenes, are the most challenging for the TROPOMI retrieval algorithm, and these results testify to the need to further investigate the underlying cause. This work provides a clear indication that the TROPOMI ALH product can under certain conditions achieve the required threshold accuracy and precision requirements of 1 km, especially when only ocean pixels are included in the comparison analysis. Furthermore, we describe and analyse three case studies in detail, one dust and two smoke episodes, in order to illustrate the strengths and limitations of the TROPOMI ALH product and demonstrate the presented validation methodology. The present analysis provides important additions to the existing validation studies that have been performed so far for the TROPOMI S5P ALH product, which were based only on satellite-to-satellite comparisons., "Panhellenic Infrastructure for Atmospheric Composition and Climate Change" project MIS 5021516, European Commission European Space Agency European Commission, SIROCCO project EXCELLENCE/1216/0217, AQ-SERVE project - Republic of Cyprus INTEGRATED/0916/0016, European Commission, Federal Ministry of Education & Research (BMBF), EU H2020 EXCELSIOR project, European Research Council (ERC) under Community's Horizon 2020 research and innovation framework programme (ERC) 725698

Due to its geographical location, Cyprus is often affected by dust storms arriving from the largest deserts of the planet, the Sahara, the Arabian Peninsula and the Syrian. In order to characterize dust properties, the Cyprus Atmospheric Observatory (CAO) and the Unmanned Research Laboratory (USRL) of the Cyprus Institute (CYI), in collaboration with the Cyprus Atmospheric Remote sensing Observatory (CARO) of the ERATOSTHENES Centre of Excellence (ECoE) of the Cyprus University of Technology (CUT), performed a research campaign in Fall 2021. Measurements were performed with ground-based aerosol remote sensing systems (lidars, ceilometers and sunphotometers), and UAV based in-situ instruments (OPCs, backscatter sondes, and impactors able to collect dust samples). As part of the remote sensing observations, two depolarized lidars performed measurements from different locations, one from CYI premises in Nicosia and the second one from ECoE-CUT premises in Limassol. The lidar signals provide information about the vertical aerosol profile at the two locations, which can be used to derive the optical properties of dust at different altitudes. Here, we will present first results on the synergy between the continuous vertically extended measurements of lidars and the in-situ measurements from UAV instrumentation during the periods of dust outbreaks. Two dust events occurred from 25 October to 1 November and from 13 to 18 November 2021. During these dust events, the lidars observed depolarized aerosol layers from ground up to 5 km above sea level. The lidar measurements provided the temporal and spatial development of these dust layers, and were also used in real-time for planning the UAV flight schedule. According to backward trajectory analyses, the two dust events had different origins with the first arriving from the Sahara and the second one from the Middle East.

Cyprus focuses on increasing the share of its renewable energy resources from 13.9% in 2020 to 22.9% in 2030, with solar energy exploitation systems to be one of the main pillars of this effort, due to the high solar potential of the island. In this study, we investigated the effect of clouds as well as aerosols, and especially dust, on the downwelling surface solar irradiation in terms of Global Horizontal Irradiation (GHI) and Direct Normal Irradiation (DNI). In order to quantify the effects of clouds, aerosols and dust on different surface solar radiation components, we used the synergy of satellite derived products for clouds, high quality and fine resolution satellite retrievals of aerosols and dust from the newly developed MIDAS dataset, and radiative transfer modeling (RTM). GHI and DNI climatologies have been also developed based on the above information. According to our findings, clouds attenuate ~25 – 30% of annual GHI and 35 – 50% of annual DNI, aerosols attenuate 5 – 10% and 15 – 35% respectively, with dust being responsible for 30 – 50% of the overall attenuation by aerosols. The outcomes of this study are useful for installation planning and for estimating the PV and CSP performance on a short-term future basis, helping towards improved penetration of solar energy exploitation systems in the electric grid of Cyprus. Furthermore, they are strongly linked to Affordable and Clean Energy (SDG 7) which has a central role in national climate plans and requires services in energy meteorology, climate applications of satellite data, and providing high quality wind and radiation data. AcknowledgementsThis study was funded by the EuroGEO e-shape (grant agreement No 820852) and EXCELSIOR (grant agreement No 857510)

A new generation PollyXT lidar system start on 27th of October 2020, continuous operation, at Limassol, Cyprus.The lidar system will become a key component within the EXCELSIOR H2020 EU Teaming project coordinated by the Cyprus University of Technology. The mission of the EXCELSIOR project is to upgrade the Remote Sensing & Geo-Environment Lab, established within the Faculty of Engineering & Technology of the Cyprus University of Technology, into a sustainable, viable and autonomous Centre of Excellence, called the ERATOSTHENES Center of Excellence (ECoE).The PollyXT-CYP will be hosted by the ERATOSTHENES CoE for its permanent operation aiming to link the Centre to ACTRIS and PollyNet. Its task will be to document the complex mixture of the different aerosol species and clouds over the Eastern Mediterranean.The system is continuously running and since the first observations in Limassol, PollyXT-CYP demostrates the complex aerosol conditions over Cyprus. For eaxample, between the 27th of October to the 1st of November 2020, the lidar observed smoke plumes from the extreme wildfires on the west coast of the U.S. The smoke travelled over the Atlantic Ocean and triggered the heterogenous ice formation at the height of 10km. Saharan dust was also detected between 2-5km and liquid clouds were formed on the top of the dust layer.In this study we will present selected cases of unique atmospheric structures from the first months of continuous operation over Cyprus as well as optical and geometrical properties of the aerosol layers.The PollyXT-CYP will be a key research infrastructure of the Cyprus Atmospheric Remote Sensing Observatory (CARO). CARO will consist of two high-tech containers housing the PollyXT-CYP lidar and state-of-the art doppler lidar, cloud radar and radiometric equipment which will be used to measure the air quality, the dust transport, and the cloud properties over Cyprus. The CARO is planned to become National Facility of the Republic of Cyprus for Aerosol and Cloud Remote Sensing Observations.AcknowledgementsThe authors acknowledge the EXCELSIOR project that received funding from the European Union [H2020-WIDESPREAD-04-2017:Teaming Phase2] project under grant agreement no. 857510, and from the Republic of Cyprus. CUT team acknowledge the Research and Innovation Foundation of Cyprus for the financial support through the SIROCCO (EXCELLENCE/1216/0217) and AQ-SERVE (INTERGRATED/0916/0016) projects. The PollyXT-CYP was funded by the German Federal Ministry of Education and Research (BMBF) via the PoLiCyTa project.

Atmospheric mineral dust has a rich tri-dimensional spatial and temporal structure that is poorly constrained in forecasts and analyses when only column-integrated aerosol optical depth (AOD) is assimilated. At present, this is the case of most operational global aerosol assimilation products. Aerosol vertical distributions obtained from space-borne lidars can be assimilated in aerosol models, but questions about the extent of their benefit upon analyses and forecasts along with their consistency with AOD assimilation remain unresolved. Our study thoroughly explores the added value of assimilating space-borne vertical dust profiles, with and without the joint assimilation of dust optical depth (DOD). We also discuss the consistency in the assimilation of both sources of information and analyse the role of the smaller footprint of the space-borne lidar profiles upon the results. To that end, we have performed data assimilation experiments using dedicated dust observations for a period of two months over Northern Africa, the Middle East and Europe. We assimilate DOD derived from VIIRS/SUOMI-NPP Deep Blue, and for the first time CALIOP-based LIVAS pure-dust extinction coefficient profiles on an aerosol model. The evaluation is performed against independent ground-based DOD derived from AERONET Sun photometers and ground-based lidar dust extinction profiles from field campaigns (CyCARE and Pre-TECT). Jointly assimilating LIVAS and Deep Blue data reduces the root mean square error (RMSE) in the DOD by 39 % and in the dust extinction coefficient by 65 % compared to a control simulation that excludes assimilation. We show that the assimilation of dust extinction coefficient profiles provides a strong added value to the analyses and forecasts. When only Deep Blue data are assimilated the RMSE in the DOD is reduced further, by 42 %. However, when only LIVAS data are assimilated the RMSE in the dust extinction coefficient decreases by 72 %, the largest improvement across experiments. We also show that the assimilation of dust extinction profiles yields better skill scores than the assimilation of DOD under equivalent sensor footprint. Our results demonstrate the strong potential of future lidar space missions to improve desert dust forecasts, particularly if they foresee a depolarization lidar channel to allow discriminating desert dust from other aerosol types.

Depolarization ratio is a valuable parameter for lidar-based aerosol categorization. Usually, aerosol particle depolarization ratio is determined at relatively short wavelengths of 355 nm and/or 532 nm, but some multi-wavelength studies including longer wavelengths indicate strong spectral dependency. Here, we investigate the capabilities of Halo Photonics Stream Line Doppler lidars to retrieve the particle linear depolarization ratio at 1565 nm wavelength. We utilize collocated measurements with another lidar system, PollyXT at Limassol, Cyprus, and at Kuopio, Finland, to compare the depolarization ratio observed by the two systems. For mineral dust-dominated cases we find typically a little lower depolarization ratio at 1565 nm than at 355 nm and 532 nm. However, for dust mixed with other aerosol we find higher depolarization ratio at 1565 nm. For polluted marine aerosol we find marginally lower depolarization ratio at 1565 nm compared to 355 nm and 532 nm. For mixed spruce and birch pollen we find a little higher depolarization ratio at 1565 nm compared to 532 nm. Overall, we conclude that Halo Doppler lidars can provide particle linear depolarization ratio at 1565 nm wavelength at least in the lowest 2–3 km above ground.

Remote sensing measurements of aerosols using depolarization Raman Lidar systems from 4 EARLINET (European Aerosol research Lidar Network) stations are used for a comprehensive analysis of Saharan dust events over the Mediterranean basin in the period 2014–2017. In this period, we selected to study 51 dust events regarding the geometrical, optical and microphysical properties of dust particles, classifying them and assessing their radiative forcing effect on the atmosphere. From West to East, the stations of Granada, Potenza, Athens and Limassol were selected as representative Mediterranean cities regularly affected by Saharan dust intrusions. Emphasis was given on lidar measurements in the visible (532 nm) and specifically on the consistency of the particle linear depolarization ratio (δp532), the extinction-to-backscatter lidar ratio (LR532) and the Aerosol Optical Thickness (AOT532) within the observed dust layers. We found mean δp532 values of 0.24 ± 0.05, 0.26 ± 0.06, 0.28 ± 0.05 and 0.28 ± 0.04, mean LR532 values of 52 ± 8 sr, 51 ± 9 sr, 52 ± 9 sr and 49 ± 6 sr, and mean AOT532 values of 0.40 ± 0.31, 0.11 ± 0.07, 0.12 ± 0.10 and 0.32 ± 0.17, for Granada, Potenza, Athens and Limassol, respectively. The mean layer thickness values were found to range from ~1700 to ~3400 m. Additionally, based also on a previous aerosol type classification scheme provided by airborne High Spectral Resolution Lidar (HSRL) observations and on air mass backward trajectory analysis, a clustering analysis was performed in order to identify the major mixing aerosol types over the studied area. Furthermore, a synergy of lidar measurements and modeling was used to deeply analyze the solar and thermal radiative forcing of airborne dust. In total, a cooling behavior in the solar range and a significantly lower heating behavior in the thermal range was estimated. Depending on the dust optical and geometrical properties, the load intensity and the solar zenith angle (SZA), the estimated solar radiative forcing values range from −59 to −22 W m−2 at the surface and from −24 to −1 W m−2 at the top of the atmosphere (TOA). Similarly, in the thermal spectral range these values range from +2 to +4 W m−2 for the surface and from +1 to +3 W m−2 for the TOA. Finally, the radiative forcing seems to be inversely proportional to the dust mixing ratio, since higher absolute values are estimated for less mixed dust layers.

The Mediterranean Basin is well recognized by IPCC as a hot spot for climate change. Severe consequences are expected for the future in the Eastern Mediterranean, the Middle East and North Africa (EMMENA) region.The increased urbanization, high pollution, dust storms and decreasing precipitation in the region dramatically affect climate change. Current prediction models for weather, climate, and environment are based on sophisticated modeling in close connection with state-of-the-art observations.A modern observational super-site in Cyprus is of fundamental importance to understanding the atmospheric system in the EMMENA region. The presence of such a super site will be able to effectively monitor atmospheric conditions and provide relevant data for atmospheric prediction modeling.This contribution reports on the recent progress regarding the buildup of a permanent, state-of-the-art atmospheric remote sensing station in Limassol, Cyprus. Through the EU H2020 Teaming project EXCELSIOR, the ERATOSTHENES Centre of Excellence (ECoE) will be established as a Centre of Excellence for Earth Surveillance and Space-Based Monitoring of the Environment.The ECoE modern in-situ observational super site will be established in Cyprus for long-term profiling of the atmosphere, including wind, humidity, aerosol and cloud properties and precipitation fields. The ECoE will be fully in line with ESFRI networks, such as ACTRIS, as it will utilize state-of-the-art infrastructure and techniques to provide cutting-edge data regarding atmospheric processes.As a demonstration initiative, an 18-month field campaign (Cy-CARE (Cyprus Cloud Aerosol and pRecipitation Experiment)) has been designed by the Leibniz Institute for Tropospheric Research (TROPOS) and was implemented by the ERATOSTHENES group at Cyprus University of Technology (CUT) between October 2016 and March 2018, with the main focus on lidar/radar-based studies of aerosol-cloud-precipitation relationships. Case studies of the Cy-CARE campaign will be presented to demonstrate the importance of the ground based atmospheric remote sensing observations in the region.AcknowledgementsThe authors acknowledge the EXCELSIOR project that received funding from the European Union [H2020-WIDESPREAD-04-2017:Teaming Phase2] project under grant agreement no. 857510, and from the Republic of Cyprus. CUT team acknowledge ACTRIS-2 project (H2020-INFRAIA-2014-2015, GA no. 654109) and the Research and Innovation Foundation of Cyprus for the financial support through the SIROCCO (EXCELLENCE/1216/0217) and AQ-SERVE (INTERGRATED/0916/0016) projects.

Cyprus is strategically located in the region of the Eastern Mediterranean, the Middle East and North Africa (EMMENA). As a crossroad between Europe, Asia and Africa, it is representative of meteorological conditions and coastal areas in the EMMENA region.Incomplete coverage with ground monitoring stations is the main limitation to make fast and significant progress in understanding the complex climate-relevant atmospheric processes around the globe and thus to improve atmospheric models used for climate change projections and extreme weather predictions. Although satellites can continuously monitor the atmosphere on a regional to global scale, they must be ground-calibrated and validated in order to incorporate satellite data into atmospheric models.Cyprus, and especially Limassol as a coastal city, can be considered an ideal natural laboratory for advanced and comprehensive field studies on climate change, aerosol-cloud-dynamics-precipitation interaction, and the weather-precipitation-dryness complex, providing additionally valuable ground truthing observations for satellite missions.The vision of the ERATOSTHENES Research Centre (ERC) in Cyprus is to become a Centre of Excellence for Earth Surveillance and Space-Based Monitoring of the Environment, in the framework of the EU H2020 Teaming project EXCELSIOR. Within this vision, a modern observational super site in Cyprus is of fundamental importance and will be build up for long-term profiling of the atmosphere (wind, humidity, aerosol and cloud properties, precipitation fields), in one of the hot spots of climate change increasing extreme weather events.The ERATOSTHENES station in Limassol, Cyprus with the current instrumentation (EARLINET Raman depolarization lidar) follows the CAL/VAL activities of the AEOLUS satellite launched August 2018 through the participation to the VADAM project. Selected cases that demonstrate the complex aerosol and meteorological conditions over Eastern Mediterranean will be presented as well as lidar observations during AEOLUS overpasses over Cyprus.AcknowledgementsThe authors acknowledge the EXCELSIOR H2020-WIDESPREAD-04-2017: Teaming Phase2 project under grant agreement No 857510, ACTRIS and the ESA AEOLUS CAL/VAL VADAM project (27409). CUT team acknowledge Research and Innovation Foundation for the financial support through the SIROCCO (EXCELLENCE/1216/0217) and AQ-SERVE (INTERGRATED/0916/0016) projects.

The Mediterranean region is a unique area characterized by a large spectrum of atmospheric phenomena, some of which have a high impact on many aspects of human activities, safety and wellbeing. The area is long considered as a hot spot of such atmospheric phenomena deserving multidisciplinary scientific attention. The scientific research that has been carried out on these high impact atmospheric processes that occur in the Mediterranean area is indeed widespread and the available international literature is very extensive. The paper touches initially the temperature and precipitation regimes, followed by a discussion of floods and droughts. The exciting cyclogenetic patterns of explosive cyclones and medicanes are presented in separate sections. The lightning activity and the presence of dust and other pollutants are also presented herein. The atmospheric chemistry of the region which is increasingly becoming of utmost importance for the area under study is distinctly discussed. Attempts to modify the weather (the precipitation, in particular) are outlined too. The effects of climatic change on various atmospheric processes are considered throughout this paper, in addition to a dedicated section on temperature and precipitation.

For the first time, a closure study of the relationship between ice-nucleating particle concentration (INPC) and ice crystal number concentration (ICNC) in altocumulus and cirrus layers, solely based on ground-based active remote sensing, is presented. Such aerosol-cloud closure experiments are required (a) to better understand aerosol-cloud interaction in the case of mixed-phase clouds, (b) to explore to what extend heterogeneous ice nucleation can contribute to cirrus formation which is usually controlled by homogeneous freezing, and (c) to check the usefulness of available INPC parameterization schemes, applied to lidar profiles of aerosol optical and microphysical properties up to tropopause level. The INPC-vs-ICNC closure studies were conducted in Cyprus (Limassol and Nicosia) during a six-week field campaign in March–April 2015 and during the 17-month CyCARE (Cyprus Clouds Aerosol and Rain Experiment) campaign. Focus is on altocumulus and cirrus layers which developed in pronounced Saharan dust layers at heights from 5–11 km. Cloud top temperatures ranged from −20 °C to −57 °C. INPC was estimated from polarization/Raman lidar observations in combination with published INPC parameterization schemes for immersion and deposition nucleation. ICNC was estimated from combined Doppler lidar, aerosol lidar, and cloud radar observations of the terminal velocity of falling ice crystals, radar reflectivity and lidar backscatter in combination with modeling of backscattering at 532 nm and 8.5 mm wavelength. Good to acceptable agreement between INPC (observed before and after the occurrence of the cloud layer under investigation) and ICNC values was found in three proof-of-concept closure experiments. In these case studies, INPC and ICNC values matched within an order of magnitude (i.e., within the uncertainty ranges of the INPC and ICNC estimates), and ranged from 0.1–10 per liter in the altocumulus layers and 1–50 per liter in the cirrus layers observed between 8–11 km height.

We present the first attempt of a closure experiment regarding the relationship between ice nucleating particle concentration (INPC) and ice crystal number concentration (ICNC), solely based on active remote sensing. The approach combines aerosol and cloud observations with polarization lidar, Doppler lidar, and cloud radar. Several field campaigns were conducted on the island of Cyprus in the Eastern Mediterranean from 2015-2018 to study heterogeneous ice formation in altocumulus and cirrus layers embedded in Saharan dust. A case study observed on 10 April 2017 is discussed in this contribution.

Four years (2010–2013) of observations with polarization lidar and sun/sky photometer at the combined European Aerosol Research Lidar Network (EARLINET) and Aerosol Robotic Network (AERONET) site of Limassol (34.7° N, 33° E), Cyprus, were used to compare extinction-to-backscatter ratios (lidar ratios) for desert dust from Middle East deserts and the Sahara. In an earlier article, we analyzed one case only and found comparably low lidar ratios < 40 sr for Middle East dust. The complex data analysis scheme is presented. The quality of the retrieval is checked within a case study by comparing the results with respective Raman lidar solutions for particle backscatter, extinction, and lidar ratio. The applied combined lidar/photometer retrievals corroborate recent findings regarding the difference between Middle East and Saharan dust lidar ratios. We found values from 43–65 sr with a mean (±standard deviation) of 53 ± 6 sr for Saharan dust and from 33–48 sr with a mean of 41 ± 4 sr for Middle East dust for the wavelength of 532 nm. The presented data analysis, however, also demonstrates the difficulties in identifying the optical properties of dust even during outbreak situations in the presence of complex aerosol mixtures of desert dust, marine particles, fire smoke, and anthropogenic haze.

A novel procedure has been developed to retrieve, simultaneously, the optical, microphysical and chemical properties of tropospheric aerosols with a multi-wavelength Raman lidar system in the troposphere over an urban site (Athens, Greece: 37.9° N, 23.6° E, 200 m a.s.l.) using data obtained during the European Space Agency (ESA) THERMOPOLIS project, which took place between 15–31 July 2009 over the Greater Athens Area (GAA). We selected to apply our procedure for a case study of intense aerosol layers that occurred on 20–21 July 2009. The National Technical University of Athens (NTUA) EOLE 6-wavelength Raman lidar system has been used to provide the vertical profiles of the optical properties of aerosols (extinction and backscatter coefficients, lidar ratio) and the water vapor mixing ratio. An inversion algorithm was used to derive the mean aerosol microphysical properties (mean effective radius (reff), single-scattering albedo ω) and mean complex refractive index (m)) at selected heights in the 2–3 km height region. We found that reff was 0.14–0.4 (±0.14) μm, ω was 0.63–0.88 (±0.08) (at 532 nm) and m ranged from 1.44 (±0.10) + 0.01 (±0.01)i to 1.55 (±0.12) + 0.06 (±0.02)i, in good agreement (only for the reff values) with in situ aircraft measurements. The water vapor and temperature profiles were incorporated into the ISORROPIA II model to propose a possible in situ aerosol composition consistent with the retrieved m and ω values. The retrieved aerosol chemical composition in the 2–3 km height region gave a variable range of sulfate (0–60%) and organic carbon (OC) content (0–50%), although the OC content increased (up to 50%) and the sulfate content dropped (up to 30%) around 3 km height; the retrieved low ω value (0.63), indicates the presence of absorbing biomass burning smoke mixed with urban haze. Finally, the retrieved aerosol microphysical properties were compared with column-integrated sun photometer CIMEL data.

Proceedings of SPIE - The International Society for Optical Engineering, 2017, Volume 10429, Article number 1042906 The aim of this article is to present the importance of a permanent state-of-the-art atmospheric remote sensing ground based station in the region of the Eastern Mediterranean and Middle East (EMME). The Eratosthenes Research Centre (ERC) with the vision to become a Centre of Excellence for Earth Surveillance and Space-Based Monitoring of the Environment (EXCELSIOR H2020: Teaming project) already operates (within Phase 1) a fully established EARLINETt-Cloudnet supersite at Limassol, Cyprus, for a period of 2 years, in close collaboration with the German Leibniz Institute for Tropospheric Research (TROPOS), The scientific aspects of this prototype-like field campaign CyCARE (Cyprus Cloud Aerosol and Rain Experiment) - a common initiative between the Cyprus University of Technology (CUT), Limassol and TROPOS- are presented in this paper. Cy-CARE has been designed by TROPOS and CUT to fill a gap in the understanding of aerosol-cloud interaction in one of the key regions of climate change and how precipitation formation is influenced by varying aerosol/pollution and meteorological conditions The guiding questions are: How may rain patterns change in future and what may be the consequences of climate change in arid regions such as EMME. EXCELSIOR is a team effort between CUT (acting as the coordinator), the German Aerospace Centre (DLR), the Institute for Astronomy and Astrophysics Space Applications and Remote Sensing of the National Observatory of Athens (NOA), TROPOS and the Cyprus Department of Electronic Communications of the Ministry of Transport, Communications and Works (DEC-MTCW) who will work together to improve the network structures significantly, resulting in Cyprus being regarded as a cornerstone of a European Network of active remote sensing of the atmosphere.

We applied the recently introduced polarization lidar–photometer networking (POLIPHON) technique for the first time to triple-wavelength polarization lidar measurements at 355, 532, and 1064 nm. The lidar observations were performed at Barbados during the Saharan Aerosol Long-Range Transport and Aerosol-Cloud-Interaction Experiment (SALTRACE) in the summer of 2014. The POLIPHON method comprises the traditional lidar technique to separate mineral dust and non-dust backscatter contributions and the new, extended approach to separate even the fine and coarse dust backscatter fractions. We show that the traditional and the advanced method are compatible and lead to a consistent set of dust and non-dust profiles at simplified, less complex aerosol layering and mixing conditions as is the case over the remote tropical Atlantic. To derive dust mass concentration profiles from the lidar observations, trustworthy extinction-to-volume conversion factors for fine, coarse, and total dust are needed and obtained from an updated, extended Aerosol Robotic Network sun photometer data analysis of the correlation between the fine, coarse and total dust volume concentration and the respective fine, coarse, and total dust extinction coefficient for all three laser wavelengths. Conversion factors (total volume to extinction) for pure marine aerosol conditions and continental anthropogenic aerosol situations are presented in addition. As a new feature of the POLIPHON data analysis, the Raman lidar method for particle extinction profiling is used to identify the aerosol type (marine or anthropogenic) of the non-dust aerosol fraction. The full POLIPHON methodology was successfully applied to a SALTRACE case and the results are discussed. We conclude that the 532 nm polarization lidar technique has many advantages in comparison to 355 and 1064 nm polarization lidar approaches and leads to the most robust and accurate POLIPHON products.

Four-year observations (2010–2014) with EARLINET polarization lidar and AERONET sun/sky photometer at Limassol (34.7° N, 33° E), Cyprus, were used to study the soil dust content in lofted fire smoke plumes advected from Turkey. This first systematic attempt to characterize less than 3-day-old smoke plumes in terms of particle linear depolarization ratio (PDR), measured with lidar, contributes to the more general effort to properly describe the life cycle of free-tropospheric smoke–dust mixtures from the emission event to phases of long-range transport (> 4 days after emission). We found significant PDR differences with values from 9 to 18% in lofted aerosol layers when Turkish fires contributed to the aerosol burden and of 3–13 % when Turkish fires were absent. High Ångström exponents of 1.4–2.2 during all these events with lofted smoke layers, occurring between 1 and 3 km height, suggest the absence of a pronounced particle coarse mode. When plotted vs. travel time (spatial distance between Limassol and last fire area), PDR decreased strongly from initial values around 16–18% (1 day travel) to 4–8% after 4 days of travel caused by deposition processes. This behavior was found to be in close agreement with findings described in the literature. Computation of particle extinction coefficient and mass concentrations, derived from the lidar observations, separately for fine-mode dust, coarse-mode dust, and non-dust aerosol components show extinction-related dust fractions on the order of 10% (for PDR =4%, travel times > 4 days) and 50% (PDR =15%, 1 day travel time) and respective mass-related dust fractions of 25% (PDR =4%) to 80% (PDR =15%). Biomass burning should therefore be considered as another source of free tropospheric soil dust.

The polarization-lidar photometer networking (POLIPHON) method for separating dust and non-dust aerosol backscatter and extinction, volume, and mass concentration is extended to allow for a height-resolved separation of fine-mode and coarse-mode dust properties in addition. The method is applied to a period with complex aerosol layering of fine-mode background dust from Turkey and Arabian desert dust from Syria. The observation was performed at the combined European Aerosol Research Lidar Network (EARLINET) and Aerosol Robotic Network (AERONET) site of Limassol (34.7° N, 33° E), Cyprus, in September 2011. The dust profiling methodology and case studies are presented. Consistency between the column-integrated optical properties obtained with sun/sky photometer and the respective results derived by means of the new lidar-based method corroborate the applicability of the extended POLIPHON version.

[1] Compared to typical values of 50–60 sr of the extinction-to-backscatter ratio (lidar ratio) at 532 nm of western Saharan mineral dust, low dust lidar ratios from 33.7±6.7 to 39.1±5.1 sr were derived from polarization lidar observations at Limassol, Cyprus (34°N, 33°E) during an outbreak of Arabian dust mainly from Syria in September 2011, indicated by particle linear depolarization ratios up to 28%–35%. The applied new polarization-lidar/photometer method for the extraction of the dust-related lidar-ratio information from the lidar data is outlined, and the results of the dust outbreak which lasted over several days are discussed. The results confirm an Aerosol Robotic Network photometer study on Arabian dust lidar ratios.

The extreme dust storm that affected Middle East and the Eastern Mediterranean in September 2015 resulted in record-breaking dust loads over Cyprus with aerosol optical depth exceeding 5.0 at 550 nm. We analyze this event using profiles from the European Aerosol Research Lidar Network (EARLINET), the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO), geostationary observations from the Meteosat Second Generation – Spinning Enhanced Visible and Infrared Imager (MSG-SEVIRI) and high resolution simulations with the Regional Atmospheric Modeling System (RAMS). The analysis reveals the main mechanisms that resulted in the generation and persistence of the dust cloud over Middle-East and Cyprus. A combination of meteorological and surface processes is found: (a) the development of a thermal low at the area of Syria that results in unstable atmospheric conditions and dust mobilization at this area; (b) the convective activity over North Iraq that triggers the formation of a westward moving haboob that merges with the previously elevated dust layer; and (c) the changes in land use due to war at the areas of North Iraq and Syria that enhances dust erodibility.

An unusually strong dust outbreak towards Cyprus occurred in September 2015. Mass concentrations exceeding 10 000 μg/m3 were estimated from visibility studies at Limassol (visibilities around 500 m on 8 September). Surprisingly, dust transport models failed to predict this record dust event. We present MODIS products (aerosol optical thickness AOT), surface PM10 observations, visibility studies, and lidar profiling results (covering the main dust period from 7–11 September 2015). Vertical aerosol layering was dominated by a two-layer structure with layers from the ground to 1500 m and from about 1500–3500 m height. The maximum dust AOT reached probably values between 6–10 and was higher than 1 over Cyprus for more than three days. Dust particle extinction coefficients (532 nm) and mass concentrations up to 1300 Mm−1 and 2700 μg/m3, respectively, were observed with lidar in the elevated layers on 7 September, when first dense dust plumes crossed the EARLINET lidar station at Limassol. Raman lidar retrievals yield typical Middle East dust lidar ratios of 35–45 sr at 532 nm. The 532 nm particle linear depolarization ratio assumed values around 0.3.

A global vertically resolved aerosol data set covering more than 10 years of observations at more than 20 measurement sites distributed from 63° N to 52° S and 72° W to 124° E has been achieved within the Raman and polarization lidar network PollyNET. This network consists of portable, remote-controlled multiwavelength-polarization-Raman lidars (Polly) for automated and continuous 24/7 observations of clouds and aerosols. PollyNET is an independent, voluntary, and scientific network. All Polly lidars feature a standardized instrument design with different capabilities ranging from single wavelength to multiwavelength systems, and now apply unified calibration, quality control, and data analysis. The observations are processed in near-real time without manual intervention, and are presented online at http://polly.tropos.de/. The paper gives an overview of the observations on four continents and two research vessels obtained with eight Polly systems. The specific aerosol types at these locations (mineral dust, smoke, dust-smoke and other dusty mixtures, urban haze, and volcanic ash) are identified by their Ångström exponent, lidar ratio, and depolarization ratio. The vertical aerosol distribution at the PollyNET locations is discussed on the basis of more than 55 000 automatically retrieved 30 min particle backscatter coefficient profiles at 532 nm as this operating wavelength is available for all Polly lidar systems. A seasonal analysis of measurements at selected sites revealed typical and extraordinary aerosol conditions as well as seasonal differences. These studies show the potential of PollyNET to support the establishment of a global aerosol climatology that covers the entire troposphere.

A strong Saharan dust event that occurred over the city of Athens, Greece (37.9° N, 23.6° E) between 27 March and 3 April 2009 was followed by a synergy of three instruments: a 6-wavelength Raman lidar, a CIMEL sun-sky radiometer and the MODIS sensor. The BSC-DREAM model was used to forecast the dust event and to simulate the vertical profiles of the aerosol concentration. Due to mixture of dust particles with low clouds during most of the reported period, the dust event could be followed by the lidar only during the cloud-free day of 2 April 2009. The lidar data obtained were used to retrieve the vertical profile of the optical (extinction and backscatter coefficients) properties of aerosols in the troposphere. The aerosol optical depth (AOD) values derived from the CIMEL ranged from 0.33–0.91 (355 nm) to 0.18–0.60 (532 nm), while the lidar ratio (LR) values retrieved from the Raman lidar ranged within 75–100 sr (355 nm) and 45–75 sr (532 nm). Inside a selected dust layer region, between 1.8 and 3.5 km height, mean LR values were 83 ± 7 and 54 ± 7 sr, at 355 and 532 nm, respectively, while the Ångström-backscatter-related (ABR355/532) and Ångström-extinction-related (AER355/532) were found larger than 1 (1.17 ± 0.08 and 1.11 ± 0.02, respectively), indicating mixing of dust with other particles. Additionally, a retrieval technique representing dust as a mixture of spheres and spheroids was used to derive the mean aerosol microphysical properties (mean and effective radius, number, surface and volume density, and mean refractive index) inside the selected atmospheric layers. Thus, the mean value of the retrieved refractive index was found to be 1.49( ± 0.10) + 0.007( ± 0.007)i, and that of the effective radiuses was 0.30 ± 0.18 μm. The final data set of the aerosol optical and microphysical properties along with the water vapor profiles obtained by Raman lidar were incorporated into the ISORROPIA II model to provide a possible aerosol composition consistent with the retrieved refractive index values. Thus, the inferred chemical properties showed 12–40% of dust content, sulfate composition of 16–60%, and organic carbon content of 15–64%, indicating a possible mixing of dust with haze and smoke. PM10 concentrations levels, PM10 composition results and SEM-EDX (Scanning Electron Microscope-Energy Dispersive X-ray) analysis results on sizes and mineralogy of particles from samples during the Saharan dust transport event were used to evaluate the retrieval.

We propose a new iterative algorithm for the retrieval of the microphysical properties of stratospheric and tropospheric aerosols from multiwavelength lidar data. We consider the basic equation as an ill-posed problem and solve the system derived from spline collocation via a Padé iteration. The algorithm takes special care of the fact that the reconstruction of the distribution via spline collocation is very sensitive to the choice of base points of the chosen spline basis. The algorithm makes use of this fact by changing the base points used for the spline collocation at certain iteration steps. In addition, the effects of projection to ensure a nonnegative solution are examined. We tested how well this and other algorithms are suitable for retrieving the complex refractive index of the particles as well. We also examine whether the algorithm is capable of distinguishing between different, very small imaginary parts of the refractive index, which is often a main problem in practice. Finally, the algorithm is applied to real multiwavelength Raman lidar data and our results are partially validated by the thermodynamic chemical model Isorropia II.

An investigation of the Planetary Boundary Layer (PBL) height evolution over Greece, during the solar eclipse of 29 March 2006, is presented. Ground based observations were carried out using lidar detection and ranging devices (Lidars) and ground meteorological instruments, to estimate the height of the Mixing Layer (ML) before, during and after the solar eclipse in Northern and Southern parts of Greece exhibiting different sun obscuration. Data demonstrate that the solar eclipse has induced a decrease of the PBL height, indicating a suppression of turbulence activity similar to that during the sunset hours. The changes in PBL height were associated with a very shallow entrainment zone, indicating a significant weakening of the penetrative convection. Heat transfer was confined to a thinner layer above ground. The thickness of the entrainment zone exhibited its minimum during the maximum of the eclipse, demonstrative of turbulence mechanisms suppression at that time. Model estimations of the PBL evolution were additionally conducted using the Comprehensive Air Quality Model with extensions (CAMx) coupled with the Weather Research and Forecasting model (WRF). Model diagnosed PBL height decrease during the solar eclipse due to vertical transport decay, in agreement with the experimental findings; vertical profiles of atmospheric particles and gaseous species showed an important vertical mixing attenuation.

Marine Spatial Planning (MSP), which is in concept similar to land-use planning, is a public process by which the relevant Member State’s authorities analyse and organise human activities in marine areas to achieve ecological, economic and social objectives. MSP aims to promote sustainable growth of maritime economies, sustainable development of marine areas and sustainable use of marine resources. This paper highlights the importance of MSP and provides basic outcomes of the main European marine development. The already successful MSP plans can provide useful feedback and guidelines for other countries that are in the process of implementation of an integrated MSP, such as Cyprus. This paper presents part of the MSP project, of which 80% funded by the European Regional Development Fund (ERDF) and 20% from national contribution. An overview of the project is presented, including data acquisition, methodology and preliminary results for the implementation of MSP in Cyprus.

Mixing height is one of the key parameters in describing lower tropospheric dynamics, and capturing the diurnal variability is crucial, especially in interpreting surface observations. In this paper we introduce a method for identifying mixing heights below the vertical minimum range of a scanning Doppler lidar. The method we propose is based on velocity variance in low elevation angle conical scanning, and is applied to measurements in two very different coastal environments: Limassol, Cyprus during summer; and Loviisa, Finland during winter. At both locations, the new method agrees well with mixing heights derived from turbulent kinetic energy dissipation rate profiles obtained from vertically-pointing measurements. The low-level scanning routine frequently indicated non-zero mixing heights less than 100 m above the surface. Such low mixing heights were more common at wintertime Loviisa on the Baltic Sea coast than during summertime in Mediterranean Limassol.

The eruption of the Icelandic volcano Eyjafjallajökull in April–May 2010 represents a "natural experiment" to study the impact of volcanic emissions on a continental scale. For the first time, quantitative data about the presence, altitude, and layering of the volcanic cloud, in conjunction with optical information, are available for most parts of Europe derived from the observations by the European Aerosol Research Lidar NETwork (EARLINET). Based on multi-wavelength Raman lidar systems, EARLINET is the only instrument worldwide that is able to provide dense time series of high-quality optical data to be used for aerosol typing and for the retrieval of particle microphysical properties as a function of altitude. In this work we show the four-dimensional (4-D) distribution of the Eyjafjallajökull volcanic cloud in the troposphere over Europe as observed by EARLINET during the entire volcanic event (15 April–26 May 2010). All optical properties directly measured (backscatter, extinction, and particle linear depolarization ratio) are stored in the EARLINET database available at http://www.earlinet.org. A specific relational database providing the volcanic mask over Europe, realized ad hoc for this specific event, has been developed and is available on request at http://www.earlinet.org. During the first days after the eruption, volcanic particles were detected over Central Europe within a wide range of altitudes, from the upper troposphere down to the local planetary boundary layer (PBL). After 19 April 2010, volcanic particles were detected over southern and south-eastern Europe. During the first half of May (5–15 May), material emitted by the Eyjafjallajökull volcano was detected over Spain and Portugal and then over the Mediterranean and the Balkans. The last observations of the event were recorded until 25 May in Central Europe and in the Eastern Mediterranean area. The 4-D distribution of volcanic aerosol layering and optical properties on European scale reported here provides an unprecedented data set for evaluating satellite data and aerosol dispersion models for this kind of volcanic events., The financial support for EARLINET by the European Union under grant RICA 025991 in the Sixth Framework Programme is gratefully acknowledged. Since 2011 EARLINET has been integrated in the ACTRIS Research Infrastructure Project supported by the European Union Seventh Framework Programme (FP7/2007-2013) under grant agreement no. 262254. The authors acknowledge the ESA financial support under the ESRIN contract 21769/08/I-OL and 22202/09/I-EC. Additional financial support has been received from the Andalusia Regional Government through project P10-RNM-6299 and from the Spanish Ministry of Science and Technology through projects CGL2010-18782, and CSD2007-00067.

The potential of spaceborne lidar to monitor aerosol layering and mixing with high vertical resolution is reviewed. An overview is presented on aerosol lidar techniques of past, present, and future NASA and ESA lidar missions. The potential of a standard backscatter lidar (LITE, 1994), a backscatter/ polarization lidar (CALIPSO, since 2006), a polarization High Spectral Resolution Lidar (HSRL, ATLID, EARTHCARE), and of a multiwavelength polarization HSRL are discussed regarding their ability to derive height profiles of optical and microphysical properties of aerosols and to resolve aerosol types and mixtures as a function of height. The important role of ground-truth activities is emphasized. Measurement examples taken with ground-based lidars illustrate that these systems provide a detailed characterization of complex aerosol scenarios in contrast to the snapshot-like observations with spaceborne lidars.

We present first retrievals of the Lidar-Radiometer Inversion Code (LIRIC), applied on combined lidar and sunphotometer data during a Saharan dust episode over Athens, Greece, on July 20, 2011. A full lidar dataset in terms of backscatter signals at 355, 532 and 1064 nm, as well as depolarization at 532 nm was acquired from the European Aerosol Research Network (EARLINET) station of Athens and combined with Aerosol Robotic Network (AERONET) data, in order to retrieve the concentration and extinction coefficient profiles of dust. The lidar measurements showed a free tropospheric layer between 1-5 km above Athens, with low Ångström exponent of ~0.5 and high particle depolarization ratio, ~25-30%, both values characteristic of dust particles. The application of LIRIC revealed high concentration profiles of non-spherical coarse particles in the layer, in the range of 0.04-0.07 ppb and a smaller fine particle component with concentrations of ~0.01 ppb. The extinction coefficients at 532 nm ranged between 50 and 90 Mm-1 for coarse non-spherical particles and between 25 and 50Mm-1 for fine particles. The retrievals were compared with modeled dust concentration and extinction coefficient profiles from the Dust Regional Atmospheric Modeling (BSC-DREAM8b), showing good agreement, especially for the coarse mode

Vertical profiles of the optical (extinction and backscatter coefficients, lidar ratio and Ångström exponent), microphysical (mean effective radius, mean refractive index, mean number concentration) and geometrical properties as well as the mass concentration of volcanic particles from the Eyjafjallajökull eruption were retrieved at selected heights over Athens, Greece, using multi-wavelength Raman lidar measurements performed during the period 21–24 April 2010. Aerosol Robotic Network (AERONET) particulate columnar measurements along with inversion schemes were initialized together with lidar observations to deliver the aforementioned products. The well-known FLEXPART (FLEXible PARTicle dispersion model) model used for volcanic dispersion simulations is initiated as well in order to estimate the horizontal and vertical distribution of volcanic particles. Compared with the lidar measurements within the planetary boundary layer over Athens, FLEXPART proved to be a useful tool for determining the state of mixing of ash with other, locally emitted aerosol types. The major findings presented in our work concern the identification of volcanic particles layers in the form of filaments after 7-day transport from the volcanic source (approximately 4000 km away from our site) from the surface and up to 10 km according to the lidar measurements. Mean hourly averaged lidar signals indicated that the layer thickness of volcanic particles ranged between 1.5 and 2.2 km. The corresponding aerosol optical depth was found to vary from 0.01 to 0.18 at 355 nm and from 0.02 up to 0.17 at 532 nm. Furthermore, the corresponding lidar ratios (S) ranged between 60 and 80 sr at 355 nm and 44 and 88 sr at 532 nm. The mean effective radius of the volcanic particles estimated by applying inversion scheme to the lidar data found to vary within the range 0.13–0.38 μm and the refractive index ranged from 1.39+0.009i to 1.48+0.006i. This high variability is most probably attributed to the mixing of aged volcanic particles with other aerosol types of local origin. Finally, the LIRIC (LIdar/Radiometer Inversion Code) lidar/sunphotometric combined inversion algorithm has been applied in order to retrieve particle concentrations. These have been compared with FLEXPART simulations of the vertical distribution of ash showing good agreement concerning not only the geometrical properties of the volcanic particles layers but also the particles mass concentration.

WebAir-2 EUREKA project aims to expand the basic air quality modelling technology (web-based client server) developed in E!3266 WebAir project. WebAir-2 will incorporate different technologies such as satellite remote sensing data and ground PM samples for monitoring air pollution and in addition 3G mobile phone technology will be used for personalized health related information, warnings and exposure reports. Emphasis will be given to the development of statistical models for PM against AOT derived from MODIS data. Due to inadequate spatial-temporal coverage of air pollution from existing air pollution stations, MODIS products can assist to this task both spatial and temporal. The statistical AOT model will be cross-validated during satellite overpass based on handheld sun-photometers and daily CIMEL sun-photometer (NASA/AERONET network) measurements. Moreover ground LIDAR measurements for vertical distribution of the aerosols will be carried out. Based on these data, a 3D nested grid Eurelian model CAMx will be used to generate the dynamic boundary conditions for the Cyprus model domain.

A strong dust event over Abastumani, Georgia, during May 2009 was studied using light detection and ranging (lidar), satellite and sun photometric measurements. High aerosol optical depth (AOD) values (0.45-0.57) at 500 nm were measured over the closest Aerosol Robotic Network (AERONET) site (Erdemli, Turkey), whereas over Georgia, the AOD measured by the Moderate Resolution Imaging Spectroradiometer (MODIS) was about 0.9 at 550 nm. The AERONET data analysis showed a mean aerosol effective radius of about 2.5 μm, whereas the mean value of the Ångström exponent (α) (wavelength pair 440/870 nm) was smaller than 1, indicating the dominance of large aerosols. The aerosol lidar over Abastumani showed the existence of a strong particle load from the near ground up to a height of 3.5 km. The BSC-DREAM8b forecast model showed that the dust aerosols travelled from the Saharan and the Arabic deserts to the studied area, even reaching southern Russia, covering a total distance of about 5500 km, in the height region from about 2 to 11.5 km.

At the end of August 2009, wild fires ravaged the north-eastern fringes of Athens destroying invaluable forest wealth of the Greek capital. In this work, the impact of these fires on the air quality of Athens and surface radiation levels is examined. Satellite imagery, smoke dispersion modeling and meteorological data confirm the advection of smoke under cloud-free conditions over the city of Athens. Lidar measurements showed that the smoke plume dispersed in the free troposphere and lofted over the city reaching heights between 2 and 4 km. Ground-based sunphotometric measurements showed extreme aerosol optical depth, reaching nearly 6 in the UV wavelength range, accompanied by a reduction up to 70% of solar irradiance at ground. The intensive aerosol optical properties, namely the Angstrom exponent, the lidar ratio, and the single scattering albedo, showed typical values for highly absorbing fresh smoke particles. In-situ air quality measurements revealed the impact of the smoke plume down to the surface with a slight delay on both the particulate and gaseous phase. Surface aerosols increase was encountered mainly in the fine mode with prominent elevation of OC and EC levels. Photochemical processes, studied via NO x titration of O3, were also shown to be different compared to typical urban photochemistry.

The influence of Saharan dust on the air quality of Southern European big cities became a priority during the last decade. The present study reports results on PM(10) monitored at an urban site at 14 m above ground level during an intense Saharan dust transport event. The elemental composition was determined by Energy Dispersive X-ray Fluorescence Spectrometry (EDXRF) for 12 elements: Si, Al, Fe, K, Ca, Mg, Ti, S, Ni, Cu, Zn and Mn. PM(10) concentrations exceeded the EU limit (50 μg/m(3)) several times during the sampling period. Simultaneous maxima have been observed for the elements of crustal origin. The concentrations of all the elements presented a common maximum, corresponding to the date where the atmosphere was heavily charged with particulate matter permanently for an interval of about 10h. Sulfur and heavy metal concentrations were also associated to local emissions. Mineral dust represented the largest fraction of PM(10) reaching 79%. Seven days back trajectories have shown that the air masses arriving over Athens, originated from Western Sahara. Scanning Electron Microscopy coupled with Energy Dispersive X-ray analysis (SEM-EDX) revealed that particle agglomerates were abundant, most of them having sizes2 μm. Aluminosilicates were predominant in dust particles also rich in calcium which was distributed between calcite, dolomite, gypsum and Ca-Si particles. These results were consistent with the origin of the dust particles and the elemental composition results. Sulfur and heavy metals were associated to very fine particles1 μm.

This study presents an inter-comparison of two active remote sensors (lidar and ceilometer) in determining the structure of the Planetary Boundary Layer (PBL) and in retrieving tropospheric aerosol vertical profiles over Athens, Greece. This inter-comparison was performed under various strongly different aerosol concentrations (urban air pollution, biomass burning and Saharan dust event), implementing two different lidar systems (one portable Raymetrics S.A. lidar system running at 355 nm and one multi-wavelength Raman lidar system running at 355 nm, 532 nm and 1064 nm) and one CL31 Vaisala S.A. ceilometer (running at 910 nm). To convert the ceilometer data to data having the same wavelengths as those from the lidar, the backscatter-related Ångström exponent was estimated using ultraviolet multi-filter radiometer (UV-MFR) data. The inter-comparison was based on two parameters: the mixing layer structure and height determined by the presence of the suspended aerosols and the aerosol backscatter coefficient. Additionally, radiosonde data were used to derive the PBL height. In general a good agreement is found between the ceilometer and the lidar techniques in both inter-compared parameters in the height range from 500 m to 5000 m, while the limitations of each instrument are also examined.

In this article a statistical assessment concerning the relationship between the aerosol backscatter coefficient (β aer) and the relative humidity (RH) in the lower andmiddle troposphere, over Athens (Greece), is presented. For the purpose of this study, correlative radiosonde and aerosol backscatter lidar data were analysed for a period of 4 years (January 2003-December 2006), as obtained in the framework of the European Aerosol Lidar Network (EARLINET) project. The vertical profiles of the aerosol backscatter coefficients were measured by a combined Raman/elastic lidar system at ultraviolet (355 nm) and visible (532 nm) wavelengths. The correlation coefficient (R) of the vertical profiles of the RH against the backscatter coefficient of aerosols was investigated in altitudes within the free troposphere (0-6000 m). The altitude range was divided into three areas: 0 m up to the top of the Planetary Boundary Layer (PBL); PBL up to PBL + 2000 m; and PBL + 2000 m up to 6000 m. The properties and seasonal variations of the height of the PBL were also studied. The annual mean PBL height over Athens was found to be (1320 ± 480) m, while during the warm period of the year (spring-summer) the PBL was higher than during the cold period (autumn-winter). Regarding the correlation coefficient (R), low (0-0.5) and medium (0.5-0.8) R values were mostly observed during the warmmonths of the year. For the aerosols originating from the Balkan area the highest correlation was observed at both wavelengths (R = 0.71 at 355 nm and R = 0.41 at 532 nm), especially during the years 2003 and 2005 (R = 0.61 at 355 nm and R = 0.93 at 532 nm). The almost linear correlation of this type of aerosols can be attributed to the fact that these remained for a longer time in a coherently alternating atmosphere, therefore having the tendency to become homogenized.