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We report on the performance improvements of the L1 Allegra laser system. The pump laser upgrade with the thin-disk multipass amplifier allows for the energy ramp-up, while a newly developed synchronized auxiliary laser system provides the capability of the pump-probe experiments at arbitrary delays.

We report on a 1 kHz, 515 nm laser system, based on a commercially available 230 W average power Yb:YAG thin-disk regenerative amplifier, developed for pumping one of the last optical parametric chirped pulse amplification (OPCPA) stages of the Allegra laser system at ELI Beamlines. To avoid problems with self-focusing of picosecond pulses, the 1030 nm output pulses are compressed and frequency doubled with an LBO crystal in vacuum. Additionally, development of a thermal management system was needed to ensure stable phase matching conditions at high average power. The resulting 515 nm pulses have an energy of more than 120 mJ with SHG efficiency of 60% and an average RMS stability of 1.1% for more than 8 h.

The L1 Allegra is an OPCPA-based, high average power, high repetition rate laser system pumped by thin-disc based regenerative amplifiers currently under development at the ELI-Beamlines center in Czech Republic. The repetition rate is 1 kHz, pulse duration is below 15 fs and the wavelength centered around 820 nm with a maximum design pulse energy of 100 mJ. To avoid problems with self-focusing, a large portion of the system was placed inside vacuum, including the compressors and second-harmonic crystals for the last three 1030 nm pump lasers, the final three OPA stages, and the chirped mirror compressor. In order to reach the designed output energy of the whole system, the pump lasers need to be efficient, stable, and providing enough pump power for each of the amplification stages. Pulse compression of the final three pump lasers as well as efficient conversion to the second harmonic frequency in vacuum has posed several challenges and we report on their solutions and results. The vacuum environment causes difficulties for two main reasons. The first one is laser-induced-contamination (LIC) degrading the optical surfaces of dielectric gratings, mirrors and crystals, due to the presence of degassing components contaminating the vacuum chambers. The second reason is second-harmonic generation crystal mounts heating up, requiring regular phase matching corrections by rotation of the crystal mounts. The LIC problem was solved by regular cleaning of the chambers by means of an RF-plasma source, and the heating problem was solved by implementing active temperature stabilization by means of installing thermo-electric coolers on the crystal holders. To increase the efficiency of the second-harmonic generation, beam profiles of the pump lasers had to be improved. The original Faraday rotators, present in the linearly-designed regenerative amplifiers, caused non-Gaussian beam profiles due to the self focusing inside the rotators. By using KTF crystals inside a new type of rotators, the spatial profile of the pump lasers is more Gaussian, allowing the efficiency of the SHG to be higher, almost by 25%. All the solved problems recently allowed the system to reach a short pulse output energy of 56 mJ, paving a way to reach 100 mJ successfuly in the future.

Vacuum chambers are frequently used in high-energy, high-peak-power laser systems to prevent deleterious nonlinear effects, which can result from propagation in air. In the vacuum sections of the Allegra laser system at ELI-Beamlines, we observed degradation of several optical elements due to laser-induced contamination (LIC). This contamination is present on surfaces with laser intensity above 30 G W / c m 2 with wavelengths of 515, 800, and 1030 nm. It can lead to undesired absorption on diffraction gratings, mirrors, and crystals and ultimately to degradation of the laser beam profile. Because the Allegra laser is intended to be a high-uptime source for users, such progressive degradation is unacceptable for operation. Here, we evaluate three methods of removing LIC from optics in vacuum. One of them, the radio-frequency-generated plasma cleaning, appears to be a suitable solution from the perspective of operating a reliable, on-demand source for users.

We report on the current state of readiness of the 1 kHz, 15 fs L1 ALLEGRA laser system for long term reliable operation driving user experiments based on HHG. The highly automated system, based on short pulse OPCPA, currently generates pulses with energy of 30 mJ at central wavelength of 820 nm.

We present experimental setup for user-oriented high-harmonic source with a description of different focusing and interaction geometries. Infrared rejection system and resulting extreme ultraviolet beam characterization are also described. Beamline is designed to be driven with 100 mJ

We report on the status of the Allegra laser beamline currently being commissioned at the ELI-Beamlines facility. The beamline will be used to drive X-ray sources for research in material science, molecular physics, and biophysics, where a high repetition rate is essential. Designed for user operation, significant attention is given to stability, reliability, and automation of the system. A photo of the beamline is shown in Fig. 1(a).

The Allegra femtosecond laser system is the main driver for high harmonic and plasma x-ray secondary sources at ELI-Beamlines operating at a 1 kHz rep rate. The system is based on OPCPA technology and consists of seven amplification stages pumped by thin-disk picosecond lasers. It is designed to reach 30 mJ output in the first phase of operation and to be ramped up to 50 mJ by engaging an additional pump laser. The amplified pulse is compressed to sub-20fs by an array of chirped mirrors and higher order dispersion is pre-compensated for by a Dazzler AOPDF in the front-end. In this paper we present the overview of Allegra system and the current status of deployment with a special focus on the high average power OPCPA in vacuum.

We report on the status of the Allegra laser beamline, which is designed to provide ub-20 fs pulses with tens of mJ of energy with exceptionally high contrast at a 1 kHz repetition rate.

We discuss the performance of several stages of high energy, high average power SHG and OPCPA with picosecond pulses in vacuum as part of the ALLEGRA laser at ELI-Beamlines.

For most extreme light applications, a reliable and stable driver laser is crucial to successful experiments. As lasers grow in energy and peak power they become increasingly complex and more failure modes are introduced to the system as a whole. For this reason it is prudent to develop a laser with simplicity, repeatability, and durability in mind. With the wide commercial availability of high quality, inexpensive fiber components, much of the required pulse conditioning for seeding high energy laser systems can take place entirely in fiber. This allows for much of the laser front end to be compact, alignment-free, and computer controlled with potentially dramatic savings in cost and space on the optical table. Here we explore some of the current trends in fiberbased front ends for high peak power laser systems. The requirements for any given high peak power laser are always quite different and fiber front ends are enormously customizable, so here we present two basic versions of fiber front ends which are used at the ELI-Beamlines facility which resemble other common fiber front end architectures.

We present photoemission time-delay measurements between electrons originating from the valence shells of neon and argon obtained by attosecond streaking. After giving a brief review of the different techniques, we focus on more detailed analysis using the attosecond streaking technique. We show that the temporal structure of the ionizing single attosecond pulse may significantly affect the obtained time delays, and we propose a procedure how to take this contribution properly into account. Our analysis reveals a delay of a few tens of attoseconds in a photon energy range between 28 and 40 eV in the emission of electrons ionized from argon with respect to those liberated from neon.

Overview of progress in construction and testing of the laser systems of ELI-Beamlines, accomplished since 2015, is presented. Good progress has been achieved in construction of all four lasers based largely on the technology of diode-pumped solid state lasers (DPSSL). The first part of the L1 laser, designed to provide 200 mJ

We report on the status of the high repetition rate, high energy, L1 laser beamline at the ELI-Beamlines facility. The beamline is based on picosecond optical parametric chirped pulse amplification (OPCPA) of pulses from a mode-locked Ti:Sapphire oscillator and has a target energy/repetition rate of 100 mJ/1 kHz with < 15fs pulse duration. The OPCPA pump lasers use thin disk technology to achieve the high energy and average power required to pump such a high energy, high repetition rate broadband amplifier. Here we report on the progress in beamline development and discuss the technical challenges involved in producing such a system and their solutions. A major focus of the laser development is reliable, robust operation and long term stability; mechanical, optical, and control system architecture design considerations to achieve our goals of long term stability are discussed.

We present an active cavity pointing stabilization system based on a novel method that tracks the cavity mode position directly on the thin disk gain medium itself. Here, the overlap of the lasing cavity with the pump, visible as a depletion within the pumped area, is most crucial to the stability of the laser. Short term stability as well as long term stability are significantly increased enabling day long operation, directly from a cold start of the laser system, without the need for thermalization and manual alignment.

We present a stable supercontinuum (SC) generated in a bulk YAG crystal, pumped by 3 ps chirped pulses at 1030 nm. The SC is generated in a loose focus geometry in a 13 cm long YAG crystal, allowing for stable and robust single-filament generation. The SC energy stability exceeds that of the pump laser by almost a factor of 3. Additionally, we show that the SC spectrum has long-term stability and that the SC is coherent and compressible by compressing the portions of SC spectra close to the corresponding Fourier limit. This makes the picosecond-pulse-driven SC a suitable stable seed for OPCPA amplifiers.

We report on the design and performance of a fiber-based, multi-channel laser amplifier seed pulse distribution system. The device is designed to condition and distribute low energy laser pulses from a mode-locked oscillator to multiple, highly synchronized, high energy amplifiers integrated into a laser beamline. Critical functions such as temporal pulse stretching well beyond 100 ps/nm, pulse picking, and fine control over the pulse delay up to 300 ps are all performed in fiber eliminating the need for bulky and expensive grating stretchers, Pockels cells, and delay lines. These functions are characterized and the system as a whole is demonstrated by seeding two high energy amplifiers in the laser beamline. The design of this system allows for complete computer control of all functions, including tuning of dispersion, and is entirely hands-free. The performance of this device and its subsystems will be relevant to those developing lasers where reliability, size, and cost are key concerns in addition to performance; this includes those developing large-scale laser systems similar to ours and also those developing table-top experiments and commercial systems.

We report on a broadband OPCPA system, pumped at 515 nm by frequency doubled Yb:YAG thin disk lasers. The system delivers 11.3 mJ pulses at a central wavelength of 800 nm with a spatial beam quality of Msup2/sup= 1.25 and25% pump-to-signal conversion efficiency. The broadband pulses were demonstrated to be compressible to 12 fs using a chirped mirror compressor.

We report on a frequency-doubled picosecond Yb:YAG thin disk regenerative amplifier, developed as a pump laser for a kilohertz repetition rate OPCPA. At a repetition rate of 1 kHz, the compressed output of the regenerative amplifier has a pulse duration of 1.2 ps and pulse energy of 90 mJ with energy stability of σ < 0.8% and M2 < 1.2. The pulses are frequency doubled in an LBO crystal yielding 42 mJ at 515 nm.

Time delays of electrons emitted from an isotropic initial state with the absorption of a single photon and leaving behind an isotropic ion are angle independent. Using an interferometric method involving XUV attosecond pulse trains and an IR-probe field in combination with a detection scheme, which allows for full three-dimensional momentum resolution, we show that measured time delays between electrons liberated from the 1s2 spherically symmetric ground state of helium depend on the emission direction of the electrons relative to the common linear polarization axis of the ionizing XUV light and the IR-probing field. Such time delay anisotropy, for which we measure values as large as 60 as, is caused by the interplay between final quantum states with different symmetry and arises naturally whenever the photoionization process involves the exchange of more than one photon. With the support of accurate theoretical models, the angular dependence of the time delay is attributed to small phase differences that are induced in the laser-driven continuum transitions to the final states. Since most measurement techniques tracing attosecond electron dynamics involve the exchange of at least two photons, this is a general and significant effect that must be taken into account in all measurements of time delays involving photoionization processes, S.H, C.C, L.G., and U.K. acknowledge support by the ERC advanced Grant No. ERC-2012-ADG_20120216 within the seventh framework program of the European Union and by the NCCR MUST, funded by the Swiss National Science Foundation. M.L. acknowledges support from the ETH Zurich Postdoctoral Fellowship Program. A.J.G., L.A., and F.M. acknowledge the support from the European Research Council under the ERC Grant No. 290853 XCHEM, from the European COST Action No. CM1204 XLIC, the MINECO Project No. FIS2013-42002-R, the ERA-Chemistry Project No. PIM2010EEC- 00751, and the European Grant No. MC-ITN CORINF. Calculations were performed at the Centro de Computacion Científica of the Universidad Autónoma de Madrid (CC-UAM) and the Barcelona Supercomputing Center (BSC). I.I. and A.S.K. acknowledge support of the Australian Research Council (Grant No. DP120101805) and the use of the National Computational Infrastructure Facility. J.M.D. acknowledges support from the Swedish Research Grants No. 2013-344 and No. 2014-3724. E.L. acknowledges support from the Swedish Research Council, Grant No. 2012-3668. Moreover, this research was supported in part by the Kavli Institute for Theoretical Physics (National Science Foundation under Grant No. NSF PHY11-25915) and by NORDITA, the Nordic Institute for Theoretical Physics

Here, we present the first experiments addressing the single-photon ionization time delay for randomly oriented molecular hydrogen (H2), the simplest non-charged molecule. We measure the difference \( \varDelta \tau_{\text{m}}^{\text{Ar,H2}} \) in time delays between electrons emitted from the 3p6 shell of argon (Ar) and the highest occupied molecular orbital of H2 by means of two distinct methods, employing attosecond streaking and RABBITT.

In contrast to expectations, we observe that the photoionization time delay from the 1s2 spherically symmetric ground state of He depend on the electron emission direction with respect to an external reference. We attribute the observed anisotropy to the interplay between different final quantum states, which become accessible once two photons are involved in the photoionization process. This is a universal effect, which needs to be taken into account for any study dealing with photoionization dynamics.

For the first time, we implemented both RABBITT and attosecond energy streaking using an AttoCOLTRIMS apparatus and exploit its advantages to determine energy- and angle-resolved single-photon ionization time delays for different noble gases.

We present measurements of single-photon ionization time delays between the outermost valence electrons of argon and neon using a coincidence detection technique that allows for the simultaneous measurement of both species under identical conditions. The analysis of the measured traces reveals energy-dependent time delays of a few tens of attoseconds with high energy resolution. In contrast to photoelectrons ejected through tunneling, single-photon ionization can be well described in the framework of Wigner time delays. Accordingly, the overall trend of our data is reproduced by recent Wigner time delay calculations. However, besides the general trend we observe resonance features occurring at specific photon energies. These features have been qualitatively reproduced and identified by a calculation using the multiconfigurational Hartree-Fock method, including the influence of doubly excited states and ionization thresholds.

We report on the first experiments characterizing the complete time-dependent 2D vector potential of a few-cycle laser pulse. The instantaneous amplitude and orientation of the electric field is determined with sub-cycle resolution, directly giving access to the polarization state of the pulse at any instant in time. This is achieved by performing an attosecond streaking experiment using a reaction microscope, where the full pulse characterization is performed directly in the target region.

Here we present a successful combination of an attosecond beamline with a COLTRIMS apparatus, which we refer to as AttoCOLTRIMS. The setup provides either single attosecond pulses or attosecond pulse trains for extreme ultraviolet-infrared pump-probe experiments. We achieve full attosecond stability by using an active interferometer stabilization. The capability of the setup is demonstrated by means of two measurements, which lie at the heart of the COLTRIMS detector: firstly, we resolve the rotating electric field vector of an elliptically polarized few-cycle infrared laser field by attosecond streaking exploiting the access to the 3D momentum space of the charged particles. Secondly, we show streaking measurements on different atomic species obtained simultaneously in a single measurement making use of the advantage of measuring ions and electrons in coincidence. Both of these studies demonstrate the potential of the AttoCOLTRIMS for attosecond science., Review of Scientific Instruments, 85 (10), ISSN:0034-6748, ISSN:1089-7623

Strong field ionization momentum distribution contains much information. The angular distribution indicates real tunneling delay time, the center shows ellipticity dependent Coulomb effects, and the longitudinal momentum spread challenges the assumption of zero initial momentum.

We combine an attosecond beam line with a 3D momentum imaging spectrometer to achieve coincidence pump probe experiments with unprecedented attosecond time-resolution. Besides technical details, first coincidence and pump-probe experiments are presented.

We investigate experimentally the validity of proposed theories extending the tunneling approximation towards the multiphoton regime in strong-field ionization of helium. We employ elliptically polarized laser pulses and demonstrate how the influence of the ion potential on the released electron encoded in the measured observable provides the desired sensitivity to detect nonadiabatic effects in tunnel ionization. Our results show that for a large intensity range the proposed nonadiabatic theories contradict the experimental trends of the data, while adiabatic assumptions are confirmed.

We compare the main competing theories of tunneling time against experimental measurements using the attoclock in strong laser field ionization of helium atoms. Refined attoclock measurements reveal a real and not instantaneous tunneling delay time over a large intensity regime, using two different experimental apparatus. Only two of the theoretical predictions are compatible within our experimental error: the Larmor time, and the probability distribution of tunneling times constructed using a Feynman Path Integral (FPI) formulation. The latter better matches the observed qualitative change in tunneling time over a wide intensity range, and predicts a broad tunneling time distribution with a long tail. The implication of such a probability distribution of tunneling times, as opposed to a distinct tunneling time, challenges how valence electron dynamics are currently reconstructed in attosecond science. It means that one must account for a significant uncertainty as to when the hole dynamics begin to evolve., 11 pages, 4 figures

The question of how long a tunneling particle spends inside the barrier region has remained unresolved since the early days of quantum mechanics. The main theoretical contenders, such as the Buttiker–Landauer, Eisenbud–Wigner, and Larmor time, give contradictory answers. On the other hand, recent attempts at reconstructing valence electron dynamics in atoms and molecules have entered a regime where the tunneling time genuinely matters. Here, we compare the main competing theories of tunneling time against experimental measurements using the attoclock in strong laser field ionization of helium atoms. The attoclock uses a close to circularly polarized femtosecond laser pulse, mapping the angle of rotation of the laser field vector to time similar to the hand of a watch. Refined attoclock measurements reveal a real (not instantaneous) tunneling delay time over a large intensity regime, using two independent experimental apparatus. Only two theoretical predictions are compatible within our experimental error: the Larmor time and the probability distribution of tunneling times constructed using a Feynman Path Integral formulation. The latter better matches the observed qualitative change in tunneling time over a wide intensity range, and predicts a broad tunneling time distribution with a long tail. The implication of such a probability distribution of tunneling times, as opposed to a distinct tunneling time, would imply that one must account for a significant, though bounded and measurable, uncertainty as to when the hole dynamics begin to evolve. We therefore expect our results to impact the reconstruction of attosecond electron dynamics following tunnel ionization.

We present a multistage 1 kHz OPCPA system, pumped by two frequency doubled thin disk regenerative amplifiers, delivering together 57 mJ at 515 nm. The OPCPA produces 8 mJ of amplified signal and is compressible to < 27 fs.