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We study the Hanle and spin polarization recovery effects on resident electrons in a monolayer MoSe$_2$ on EuS. We demonstrate that localized electrons provide the main contribution to the spin dynamics signal at low temperatures below 15~K for small magnetic fields of only a few mT. The spin relaxation of these electrons is determined by random effective magnetic fields due to a contact spin interaction, namely the hyperfine interaction with the nuclei in MoSe$_2$ or the exchange interaction with the magnetic ions of the EuS film. From the magnetic field angular dependence of the spin polarization we evaluate the anisotropy of the intervalley electron $g$-factor and the spin relaxation time. The non-zero in-plane $g$-factor $|g_x|\approx 0.1$, the value of which is comparable to its dispersion, is attributed to randomly localized electrons in the MoSe$_2$ layer., Comment: 6 pages, 4 figures

Here, we report the observation of strong coupling between magnons and surface acoustic wave (SAW) phonons in a thin CoFeB film constructed in an on-chip SAW resonator by analyzing SAW phonon dispersion anticrossings. Our device design provides the tunability of the film thickness with a fixed phonon wavelength, which is a departure from the conventional approach in strong magnon--phonon coupling research. We detect a monotonic increase in the coupling strength by expanding the film thickness, which agrees with our theoretical model. Our work offers a significant way to advance fundamental research and the development of devices based on magnon--phonon hybrid quasiparticles., Comment: Main text 6 pages, 4 figures, plus supplemental materials

A key phenomenon that enables nanoscale spintronic devices is the efficient inter-conversion between spin and charge degrees of freedom. Here, we experimentally demonstrate a pathway to generate current-induced spin polarization at the interface between an insulating ferromagnet and a non-magnetic metal using interfacial exchange-field spin filtering. Measuring current-in-plane giant magnetoresistance in Py$|$Cu$|$EuS trilayer Hall cross devices, we induce a non-equilibrium spin polarization of $P_\text{neq}^\text{Cu|EuS}$=0.6% at a low charge current density of 1.88$\times$10$^3$ A/cm$^2$. This efficiency is comparable to that of conventional charge-to-spin conversion of spin-Hall or Rashba-Edelstein effects enabled by relativistic spin-orbit coupling. Interfacial exchange field filtering allows operation with largely reduced power consumption and magnetic reconfigurability, opening new pathways to nanoscale low-power insulator spintronics., Comment: 8 pages, 4 figures and 2 tables; Supplemental Material 4 pages, 3 figures

Phonons and magnons are engineered by periodic potential landscapes in phononic and magnonic crystals, and their combined studies may enable valley phonon transport tunable by the magnetic field. Through nonreciprocal surface acoustic wave transmission, we demonstrate valley-selective phonon-magnon scattering in magnetoelastic superlattices. The lattice symmetry and the out-of-plane magnetization component control the sign of nonreciprocity. The phonons in the valleys play a crucial role in generating nonreciprocal transmission by inducing circularly polarized strains that couple with the magnons. The transmission spectra show a nonreciprocity peak near a transmission gap, matching the phononic band structure. Our results open the way for manipulating valley phonon transport through periodically varying magnon-phonon coupling.

Harnessing the causal relationships between mechanical and magnetic properties of van der Waals materials presents a wealth of untapped opportunity for scientific and technological advancement, from precision sensing to novel memories. This can, however, only be exploited if the means exist to efficiently interface with the magnetoelastic interaction. Here, we demonstrate acoustically-driven spin-wave resonance in a crystalline antiferromagnet, chromium trichloride, via surface acoustic wave irradiation. The resulting magnon-phonon coupling is found to depend strongly on sample temperature and external magnetic field orientation, and displays a high sensitivity to extremely weak magnetic anisotropy fields in the few~mT range. Our work demonstrates a natural pairing between power-efficient strain-wave technology and the excellent mechanical properties of van der Waals materials, representing a foothold towards widespread future adoption of dynamic magneto-acoustics., Comment: 14 pages, 7 figures (main text + supplemental material)

Deep in the ultrastrong light-matter coupling regime, it has been predicted that the ground state of a two-level atom interacting with a cavity mode takes the form of a "virtual" Schr\"odinger cat entangled state between light and matter. We propose a method to convert this Schr\"odinger cat state from virtual to real, and back again, by driving the atom with optimally chosen pulses. Our system consists of a four-level atom, with two of these levels ultrastrongly coupled to a cavity mode. We show that the Schr\"odinger cat state can be converted between virtual and real by making use of either an ideal ultrafast pulse or a multi-tone {\pi}-pulse. In addition to allowing us to observe these unusual virtual states this method could also be used to generate entangled cat states on demand for quantum information processing.

Surface acoustic waves (SAWs) in the GHz frequency range can inject spin currents dynamically into adjacent nonmagnetic layers via spin pumping effect associated with ferromagnetic resonance. Here, we demonstrate an enhancement of acoustic ferromagnetic resonance and spin current generation by a pair of SAW reflector gratings, which form an acoustic analogue of the distributed Bragg reflector cavity. In the experiment, we confirmed 2.04 $\pm$ 0.02 times larger SAW power absorption in a device with cavity than in case of no acoustic cavity. We confirmed up to 2.96 $\pm$ 0.02 times larger spin current generation by measuring electric voltages generated by the inverse Edelstein effect (IEE) at the interface between Cu and Bi$_2$O$_3$. The results suggest that acoustic cavities would be useful to enhance the conversion efficiency in SAW driven coupled magnon-phonon dynamics., Comment: Main text and Supplemental Material

Voltage induced magnetization dynamics of magnetic thin films is a valuable tool to study anisotropic fields, exchange couplings, magnetization damping and spin pumping mechanism. A particularly well established technique is the ferromagnetic resonance (FMR) generated by the coupling of microwave photons and magnetization eigenmodes in the GHz range. Here we review the basic concepts of the so-called acoustic ferromagnetic resonance technique (a-FMR) induced by the coupling of surface acoustic waves (SAW) and magnetization of thin films. Interestingly, additional to the benefits of the microwave excited FMR technique, the coupling between SAW and magnetization also offers fertile ground to study magnon-phonon and spin rotation couplings. We describe the in-plane magnetic field angle dependence of the a-FMR by measuring the absorption / transmission of SAW and the attenuation of SAW in the presence of rotational motion of the lattice, and show the consequent generation of spin current by acoustic spin pumping., Comment: 6 pages, 6 figures, short review

One of the most fundamental forms of magnon-phonon interaction is an intrinsic property of magnetic materials, the "magnetoelastic coupling". This particular form of interaction has been the basis for describing magnetic materials and their strain related applications, where strain induces changes of internal magnetic fields. Different from the magnetoelastic coupling, more than 40 years ago, it was proposed that surface acoustic waves may induce surface magnons via rotational motion of the lattice in anisotropic magnets. However, a signature of this magnon-phonon coupling mechanism, termed magneto-rotation coupling, has been elusive. Here, we report the first observation and theoretical framework of the magneto-rotation coupling in a perpendicularly anisotropic ultra-thin film Ta/CoFeB(1.6 nm)/MgO, which consequently induces nonreciprocal acoustic wave attenuation with a unprecedented ratio up to 100$\%$ rectification at the theoretically predicted optimized condition. Our work not only experimentally demonstrates a fundamentally new path for investigating magnon-phonon coupling, but also justify the feasibility of the magneto-rotation coupling based application., Comment: 30 pages, 12 figures

At interfaces with inversion symmetry breaking, Rashba effect couples the motion of electrons to their spin; as a result, spin-charge interconversion mechanism can occur. These interconversion mechanisms commonly exploit Rashba spin splitting at the Fermi level by spin pumping or spin torque ferromagnetic resonance. Here, we report evidence of significant photoinduced spin to charge conversion via Rashba spin splitting in an unoccupied state above the Fermi level at the Cu(111)/$\alpha$-Bi$_{2}$O$_{3}$ interface. We predict an average Rashba coefficient of $1.72\times 10^{-10}eV.m$ at 1.98 eV above the Fermi level, by fully relativistic first-principles analysis of the interfacial electronic structure with spin orbit interaction. We find agreement with our observation of helicity dependent photoinduced spin to charge conversion excited at 1.96 eV at room temperature, with spin current generation of $J_{s}=10^{6}A/m^{2}$. The present letter shows evidence of efficient spin-charge conversion exploiting Rashba spin splitting at excited states, harvesting light energy without magnetic materials or external magnetic fields., Comment: 7 pages, 4 figures in main text and 5 figures in appendix

The formation of novel two-dimensional electron gas (2DEG) with high mobility in metal/amorphous interfaces has motivated an ongoing debate regarding the formation and novel characteristics of these 2DEGs. Here we report an optical study, based on infrared spectroscopic ellipsometry, of nonmagnetic metal and amorphous semiconducting oxide (Cu/Bi$_2$O$_3$) interfaces that confirms the formation of a 2DEG with spin orbit coupling (SOC). The 2DEG optical response was simulated with a uniaxial diagonal dielectric tensor within a sub-nanometer thin layer, where its $x$ and $z$ components lineshapes resolved in both free-electron and peak-like contributions, resulted very similar to theoretical predictions [M. Xie et al., Phys. Rev. B $\bf{89}$, 245417 (2014)] of a two dimensional electron gas confined in the normal direction of a perovskite interface. In particular, the small but finite conducting character of the $z$ component provides a unambiguous signature of the presence of the 2DEG in the Cu/Bi$_2$O$_3$ system. Although the original constituent materials do not possess spin-orbit coupling (SOC), the resulting interfacial hybridization of such states induce electronic asymmetric wave functions. This work demonstrates the detection of 2DEG in amorphous crystals allowing to study its challenging interfacial phenomena such as SOC and interface-bulk coupling, overcoming an experimental impediment which has hold back for decades important advancements for the understanding of 2DEGs in amorphous materials., Comment: 10 pages main text, under review at Phys. Rev. B

We demonstrate a spin to charge current conversion via magnon-phonon coupling and inverse Edelstein effect on the hybrid device Ni/Cu(Ag)/Bi$_{2}$O$_{3}$. The generation of spin current ($J_{s}\approx 10^{8}A/m^{2}$) due to magnon - phonon coupling reveals the viability of acoustic spin pumping as mechanism for the development of spintronic devices. A full in-plane magnetic field angle dependence of the power absorption and a combination of longitudinal and transverse voltage detection reveals the symmetric and asymmetric components of the inverse Edelstein effect voltage induced by Rayleigh type surface acoustic waves. While the symmetric components are well studied, asymmetric components are widely unexplored. We assign the asymmetric contributions to the interference between longitudinal and shear waves and an anisotropic charge distribution in our hybrid device., Comment: 4 figures. 5 pages

Rashba effect describes how electrons moving in an electric field experience a momentum dependent magnetic field that couples to the electron angular momentum (spin). This physical phenomenon permits the generation of spin polarization from charge current (Edelstein effect), which leads to the buildup of spin accumulation. Spin accumulation due to Rashba Edelstein effect has been recently reported to be uniform and oriented in plane, which has been suggested for applications as spin filter device and efficient driving force for magnetization switching. Here, we report the X-ray spectroscopy characterization Rashba interface formed between nonmagnetic metal (Cu, Ag) and oxide (Bi$_{2}$O$_{3}$) at grazing incidence angles. We further discuss the generation of spin accumulation by injection of electrical current at these Rashba interfaces, and its optical detection by time resolved magneto optical Kerr effect. We provide details of our characterization which can be extended to other Rashba type systems beyond those reported here., Comment: 13 pages, 5 figures

We present a method to implement two-phonon interactions between mechanical resonators and spin qubits in hybrid setups, and show that these systems can be applied for the generation of nonclassical mechanical states even in the presence of dissipation. In particular, we demonstrate that the implementation of a two-phonon Jaynes-Cummings Hamiltonian under coherent driving of the qubit yields a dissipative phase transition with similarities to the one predicted in the model of the degenerate parametric oscillator: beyond a certain threshold in the driving amplitude, the driven-dissipative system sustains a mixed steady state consisting of a `jumping cat', i.e., a cat state undergoing random jumps between two phases. We consider realistic setups and show that, in samples within reach of current technology, the system features non-classical transient states, characterized by a negative Wigner function, that persist during timescales of fractions of a second.

We report on state-of-the-art scanning probe microscopy measurements performed in a pulse tube based top-loading closed-cycle cryostat with a base temperature of 4 K and a 9 T magnet. We decoupled the sample space from the mechanical and acoustic noise from the cryocooling system to enable scanning probe experiments. The extremely low vibration amplitudes in our system enabled successful imaging of 0.39 nm lattice steps on single crystalline SrTiO$_{3}$ as well as magnetic vortices in Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$ superconductor. Fine control over sample temperature and applied magnetic field further enabled us to probe the helimagnetic and the skyrmion-lattice phases in Fe$_{0.5}$Co$_{0.5}$Si with unprecedented signal-to-noise ratio of 20:1. Finally, we demonstrate for the first time quartz-crystal tuning fork shear-force microscopy in a closed-cycle cryostat.