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An intense and long-lasting Saharan dust outbreak crossed the Iberian Peninsula (IP) from the southwest (SW) to the northeast (NE) from 25 March until 7 April 2021. This work aims to assess the optical and mass contribution of both fine and coarse dust particles along their transport. Five Iberian lidar stations were monitoring the transport and evolution of the Saharan dust particles, i.e. El Arenosillo/Huelva, Granada, Torrejón/Madrid and Barcelona in Spain, and Évora in Portugal. The particular meteorological conditions determined the aerosol scenario along the overall dust event, differing in the first part of the event (25–31 March), in which the strongest dust incidence occurred on 29–31 March at the south and central stations and 1 April at Barcelona, from the second one (1–7 April). The use of the two-step POLIPHON algorithm showed the relevance of using polarized lidar measurements for separating the aerosol properties of dust fine and coarse particles as an added value. Both the fine dust (Df) and coarse dust (Dc) components of the total particle backscatter coefficient (total dust, DD = Dc + Df) were separately derived. The dust plume was well-mixed with height and no significant differences were found in the vertical structure of both the Dc and Df particle backscatter coefficients. From the beginning of the dust outbreak until 1 April, the vertical Df /DD mass ratio was nearly constant in time at each station and also in altitude with values of ∼ 10 %. Moreover, the mean dust optical depth at 532 nm was decreasing along that dust pathway, reporting values from SW to NE stations of 0.34 at El Arenosillo/Huelva, 0.28 at Granada, 0.20 at Évora, 0.28 at Torrejón/Madrid, and 0.14 at Barcelona, although its Df / DD ratio remained almost constant (28 %–30 %). A similar pattern was found for the total dust mass loading and its Df/ DD ratio, i.e. mostly decreasing mean mass values were reported, being constant in its Df /DD ratio (∼ 10 %) along the SW–NE dust pa

Megacities and other major population centres (MPCs) worldwide are major sources of air pollution, both locally as well as downwind. The overall assessment and prediction of the impact of MPC pollution on tropospheric chemistry are challenging. The present work provides an overview of the highlights of a major new contribution to the understanding of this issue based on the data and analysis of the EMeRGe (Effect of Megacities on the transport and transformation of pollutants on the Regional to Global scales) international project. EMeRGe focuses on atmospheric chemistry, dynamics, and transport of local and regional pollution originating in MPCs. Airborne measurements, taking advantage of the long range capabilities of the High Altitude and LOng Range Research Aircraft (HALO, https://www.halo-spp.de, last access: 22 March 2022), are a central part of the project. The synergistic use and consistent interpretation of observational data sets of different spatial and temporal resolution (e.g. from ground-based networks, airborne campaigns, and satellite measurements) supported by modelling within EMeRGe provide unique insight to test the current understanding of MPC pollution outflows. In order to obtain an adequate set of measurements at different spatial scales, two field experiments were positioned in time and space to contrast situations when the photochemical transformation of plumes emerging from MPCs is large. These experiments were conducted in summer 2017 over Europe and in the inter-monsoon period over Asia in spring 2018. The intensive observational periods (IOPs) involved HALO airborne measurements of ozone and its precursors, volatile organic compounds, aerosol particles, and related species as well as coordinated ground-based ancillary observations at different sites. Perfluorocarbon (PFC) tracer releases and model forecasts supported the flight planning, the identification of pollution plumes, and the analysis of chemical transformations during transport

An unprecedented extreme Saharan dust event was registered in winter time from 20 to 23 February 2017 over the Iberian Peninsula (IP). We report on aerosol optical properties observed under this extreme dust intrusion through passive and active remote sensing techniques. For that, AERONET (AErosol RObotic NETwork) and EARLINET (European Aerosol Research LIdar NETwork) databases are used. The sites considered are: Barcelona (41.38°N, 2.17°E), Burjassot (39.51°N, 0.42°W), Cabo da Roca (38.78°N, 9.50°W), Évora (38.57°N, 7.91°W), Granada (37.16°N, 3.61°W) and Madrid (40.45°N, 3.72°W). Large aerosol optical depths (AOD) and low Ångström exponents (AE) are observed. An AOD of 2.0 at 675 nm is reached in several stations. A maximum peak of 2.5 is registered in Évora. During and around the peak of AOD, AEs close to 0 and even slightly negative are measured. With regard to vertically-resolved aerosol optical properties, particle backscatter coefficients as high as 15 Mm−1 sr−1 at 355 nm are recorded at the lidar stations. Layer-mean lidar ratios are found in the range 40–55 sr at 355 nm and 34–61 sr at 532 nm during the event. The particle depolarization ratios are found to be constant inside the dust layer, and consistent from one site to another. Layer-mean values vary in the range 0.19–0.31. Another remarkable aspect of the event is the limited vertical distribution of the dust plume which never exceeds 5 km. The extreme aspect of the event also presented a nice case for testing the ability of two dust forecast models, BSC-DREAM8b and NMMB/BSC-Dust, to reproduce the arrival, the vertical distribution and the intensity of the dust plume over a long-range transport region. In the particular case of the February 2017 dust event, we found a large underestimation in the forecast of the extinction coefficient provided by BSC-DREAM8b at all heights independently of the site. In contrast NMMB/BSC-Dust forecasts presented a better agreement with the observations, especially in sou, The research leading to these results has received funding from the H2020 program from the European Union (grant agreement no. 654109, 778349) and also from the Spanish Ministry of Industry, Economy and Competitiviness (MINECO, ref. CGL2013-45410-R, CGL2016-81092-R, CGL2017-85344-R, TEC2015-63832-P), the Spanish Ministry of Science, Innovation and Universities (ref. CGL2017-90884-REDT); the CommSensLab "Maria de Maeztu" Unity of Excellence (ref. MDM-2016-0600) financed by the Spanish Agencia Estatal de Investigación. Co-funding was also provided by the European Union through the European Regional Development Fund (ref. POCI-01-0145-FEDER-007690, ALT20-03-0145-FEDER-000004, ALT20-03-0145-FEDER-000011); by the Andalusia Regional Government (ref. P12-RNM-2409); by the Madrid Regional Government (projects TIGAS-CM, ref. Y2018/EMT-5177 and AIRTEC-CM, ref. P2018/EMT4329); by the University of Granada through “Plan Propio. Programa 9 Convocatoria 2013” and by the Portuguese Foundation for Science and Technology and national funding (ref. SFRH/BSAB/143164/2019). The BSC-DREAM8b and NNMB/BSC-Dust (now NMMB-MONARCH) model simulations were performed by the Mare Nostrum supercomputer hosted by the Barcelona Supercomputer Center (BSC). S. Basart acknowledges the AXA Research Fund for supporting aerosol research at the BSC through the AXA Chair on Sand and Dust Storms Fund, as well as the InDust project (COST Action CA16202). The authors gratefully acknowledge the NOAA Air Resources Laboratory (ARL) for the provision of the HYSPLIT transport and dispersion model and/or READY website (http://www.ready.noaa.gov) used in this publication., Peer Reviewed, Postprint (published version)

Cuatro sistemas lidar Raman multifrecuencia (Madrid, Granada, Barcelona y Evora), tomaron medidas simultáneamente a un sistema de referencia (Potenza) para verificar su funcionamiento durante la campaña de intercomparación: SPALI10, (SPAin Lidar Intercomparison 2010) que tuvo lugar en Madrid entre el 18 de Octubre y el 5 de Noviembre de 2010. Estos sistemas lidar Raman multifrecuencia proporcionan propiedades ópticas de los aerosoles con resolución vertical. Los perfiles suministrados por los sistemas lidar se compararon con información complementaria proporcionada por otra instrumentación, tal como la distribución de tamaños de los aerosoles medida de manera continua a nivel de superficie o la caracterización de la columna de aerosoles, Postprint (published version)

To extend and reinforce the action of the European network EARLINET (supported by the EARLINET-ASOS European project), a network of Spanish and Portuguese aerosol lidars (SPALINET) was created. In the first three years of the project six out of the ten systems have been successfully intercompared, seven elastic algorithms and six Raman algorithms have also been validated. Now the network focuses on future scientific objectives aiming at performing coordinated measurements. This paper presents the scientific context and a description of the network, as well as the results from the first three years of activity., Postprint (published version)

Lidar and sun-photometer measurements were performed intensively over the Iberian Peninsula (IP) during the eruption of Eyjafjallaj ¨ okull volcano (Iceland) in April–May 2010. The volcanic plume hit all the IP stations for the first time on 5 May 2010. A thorough study of the event is conducted for the period 5–8 May. Firstly the spatial and temporal evolution of the plume is described by means of lidar and sun-photometer measurements supported with backtrajectories. The volcanic aerosol layers observed over the IP were rather thin (< 1000 m) with a top height up to 11–12 km. The mean optical thicknesses associated to those layers were rather low (between 0.013 and 0.020 over the whole period). Punctually on 7 May the optical thickness reached peak values near 0.10. Secondly the volcanic aerosols are characterized in terms of extinction and backscatter coefficients, lidar ratios, A° ngstro¨m exponents and linear particle depolarization ratio. Lidar ratios at different sites varied between 30 and 50 sr without a marked spectral dependency. Similar extinction-related A° ngstro¨m exponents varying between 0.6 and 0.8 were observed at different sites. The temporal evolution of the backscatter-related A° ngstro¨m exponents points out a possible decrease of the volcanic particle size as the plume moves from west to east. Particle depolarization ratios on the order of 0.06–0.08 confirmed the coexistence of both ash and non-ash particles. Additionally profiles of mass concentration were obtained with a method using the opposite depolarizing effects of ash particles (strongly depolarizing) and non-ash particles (very weakly depolarizing), and sun-photometer observations. In Granada the ash mass concentration was found approximately 1.5 higher than that of non-ash particles, and probably did not exceed the value of 200 μgm−3 during the whole event., Peer Reviewed, Postprint (published version)

This work presents the characterization of atmospheric aerosols performed over the Iberian Peninsula in the framework of EARLINET for a special episode on 20th August 2007. The assessment of aerosol radiative impact requires an accurate determination of their optical and microphysical properties, which are presented here for a variety of instrumentation including passive remote sensors, as sun-photometers, and active systems both ground-based and on board CALIPSO satellite. Measurements highlight the presence of a multilayered structure with a well-defined planetary boundary layer and biomass-particles in elevated layers, extending up to 7 km asl over the central Iberian Peninsula, and even higher, up to 9 km asl, at the southeastern part of the peninsula. Lidar computations reveal a contribution to the aerosol optical depth around 10-40% for these biomass-burning particles, with backscatter-related Angströ, Postprint (published version)

La reciente erupción del volcán Eyjafjallajökull es una muestra – extremada, pero de probabilidad no despreciable – de la influencia que los aerosoles atmosféricos pueden tener en la vida diaria de miles de personas y en la economía mundial. Este acontecimiento ha sido seguido desde tierra por – entre otros instrumentos – radares láser (lidares) que han permitido determinar la evolución en el espacio y el tiempo de las nubes de ceniza proyectadas por el volcán y han proporcionado información de valor a las agencias meteorológicas y a las administraciones responsables de la seguridad de la navegación aérea., Postprint (published version)

This work presents the assessment of the aerosol direct radiative effects for a special episode of transatlantic transport of a biomass burning plume, performed over Granada, south-eastern Iberian Peninsula, on 20th August 2007. The knowledge of aerosol radiative impact requires an accurate determination of their optical and microphysical properties, which are obtained here using ground-based remote sensing instrumentation by means of a combination of lidar and sun-photometer. Our data highlight the presence of a multilayered structure with a well-defined planetary boundary layer and biomass-particles in elevated layers, extending up to 9 km asl, at the south-eastern part of the Iberian Peninsula. The aerosol direct shortwave radiative effects, evaluated from simulations with SBDART code, show that the biomass burning plume increases the heating rate up to 0.5 K/day in spite of the small contribution of these particles to the total aerosol optical depth (10-20%). In addition, our results indicate that the biomass burning plume strengths the negative radiative forcing about -5 down to -8 W/m2 at the surface, between noon and evening. At the TOA, radiative forcing appeared slightly positive but very close to zero at noon, and negative in the evening with a decrease of 1.5 W/m2 caused by the presence of the biomass burning plume., Postprint (published version)

The European Aerosol Research Lidar Network, EARLINET, performs correlative observations during CALIPSO overpasses based on a sophisticated measurement strategy since June 2006. Within a dedicated activity supported by the European Space Agency (ESA), sixteen EARLINET stations contributed about 1500 measurements during an intensive observational period from May 2008 to October 2009. From these measurements, we establish a long-term aerosol and cloud database of correlative EARLINET-CALIPSO observations. This database shall provide a basis for homogenizing long-term space-borne observations conducted with different lidar instruments operating at different wavelengths on various platforms over the next decade(s). The database is also used to study the quality and representativeness of satellite lidar cross sections along an orbit against long-term lidar network observations on a continental scale., Postprint (published version)

Lidar measurements were performed in the framework of the EARLINET and SPALINET networks during the eruption of Eyjafjalla volcano (Iceland) since 14 April 2010. The profiles of the aerosol optical properties, namely backscatter and extinction coefficients, lidar ratio and Angström exponent, show the presence of volcanic aerosol layers over all SPALINET stations since 5 May. The volcanic particles were monitored both within the planetary boundary layer and in decoupled layers up to 8 km agl over the Iberian Peninsula. This is the first time that the spatial and temporal distributions of volcanic aerosols have been studied with active remote sensing techniques over the Iberian Peninsula., Postprint (published version)

The high variability of tropospheric aerosols, both in space and time, is the main cause of the high uncertainty about radiative forcing related to tropospheric aerosols and their interaction with clouds. Because of the lack of high resolution aerosol global vertical profiles, the vertical mixing has not been considered so far in studies of spatial and temporal variability. The CALIPSO mission provides the first opportunity to investigate the 4-D aerosol and cloud fields in detail. However, because of the CALIOP small footprint and the revisit time of 16 days, correlative ground-based lidar observations are necessary in order to investigate the representativeness of these satellite observations. EARLINET, the European Aerosol Research Lidar Network, started correlative measurements for CALIPSO in June 2006, right after the CALIPSO launch. An integrated study of CALIPSO and EARLINET correlative measurements opens new possibilities for spatial (both horizontal and vertical) and temporal representativeness investigation of polar-orbit satellite measurements also in terms of revisit time., Postprint (published version)

Postprint (author’s final draft)