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Default aerosol extinction coefficient profiles are commonly used instead of measured profiles in radiative transfer modeling, increasing the uncertainties in the simulations. The present study aimed to determine the magnitude of these uncertainties and contribute towards the understanding of the complex interactions between aerosols and solar radiation. Default, artificial and measured profiles of the aerosol extinction coefficient were used to simulate the profiles of different radiometric quantities in the atmosphere for different surface, atmospheric, and aerosol properties and for four spectral bands: ultraviolet-B, ultraviolet-A, visible, and near-infrared. Case studies were performed over different areas in Europe and North Africa. Analysis of the results showed that under cloudless skies, changing the altitude of an artificial aerosol layer has minor impact on the levels of shortwave radiation at the top and bottom of the atmosphere, even for high aerosol loads. Differences of up to 30% were, however, detected for individual spectral bands. Using measured instead of default profiles for the simulations led to more significant differences in the atmosphere, which became very large during dust episodes (10–60% for actinic flux at altitudes between 1 and 2 km, and up to 15 K/day for heating rates depending on the site and solar elevation). © 2022 by the authors. Licensee MDPI, Basel, Switzerland.

The retrieval of aerosol properties from satellite observations provides their spatial distribution over a wide area in cloud-free conditions. As such, they complement ground-based measurements by providing information over sparsely instrumented areas, albeit that significant differences may exist in both the type of information obtained and the temporal information from satellite and ground-based observations. In this paper, information from different types of satellite-based instruments is used to provide a 3-D climatology of aerosol properties over mainland China, i.e., vertical profiles of extinction coefficients from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP), a lidar flying aboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite and the column-integrated extinction (aerosol optical depth – AOD) available from three radiometers: the European Space Agency (ESA)'s Along-Track Scanning Radiometer version 2 (ATSR-2), Advanced Along-Track Scanning Radiometer (AATSR) (together referred to as ATSR) and NASA's Moderate Resolution Imaging Spectroradiometer (MODIS) aboard the Terra satellite, together spanning the period 1995–2015. AOD data are retrieved from ATSR using the ATSR dual view (ADV) v2.31 algorithm, while for MODIS Collection 6 (C6) the AOD data set is used that was obtained from merging the AODs obtained from the dark target (DT) and deep blue (DB) algorithms, further referred to as the DTDB merged AOD product. These data sets are validated and differences are compared using Aerosol Robotic Network (AERONET) version 2 L2.0 AOD data as reference. The results show that, over China, ATSR slightly underestimates the AOD and MODIS slightly overestimates the AOD. Consequently, ATSR AOD is overall lower than that from MODIS, and the difference increases with increasing AOD. The comparison also shows that neither of the ATSR and MODIS AOD data sets is better than the other one everywhere. However, ATSR ADV has limitations over bright surfaces which the MODIS DB was designed for. To allow for comparison of MODIS C6 results with previous analyses where MODIS Collection 5.1 (C5.1) data were used, also the difference between the C6 and C5.1 merged DTDB data sets from MODIS/Terra over China is briefly discussed. The AOD data sets show strong seasonal differences and the seasonal features vary with latitude and longitude across China. Two-decadal AOD time series, averaged over all of mainland China, are presented and briefly discussed. Using the 17 years of ATSR data as the basis and MODIS/Terra to follow the temporal evolution in recent years when the environmental satellite Envisat was lost requires a comparison of the data sets for the overlapping period to show their complementarity. ATSR precedes the MODIS time series between 1995 and 2000 and shows a distinct increase in the AOD over this period. The two data series show similar variations during the overlapping period between 2000 and 2011, with minima and maxima in the same years. MODIS extends this time series beyond the end of the Envisat period in 2012, showing decreasing AOD.

We present a 3-D climatology of the desert dust distribution over South and East Asia derived using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) data. To distinguish desert dust from total aerosol load we apply a methodology developed in the framework of EARLINET (European Aerosol Research Lidar Network). The method involves the use of the particle linear depolarization ratio and updated lidar ratio values suitable for Asian dust, applied to multiyear CALIPSO observations (January 2007–December 2015). The resulting dust product provides information on the horizontal and vertical distribution of dust aerosols over South and East Asia along with the seasonal transition of dust transport pathways. Persistent high D_AOD (dust aerosol optical depth) values at 532 nm, of the order of 0.6, are present over the arid and semi-arid desert regions. Dust aerosol transport (range, height and intensity) is subject to high seasonality, with the highest values observed during spring for northern China (Taklimakan and Gobi deserts) and during summer over the Indian subcontinent (Thar Desert). Additionally, we decompose the CALIPSO AOD (aerosol optical depth) into dust and non-dust aerosol components to reveal the non-dust AOD over the highly industrialized and densely populated regions of South and East Asia, where the non-dust aerosols yield AOD values of the order of 0.5. Furthermore, the CALIPSO-based short-term AOD and D_AOD time series and trends between January 2007 and December 2015 are calculated over South and East Asia and over selected subregions. Positive trends are observed over northwest and east China and the Indian subcontinent, whereas over southeast China trends are mostly negative. The calculated AOD trends agree well with the trends derived from Aqua MODIS (Moderate Resolution Imaging Spectroradiometer), although significant differences are observed over specific regions.

A record-breaking dust episode took place in Crete on 22 March 2018. The event was characterized by surface concentrations exceeding 1 mg m-3 for a period of 4-7 h, reaching record values higher than 6 mg m-3 at the background station of Finokalia. We present here a detailed analysis of the atmospheric dynamical processes during this period, to identify the main reasons for such extreme dust advection over Crete. At the synoptic scale, the weakening of the polar vortex and the meridional transport of polar air masses at upper tropospheric layers resulted in a strong jet streak over north Africa and Central Mediterranean and corresponding tropospheric folding that brought cold stratospheric air in mid and upper troposphere. Cyclogenesis occurred at the Gulf of Sirte in Libya, resulting in strong winds over the north-east parts of Libya, enhancing particle emissions. The dust plume traveled at low altitude (0.5-3 km) along the warm conveyor belt preceding the depression cold front. This type of dusty southerly wind is commonly known as "Khamsin". As the flow approached Crete, Foehn winds at the lee side of the island favored the downward mixing of dust towards the surface, resulting in local maxima of PM10 in Heraklion and Finokalia. The analysis is based on the combination of high-resolution WRF-Chem simulations reaching up to 1 × 1 km grid space over Crete, ground-based and satellite remote sensing of the dust plumes (PollyXT LiDAR, MSG-SEVIRI, MODIS) and detailed surface aerosol in situ measurements at urban (Heraklion, Chania, Greece) and background (Finokalia) stations in Crete. © 2018 by the authors.

During August 2016, a quasi-stationary high-pressure system spreading over Central and North-Eastern Europe, caused weather conditions that allowed for 24/7 observations of aerosol optical properties by using a complex multi-wavelength PollyXT lidar system with Raman, polarization and water vapour capabilities, based at the European Aerosol Research Lidar Network (EARLINET network) urban site in Warsaw, Poland. During 24-30 August 2016, the lidar-derived products (boundary layer height, aerosol optical depth, Ångström exponent, lidar ratio, depolarization ratio) were analysed in terms of air mass transport (HYSPLIT model), aerosol load (CAMS data) and type (NAAPS model) and confronted with active and passive remote sensing at the ground level (PolandAOD, AERONET, WIOS-AQ networks) and aboard satellites (SEVIRI, MODIS, CATS sensors). Optical properties for less than a day-old fresh biomass burning aerosol, advected into Warsaw's boundary layer from over Ukraine, were compared with the properties of long-range transported 3-5 day-old aged biomass burning aerosol detected in the free troposphere over Warsaw. Analyses of temporal changes of aerosol properties within the boundary layer, revealed an increase of aerosol optical depth and Ångström exponent accompanied by an increase of surface PM10 and PM2.5. Intrusions of advected biomass burning particles into the urban boundary layer seem to affect not only the optical properties observed but also the top height of the boundary layer, by moderating its increase. © 2018 by the authors.

In this study we use a new dust product developed using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) observations and EARLINET (European Aerosol Research Lidar Network) measurements and methods to provide a 3-D multiyear analysis on the evolution of Saharan dust over North Africa and Europe. The product uses a CALIPSO L2 backscatter product corrected with a depolarization-based method to separate pure dust in external aerosol mixtures and a Saharan dust lidar ratio (LR) based on long-term EARLINET measurements to calculate the dust extinction profiles. The methodology is applied on a 9-year CALIPSO dataset (2007–2015) and the results are analyzed here to reveal for the first time the 3-D dust evolution and the seasonal patterns of dust over its transportation paths from the Sahara towards the Mediterranean and Continental Europe. During spring, the spatial distribution of dust shows a uniform pattern over the Sahara desert. The dust transport over the Mediterranean Sea results in mean dust optical depth (DOD) values up to 0.1. During summer, the dust activity is mostly shifted to the western part of the desert where mean DOD near the source is up to 0.6. Elevated dust plumes with mean extinction values between 10 and 75 Mm−1 are observed throughout the year at various heights between 2 and 6 km, extending up to latitudes of 40° N. Dust advection is identified even at latitudes of about 60° N, but this is due to rare events of episodic nature. Dust plumes of high DOD are also observed above the Balkans during the winter period and above northwest Europe during autumn at heights between 2 and 4 km, reaching mean extinction values up to 50 Mm−1. The dataset is considered unique with respect to its potential applications, including the evaluation of dust transport models and the estimation of cloud condensation nuclei (CCN) and ice nuclei (IN) concentration profiles. Finally, the product can be used to study dust dynamics during transportation, since it is capable of revealing even fine dynamical features such as the particle uplifting and deposition on European mountainous ridges such as the Alps and Carpathian Mountains.

In this study we use a new dust product developed using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) observations and EARLINET (European Aerosol Research Lidar Network) measurements and methods to provide a 3-D multiyear analysis on the evolution of Saharan dust over North Africa and Europe. The product uses a CALIPSO L2 backscatter product corrected with a depolarization-based method to separate pure dust in external aerosol mixtures and a Saharan dust lidar ratio (LR) based on long-term EARLINET measurements to calculate the dust extinction profiles. The methodology is applied on a 9-year CALIPSO dataset (2007-2015) and the results are analyzed here to reveal for the first time the 3-D dust evolution and the seasonal patterns of dust over its transportation paths from the Sahara towards the Mediterranean and Continental Europe. During spring, the spatial distribution of dust shows a uniform pattern over the Sahara desert. The dust transport over the Mediterranean Sea results in mean dust optical depth (DOD) values up to 0.1. During summer, the dust activity is mostly shifted to the western part of the desert where mean DOD near the source is up to 0.6. Elevated dust plumes with mean extinction values between 10 and 75 Mm-1 are observed throughout the year at various heights between 2 and 6 km, extending up to latitudes of 40° N. Dust advection is identified even at latitudes of about 60° N, but this is due to rare events of episodic nature. Dust plumes of high DOD are also observed above the Balkans during the winter period and above northwest Europe during autumn at heights between 2 and 4 km, reaching mean extinction values up to 50 Mm-1. The dataset is considered unique with respect to its potential applications, including the evaluation of dust transport models and the estimation of cloud condensation nuclei (CCN) and ice nuclei (IN) concentration profiles. Finally, the product can be used to study dust dynamics during transportation, since it is capable of revealing even fine dynamical features such as the particle uplifting and deposition on European mountainous ridges such as the Alps and Carpathian Mountains. © Author(s) 2017.