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The recognition criterion for discovery of a new chemical element includes two aspects, the characterization properties and the assignment properties. In this paper, we will discuss the status of element 115 experiments that have been performed in Dubna, Russia, highlighting the characterization and assignment properties as they specifically relate to a recent experiment. After discussing the status of what is known about the decay properties of element 115 [Yu.Ts. Oganessian et al. Phys. Rev. C 72 (2005) Art. No 034611], observed previously using the Dubna Gas-Filled Recoil Separator, we will discuss the prior chemical studies that have been performed on the Db descendant of element 115 [S.N. Dmitriev et al. Mendeleev Commun.(1) (2005) 1–4]. Following the success of that experiment, some additional chemical information was desired. Two separation chemistries were then developed at LLNL and JINR. LLNL utilized reversed phase chromatography and JINR utilized anion exchange chromotography to perform not only +4/+5 separations, but also intra-group separations, where Nb-like and Ta-like fractions were eluted. The results from an experiment using these chemistries for the first time during December 2005 in Dubna, Russia, will be compared with prior chemical results. We will conclude with a discussion of possible enhancements to the work already performed and the current status of the future experimental plans.

We have studied the dependence of the production cross-sections of the isotopes 282,283112 and 286–288114 on the excitation energy of the compound nuclei 286112 and 290114. The maximum cross-sections of the xn-evaporation channels for the reaction 238U(48Ca,xn)286-x 112 were measured to be: σ 3n = 2.5 -1.1 +1.8 pb and σ 4n = 0.6 -0.5 +1.6 pb; for the reaction 242Pu(48Ca,xn)290-x 114: σ 2n ∼ 0.5 pb, σ 3n = 3.6 -1.7 +3.4 pb and σ 4n = 4.5 -1.9 +3.6 pb. In the reaction 233U(48Ca, 2-4n)277–279 112 we measured an upper cross-section limit of σ xn ≤ 0.6 pb. An increase of σ ER in the reactions of actinide targets with 48Ca can be due to the expected increase of the survivability of the excited compound nucleus upon closer approach to the closed neutron shell N = 184. The observed nuclear decay properties of the nuclides with Z = 104–118 are compared with theoretical nuclear mass calculations and the systematic trends of α-decay properties. As a whole, they give a consistent pattern of decay of the 18 even-Z neutron-rich nuclides with Z = 104–118 and N = 163–177.

neutron-rich isotopes 242,244 Pu, 243 Am, 245,248 Cm and 249 Cf with 48 Ca projectiles. The decay properties of the synthesized nuclei are consistent with the consecutive α-decays originating in the decays of parent nuclides 286,287,288,289 114, 287,288 115, 290,291,293 116 and 294 118 produced in the 2n- to 5n-evaporation channels. The present observations can be considered to be experimental evidence of the existence of the “island of stability” of superheavy elements.

Summary We measured the (n, 2n) cross sections for neutron energies from 13.7 to 15.1 MeV on 239Pu and 241Am by α- and γ-spectroscopy measurements of the post–irradiation 238Pu/239Pu and 240Am/241Am ratios relative to the (n, 2n) cross sections of 196Au and other calibration reactions. Statistical errors on the measurements were not more than a few percent. Cross–section values ranged from 228 to 214 millibarns for the reaction on 239Pu and from 260 to 222 millibarns for the 241Am reaction for neutron energies from 13.7 to 15.1 MeV.

This paper presents results of the experiments aimed at producing long-lived superheavy elements located near the spherical-shell closures with Z ⩾ 114 and N ⩾ 172 in the 244Pu + 48Ca and 248Cm + 48Ca reactions. The large measured α-particle energies of the newly observed nuclei, together with the long decay times and spontaneous fission terminating the chains, offer evidence of the decay of nuclei with high atomic numbers. The decay properties of the synthesized nuclei are consistent with the consecutive α-decays originating from the parent nuclides 288, 289114 and 292116, produced in the 3n and 4n evaporation channels with cross-sections of about a picobarn. The present observations can be considered as experimental evidence of the existence of the “island of stability” of superheavy elements.

In this paper, we present the Monte Carlo Random Probability (MCRP) calculational method details that were developed for the determination of random correlations in a set of unrelated data. After finding random correlations, we further process the correlations by applying nuclear property systematics. We compare the results of MCRP with methods presented in other references. The MCRP method can provide a conservative estimate of the random probability associated with observed events that takes into account the entire background observed in the experiment and any other running conditions (noise, decay of long-lived species, etc.) which may have been sporadic or intermittent. We discuss a particular example of a set of correlated alpha decays and its interpretation as a candidate decay chain.

This article reports the results of experiments aimed at producing hypothetical long-lived superheavy elements located near the spherical-shell closures with Z≥114 and N≥72. For the synthesis of superheavy nuclei, we used a combination of neutron-rich reaction partners, with a 244Pu target and a 48Ca projectile. The sensitivity of the present experiment exceeded by more than two orders of magnitude previous attempts at synthesizing superheavy nuclides in reactions of 48Ca projectiles with actinide targets. We observed new decay sequences of genetically linked alpha decays terminated by spontaneous fission. The high measured alpha-particle energies, together with the long decay times and spontaneous fission terminating the chains, offer evidence for the decay of nuclei with high atomic numbers. The decay properties of the synthesized nuclei are consistent with the consecutive alpha decays originating from the parent nuclides 288,289114, produced in the 3n-and 4n-evaporation channels with cross sections of about a picobarn. The present observations can be considered experimental evidence for the existence of the “island of stability” of superheavy elements and are discussed in terms of modern theoretical approaches.

In bombardment of ${}^{244}\mathrm{Pu}$ with ${}^{48}\mathrm{Ca}$, we observed a decay sequence consisting of an implanted heavy atom, three subsequent $\ensuremath{\alpha}$ decays, and a spontaneous fission (SF), all correlated in time and position. The measured $\ensuremath{\alpha}$ energies and corresponding time intervals were ${E}_{\ensuremath{\alpha}}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}9.71$ MeV ( $\ensuremath{\Delta}t\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}30.4$ s), 8.67 MeV ( $\ensuremath{\Delta}t\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}15.4$ min), and 8.83 MeV ( $\ensuremath{\Delta}t\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}1.6$ min); for the SF ( $\ensuremath{\Delta}t\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}16.5$ min), the total deposited energy was approximately 190 MeV. The $\ensuremath{\alpha}$-particle energies together with the decay times and SF terminating the chain offer evidence of the decay of nuclei with high atomic numbers. This decay chain is a good candidate for originating from the $\ensuremath{\alpha}$ decay of the parent nucleus ${}^{289}114$, produced with a cross section of about 1 pb.

Several new high-spin states are observed in the prompt $\ensuremath{\gamma}$-rays emitted from the neutron-rich, odd-$Z$ ${}^{145,147}\mathrm{La}$ fragments produced in the spontaneous fission of ${}^{252}\mathrm{Cf}.$ Alternating parity bands are extended up to spins 41/2 and 43/2 in ${}^{145,147}\mathrm{La},$ respectively. A new band completes the evidence for two sets of parity doublets expected for octupole correlations. Eight $B(E1)/B(E2)$ ratios (four new) between two bands in ${}^{145}\mathrm{La}$ are all essentially constant and somewhat larger than similar ratios in ${}^{143,144}\mathrm{Ba},$ where stable octupole deformation and/or correlations are reported. The new ratios out of the ${31/2}^{\ensuremath{-}}$ levels in both nuclei show a sharp spike compared to other states, presumably from a strong reduction in $E2$ strengths in this backbending region. In ${}^{145}\mathrm{La},$ collective bands show competition and coexistence between symmetric and asymmetric shapes. Band crossings occur in both nuclei around $\ensuremath{\Elzxh}\ensuremath{\omega}\ensuremath{\approx}0.26--0.30 \mathrm{MeV}.$ Their backbends are associated with the alignment of two ${i}_{13/2}$ neutrons according to cranked shell model calculations.

Optical measurements of a clean, $2\ensuremath{-}\ensuremath{\mu}\mathrm{C}$ ${}^{233}\mathrm{U}$ sample were made to verify light emission from gamma ray decay of the first excited nuclear level in ${}^{229}\mathrm{Th}$. The results showed that the light observed in earlier studies was likely to be caused by alpha-particle induced fluorescence of air. In vacuo, no light emission was discernable. The ${}^{229}\mathrm{Th}$ system, therefore, does not appear to provide the level of access for studying atomic-nuclear interactions suggested by the previous measurements.

From γ-γ-γ coincidence measurements in the spontaneous fission of252Cf, level energies were established for spins 14+ to 20+ in many neutron-rich nuclei. New isotopes160Sm and162Gd were identified. The yrast bands of152,154,156Nd,156,158,160Sm, and160,162Gd exhibit remarkably near-identical transition energies and moments of inertia which are shifted by the same constant amounts for every spin state from 2+ to 12+ or 14+ for nuclei differing by 2n, 4n, 2p, 4p, α, α+2p, and α+2n. These shifted identical bands (SIB) are a new phenomenon. Analysis of all known even-even proton- to neutron-rich nuclei from Ba (Z = 56) to Os (Z = 76) reveal no SIB for proton-rich nuclei and only a few additional cases of SIB for the most neutron-rich pairs aroundN = 98–102 separated by 2n and 2p. The levels in8107Mo were extended and levels in109Mo identified for the first time.

The phenomenon of cold (neutronless) alpha ternary fission in spontaneous fission of {sup 252}Cf was experimentally observed by triple gamma coincidence technique with Gammasphere with 72 gamma-ray detectors. Correlated pairs of {sub 36}Kr-{sub 60}Nd, {sub 38}Sr-{sub 58}Ce, {sub 40}Zr-{sub 56}Ba, {sub 42}Mo-{sub 54}Xe, {sub 44}Ru-{sub 52}Te, and {sub 46}Pd-{sub 50}Sn were observed to be associated with {alpha} ternary fission of {sup 252}Cf. Yields of cold {alpha} ternary fission were extracted. {copyright} {ital 1998} {ital The American Physical Society}

The phenomenon of cold (neutronless) binary and ternary fission in spontaneous fission of252 Cf was experimentally observed by triple gamma coincidence technique with Gammasphere with 72 gamma-ray detectors. Many correlated pairs for both binary and ternary (4He,10Be) fission were observed in the spontaneous fission of252 Cf. Yields of cold ternary and cold binary fission were extracted. These results are compared with the theoretical calculations using M3Y nucleon-nucleon potential and WKB approximation for barrier penetration.

Ten new transitions in {sup 107}Mo have been observed and levels in {sup 109}Mo are identified for the first time in a {gamma}-{gamma}-{gamma} coincidence study from the spontaneous fission of {sup 252}Cf with 72 Compton suppressed Ge detectors in Gammasphere. Two sets of bands, each set intertwined by E1 transitions are observed in {sup 107}Mo and one such set in {sup 109}Mo. The observed level schemes are interpreted in terms of possible octupole deformation originating from the strong interaction of the h{sub 11/2} and d{sub 5/2} neutron shells. {copyright} {ital 1997} {ital The American Physical Society}

Spontaneous fission of252Cm was studied with 72 large Compton suppressed Ge detectors in Gammasphere. New isotopes160Sm and162Gd were identified. Through X-ray-γ and γ-γ-γ coincidence measurements, level energies were established to spins 14+ to 20+ in152, 154, 15660Nd92, 94, 96156, 158, 16062Sm94, 96, 98 and160, 16264Gd96, 98. These nuclei exhibit a remarkable variety of identical bands and bands where the energies and moments of inertia are shifted by the same constant amounts for every spin state from 2+ to 12+ for various combinations of nuclei differing by 2n, 4n, 2p, 4p and α.

From an experiment with Gammasphere and a 252 C spontaneous fission source, two bands with signatures -i and +i are identified in 153 Nd Also several new transitions in 149 Nd are observed for the first time. The band with signature -i in 153 Nd shows no back bending, similar to the one observed in 161 Er . The signature splitting observed in the ground band of 153 Nd is similar to the ones observed in N=93 isotones in this mass region. In 149 Nd the new transitions are placed into a band with a proposed configuration of [Formula: see text].

In bombardments of $^{244}\mathrm{Pu}$ with $^{34}\mathrm{S}$ we discovered the \ensuremath{\alpha}-decaying nuclide $^{273}110$. We conducted an extensive off-line search of the raw data for event sequences which fit the expected pattern of implantation in a position-sensitive detector and subsequent decay of $^{273}110$ and its descendants. We observed one three-member sequence of genetically linked \ensuremath{\alpha} decays, resulting in ${\mathit{E}}_{\mathrm{\ensuremath{\alpha}}}$=11.35 MeV, a half-life of 0.${3}_{\mathrm{\ensuremath{-}}0.2}^{+1.3}$ ms, and a production cross section of about 0.4 pb for $^{273}110$. Other possible $^{273}110$ event chains were also observed. The measured \ensuremath{\alpha}-particle energy for the N=163 nuclide $^{273}110$ provides direct evidence for a neutron shell closure at N=162. \textcopyright{} 1996 The American Physical Society.

The {gamma} transitions in {sup 147}Ba, {sup 149}Ce, and {sup 151,153}Nd have been identified from {gamma}-{gamma}-{gamma}, {gamma}-{gamma}, {ital x}-{gamma}, and {ital x}-{gamma}-{gamma} coincidence studies of spontaneous fission of {sup 252}Cf. The yrast positive parity band in {sup 149}Ce is assigned to an {ital i}{sub 13/2}, neutron favored signature. The yrast negative parity band in {sup 149}Ce is assigned a {ital h}{sub 9/2} proton favored signature. The positive parity band in {sup 151}Nd corresponds to the positive parity band in {sup 149}Ce. The negative parity band in {sup 153}Nd corresponds to the negative parity bands of {sup 149}Ce and {sup 161}Er. The band observed in {sup 147}Ba is built on the {ital h}{sub 9/2} orbital. The plots for {ital J}{sub 1} in these isotopes are remarkably similar, supporting our assignments. {copyright} {ital 1996 The American Physical Society.}

Coincidence \ensuremath{\gamma}-ray data from the spontaneous fission of $^{242}\mathrm{Pu}$ were collected at the Lawrence Berkeley Laboratory high purity Ge (HPGe) array, GAMMASPHERE. Data from several cold-fission (0 neutron emission) isotopic pairs were observed and are presented. An interesting trend in the fractional population of cold-fission events was observed and is discussed. Relative yields of Zr-Xe, Sr-Ba, and Mo-Te pairs were measured. The Zr-Xe system has the most complete data set. Some speculations on the trend in the number of neutrons emitted as a function of the mass of the Xe isotope populated are presented. Comparisons between the yields from the spontaneous fission of $^{242}\mathrm{Pu}$ and the yields from thermal-neutron-induced fission of $^{241}\mathrm{Pu}$ are also presented. \textcopyright{} 1996 The American Physical Society.

In bombardments of ${}^{238}$U targets with 186-MeV ${}^{34}$S projectiles we discovered the $\ensuremath{\alpha}$-decaying nuclide ${}^{267}$108 with a half-life of ${19}_{\ensuremath{-}10}^{+29}$ ms, ${E}_{\ensuremath{\alpha}}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}9.74$ to 9.87 MeV, and a production cross section of about 2.5 pb. The new nuclide was identified by measuring correlations in energy, time, and position to establish genetic links between its implantation in a position-sensitive silicon detector and subsequent $\ensuremath{\alpha}$ decay followed by $\ensuremath{\alpha}$ decays of known descendant nuclides.

With prompt \ensuremath{\gamma}-ray and x-ray spectroscopy on fission fragments, several new transitions in $^{109,111}\mathrm{Ru}$ have been identified. Angular correlation analysis of several of the new transitions yield evidence of a stretched E2 band structure. Qualitative Nilsson model arguments, systematics, and triaxial rotor+particle calculations support our hypothesis that the observed band is built on the unique parity \ensuremath{\nu}${\mathit{h}}_{11/2}$ orbital.

In bombardments of 248Cm with 22Ne we discovered two new isotopes, 265106 and 266106, by establishing genetic links between α decays of the 106 nuclides and spontaneous fission (SF) or α decays of the daughter (or granddaughter) nuclides. For 266106 we measured Eα = 8.63 ± 0.05 MeV followed by the SF decay of 262104 for which we measured a half-life value of 1.2+1.00.5 s. For 265106 we measured Eα = 8.71–8.91 MeV. We estimated α half-lives of 10–30 s for 266106 and 2–30 s for 265106 with SF branches of approximately 50% or less. The decay properties of 266106 indicate a large enhancement in the SF stability of this N = 160 nuclide and confirm the existence of the predicted deformed shells N = 162 and Z = 108.

We have measured the mass and total kinetic energy distributions from the spontaneous fission of 252No, 254No, 256[104] and 258[104]. The results, in combination with earlier measurements for 256No, 258No and 262No, show a sharp transition from asymmetrical mass division in 256No to symmetrical division for 258No and 262No. However, all isotopes of element 104, including 260[104], appear to yield broadly symmetrical mass distributions. The total kinetic energies around 200 MeV for the element 104 isotopes indicate that they fission by the low-energy mode of bimodal fission. Recent calculations of static potential energy surfaces including higher-order asymmetric deformations suggest that the outer fission barrier is well below the ground state in energy, which accounts for the observance of the symmetric mass division.

We investigated the nuclear properties of several mendelevium isotopes produced in the reactions of heavy ions with 245Esg. We measured the alpha particles, spontaneous fissions (SF), and photons emitted by counting samples resulting from chemical and/or mass separations. The 256Md half-life is (78.1 ± 1.8) min; it decays primarily by electron capture (EC), but also by alpha emission (11 ± 3)% of the time. The 256Md ground state has J ⩽ 2 (probably Jπ = 1−), and a mass excess of (87.611 ± 0.053) MeV. The 257Md half-life is (5.523 ± 0.050) h; it decays primarily by EC, but also by alpha emission (15.2 ± 2.6)% of the time and by SF less than 1% of the time. The 256Md mass excess is (88.989 ± 0.003) MeV. The 258Mdg (Jπ = 8−) half-life is (51.50 ± 0.29) d. It decays by alpha emission; the sum of SF, EC, and β− decay branches is less than 3 × 10−3 %. The alpha decay of 258Mdg populates 254Esm (0.60 ± 0.08)% of the time. The 256Mdg mass excess is (91.691 ± 0.007) MeV. The half-life of J π = 1 − 258 Md m is (57.0 ± 0.9) min. It decays by EC; the branch for decay by alpha emission is less than 1.2%. The sum of SF and β− decay branches is less than 30%. The half-life of 259Md is (1.60 ± 0.06) h; it decays primarily by SF. The alpha decay branch of 259Md is less than 1.3%. From the 259Md half-life we calculated a SF hindrance factor associated with the 7 2 − [514] proton configuration of 3.6 × 106. From our data we proposed partial level schemes for 252Es, 253Es, and 254Es.

The fission cross sections of 247Cm, 254Es, and 250Cf are measured with the Rensselaer intense neutron spectrometer from 0.1 eV to 80 keV. The cross sections are normalized to the 235U ENDF/B-V bro...

Thirty‐four new nuclides with Z = 104–116, 118 and N = 161–177 have been synthesized in the complete‐fusion reactions of 238U, 237Np, 242,244Pu, 243Am, 245,248Cm, and 249Cf targets with 48Ca beams. The masses of evaporation residues were identified through measurements of the excitation functions of the xn‐evaporation channels and from cross bombardments. The decay properties of the new nuclei agree with those of previously known heavy nuclei and with predictions from different theoretical models. A discussion of self‐consistent interpretations of all observed decay chains originating from the parent isotopes 282,283112, 282113, 286–289114, 287,288115, 290–293116, and 294118 is presented. Decay energies and lifetimes of the neutron‐rich superheavy nuclei as well as their production cross sections indicate a considerable increase in the stability of nuclei with the approach to the theoretically predicted nuclear shells with N = 184 and Z = 114.

This project consisted of three major research areas: (1) development of a solid Pu ceramic target for the MASHA separator, (2) chemical separation of nuclear decay products, and (3) production of new isotopes and elements through nuclear reactions. There have been 16 publications as a result of this project, and this collection of papers summarizes our accomplishments in each of the three areas of research listed above. The MASHA (Mass Analyzer for Super-Heavy Atoms) separator is being constructed at the U400 Cyclotron at the Flerov Laboratory of Nuclear Reactions in Dubna, Russia. The purpose of the separator is to physically separate the products from nuclear reactions based on their isotopic masses rather than their decay characteristics. The separator was designed to have a separation between isotopic masses of {+-}0.25 amu, which would enable the mass of element 114 isotopes to be measured with outstanding resolution, thereby confirming their discovery. In order to increase the production rate of element 114 nuclides produced via the {sup 244}Pu+{sup 48}Ca reaction, a new target technology was required. Instead of a traditional thin actinide target, the MASHA separator required a thick, ceramic-based Pu target that was thick enough to increase element 114 production while stillmore » being porous enough to allow reaction products to migrate out of the target and travel through the separator to the detector array located at the back end. In collaboration with UNLV, we began work on development of the Pu target for MASHA. Using waste-form synthesis technology, we began by creating zirconia-based matrices that would form a ceramic with plutonium oxide. We used samarium oxide as a surrogate for Pu and created ceramics that had varying amounts of the starting materials in order to establish trends in material density and porosity. The results from this work are described in more detail in Refs. [1,4,10]. Unfortunately, work on MASHA was delayed in Russia because it was found that the efficiency of transporting products from the target chamber to the detector array was much too low for applications in heavy element experiments where production rates are on the order of one atom per day or less. Work continues on the MASHA separator, and once the efficiency has been improved, we plan to continue our work on the Pu target for future element 114 experiments. Due to the delays of the MASHA separator, work on establishing the identity of heavy element species produced through nuclear reactions focused instead on chemical separations. In particular, element 115 decays through a series of alpha decays, terminating with an element 105 isotope with a long half-life ({approx} 1 day). By chemically separating the element 105 daughter and observing its subsequent fission decay, the identity of the original parent nucleus can be established through the genetic correlation of the initial series of alpha decays. Chemical separations of element 105 were developed in Switzerland, Russia, and at LLNL. Over the course of two experiments, reaction products from the {sup 243}Am+{sup 48}Ca reaction were collected in a copper block and subsequently processed for chemical separation of the Group Five elements [8,9,13,15]. The Group Five elements were initially separated from the Group Four species, and then the samples were sub-divided into tantalum and niobium fractions. All of the fission events were observed in the tantalum fractions, which implied that element 105 behaved more like tantalum under the chemical conditions of these experiments. These experiments were very successful, and not only demonstrated that chemical separation could be performed on single atoms of interest, but also lent proof to the identity of the parent nucleus as element 115. Subsequent analysis of the alpha spectra taken during the experiment further prove that the fission events observed during the two experiments came from element 105 as the decay daughter of element 115 and could not attributed to interference from other background species [16]. The final aspect of this project was the production of new isotopes and elements. All of the experiments were performed in Dubna at the U400 Cyclotron and the results are described in more detail in Refs. [2,3,5-8,11,12,14]. The first experiments were designed to establish the decay properties of isotopes of elements 112, 114, and 116 [5]. Because these isotopic signatures were established through these initial experiments, the discovery of element 118 [11] was possible, since the 118 nuclides decayed into these previously studied isotopes. This was the first successful report of the discovery of element 118, which was reported by the media to a large extent. The last experiment that was performed for this project was the production and detection of a new isotope of element 113 [14].« less

We have made the first measurement of the number of neutrons emitted from the spontaneous fission of a nuclide in which very high fragment energies dominate the fission process. In bombardments of {sup 254}Es, we produced a large sample of 28-d {sup 260}Md, which was neutron counted in a 1-m-diameter spherical tank containing a Gd-doped scintillator solution. The average number of neutrons emitted per fission is only 2.58{plus minus}0.11, substantially less than for other actinides. A linear dependence of neutron multiplicity on fragment-excitation energy is observed to the highest values of total kinetic energy.

We have measured cross sections for the formation of actinide transfer products in the reaction of 72-MeV $^{13}\mathrm{C}$ projectiles with $^{254}\mathrm{Es}^{\mathrm{g}}$ targets. The pattern of nuclide yields is similar to those observed in the reactions of heavier ions with $^{254}\mathrm{Es}^{\mathrm{g}}$. We have constructed the primary element yields from these results and show that the total cross section for transfer reactions is 58 mb. The total reaction cross section is about 300 mb. Lawrencium isotopes are formed with larger cross sections than are consistent with the trends of the transfer-product distributions; we explain this in terms of massive transfer, and model the lawrencium yields with an evaporation code.

Thirty‐four new nuclides with Z = 104–116, 118 and N = 161–177 have been synthesized in the complete‐fusion reactions of 238U, 237Np, 242,244Pu, 243Am, 245,248Cm, and 249Cf targets with 48Ca beams. The masses of evaporation residues were identified through measurements of the excitation functions of the xn‐evaporation channels and from cross bombardments. The decay properties of the new nuclei agree with those of previously known heavy nuclei and with predictions from different theoretical models. A discussion of self‐consistent interpretations of all observed decay chains originating from the parent isotopes 282,283112, 282113, 286–289114, 287,288115, 290–293116, and 294118 is presented. Decay energies and lifetimes of the neutron‐rich superheavy nuclei as well as their production cross sections indicate a considerable increase in the stability of nuclei with the approach to the theoretically predicted nuclear shells with N = 184 and Z = 114.

From an experiment with Gammasphere and a ${}^{252}\mathrm{Cf}$ spontaneous fission source, a new negative-parity band in ${}^{154}\mathrm{Nd}$ and new negative-parity levels in ${}^{152}\mathrm{Nd}$ were identified and the yrast bands were extended to ${18}^{+}$ in ${}^{154}\mathrm{Nd}$ and ${20}^{+}$ in ${}^{152}\mathrm{Nd}$ in a triple gamma coincidence study. These new negative-parity bands are consistent with octupole vibrational mode. There is a constant difference as a function of spin between the ${J}_{1}$ values for the negative-parity band in ${}^{152}\mathrm{Nd}$ and ${J}_{1}$ for the similar negative-parity band in ${}^{154}\mathrm{Nd},$ however, their ${J}_{2}$ values are essentially identical. These bands indicate a new kind of identical band.

The decay properties of {sup 290}116 and {sup 291}116, and the dependence of their production cross sections on the excitation energies of the compound nucleus, {sup 293}116, have been measured in the {sup 245}Cm({sup 48}Ca,xn){sup 293-x}116 reaction. These isotopes of element 116 are the decay daughters of element 118 isotopes, which are produced via the {sup 249}Cf+{sup 48}Ca reaction. They performed the element 118 experiment at two projectile energies, corresponding to {sup 297}118 compound nucleus excitation energies of E* = 29.2 {+-} 2.5 and 34.4 {+-} 2.3 MeV. During an irradiation with a total beam dose of 4.1 x 10{sup 19} {sup 48}Ca projectiles, three similar decay chains consisting of two or three consecutive {alpha} decays and terminated by a spontaneous fission (SF) with high total kinetic energy of about 230 MeV were observed. The three decay chains originated from the even-even isotope {sup 294}118 (E{sub {alpha}} = 11.65 {+-} 0.06 MeV, T{sub {alpha}} = 0.89{sub -0.31}{sup +1.07} ms) produced in the 3n-evaporation channel of the {sup 249}Cf+{sup 48}Ca reaction with a maximum cross section of 0.5{sub -0.3}{sup +1.6} pb.

The results of two experiments designed to synthesize element 115 isotopes in the {sup 243}Am+{sup 48}Ca reaction are presented. Two new elements with atomic numbers 113 and 115 were observed for the first time. With 248-MeV {sup 48}Ca projectiles, we observed three similar decay chains consisting of five consecutive {alpha} decays, all detected in a total time interval of 30 s. Each chain was terminated by a spontaneous fission (SF) with a high-energy release and a lifetime of about a day. With 253-MeV {sup 48}Ca projectiles, we registered a different decay chain of consecutive {alpha} decays detected in a time interval of 0.5 s, also terminated by spontaneous fission, but after 1.8 h. The decay properties of the eleven new {alpha}- and SF-decaying nuclei are consistent with expectations for consecutive {alpha} decays originating from the parent isotopes {sup 288}115 and {sup 287}115, produced in the 3n- and 4n-evaporation channels, respectively. Support for the assignment of the atomic numbers of all of the nuclei in the {sup 288}115 decay chain was obtained in an independent experiment in which a long-lived spontaneous fission activity, {sup 268}Db (15 events), was found to be chemically consistent with the fifth group of the periodic table.more » The odd-odd isotope {sup 288}115 was observed with largest cross section of about 4 pb. In the SF decay of {sup 268}Db, a total kinetic energy of 230 MeV and a neutron multiplicity per fission of 4.2 were measured. The decay properties of the 11 new isotopes with Z=105-115 and the production cross sections are in agreement with modern concepts of the role of nuclear shells in the stability of superheavy nuclei. The experiments were carried out at the Flerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research.« less

The level structure of $^{249}\mathrm{Bk}$ has been investigated by measuring the \ensuremath{\gamma}-ray spectra of an extremely pure $^{253}\mathrm{Es}$ sample obtained by milking this nuclide from $^{253}\mathrm{Cf}$ source material produced in the High Flux Isotope Reactor at Oak Ridge National Laboratory. Additional information on the $^{249}\mathrm{Bk}$ levels was obtained from the ${\ensuremath{\beta}}^{\ensuremath{-}}$-decay study of $^{249}\mathrm{Cm}$, produced by neutron irradiation of $^{248}\mathrm{Cm}$. Using the results of the present study together with the data from previous $^{248}\mathrm{Cm}$($\ensuremath{\alpha},t$) and $^{248}\mathrm{Cm}$($^{3}\mathrm{He},d$) reactions, the following single-particle states have been identified in $^{249}\mathrm{Bk}$: 7/2${}^{+}$[633], 0.0 keV; 3/2${}^{\ensuremath{-}}$[521], 8.78 keV; 1/2${}^{+}$[400], 377.55 keV; 5/2${}^{+}$[642], 389.17 keV; 1/2${}^{\ensuremath{-}}$[530], 569.20 keV; 1/2${}^{\ensuremath{-}}$[521], 643.0 keV; 5/2${}^{\ensuremath{-}}$[523], 672.9 keV; and 9/2${}^{+}$[624], 1075.1 keV. Four vibrational bands were identified at 767.9, 932.2, 1150.7, and 1223.0 keV with tentative assignments of {7/2${}^{+}$ [633] $\ensuremath{\bigotimes}{1}^{\ensuremath{-}}$}9/2${}^{\ensuremath{-}}$, {7/2${}^{+}$ [633] $\ensuremath{\bigotimes} {0}^{\ensuremath{-}}$}7/2${}^{\ensuremath{-}}$, {7/2${}^{+}$ [633] $\ensuremath{\bigotimes} {1}^{\ensuremath{-}}$}5/2${}^{\ensuremath{-}}$, and {7/2${}^{+}$ [633] $\ensuremath{\bigotimes} {0}^{+}$}7/2${}^{+}$, respectively. A band at 899.9 keV was observed in $\ensuremath{\gamma}\text{\ensuremath{-}}\ensuremath{\gamma}$ coincidence measurements and given a tentative spin assignment of 3/2. It is possibly associated with a 2${}^{\ensuremath{-}}$ phonon coupled to the ground state, with configuration {7/2${}^{+}$ [633] $\ensuremath{\bigotimes} {2}^{\ensuremath{-}}$}3/2${}^{\ensuremath{-}}$. Three levels at 624.3, 703.5, and 769.1 keV were assigned spins of 5/2, 7/2, and 9/2, respectively. These could be the members of the 3/2${}^{+}$ [651] band, expected in this energy region.

The level structure of 249Bk has been investigated by measuring the γ‐ray spectra following the α decay of a chemically and isotopically pure 253Es sample. Alpha‐gamma coincidence measurement was performed using a Si detector for α particles and a 25% Ge detector for γ rays. A gamma‐gamma coincidence measurement was performed with the Gammasphere spectrometer. The Es sample was obtained by extracting the 253Es which grew in a 253Cf source material produced in the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory. Additional information on the 249Bk levels was obtained from the study of γ rays produced in the β− decay of 249Cm. The 249Cm sample was produced by neutron irradiation of 248Cm. Using the results of the present study and the results of previous 248Cm(α,t) and 248Cm(3He,d) reaction spectra, the following single‐particle states have been identified in 249Bk: 7/2+[633], 0.0 keV; 3/2−[521], 8.78 keV; 1/2+[400], 377.55 keV: 5/2+[642], 389.17 keV; 1/2−[530], 569.19 keV; 1/2−[521], 643....

We have studied the dependence of the production cross sections of the isotopes {sup 282,283}112 and {sup 286,287}114 on the excitation energy of the compound nuclei {sup 286}112 and {sup 290}114. The maximum cross section values of the xn-evaporation channels for the reaction {sup 238}U({sup 48}Ca,xn){sup 286-x}112 were measured to be {sigma}{sub 3n}=2.5{sub -1.1}{sup +1.8} pb and {sigma}{sub 4n}=0.6{sub -0.5}{sup +1.6} pb; for the reaction {sup 242}Pu({sup 48}Ca,xn){sup 290-x}114: {sigma}{sub 2n}{approx}0.5 pb, {sigma}{sub 3n}=3.6{sub -1.7}{sup +3.4} pb, and {sigma}{sub 4n}=4.5{sub -1.9}{sup +3.6} pb. In the reaction {sup 233}U({sup 48}Ca,2-4n){sup 277-279}112 at E*=34.9=2.2 MeV we measured an upper cross section limit of {sigma}{sub xn}{

We have studied the excitation functions of the reactions $^{244}\mathrm{Pu}$($^{48}\mathrm{Ca}$,$xn$). Maximum cross sections for the evaporation of 3--5 neutrons in the complete-fusion reaction $^{244}\mathrm{Pu+}^{48}\mathrm{Ca}$ were measured to be ${\ensuremath{\sigma}}_{3n}=2\phantom{\rule{0.3em}{0ex}}\text{pb}$, ${\ensuremath{\sigma}}_{4n}=5\phantom{\rule{0.3em}{0ex}}\text{pb}$, and ${\ensuremath{\sigma}}_{5n}=1\phantom{\rule{0.3em}{0ex}}\text{pb}$. The decay properties of $3n$-evaporation product $^{289}114$, in the decay chains observed at low $^{48}\mathrm{Ca}$ energy coincide well with those previously observed in the $^{244}\mathrm{Pu+}^{48}\mathrm{Ca}$ and $^{248}\mathrm{Cm+}^{48}\mathrm{Ca}$ reactions and assigned to $^{288}114$. Two isotopes of element 114 and their descendant nuclei were identified for the first time at higher bombarding energies: $^{288}114$ (${E}_{\ensuremath{\alpha}}=9.95\phantom{\rule{0.3em}{0ex}}\text{MeV}$, ${T}_{1∕2}=0.6\phantom{\rule{0.3em}{0ex}}\mathrm{s}$) and $^{287}114$ (${E}_{\ensuremath{\alpha}}=10.04\phantom{\rule{0.3em}{0ex}}\text{MeV}$, ${T}_{1∕2}=1\phantom{\rule{0.3em}{0ex}}\mathrm{s}$). We also report on the observation of new isotopes of element 116, $^{290,291}116$, produced in the $^{245}\mathrm{Cm}+^{48}\mathrm{Ca}$ reaction with cross sections of about $1\phantom{\rule{0.3em}{0ex}}\text{pb}$. A discussion of self-consistent interpretations of all observed decay chains originating at $Z=118$, 116, and 114 is presented.

This paper presents results of experiments aimed at producing long-lived superheavy elements located near the spherical shell closures with Z ≥114 and N ≥172 in the reactions of neutron-rich isotopes 244Pu, 245,248Cm and 249Cf with 48Ca projectiles. The decay properties of the synthesized nuclei are consistent with the consecutive α-decays originating in the decays of parent nuclides 289114, 290,291,293116 and 294118 produced in the 2n and 3n-evaporation channels. The present observations can be considered to be experimental evidence of the existence of the “island of stability” of superheavy elements.

The present paper reports the results of an attempt aimed at the synthesis of element 118 in the reaction {sup 249}Cf({sup 48}Ca,3n){sup 294}118. The experiment was performed employing the Dubna Gas-filled Recoil Separator and the U400 heavy-ion cyclotron at FLNR, JINR, Dubna. In the course of a 2300-hour irradiation of an enriched {sup 249}Cf target (0.23 mg/cm{sup 2}) with a beam of 245-MeV {sup 48}Ca ions, we accumulated a total beam dose of 2.5 x 10{sup 19} ions. We detected two events that may be attributed to the formation and decay of nuclei with Z=118. For one event, we observed a decay chain of two correlated {alpha}-decays with corresponding energies and correlation times of E{sub {alpha}1} = 11.65 {+-} 0.06 MeV, t{sub {alpha}1} = 2.55 ms and E{sub {alpha}2} = 10.71 {+-} 0.17 MeV, t{sub {alpha}2} = 42.1 ms and, finally, a spontaneous fission with the sum of the kinetic energies of the fission fragments E{sub tot} = 207 MeV (TKE {approx} 230 MeV) and t{sub SF} = 0.52 s. In the second event chain, the recoil nucleus decayed into two fission fragments with E{sub tot} = 223 MeV (TKE {approx} 245 MeV) 3.16 ms later, without intervening {alpha} decays.more » The probabilities that these events were caused by the chance correlations of unrelated signals are negligible. Both events were observed at an excitation energy of the compound nucleus {sup 297}118 of E* = 30.0 {+-} 2.4 MeV, close to the expected maximum of the 3n-evaporation channel. The relationship between the decay energy Q{sub {alpha}} and decay period T{sub {alpha}} shows that sequential {alpha}-transitions in the first event correspond to the decay chain with Z = 118{_}116{_}114. Decay characteristics of the newly observed nuclides are compared with radioactive decay properties of the even-even isotopes with Z = 116, 114 and 112 previously produced in the reactions {sup 244}Pu, {sup 248}Cm + {sup 48}Ca and calculations made in various nuclear models.« less