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This paper addresses the influence of land topography and cover on 3D radiative effects under cloudless skies in the Hornsund area, Spitsbergen, Svalbard. The authors used Monte Carlo simulations of solar radiation transfer over a heterogeneous surface to study the impact of a non-uniform surface on: (1) the spatial distribution of irradiance transmittance at the fjord surface under cloudless skies; (2) the spectral shortwave aerosol radiative forcing at the fjord surface; (3) normalized nadir radiance at the Top Of the Atmosphere (TOA) over the fjord. The modelled transmittances and radiances over the fjord are compared to the transmittances and radiances over the open ocean under the same conditions. The dependence of the 3D radiative effects on aerosol optical thickness, aerosol type, surface albedo distribution, solar azimuth and zenith angle and spectral channel is discussed. The analysis was done for channels 3 (459-479 nm) and 2 (841-876 nm) of the MODIS radiometer. In the simulations a flat water surface was assumed. The study shows that snow-covered land surrounding the fjord strongly modifies the radiation environment over the fjord surface. The enhancement of the mean irradiance transmittance over the fjord with respect to the open ocean is up to 0.06 for channel 3. The enhancement exceeds 0.11 in the vicinity of sunlit cliffs. The influence of the snow-covered land on the TOA radiance over the fjord in channel 3 is comparable to the impact of an increase in aerosol optical thickness of over 100%, and in lateral fjords of up to several hundred percent. The increase in TOA radiance is wavelength dependent. These effects may affect retrievals of aerosol optical thickness.

Black Carbon (BC) is a significant forcing agent in the Arctic, but substantial uncertainty remains to quantify its climate effects due to the complexity of the different mechanisms involved, in particular related to processes in the snow-pack after deposition. In this study, we provide detailed and unique information on the evolution and variability of BC content in the upper surface snow layer during the spring period in Svalbard (Ny-Ålesund). Two different snow-sampling strategies were adopted during spring 2014 and 2015, providing the refractory BC (rBC) mass concentration variability on a seasonal/daily and daily/hourly time scales. The present work aims to identify which atmospheric variables could interact and modify the mass concentration of BC in the upper snowpack, the snow layer which BC particles affects the snow albedo. Despite the low BC mass concentrations, a relatively high daily variability was observed. Atmospheric, meteorological, and snow-related physico -chemical parameters were considered in a multiple statistical model to separate the factors determining observations. Precipitation events were the main drivers of the BC variability. Snow metamorphism and activation of local sources during the snow melting periods appeared to play a non-negligible role (wind resuspension in specific Arctic areas where coal mines were present). The BC content in the snow resulted in being statistically decoupled from the atmospheric BC load. [ABSTRACT FROM AUTHOR]

Black Carbon (BC) is a major forcing agent in the Arctic but substantial uncertainty remains to quantify its climate effects due to the complexity of mechanisms involved. In this study, we provide unique information on processes driving the variability of BC mass concentration in surface snow in the Arctic. Two different snow-sampling strategies were adopted during spring 2014 and 2015, focusing on the refractory BC (rBC) mass Ny-Ålesund concentration daily/hourly variability on a seasonal/daily time scale (referred to as 80-days and 3-days experiments). Despite the low rBC mass concentrations (never exceeding 22 ng g-1), a daily variability of up to 4.5 ng g-1 was observed. Atmospheric, meteorological and snow-related physico-chemical parameters were considered in multiple statistical models to understand the factors behind the observed variation of rBC mass concentrations. Results indicate that the main drivers of the variation of rBC are the precipitations events, snow metamorphism (melting-refreezing cycles, surface hoar formation and sublimation) and the activation of local sources (wind resuspension) during the snow melting periods. The rBC in the snow seems de-coupled with the atmospheric BC load. Our results highlighted a common association of snow rBC with coarse mode particles number concentration and with snow precipitation events. [ABSTRACT FROM AUTHOR]

The aim of the presented study was to investigate the impact on the radiation budget of biomass burning smoke plume transported from Alaska to high Arctic region (Ny-Alesund, Svalbard) in early July 2015. This high aerosol load event is considered exceptional in the last 25 years with mean aerosol optical depth increased by the factor of 10 in comparison to the average summer background values. We utilised in-situ data with hygroscopic growth equations as well as remote sensing measurements as inputs to radiative transfer models with an objective to estimate biases associated with (i) hygroscopicity, (ii) variability of ω profiles and (iii) plane-parallel closure of the modelled atmosphere. A chemical weather model with satellite-derived biomass burning emissions was used to interpret the transport and transformations pathways. Provided MODTRAN simulations resulted in the mean aerosol direct radiative forcing on the level of -78.9 W m-2 and -47.0 W m-2 at the surface and the top of the atmosphere respectively for the mean value of aerosol optical depth equal to 0.64 at 550 nm. It corresponded to the average clear-sky direct radiative forcing of -43.3 W m-2 estimated by radiometers and model simulations. Furthermore, model-derived aerosol direct radiative forcing efficiency reached on average -126 W m-2 / τ550 and -71 W m-2 / τ550 at the surface and at the top of the atmosphere. Estimated heating rate up to 1.8 K day-1 inside the BB plume implied vertical mixing with the turbulent kinetic energy of 0.3 m2 s-2. Ultimately, uncertainty connected with the plane-parallel atmosphere approximation altered results by about 2 W m-2. [ABSTRACT FROM AUTHOR]