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We use an ensemble of laser-cooled strontium atoms in a high-finesse cavity to cleanly emulate the technique of rf spectroscopy employed in studies of BEC-BCS physics in fermionic superfluids of degenerate cold gases. Here, we leverage the multilevel internal structure of the atoms to study the physics of Cooper pair breaking in this system. In doing so, we observe and distinguish the properties of two distinct many-body gaps, the BCS pairing gap and the spectral gap, using nondestructive readout techniques. The latter is found to depend on the populations of the internal atomic states, reflecting the chemical potential dependence predicted in fermionic superfluids. This work opens the path for more fully exploiting the rich internal structure of atoms in cavity QED emulators to study both analogous systems and also more exotic states yet to be realized., Comment: Main Text with Supplementary Material, 15 pages, 5 figures

In cavity quantum electrodynamics (QED), emitters and a resonator are coupled together to enable precise studies of quantum light-matter interactions. Over the past few decades, this has led to a variety of quantum technologies such as more precise inertial sensors, clocks, memories, controllable qubits, and quantum simulators. Furthermore, the intrinsically dissipative nature of cavity QED platforms makes them a natural testbed for exploring driven-dissipative phenomena in open quantum systems as well as equilibrium and non-equilibrium phase transitions in quantum optics. One such model, the so-called cooperative resonance fluorescence (CRF) model, concerns the behavior of coherently driven emitters in the presence of collective dissipation (superradiance). Despite tremendous interest, this model has yet to be realized in a clean experimental system. Here we provide an observation of the continuous superradiant phase transition predicted in the CRF model using an ensemble of ultracold $^{88}$Sr atoms coupled to a driven high-finesse optical cavity on a long-lived optical transition. Below a critical drive, atoms quickly reach a steady state determined by the self-balancing of the drive and the collective dissipation. The steady state possesses a macroscopic dipole moment and corresponds to a superradiant phase. Above a critical drive strength, the atoms undergo persistent Rabi-like oscillations until other decoherence processes kick in. In fact, our platform also allows us to witness the change of this phase transition from second to first order induced by single-particle spontaneous emission, which pushes the system towards a different steady state. Our observations are a first step towards finer control of driven-dissipative systems, which have been predicted to generate quantum states that can be harnessed for quantum information processing and in particular quantum sensing., Comment: 12 pages, 7 figures (main text and methods); 11 pages, 4 figures (supplementary information); typos corrected

Quantum computation (QC) and simulation rely on long-lived qubits with controllable interactions. Early work in quantum computing made use of molecules because of their readily available intramolecular nuclear spin coupling and chemical shifts, along with mature nuclear magnetic resonance techniques. Subsequently, the pursuit of many physical platforms has flourished. Trapped polar molecules have been proposed as a promising quantum computing platform, offering scalability and single-particle addressability while still leveraging inherent complexity and strong couplings of molecules. Recent progress in the single quantum state preparation and coherence of the hyperfine-rotational states of individually trapped molecules allows them to serve as promising qubits, with intermolecular dipolar interactions creating entanglement. However, universal two-qubit gates have not been demonstrated with molecules. Here, we harness intrinsic molecular resources to implement a two-qubit iSWAP gate using individually trapped $X^{1}\Sigma^{+}$ NaCs molecules. We characterize the innate dipolar interaction between rotational states and control its strength by tuning the polarization of the traps. By allowing the molecules to interact for 664 $\mu$s at a distance of 1.9 $\mu$m, we create a maximally entangled Bell state with a fidelity of 94(3)\%, following postselection to remove trials with empty traps. Using motion-rotation coupling, we measure residual excitation of the lowest few motional states along the axial trapping direction and find them to be the primary source of decoherence. Finally, we identify two non-interacting hyperfine states within the ground rotational level in which we encode a qubit. The interaction is toggled by transferring between interacting and non-interacting states to realize an iSWAP gate. We verify the gate performance by measuring its logical truth table.

The ability to create and harness entanglement is crucial to the fields of quantum sensing and simulation, and ultracold atom-cavity systems offer pristine platforms for this undertaking. Here, we present a method for creating and controlling entanglement between solely the motional states of atoms in a cavity without the need for electronic interactions. We show this interaction arises from a general atom-cavity model, and discuss the role of the cavity frequency shift in response to atomic motion. This cavity response leads to many different squeezing interactions between the atomic momentum states. Furthermore, we show that when the atoms form a density grating, the collective motion leads to one-axis twisting, a many-body energy gap, and metrologically useful entanglement even in the presence of noise. Noteably, an experiment has recently demonstrated this regime leads to an effective momentum-exchange interaction between atoms in a common cavity mode. This system offers a highly tunable, many-body quantum sensor and simulator.

We propose protocols that probe manifestations of the mass-energy equivalence in an optical lattice clock (OLC) interrogated with spin coherent and entangled quantum states. To tune and uniquely distinguish the mass-energy equivalence effects (gravitational redshift and second order Doppler shift) in such setting, we devise a dressing protocol using an additional nuclear spin state. We then analyze the interplay between photon-mediated interactions and gravitational redshift and show that such interplay can lead to entanglement generation and frequency synchronization. In the regime where all atomic spins synchronize, we show the synchronization time depends on the initial entanglement of the state and can be used as a proxy of its metrological gain compared to a classical state. Our work opens new possibilities for exploring the effects of general relativity on quantum coherence and entanglement in OLC experiments., Comment: 7+17 pages, 4+6 figures

We propose the use of phonon$\unicode{x2013}$mediated interactions as an entanglement resource to engineer Einstein$\unicode{x2013}$Podolsky$\unicode{x2013}$Rosen (EPR) correlations and to perform teleportation of collective spin states in two$\unicode{x2013}$dimensional ion crystals. We emulate continuous variable quantum teleportation protocols between subsystems corresponding to different nuclear spin degrees of freedom. In each of them, a quantum state is encoded in an electronic spin degree of freedom that couples to the vibrational modes of the crystal. We show that high fidelity teleportation of spin-coherent states and their phase-displaced variant, entangled spin-squeezed states, and Dicke states, is possible for realistic experimental conditions in arrays from a few tens to a few hundred ions., Comment: 9 pages, 7 figure

Long-range and anisotropic dipolar interactions profoundly modify the dynamics of particles hopping in a periodic lattice potential. Here, we report the realization of a generalized t-J model with dipolar interactions using a system of ultracold fermionic molecules with spin encoded in the two lowest rotational states. We systematically explore the role of dipolar Ising and spin-exchange couplings and the effect of motion on spin dynamics. The model parameters can be controlled independently, with dipolar couplings tuned by electric fields and motion regulated by optical lattices. Using Ramsey spectroscopy, we observed interaction-driven contrast decay that depends strongly both on the strength of the anisotropy between Ising and spin-exchange couplings and on motion. These observations are supported by theory models established in different motional regimes that provide intuitive pictures of the underlying physics. This study paves the way for future exploration of kinetic spin dynamics and quantum magnetism with highly tunable molecular platforms in regimes challenging for existing numerical and analytical methods, and it could shed light on the complex behaviors observed in real materials.

We demonstrate a bipartition technique using a super-lattice architecture to access correlations between alternating planes of a mesoscopic array of spin-3 chromium atoms trapped in a 3D optical lattice. Using this method, we observe that out-of-equilibrium dynamics driven by long-range dipolar interactions lead to spin anti-correlations between the two spatially separated subsystems. Our bipartite measurements reveal a subtle interplay between the anisotropy of the 3D dipolar interactions and that of the lattice structure, without requiring single-site addressing. We compare our results to theoretical predictions based on a truncated cumulant expansion and a new cluster semi-classical method that we use to investigate correlations at the microscopic scale. Comparison with a high-temperature analytical model reveals quantum thermalization at a high negative spin temperature., Comment: Main article: 5 pages, 3 Figures Supp Mat: 4 pages, 3 Figures

Quantum simulation using synthetic quantum systems offers unique opportunities to explore open questions in many-body physics and a path for the generation of useful entangled states. Nevertheless, so far many quantum simulators have been fundamentally limited in the models they can mimic. Here, we are able to realize an all-to-all interaction with arbitrary quadratic Hamiltonian or effectively an infinite range tunable Heisenberg XYZ model. This is accomplished by engineering cavity-mediated four-photon interactions between 700 rubidium atoms in which we harness a pair of momentum states as the effective pseudo spin or qubit degree of freedom. Using this capability we realize for the first time the so-called two-axis counter-twisting model at the mean-field level. The versatility of our platform to include more than two relevant momentum states, combined with the flexibility of the simulated Hamiltonians by adding cavity tones opens rich opportunities for quantum simulation and quantum sensing in matter-wave interferometers and other quantum sensors such as optical clocks and magnetometers

Measurement science now connects strongly with engineering of quantum coherence, many-body states, and entanglement. To scale up the performance of an atomic clock using a degenerate Fermi gas loaded in a three-dimensional optical lattice, we must understand complex many-body Hamiltonians to ensure meaningful gains for metrological applications. In this work, we use a near unity filled Sr 3D lattice to study the effect of a tunable Fermi-Hubbard Hamiltonian. The clock laser introduces a spin-orbit coupling spiral phase and breaks the isotropy of superexchange interactions, changing the Heisenberg spin model into one exhibiting XXZ-type spin anisotropy. By tuning the lattice confinement and applying imaging spectroscopy we map out favorable atomic coherence regimes. With weak transverse confinement, both s- and p-wave interactions contribute to decoherence and atom loss, and their contributions can be balanced. At deep transverse confinement, we directly observe coherent superexchange interactions, tunable via on-site interaction and site-to-site energy shift, on the clock Ramsey fringe contrast over timescales of multiple seconds. This study provides a groundwork for using a 3D optical lattice clock to probe quantum magnetism and spin entanglement

We show how a driven-dissipative cavity coupled to a collective ensemble of atoms can dynamically generate metrologically useful spin-squeezed states. In contrast to other dissipative approaches, we do not rely on complex engineered dissipation or input states, nor do we require tuning the system to a critical point. Instead, we utilize a strong symmetry, a special type of symmetry that can occur in open quantum systems and emerges naturally in systems with collective dissipation, such as superradiance. This symmetry preserves coherence and allows for the accumulation of an atom number-dependent Berry phase which in turn creates spin-squeezed states via emergent one-axis twisting dynamics. This work shows that it is possible to generate entanglement in an atom-cavity resonant regime with macroscopic optical excitations of the system, going beyond the typical dispersive regime with negligible optical excitations often utilized in current cavity QED experiments., Comment: 5+14 pages, 3 figures

By leveraging the hyperfine interaction between the rotational and nuclear spin degrees of freedom, we demonstrate extensive magnetic control over the electric dipole moments, electric dipolar interactions, and ac Stark shifts of ground-state alkali-dimer molecules such as KRb$(X^1\Sigma)$. The control is enabled by narrow avoided crossings and the highly ergodic character of molecular eigenstates at low magnetic fields, offering a general and robust way of continuously tuning the intermolecular electric dipolar interaction for applications in quantum simulation and sensing.

Trapped ion systems are a leading platform for quantum information processing, but they are currently limited to 1D and 2D arrays, which imposes restrictions on both their scalability and their range of applications. Here, we propose a path to overcome this limitation by demonstrating that Penning traps can be used to realize remarkably clean bilayer crystals, wherein hundreds of ions self-organize into two well-defined layers. These bilayer crystals are made possible by the inclusion of an anharmonic trapping potential, which is readily implementable with current technology. We study the normal modes of this system and discover salient differences compared to the modes of single-plane crystals. The bilayer geometry and the unique properties of the normal modes open new opportunities, in particular in quantum sensing and quantum simulation, that are not straightforward in single-plane crystals. Furthermore, we illustrate that it may be possible to extend the ideas presented here to realize multilayer crystals with more than two layers. Our work increases the dimensionality of trapped ion systems by efficiently utilizing all three spatial dimensions and lays the foundation for a new generation of quantum information processing experiments with multilayer 3D crystals of trapped ions., Comment: 21+10 pages, 12 figures, 3 supplementary videos; Updated to version submitted to journal

We study the combined effects of measurements and unitary evolution on the preparation of spin squeezing in an ensemble of atoms interacting with a single electromagnetic field mode inside a cavity. We derive simple criteria that determine the conditions at which measurement based entanglement generation overperforms unitary protocols. We include all relevant sources of decoherence and study both their effect on the optimal spin squeezing and the overall size of the measurement noise, which limits the dynamical range of quantum-enhanced phase measurements. Our conclusions are relevant for state-of-the-art atomic clocks that aim to operate below the standard quantum limit., Comment: 6 + 10 pages, 4 + 1 figures

We utilize multilevel atoms trapped in a driven resonant optical cavity to produce scalable multi-mode squeezed states for quantum sensing and metrology. While superradiance or collective dissipative emission by itself has been typically a detrimental effect for entanglement generation in optical cavities, in the presence of additional drives it can also be used as an entanglement resource. In a recent work [Phys. Rev. Lett. 132, 033601 (2024)], we described a protocol for the dissipative generation of two-mode squeezing in the dark state of a six-level system with only one relevant polarization. There we showed that up to two quadratures can be squeezed. Here, we develop a generalized analytic treatment to calculate the squeezing in any multilevel system where atoms can collectively decay by emitting light into two polarization modes in a cavity. We show that in this more general system up to four spin squeezed quadratures can be obtained. We study how finite-size effects constrain the reachable squeezing, and analytically compute the scaling with $N$. Our findings are readily testable in current optical cavity experiments with alkaline-earth-like atoms., Comment: 14 pages, 5 figures + Appendix; References updated; Moved some sections from Appendix to main text

We analyse the properties across steady state phase transitions of two all-to-all driven-dissipative spin models that describe possible dynamics of N two-level systems inside an optical cavity. We show that the finite size behaviour around the critical points can be captured correctly by carefully identifying the relevant non-linearities in the Holstein-Primakoff representation of spin operators in terms of bosonic variables. With these tools, we calculate analytically various observables across the phase transitions and obtain their finite size scalings, including numerical prefactors. In particular, we look at the amount of spin squeezing carried by the steady states, of relevance for quantum metrology applications, and describe in analytical detail the mechanism by which the optimal spin squeezing acquires logarithmic corrections that depend on the system size. We also demonstrate that the logarithmic nature of these corrections is difficult to characterize through numerical procedures for any experimentally realistic and/or simulable values of particle number. We complement all of our analytical arguments with numerical benchmarks., Comment: 10+5 pages, 4+3 figures

We describe a theoretical scheme for generating scalable spin squeezing with nearest-neighbour interactions between spin-1/2 particles in a 3D lattice, which are naturally present in state-of-the-art 3D optical lattice clocks. We propose to use strong isotropic Heisenberg interactions within individual planes of the lattice, forcing the constituent spin-1/2s to behave as large collective spins. These large spins are then coupled with XXZ anisotropic interactions along a third direction of the lattice. This system can be realized via superexchange interactions in a 3D optical lattice subject to an external linear potential, such as gravity, and in the presence of spin-orbit coupling (SOC) to generate spin anisotropic interactions. We show there is a wide range of parameters in this setting where the spin squeezing improves with increasing system size even in the presence of holes., Comment: 13+9 pages, 8+1 figures

In conventional Bardeen-Cooper-Schrieffer (BCS) superconductors, electrons with opposite momenta bind into Cooper pairs due to an attractive interaction mediated by phonons in the material. While superconductivity naturally emerges at thermal equilibrium, it can also emerge out of equilibrium when the system's parameters are abruptly changed. The resulting out-of-equilibrium phases are predicted to occur in real materials and ultracold fermionic atoms but have not yet all been directly observed. Here we realize an alternate way to generate the proposed dynamical phases using cavity quantum electrodynamics (cavity QED). Our system encodes the presence or absence of a Cooper pair in a long-lived electronic transition in $^{88}$Sr atoms coupled to an optical cavity and represents interactions between electrons as photon-mediated interactions through the cavity. To fully explore the phase diagram, we manipulate the ratio between the single-particle dispersion and the interactions after a quench and perform real-time tracking of subsequent dynamics of the superconducting order parameter using non-destructive measurements. We observe regimes where the order parameter decays to zero (phase I), assumes a non-equilibrium steady-state value (phase II), or exhibits persistent oscillations (phase III). This opens up exciting prospects for quantum simulation, including the potential to engineer unconventional superconductors and to probe beyond mean-field effects like the spectral form factor, and for increasing coherence time for quantum sensing., Comment: Main Text with Supporting Material, 18 pages, 10 figures. The content in this version of the paper is similar to that of the article in Nature

Using a recently developed extension of the time-dependent variational principle for matrix product states, we evaluate the dynamics of 2D power-law interacting XXZ models, implementable in a variety of state-of-the-art experimental platforms. We compute the spin squeezing as a measure of correlations in the system, and compare to semiclassical phase-space calculations utilizing the discrete truncated Wigner approximation (DTWA). We find the latter efficiently and accurately captures the scaling of entanglement with system size in these systems, despite the comparatively resource-intensive tensor network representation of the dynamics. We also compare the steady-state behavior of DTWA to thermal ensemble calculations with tensor networks. Our results open a way to benchmark dynamical calculations for two-dimensional quantum systems, and allow us to rigorously validate recent predictions for the generation of scalable entangled resources for metrology in these systems., Comment: 6+4 pages, 3+1 figures

Quantum simulation and sensing hold great promise for providing new insights into nature, from understanding complex interacting systems to searching for undiscovered physics. Large ensembles of laser-cooled atoms interacting via infinite-range photon mediated interactions are a powerful platform for both endeavours. Here, we realize for the first time momentum-exchange interactions in which atoms exchange their momentum states via collective emission and absorption of photons from a common cavity mode. The momentum-exchange interaction leads to an observed all-to-all Ising-like interaction in a matter-wave interferometer, which is useful for entanglement generation. A many-body energy gap also emerges, effectively binding interferometer matter-wave packets together to suppress Doppler dephasing, akin to M\"ossbauer spectroscopy. The tunable momentum-exchange interaction provides a new capability for quantum interaction-enhanced matter-wave interferometry and for realizing exotic behaviors including simulations of superconductors and dynamical gauge fields., Comment: Main Text with Supporting Material, 17 pages, 5 figures

The control over quantum states in atomic systems has led to the most precise optical atomic clocks to date. Their sensitivity is currently bounded by the standard quantum limit, a fundamental floor set by quantum mechanics for uncorrelated particles, which can nevertheless be overcome when operated with entangled particles. Yet demonstrating a quantum advantage in real world sensors is extremely challenging and remains to be achieved aside from two remarkable examples, LIGO and more recently HAYSTAC. Here we illustrate a pathway for harnessing scalable entanglement in an optical transition using 1D chains of up to 51 ions with state-dependent interactions that decay as a power-law function of the ion separation. We show our sensor can be made to behave as a one-axis-twisting (OAT) model, an iconic fully connected model known to generate scalable squeezing. The collective nature of the state manifests itself in the preservation of the total transverse magnetization, the reduced growth of finite momentum spin-wave excitations, the generation of spin squeezing comparable to OAT (a Wineland parameter of $-3.9 \pm 0.3$ dB for only N = 12 ions) and the development of non-Gaussian states in the form of atomic multi-headed cat states in the Q-distribution. The simplicity of our protocol enables scalability to large arrays with minimal overhead, opening the door to advances in timekeeping as well as new methods for preserving coherence in quantum simulation and computation. We demonstrate this in a Ramsey-type interferometer, where we reduce the measurement uncertainty by $-3.2 \pm 0.5$ dB below the standard quantum limit for N = 51 ions., Comment: During the completion of our work, we became aware of three related experiments using dressed Rydberg interactions in tweezer and microtrap array platforms. See arXiv:2303.08053, arXiv:2303.08078 and arXiv:2303.08805. This manuscript contains 14 Pages and 5 figures

We describe a method to create and store scalable and long-lived entangled spin-squeezed states within a manifold of many-body cavity dark states using collective emission of light from multilevel atoms inside an optical cavity. We show that the system can be tuned to generate squeezing in a dark state where it will be immune to superradiance. We also show more generically that squeezing can be generated using a combination of superradiance and coherent driving in a bright state, and subsequently be transferred via single-particle rotations to a dark state where squeezing can be stored. Our findings, readily testable in current optical cavity experiments with alkaline-earth-like atoms, can open a path for dissipative generation and storage of metrologically useful states in optical transitions., Comment: 4.5 pages, 3 figures + Supplement; New sections in Supplement

We study the temporal growth and spatial propagation of quantum correlations in a two-dimensional bilayer realising a spin-1/2 quantum XXZ model with couplings mediated by long-range and anisotropic dipolar interactions. Starting with an initial state consisting of spins with opposite magnetization in each of the layers, we predict the emergence of a momentum-dependent dynamic instability in the spin structure factor that results, at short times, in the creation of pairs of excitations at exponentially fast rates. The created pairs present a characteristic momentum distribution that can be tuned by controlling the dipolar orientation, the layer separation or the dipolar couplings. The predicted behavior remains observable at very low filling fractions, making it accessible in state-of-the-art experiments with Rydberg atoms, magnetic atoms, and polar molecule arrays., Comment: 4+7 pages, 4+5 figures; comments welcome

We propose a scheme to control and enhance atomic Bloch oscillations via photon-mediated interactions in an optical lattice supported by a standing-wave cavity with incommensurate lattice and cavity wavelengths. Our scheme uses position-dependent atom-light couplings in an optical cavity to spatially prepare an array of atoms at targeted lattice sites starting from a thermal gas. On this initial state we take advantage of dispersive position-dependent atom-cavity couplings to perform non-destructive measurements of single-particle Bloch oscillations, and to generate long-range interactions self-tuned by atomic motion. The latter leads to the generation of dynamical phase transitions in the deep lattice regime and the amplification of Bloch oscillations in the shallow lattice regime. Our work introduces new possibilities accessible in state-of-the-art cavity QED experiments for the exploration of many-body dynamics in self-tunable potentials., Comment: 6+11 pages, 3+5 figures

Entangled spin squeezed states generated via dipolar interactions in lattice models provide unique opportunities for quantum enhanced sensing and are now within reach of current experiments. A critical question in this context is which parameter regimes offer the best prospects under realistic conditions. Light scattering in deep lattices can induce significant decoherence and strong Stark shifts, while shallow lattices face motional decoherence as a fundamental obstacle. Here we analyze the interplay between motion and spin squeezing in itinerant fermionic dipoles in one dimensional chains using exact matrix product state simulations. We demonstrate that shallow lattices can achieve more than 5dB of squeezing, outperforming deep lattices by up to more than 3dB, even in the presence of low filling, loss and decoherence. We relate this finding to SU(2)-symmetric superexchange interactions, which keep spins aligned and protect collective correlations. We show that the optimal regime is achieved for small repulsive off-site interactions, with a trade-off between maximal squeezing and optimal squeezing time., Comment: 4.5+5.5 pages, 4+4 figures

Penning traps have been used for performing quantum simulations and sensing with hundreds of ions and provide a promising route toward scaling up trapped ion quantum platforms because of the ability to trap and control up to thousands of ions in 2D and 3D crystals. A leading source of decoherence in laser-based multiqubit operations on trapped ions is off-resonant spontaneous emission. While many trapped ion quantum computers or simulators utilize clock qubits, other systems rely on Zeeman qubits, which require a more complex calculation of this decoherence. We examine theoretically the impacts of spontaneous emission on quantum gates performed with trapped ions in a high magnetic field. We consider two types of gates -- light-shift and Molmer-Sorensen gates -- and compare the decoherence errors in each. We also compare different detunings, polarizations, and required intensities of the laser beams used to drive the gates. We show that both gates can have similar performance at their optimal operating conditions and examine the experimental feasibility of various operating points. By examining the magnetic field dependence of each gate, we demonstrate that when the $P$ state fine structure splitting is large compared to the Zeeman splittings, the theoretical performance of the Molmer-Sorensen gate is significantly better than that of the light-shift gate. Additionally, for the light-shift gate, we make an approximate comparison between the fidelities that can be achieved at high fields with the fidelities of state-of-the-art two-qubit trapped ion quantum gates. We show that, with regard to spontaneous emission, the achievable infidelity of our current configuration is about an order of magnitude larger than that of the best low-field gates, but we also discuss alternative configurations with potential error rates that are comparable with state-of-the-art trapped ion gates., Comment: Main text: 19 pages, 13 figures, Appendix: 7 pages, 1 figure, updated to improve presentation

We study the non-equilibrium dynamics of dipoles confined in multiple stacked two-dimensional layers realising a long-range interacting quantum spin 1/2 XXZ model. We demonstrate that strong in-plane XXX interactions can protect a manifold of collective layer dynamics. This then allows us to map the many-body spin dynamics to bosonic models. In a bilayer configuration we show how to engineer the paradigmatic two-mode squeezing Hamiltonian known from quantum optics, resulting in exponential production of entangled pairs and generation of metrologically useful entanglement from initially prepared product states. In multi-layer configurations we engineer a bosonic variant of the Kitaev model displaying chiral propagation along the layer direction. Our study illustrates how the control over interactions, lattice geometry and state preparation in interacting dipolar systems uniquely afforded by AMO platforms such as Rydberg and magnetic atoms, polar molecules or trapped ions allow for the control over the temporal and spatial propagation of correlations for applications in quantum sensing and quantum simulation., Comment: 5 pages, 4 figures + references + supplement

We propose a new direction in quantum simulation that uses multilevel atoms in an optical cavity as a toolbox to engineer new types of bosonic models featuring correlated hopping processes in a synthetic ladder spanned by atomic ground states. The underlying mechanisms responsible for correlated hopping are collective cavity-mediated interactions that dress a manifold of excited levels in the far detuned limit. By weakly coupling the ground state levels to these dressed states using two laser drives with appropriate detunings, one can engineer correlated hopping processes while suppressing undesired single-particle and collective shifts of the ground state levels. We discuss the rich many-body dynamics that can be realized in the synthetic ladder including pair production processes, chiral transport and light-cone correlation spreading. The latter illustrates that an effective notion of locality can be engineered in a system with fully collective interactions., Comment: 6+9 pages, 4+4 figures

We propose a new protocol for preparing spin squeezed states in controllable atomic, molecular, and optical systems, with particular relevance to emerging optical clock platforms compatible with Rydberg interactions. By combining a short-ranged, soft-core potential with an external drive, we can transform naturally emerging Ising interactions into an XX spin model while opening a many-body gap. The gap helps maintain the system within a collective manifold of states where metrologically useful spin squeezing can be generated at a level comparable to the spin squeezing generated in systems with genuine all-to-all interactions. We examine the robustness of our protocol to experimentally-relevant decoherence and show favorable performance over typical protocols lacking gap protection., Comment: 5+4 pages, 3+3 figures

Exchange-antisymmetric pair wavefunctions in fermionic systems can give rise to unconventional superconductors and superfluids with non-trivial transport properties. The realisation of these states in controllable quantum systems, such as ultracold gases, could enable new types of quantum simulations, topological quantum gates, and exotic few-body states. However, p-wave and other antisymmetric interactions are weak in naturally occurring systems, and their enhancement via Feshbach resonances in ultracold systems has been limited by three-body loss. In this work, we create isolated pairs of spin-polarised fermionic atoms in a multi-orbital three-dimensional optical lattice. We spectroscopically measure elastic p-wave interaction energies of strongly interacting pairs of atoms near a magnetic Feshbach resonance and find pair lifetimes to be up to fifty times larger than in free space. We demonstrate that on-site interaction strengths can be widely tuned by the magnetic field and confinement strength but collapse onto a universal single-parameter curve when rescaled by the harmonic energy and length scales of a single lattice site. Since three-body processes are absent within our approach, we are able to observe elastic unitary p-wave interactions for the first time. We take the first steps towards coherent temporal control via Rabi oscillations between free-atom and interacting-pair states. All experimental observations are compared both to an exact solution for two harmonically confined atoms interacting via a p-wave pseudopotential, and to numerical solutions using an ab-initio interaction potential. The understanding and control of on-site p-wave interactions provides a necessary component for the assembly of multi-orbital lattice models, and a starting point for investigations of how to protect such a system from three-body recombination even in the presence of tunnelling., Comment: 15 pages, 4 figures

We propose a general protocol for on-demand generation of robust entangled states of nuclear and/or electron spins of ultracold $^1\Sigma$ and $^2\Sigma$ polar molecules using electric dipolar interactions. By encoding a spin-1/2 degree of freedom in a combined set of spin and rotational molecular levels, we theoretically demonstrate the emergence of effective spin-spin interactions of the Ising and XXZ forms, enabled by efficient magnetic control over electric dipolar interactions. We show how to use these interactions to create long-lived cluster and squeezed spin states.

We propose to simulate bosonic pair creation using large arrays of long-lived dipoles with multilevel internal structure coupled to an undriven optical cavity. Entanglement between the atoms, generated by the exchange of virtual photons through a common cavity mode, grows exponentially fast and is described by two-mode squeezing of effective bosonic quadratures. The mapping between an effective bosonic model and the natural spin description of the dipoles allows us to realize the analog of optical homodyne measurements via straightforward global rotations and population measurements of the electronic states, and we propose to exploit this for quantum-enhanced sensing of an optical phase (common and differential between two ensembles). We discuss a specific implementation based on Sr atoms and show that our sensing protocol is robust to sources of decoherence intrinsic to cavity platforms. Our proposal can open unique opportunities for next-generation optical atomic clocks., Comment: 5 pages + 3 figures + references + supplement; Updated parts of main text and supplement

We theoretically study the dynamics of $n$-level spin-orbit coupled alkaline-earth fermionic atoms with SU($n$) symmetric interactions. We consider three dimensional lattices with tunneling along one dimension, and the internal levels treated as a synthetic dimension, realizing an $n$-leg flux ladder. Laser driving is used to couple the internal levels and to induce an effective magnetic flux through the ladder. We focus on the dense and strongly interacting regime, where in the absence of flux the system behaves as a Mott insulator with suppressed motional dynamics. At integer and fractional ratios of the laser Rabi frequency to the onsite interactions, the system exhibits resonant features in the dynamics. These resonances occur when interactions help overcome kinetic constraints upon the tunneling of atoms, thus enabling motion. Different resonances allow for the development of complex chiral current patterns. The resonances resemble the ones appearing in the longitudinal Hall resistance when the magnetic field is varied. We characterize the dynamics by studying the system's long-time relaxation behavior as a function of flux, number of internal levels $n$, and interaction strength. We observe a series of non-trivial pre-thermal plateaus caused by the emergence of resonant processes at successive orders in perturbation theory. We discuss protocols to observe the predicted phenomena under current experimental conditions., Comment: 21+3 pages, 12+2 figures. Updated to incorporate feedback from referees, including finite size scaling analysis and improved comparison of long-time averages to thermal predictions

Two-dimensional $p+ i p$ superconductors and superfluids are systems that feature chiral behavior emerging from the Cooper pairing of electrons or neutral fermionic atoms with non-zero angular momentum. Their realization has been a longstanding goal because they offer great potential utility for quantum computation and memory. However, they have so far eluded experimental observation both in solid state systems as well as in ultracold quantum gases. Here, we propose to leverage the tremendous control offered by rotating two-dimensional trapped-ion crystals in a Penning trap to simulate the dynamical phases of two-dimensional $p+ip$ superfluids. This is accomplished by mapping the presence or absence of a Cooper pair into an effective spin-1/2 system encoded in the ions' electronic levels. We show how to infer the topological properties of the dynamical phases, and discuss the role of beyond mean-field corrections. More broadly, our work opens the door to use trapped ion systems to explore exotic models of topological superconductivity and also paves the way to generate and manipulate skyrmionic spin textures in these platforms., Comment: Main: 9 pages, 4 figures, Appendix: 14 pages, 3 figures, Improved presentation

Trapped ions boast long coherence times and excellent gate fidelities, making them a useful platform for quantum information processing. Scaling to larger numbers of ion qubits in RF Paul traps demands great effort. Another technique for trapping ions is via a Penning trap where a 2D crystal of hundreds of ions is formed by controlling the rotation of the ions in the presence of a strong magnetic field. However, the rotation of the ion crystal makes single ion addressability a significant challenge. We propose a protocol that takes advantage of a deformable mirror to introduce AC Stark shift patterns that are static in the rotating frame of the crystal. Through numerical simulations we validate the potential of this protocol to perform high-fidelity single-ion gates in crystalline arrays of hundreds of ions.

Cavity QED experiments are natural hosts for non-equilibrium phases of matter supported by photon-mediated interactions. In this work, we consider a cavity QED simulation of the BCS model of superfluidity, by studying regimes where the cavity photons act as dynamical degrees of freedom instead of mere mediators of the interaction via virtual processes. We find an enhancement of long time coherence following a quench whenever the cavity frequency is tuned into resonance with the atoms. We discuss how this is equivalent to enhancement of non-equilibrium superfluidity and highlight similarities to an analogous phenomena recently studied in solid state quantum optics. We also discuss the conditions for observing this enhanced resonant pairing in experiments by including the effect of photon losses and inhomogeneous coupling in our analysis., Comment: 5 pages, 3 figures, Supplemental Material

We propose protocols for the creation of useful entangled states in a system of spins collectively coupled to a bosonic mode, directly applicable to trapped-ion and cavity QED setups. The protocols use coherent manipulations of the spin-boson interactions naturally arising in these systems to prepare spin squeezed states exponentially fast in time. We demonstrate the robustness of the protocols by analyzing the effects of natural sources of decoherence in these systems and show their advantage compared to more standard slower approaches where entanglement is generated algebraically with time., Comment: 6 pages, 4 figures (18 pages, 8 figures with appendices)

We overview the concept of dynamical phase transitions in isolated quantum systems quenched out of equilibrium. We focus on non-equilibrium transitions characterized by an order parameter, which features qualitatively distinct temporal behaviour on the two sides of a certain dynamical critical point. Dynamical phase transitions are currently mostly understood as long-lived prethermal phenomena in a regime where inelastic collisions are incapable to thermalize the system. The latter enables the dynamics to substain phases that explicitly break detailed balance and therefore cannot be encompassed by traditional thermodynamics. Our presentation covers both cold atoms as well as condensed matter systems. We revisit a broad plethora of platforms exhibiting pre-thermal DPTs, which become theoretically tractable in a certain limit, such as for a large number of particles, large number of order parameter components, or large spatial dimension. The systems we explore include, among others, quantum magnets with collective interactions, $\phi^4$ quantum field theories, and Fermi-Hubbard models. A section dedicated to experimental explorations of DPTs in condensed matter and AMO systems connects this large variety of theoretical models., Comment: 37 pages; 10 figures; review article

We perform collective spin measurements to study the buildup of two-body correlations between $\approx10^4$ spin $s=3$ chromium atoms pinned in a 3D optical lattice. The spins interact via long range and anisotropic dipolar interactions. From the fluctuations of total magnetization, measured at the standard quantum limit, we estimate the dynamical growth of the connected pairwise correlations associated with magnetization. The quantum nature of the correlations is assessed by comparisons with short and long time expansions, and numerical simulations. Our work shows that measuring fluctuations of spin populations provides new ways to characterize correlations in quantum many-body systems, for $s>1/2$ spins, Comment: 3+4 figures