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Polarization entanglement holds significant importance for photonic quantum technologies. Recently emerging subwavelength nonlinear quantum light sources, e.g., GaP and LiNbO3 thin films, benefiting from the relaxed phase-matching constraints and volume confinement, has shown intriguing properties, such as high-dimensional hyperentanglement and robust entanglement anti-degradation. Van der Waals (vdW) NbOCl2 crystal, renowned for its superior optical nonlinearities, has emerged as one of ideal candidates for ultrathin quantum light sources [Nature 613, 53 (2023)]. However, polarization-entanglement is inaccessible in NbOCl2 crystal due to its unfavorable nonlinear susceptibility tensor. Here, by leveraging the twist-stacking degree of freedom inherently in vdW systems, we showcase the preparation of tunable polarization entanglement and quantum Bell states. Our work not only provides a new and tunable polarization-entangled vdW photon-pair source, but also introduces a new knob in engineering the entanglement state of quantum light at the nanoscale., Comment: 16 pages,4 figures

The advancing maturity of photonic integrated circuit (PIC) fabrication technology enables the high integration of an increasing number of optical components onto a single chip. With the incremental circuit complexity, the calibration of active phase shifters in a large-scale PIC becomes a crucially important issue. The traditional one-by-one calibration techniques encounter significant hurdles with the propagation of calibration errors, and achieving the decoupling of all phase shifters for independent calibration is not straightforward. To address this issue, we propose a machine-learning approach for globally calibrating the large-scale PIC. Our method utilizes a custom network to simultaneously learn the nonlinear phase-current relations for all thermo-optic phase shifters on the PIC by minimizing the negative likelihood of the measurement datasets. Moreover, the reflectivities of all static beamsplitter components can also be synchronizedly extracted using this calibration method. As an example, a quantum walk PIC with a circuit depth of 12 is calibrated, and a programmable discrete-time quantum walk is experimentally demonstrated. These results will greatly benefit the applications of large-scale PICs in photonic quantum information processing., Comment: 9 pages, 5 figures, and comments are welcome

We propose a scheme to realize quantum controlled-Z (CZ) gates through single gradient metasurface. Using its unique parallel beam-splitting feature, i.e., a series of connected beam splitters with the same splitting ratio, one metasurface can support a CZ gate, several independent CZ gates, or a cascaded CZ gates. Taking advantage of the input polarization determined output path-locking feature, both polarization-encoded and path-encoded CZ gates can be demonstrated on the same metasurface, which further improves the integration level of quantum devices. Our research paves the way for integrating quantum logical function through the metasurface.

Gradient metasurface, formed by a set of subwavelength unit cells with different phase modulation, is widely used in polarized beam splitting (BS) in the classical and quantum optics. Specifically, its phase gradient allows the path and polarization of multiple output lights to be locked by corresponding inputs.Using this unique path-polarization locked property, we demonstrate that the single metasurface can function as sequentially linked beamsplitters, enabling the parallelization of a series of BS processes. Such a parallel BS metasurface provides a multi-beam interference capability for both classical and quantum light manipulation. Taking this advantage, we first prepare path and polarization hybrid entangled states of two, three, and multi photons from unentangled photon sources. Then, the ability of parallel BS-facilitated entanglement is applied to demonstrate entanglement fusion among entangled photon pairs, which can greatly enlarge the entanglement dimension. The principle of parallel BS through the metasurface opens up a versatile way to manipulate the quantum state at the micro/nano scale, which will have potential applications in on-chip quantum optics and quantum information processing.

Symmetric informationally complete measurements are both important building blocks in many quantum information protocols and the seminal example of a generalised, non-orthogonal, quantum measurement. In higher-dimensional systems, these measurements become both increasingly interesting and increasingly complex to implement. Here, we demonstrate an integrated quantum photonic platform to realize such a measurement on three-level quantum systems. The device operates at the high fidelities necessary for verifying a genuine many-outcome quantum measurement, performing near-optimal quantum state discrimination, and beating the projective limit in quantum random number generation. Moreover, it is programmable and can readily implement other quantum measurements at similarly high quality. Our work paves the way for the implementation of sophisticated higher-dimensional quantum measurements that go beyond the traditional orthogonal projections., Comment: 21 pages,13 figures

Photon-number resolving detectors with hundreds of pixels are now readily available, while the characterization of these detectors using detector tomography is computationally intensive. Here, we present a modified detector tomography model that reduces the number of variables that need optimization. To evaluate the effectiveness and accuracy of our model, we reconstruct the photon number distribution of optical coherent and thermal states using the expectation-maximization-entropy algorithm. Our results indicate that the fidelity of the reconstructed states remains above 99%, and the second and third-order correlations agree well with the theoretical values for a mean number of photons up to 100. We also investigate the computational resources required for detector tomography and find out that our approach reduces the solving time by around a half compared to the standard detector tomography approach, and the required memory resources are the main obstacle for detector tomography of a large number of pixels. Our results suggest that detector tomography is viable on a supercomputer with 1~TB RAM for detectors with up to 340 pixels.

Interlayer electronic coupling in two-dimensional (2D) materials enables tunable and emergent properties by stacking engineering. However, it also brings significant evolution of electronic structures and attenuation of excitonic effects in 2D semiconductors as exemplified by quickly degrading excitonic photoluminescence and optical nonlinearities in transition metal dichalcogenides when monolayers are stacked into van der Waals structures. Here we report a novel van der Waals crystal, niobium oxide dichloride, featuring a vanishing interlayer electronic coupling and scalable second harmonic generation intensity of up to three orders higher than that of exciton-resonant monolayer WS2. Importantly, the strong second-order nonlinearity enables correlated parametric photon pair generation, via a spontaneous parametric down-conversion (SPDC) process, in flakes as thin as ~46 nm. To our knowledge, this is the first SPDC source unambiguously demonstrated in 2D layered materials, and the thinnest SPDC source ever reported. Our work opens an avenue towards developing van der Waals material-based ultracompact on-chip SPDC sources, and high-performance photon modulators in both classical and quantum optical technologies.

In this paper, we study the entanglement property of a 4-particle system. In this system, two initially entangled electrons A and C are scattered by two uncorrelated positrons B and D, respectively. We calculate the entanglements among the particles both before and after the double QED scattering ($AB\rightarrow AB, CD\rightarrow CD$). We find that the change of entanglement entropy between subsystems A and B during the scattering processs is proportional to the total cross section, $\sigma_{tot}=\sigma_{AB}\times\sigma_{CD}$. Even though there is no direct interaction between subsystems A and C (or B and D), the scattering process induces entanglement change among them which is also proportional to $\sigma_{tot}$. This result shows some kind of entanglement sharing property in multipartite system. In order to further investigate the entanglement sharing, we calculate the entanglement monotones which quantify the genuine multipartite entanglement in a multipartite system. For our chosen scattering process, $e^+e^-\rightarrow\mu^+\mu^-$, however, we find that the outgoing state is a W-type 4-partite entangled state which has no genuine 4-partite entanglement., Comment: 17 pages, 6 figures

As an important degree of freedom (DoF) in integrated photonic circuits, the orthogonal transverse mode provides a promising and flexible way to increasing communication capability, for both classical and quantum information processing. To construct large-scale on-chip multimode multi-DoF quantum systems, a transverse mode-encoded controlled-NOT (CNOT) gate is necessary. Here, through design and integrate transverse mode-dependent directional coupler and attenuators on a silicon photonic chip, we demonstrate the first multimode implementation of a two-qubit quantum gate. With the aid of state preparation and analysis parts, we show the ability of the gate to entangle two separated transverse mode qubits with an average fidelity of $0.89\pm0.02$ and the achievement of 10 standard deviations of violations in the quantum nonlocality verification. In addition, a fidelity of $0.82\pm0.01$ was obtained from quantum process tomography used to completely characterize the CNOT gate. Our work paves the way for universal transverse mode-encoded quantum operations and large-scale multimode multi-DoF quantum systems.

On-chip bright quantum sources with multiplexing ability are extremely high in demand for the integrated quantum networks with unprecedented scalability and complexity. Here, we demonstrate an ultrabright and broadband biphoton quantum source generated in a lithium niobate microresonator system.Without introducing the conventional domain poling, the on-chip microdisk produces entangled photon pairs covering a broad bandwidth promised by natural phase matching in spontaneous parametric down conversion.Experimentally, the multiplexed photon pairs are characterized by $30\ \rm nm$ bandwidth limited by the filtering system, which can be furthered enlarged.Meanwhile, the generation rate reaches $5.13\ {\rm MHz}/\upmu \rm W$ with a coincidence-to-accidental ratio up to $804$.Besides, the quantum source manifests the prominent purity with heralded single photon correlation $g_H^{(2)}(0)=0.0098\pm0.0021$ and energy-time entanglement with excellent interference visibility of $96.5\%\pm1.9\%$. Such quantum sources at the telecommunication band pave the way for high-dimensional entanglement and future integrated quantum information systems., Comment: 8 pages,4 figures

Non-reciprocal photonic devices are essential components of classical optical information processing. It is interesting and important to investigate their feasibility in the quantum world. In this work, the quantum properties of an on-chip silicon nitride (SiN)-based magneto-optical (MO) isolator were studied using a single-photon non-reciprocal dynamical transmission experiment. The measured isolation ratio for single photons achieved was 12.33 dB, which proved the functionality of our on-chip isolator. The quantum coherence of the passing single photons was further verified using high-visibility quantum interference. Our work will promote on-chip isolators within the integrated quantum circuits and help introduce novel phenomena in quantum information processes., Comment: 5 pages, 4figures

Path identiy induces a broad interest in recent years due to the foundation for numerous novel quantum information applications. Here, we experimentally demonstrate quantum coherent superposition of two different origins of a four-photon state, where multi-photon frustrated interference emerges from the quantum indistinguishability by path identity. The quantum state is created in four probabilistic photon-pair sources on one integrated silicon photonic chip, two combinations of which can create photon quadruplets. Coherent elimination and revival of distributed four-photons are fully controlled by tuning phases. The experiment gives rise to peculiar quantum interference of two possible ways to create photon quadruplets rather than interference of different intrinsic properties of photons. Besides many known potential applications, this new kind of multi-photon nonlinear interference enables the possibility for various fundamental studies such as nonlocality with multiple spatially separated locations., Comment: 6 pages, 4 figures, article

Topological photonics has been introduced as a powerful platform for integrated optics, since it can deal with robust light transport, and be further extended to the quantum world. Strikingly, valley-contrasting physics in topological photonic structures contributes to valley-related edge states, their unidirectional coupling, and even valley-dependent wave-division in topological junctions. Here, we design and fabricate nanophotonic topological harpoon-shaped beam splitters (HSBSs) based on $120$-deg-bending interfaces and demonstrate the first on-chip valley-dependent quantum information process. Two-photon quantum interference, namely, HongOu-Mandel (HOM) interference with a high visibility of $0.956 \pm 0.006$, is realized with our 50/50 HSBS, which is constructed by two topologically distinct domain walls. Cascading this kind of HSBS together, we also demonstrate a simple quantum photonic circuit and generation of a path-entangled state. Our work shows that the photonic valley state can be used in quantum information processing, and it is possible to realize more complex quantum circuits with valley-dependent photonic topological insulators, which provides a novel method for on-chip quantum information processing., Comment: 6 pages, 4 figures

Integrated photonics is becoming an ideal platform for generating two-photon entangled states with high brightness, high stability and scalability. This high brightness and high quality of photon pair sources encourages researchers further to study and manipulate multi-photon entangled states. Here, we experimentally demonstrate frequency-degenerate four-photon entangled state generation based on a single silicon nanowire 1 cm in length. The polarization encoded entangled states are generated with the help of a Sagnac loop using additional optical elements. The states are analyzed using quantum interference and state tomography techniques. As an example, we show that the generated quantum states can be used to achieve phase super-resolution. Our work provides a method for preparing indistinguishable multi-photon entangled states and realizing quantum algorithms in a compact on-chip setting., Comment: 9 pages, 4 figures

By harnessing the quantum states of light for illumination, precise phase and absorption estimations can be achieved with precision beyond the standard quantum limit. Despite their significance for precision measurements, quantum states are fragile in noisy environments which leads to difficulties in revealing the quantum advantage. In this work, we propose a scheme to improve optical absorption estimation precision by using the correlated photon pairs from spontaneous parametric down-conversion as the illumination. This scheme performs better than clasical illumination when the loss is below a critical value. Experimentally, the scheme is demonstrated by a scanning transmission type microscope that uses correlated photon illumination. As a result, the signal-to-noise ratio (SNR) of a two-photon image shows a $1.36$-fold enhancement over that of single-photon image for a single-layer graphene with a $0.98$ transmittance. This enhancement factor will be larger when using multi-mode squeezed state as the illumination., Comment: 7 Pages, 3 figures