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Impacts of domain textures on low-lying neutral excitations in the bulk of fractional quantum Hall effect (FQHE) systems are probed by resonant inelastic light scattering. We demonstrate that large domains of quantum fluids support long-wavelength neutral collective excitations with well-defined wave vector (momentum) dispersion that could be interpreted by theories for uniform phases. Access to dispersive low-lying neutral collective modes in large domains of FQHE fluids such as long wavelength magnetorotons at filling factor v=1/3 offer significant experimental access to strong electron correlation physics in the FQHE., Comment: 11 pages, 4 figures, and Supplemental Material

Flat bands near M points in the Brillouin zone are key features of honeycomb symmetry in artificial graphene (AG) where electrons may condense into novel correlated phases. Here we report the observation of van Hove singularity doublet of AG in GaAs quantum well transistors, which presents the evidence of flat bands in semiconductor AG. Two emerging peaks in photoluminescence spectra tuned by backgate voltages probe the singularity doublet of AG flat bands, and demonstrate their accessibility to the Fermi level. As the Fermi level crosses the doublet, the spectra display dramatic stability against electron density, indicating interplays between electron-electron interactions and honeycomb symmetry. Our results provide a new flexible platform to explore intriguing flat band physics., Comment: 11 pages, 4 figures, and Supplementary Material

Collective modes of exotic quantum fluids reveal underlying physical mechanisms responsible for emergent complex quantum ground states. We observe unexpected new collective modes in the fractional quantum Hall (FQH) regime: intra-Landau-level plasmons in the second Landau level measured by resonant inelastic light scattering. The plasmons herald rotational-symmetry-breaking phases in tilted magnetic fields and reveal long-range translational invariance in these phases. The fascinating dependence of plasmon features on filling factor provide new insights on interplays between topological quantum Hall order and nematic electronic liquid crystal phases. A marked intensity minimum in the plasmon spectrum at Landau level filling factor v = 5/2 strongly suggests that this paired state, which could support non-Abelian excitations, overwhelms competing nematic phases, unveiling the robustness of the 5/2 superfluid state for small tilt angles. At v = 7/3, a sharp and strong plasmon peak that links to emerging macroscopic coherence supports the proposed model of a FQH nematic state at this filling factor.

Photogenerated excitonic ensembles confined in coupled GaAs quantum wells are probed by a complementary approach of emission spectroscopy and resonant inelastic light scattering. Lateral electrostatic trap geometries are used to create dense systems of spatially indirect excitons and excess holes with similar densities in the order of 10$^{11}$ cm$^{-2}$. Inelastic light scattering spectra reveal a very sharp low-lying collective mode that is identified at an energy of 0.44 meV and a FWHM of only ~50 $\mu$eV. This mode is interpreted as a plasmon excitation of the excess hole system coupled to the photogenerated indirect excitons. The emission energy of the indirect excitons shifts under the application of a perpendicular applied electric field with the quantum-confined Stark effect unperturbed from the presence of free charge carriers. Our results illustrate the potential of studying low-lying collective excitations in photogenerated exciton systems to explore the many-body phase diagram, related phase transitions, and interaction physics., Comment: 19 pages, 5 figures

Quantum phases of electrons in the filling factor range $2 \leq\nu\leq 3$ are probed by the weak optical emission from the partially populated second Landau level and spin wave measurements. Observations of optical emission include a multiplet of sharp peaks that exhibit a strong filling factor dependence. Spin wave measurements by resonant inelastic light scattering probe breaking of spin rotational invariance and are used to link this optical emission with collective phases of electrons. A remarkably rapid interplay between emission peak intensities manifests phase competition in the second Landau level.

We report the observation of low-lying collective charge and spin excitations in the second Landau level at {\nu} = 2 + 1/3 and also for the very fragile states at {\nu} = 2 + 2/5, 2 + 3/8 in inelastic light scattering experiments. These modes exhibit a clear dependence on filling factor and temperature substantiating the unique access to the characteristic neutral excitation spectra of the incompressible FQHE states. A detailed mode analysis reveals low energy modes at around 70 {\mu}eV and a sharp mode slightly below the Zeeman energy interpreted as gap and spin wave excitation, respectively. The lowest energy collective charge excitation spectrum at {\nu} = 2 + 1/3 exhibits significant similarities and a universal scaling of the energies with its cousin state in the lowest Landau level at {\nu} = 1/3 suggesting similar underlying physics. The observed excitation spectra facilitate to distinguish between theoretical descriptions of the nature of those FQHE states. A striking polarization dependence in light scattering is discussed in the framework of anisotropic electron phases that allow for the stabilization of nematic FQHE states.

The unusual electronic properties of graphene, which are a direct consequence of its two-dimensional (2D) honeycomb lattice, have attracted a great deal of attention in recent years. Creation of artificial lattices that recreate graphene's honeycomb topology, known as artificial graphene, can facilitate the investigation of graphene-like phenomena, such as the existence of massless Dirac fermions, in a tunable system. In this work, we present the fabrication of artificial graphene in an ultra-high quality GaAs/AlGaAs quantum well, with lattice period as small as 50 nm, the smallest reported so far for this type of system. Electron-beam lithography is used to define an etch mask with honeycomb geometry on the surface of the sample, and different methodologies are compared and discussed. An optimized anisotropic reactive ion etching process is developed to transfer the pattern into the AlGaAs layer and create the artificial graphene. The achievement of such high-resolution artificial graphene should allow the observation for the first time of massless Dirac fermions in an engineered semiconductor., Comment: 13 pages text, 8 figures, plus references

The fractional quantum Hall effect has inspired searches for exotic emergent topological particles, such as fractionally charged excitations, composite fermions, abelian and nonabelian anyons and Majorana fermions. Fractionally charged skyrmions, which support both topological charge and topological vortex-like spin structure, have also been predicted to occur in the vicinity of 1/3 filling of the lowest Landau level. The fractional skyrmions, however, are anticipated to be exceedingly fragile, suppressed by very small Zeeman energies. Here we show that, slightly away from 1/3 filling, the smallest manifestations of the fractional skyrmion exist in the excitation spectrum for a broad range of Zeeman energies, and appear in resonant inelastic light scattering experiments as well-defined resonances slightly below the long wavelength spin wave mode. The spectroscopy of these exotic bound states serves as a sensitive tool for investigating the residual interaction between composite fermions, responsible for delicate new fractional quantum Hall states in this filling factor region., Comment: 9 pages, 8 figures

Magneto-luminescence studies in electron bilayers reveal the hallmarks of the even-denominator and other quantum Hall states in the intensities and energies of the inter-band optical recombination lines. In the presence of a small tunneling gap between the layers the magneto-optical emission from the lowest anti-symmetric subband, not populated in a single-electron picture, displays maxima at filling factors 1 and 2/3. These findings uncover a loss of pseudospin polarization, where the pseudospin describes the layer index degree of freedom, that is linked to an anomalous population of the anti-symmetric level due to excitonic correlations. The results demonstrate a new realm to probe the impact of inter-layer Coulomb interaction in quantum Hall bilayers.

The magneto-phonon resonance or MPR occurs in semiconductor materials when the energy spacing between Landau levels is continuously tuned to cross the energy of an optical phonon mode. MPRs have been largely explored in bulk semiconductors, in two-dimensional systems and in quantum dots. Recently there has been significant interest in the MPR interactions of the Dirac fermion magnetoexcitons in graphene, and a rich splitting and anti-crossing phenomena of the even parity E2g long wavelength optical phonon mode have been theoretically proposed and experimentally observed. The MPR has been found to crucially depend on disorder in the graphene layer. This is a feature that creates new venues for the study of interplays between disorder and interactions in the atomic layers. We review here the fundamentals of MRP in graphene and the experimental Raman scattering works that have led to the observation of these phenomena in graphene and graphite.

The low-lying neutral excitation spectrum of the incompressible quantum Hall fluid at $\nu=5/2$ is investigated by inelastic light scattering. Gapped modes are observable only in a very narrow filling factor range centered at 5/2 at energies that overlap estimates from transport activation gaps. The modes are interpreted as critical points in the wave-vector dispersion of excitations that preserve spin orientation. For very small changes $|\delta\nu|\lesssim 0.01$ the gapped modes disappear and a continuum of low-lying excitations takes over indicating the transition from an incompressible fluid at 5/2 to a compressible state. Observations of spin wave modes indicate spin polarization of the 5/2 and 2+1/3 quantum Hall fluids., Comment: 4 pages, 3 figures

The growth of single layer graphene nanometer size domains by solid carbon source molecular beam epitaxy on hexagonal boron nitride (h-BN) flakes is demonstrated. Formation of single-layer graphene is clearly apparent in Raman spectra which display sharp optical phonon bands. Atomic-force microscope images and Raman maps reveal that the graphene grown depends on the surface morphology of the h-BN substrates. The growth is governed by the high mobility of the carbon atoms on the h-BN surface, in a manner that is consistent with van der Waals epitaxy. The successful growth of graphene layers depends on the substrate temperature, but is independent of the incident flux of carbon atoms., Comment: Solid State Communications, 2012

We demonstrate the growth of graphene nanocrystals by molecular beam methods that employ a solid carbon source, and that can be used on a diverse class of large area dielectric substrates. Characterization by Raman and Near Edge X-ray Absorption Fine Structure spectroscopies reveal a sp2 hybridized hexagonal carbon lattice in the nanocrystals. Lower growth rates favor the formation of higher quality, larger size multi-layer graphene crystallites on all investigated substrates. The surface morphology is determined by the roughness of the underlying substrate and graphitic monolayer steps are observed by ambient scanning tunneling microscopy., Comment: Accepted in Carbon; Discussion section added; 20 pages, 6 figures (1 updated)

We observe a low-lying sharp spin mode of three interacting electrons in an array of nanofabricated AlGaAs/GaAs quantum dots by means of resonant inelastic light scattering. The finding is enabled by a suppression of the inhomogeneous contribution to the excitation spectra obtained by reducing the number of optically-probed quantum dots. Supported by configuration-interaction calculations we argue that the observed spin mode offers a direct probe of Stoner ferromagnetism in the simplest case of three interacting spin one-half fermions.

In monolayer graphene, substitutional doping during growth can be used to alter its electronic properties. We used scanning tunneling microscopy (STM), Raman spectroscopy, x-ray spectroscopy, and first principles calculations to characterize individual nitrogen dopants in monolayer graphene grown on a copper substrate. Individual nitrogen atoms were incorporated as graphitic dopants, and a fraction of the extra electron on each nitrogen atom was delocalized into the graphene lattice. The electronic structure of nitrogen-doped graphene was strongly modified only within a few lattice spacings of the site of the nitrogen dopant. These findings show that chemical doping is a promising route to achieving high-quality graphene films with a large carrier concentration., Comment: Science 2011

Even though composite fermions in the fractional quantum Hall liquid are well established, it is not yet known up to what energies they remain intact. We probe the high-energy spectrum of the 1/3 liquid directly by resonant inelastic light scattering, and report the observation of a large number of new collective modes. Supported by our theoretical calculations, we associate these with transitions across two or more composite fermions levels. The formation of quasiparticle levels up to high energies is direct evidence for the robustness of topological order in the fractional quantum Hall effect., Comment: 4 pages, 5 figures

We find unexpected low energy excitations of fully spin-polarized composite-fermion ferromagnets in the fractional quantum Hall liquid, resulting from a complex interplay between a topological order manifesting through new energy levels and a magnetic order due to spin polarization. The lowest energy modes, which involve spin reversal, are remarkable in displaying unconventional negative dispersion at small momenta followed by a deep roton minimum at larger momenta. This behavior results from a nontrivial mixing of spin-wave and spin-flip modes creating a spin-flip excitonic state of composite-fermion particle-hole pairs. The striking properties of spin-flip excitons imply highly tunable mode couplings that enable fine control of topological states of itinerant two-dimensional ferromagnets., Comment: 4 pages, 4 figures

Electrons in artificial lattices enable explorations of the impact of repulsive Coulomb interactions in a tunable system. We have trapped two-dimensional electrons belonging to a gallium arsenide quantum well in a nanofabricated lattice with honeycomb geometry. We probe the excitation spectrum in a magnetic field identifying novel collective modes that emerge from the Coulomb interaction in the artificial lattice as predicted by the Mott-Hubbard model. These observations allow us to determine the Hubbard gap and suggest the existence of a novel Coulomb-driven ground state. This approach offers new venues for the study of quantum phenomena in a controllable solid-state system., Comment: 10 pages, 10 figures

The spin degree of freedom in quantum phases of the second Landau level is probed by resonant light scattering. The long wavelength spin wave, which monitors the degree of spin polarization, is at the Zeeman energy in the fully spin-polarized state at $\nu$=3. At lower filling factors the intensity of the Zeeman mode collapses indicating loss of polarization. A novel continuum of low-lying excitations emerges that dominates near $\nu$=8/3 and $\nu$=5/2. Resonant Rayleigh scattering reveals that quantum fluids for $\nu<3$ break up into robust domain structures. While the state at $\nu$=5/2 is considered to be fully polarized, these results reveal unprecedented roles for spin degrees of freedom., Comment: 4 pages, 5 figures

Coulomb exchange interactions of electrons in the nu=3 quantum Hall state are determined from two inter-Landau level spin-flip excitations measured by resonant inelastic light scattering. The two coupled collective excitations are linked to inter-Landau level spin-flip transitions arising from the N=0 and N=1 Landau levels. The strong repulsion between the two spin-flip modes in the long-wave limit is clearly manifested in spectra displaying Coulomb exchange contributions that are comparable to the exchange energy for the quantum Hall state at nu=1. Theoretical calculations within the Hartree-Fock approximation are in a good agreement with measured energies of spin-flip collective excitations., Comment: 5 pages, 3 figures, to appear in PRB Rapid Communications

We study the growth and microscopic structure of large-area graphene monolayers, grown on copper single crystals by chemical vapor deposition (CVD) in ultra-high vacuum (UHV). Using atomic-resolution scanning tunneling microscopy (STM), we find that graphene grows primarily in registry with the underlying copper lattice for both Cu(111) and Cu(100). The graphene has a hexagonal superstructure on Cu(111) with a significant electronic component, whereas it has a linear superstructure on Cu(100). The film quality is limited by grain boundaries, and the best growth is obtained on the Cu(111) surface.

Coherent coupling of Dirac fermion magneto-excitons with an optical phonon is observed in graphite as marked magnetic-field dependent splittings and anti-crossing behavior of the two coupled modes. The sharp magneto-phonon resonance occurs in regions of the graphite sample with properties of superior single-layer graphene having enhanced lifetimes of Dirac fermions. The greatly reduced carrier broadening to values below the graphene electron-phonon coupling constant explains the appearance of sharp resonances that reveal a fundamental interaction of Dirac fermions., Comment: 5 figures, supplementary material section included

We observe the low-lying excitations of a molecular dimer formed by two electrons in a GaAs semiconductor quantum dot in which the number of confined electrons is tuned by optical illumination. By employing inelastic light scattering we identify the inter-shell excitations in the one-electron regime and the distinct spin and charge modes in the interacting few-body configuration. In the case of two electrons a comparison with configuration-interaction calculations allows us to link the observed excitations with the breathing mode of the molecular dimer and to determine the singlet-triplet energy splitting., Comment: RevTeX 4.0, 6 pages, 6 color PDF figures. Revised version including Supplementary Discussion of Wigner localisation (2 new figures + new version of Fig. 2). To appear in Physical Review Letters

Inter-layer excitonic coherence in a quantum Hall bilayer with negligible tunneling is monitored by measurements of low-lying spin excitations. At $\nu_T =1$ new quasiparticle excitations are observed above a transition temperature revealing a competing metallic phase. For magnetic fields above an onset Zeeman energy this metallic phase has full spin polarization. A phase diagram in the parameter space of temperature and Zeeman energy reveals that the transition temperature increases at higher fields. This unexpected result suggests intriguing impacts of spin polarization in the highly correlated phases., Comment: 5 pages and 5 figures

At low energy, electrons in doped graphene sheets behave like massless Dirac fermions with a Fermi velocity which does not depend on carrier density. Here we show that modulating a two-dimensional electron gas with a long-wavelength periodic potential with honeycomb symmetry can lead to the creation of isolated massless Dirac points with tunable Fermi velocity. We provide detailed theoretical estimates to realize such artificial graphene-like system and discuss an experimental realization in a modulation-doped GaAs quantum well. Ultra high-mobility electrons with linearly-dispersing bands might open new venues for the studies of Dirac-fermion physics in semiconductors., Comment: 4 + epsilon pages, 3 figures, submitted to PRB

Correlation among particles in finite quantum systems leads to complex behaviour and novel states of matter. One remarkable example is predicted to occur in a semiconductor quantum dot (QD) where at vanishing density the Coulomb correlation among electrons rigidly fixes their relative position as that of the nuclei in a molecule. In this limit, the neutral few-body excitations are roto-vibrations, which have either rigid-rotor or relative-motion character. In the weak-correlation regime, on the contrary, the Coriolis force mixes rotational and vibrational motions. Here we report evidence of roto-vibrational modes of an electron molecular state at densities for which electron localization is not yet fully achieved. We probe these collective modes by inelastic light scattering in QDs containing four electrons. Spectra of low-lying excitations associated to changes of the relative-motion wave function -the analogues of the vibration modes of a conventional molecule- do not depend on the rotational state represented by the total angular momentum. Theoretical simulations via the configuration-interaction (CI) method are in agreement with the observed roto-vibrational modes and indicate that such molecular excitations develop at the onset of short-range correlation., Comment: PDF file only; 24 pages, 7 figures, 2 table. Supplementary Information included

Optical absorption measurements are used to probe the spin polarization in the integer and fractional quantum Hall effect regimes. The system is fully spin polarized only at filling factor $\nu=1$ and at very low temperatures($\sim40$ mK). A small change in filling factor ($\delta\nu\approx\pm0.01$) leads to a significant depolarization. This suggests that the itinerant quantum Hall ferromagnet at $\nu=1$ is surprisingly fragile against increasing temperature, or against small changes in filling factor., Comment: 4 pages, 2 figures

The authors report that anisotropic confining potentials in laterally-coupled semiconductor quantum dots (QDs) have large impacts in optical transitions and energies of inter-shell collective electronic excitations. The observed anisotropies are revealed by inelastic light scattering as a function of the in-plane direction of light polarization and can be finely controlled by modifying the geometrical shape of the QDs. These experiments show that the tuning of the QD confinement potential offers a powerful method to manipulate electronic states and far-infrared inter-shell optical transitions in quantum dots., Comment: 8 pages, 4 figures

Complexity in many-particle systems occurs through processes of qualitative differentiation. These are described by concepts such as emerging states with specific symmetries that are linked to order parameters. In quantum Hall phases of electrons in semiconductor double layers with large inter-layer electron correlation there is an emergent many body exciton phase with an order parameter that measures the condensate fraction of excitons across the tunneling gap. As the inter-layer coupling is reduced by application of an in-plane magnetic field, this excitonic insulating state is brought in competition with a Fermi-metal phase of composite fermions (loosely, electrons with two magnetic flux quanta attached) stabilized by intra-layer electron correlation. Here we show that the quantum phase transformation between metallic and excitonic insulating states in the coupled bilayers becomes discontinuous (first-order) by impacts of different terms of the electron-electron interactions that prevail on weak residual disorder. The evidence is based on precise determinations of the excitonic order parameter by inelastic light scattering measurements close to the phase boundary. While there is marked softening of low-lying excitations, our experiments underpin the roles of competing orders linked to quasi-particle correlations in removing the divergence of quantum fluctuations., Comment: 18 pages, 4 figures, supp. mat. contains 3 figures

Optical control of the lateral quantum confinement and number of electrons confined in nanofabricated GaAs/AlGaAs quantum dots is achieved by illumination with a weak laser beam that is absorbed in the AlGaAs barrier. Precise tuning of energy-level structure and electron population is demonstrated by monitoring the low-lying transitions of the electrons from the lowest quantum-dot energy shells by resonant inelastic light scattering. These findings open the way to the manipulation of single electrons in these quantum dots without the need of external metallic gates., Comment: To appear in NanoLetters

The interaction of electron-hole pairs with lattice vibrations exhibits a wealth of intriguing physical phenomena. The Kohn anomaly is a renowned example where electron-phonon coupling leads to non-analytic phonon dispersion at specific momentum nesting the Fermi surface. Here we report evidence of another type of phonon anomaly discovered by low temperature Raman spectroscopy in bilayer graphene where the charge density is modulated by the electric field effect. This anomaly, arising from charge-tunable modulations of particle-hole pairs that are resonantly coupled to lattice vibrations, is predicted to exhibit a logarithmic divergence in the long-wavelength optical-phonon energy. In a non-uniform bilayer of graphene, the logarithmic divergence is abated by charge density inhomogeneity leaving as a vestige an anomalous phonon softening. The observed softening marks the first confirmation of the phonon anomaly as a key signature of the resonant deformation-potential electron-phonon coupling. The high sensitivity of the phonon softening to charge density non-uniformity creates significant venues to explore the interplay between fundamental interactions and disorder in the atomic layers., Comment: 4 figures

Neutral spin texture ST excitations at nu=1/3 are directly observed for the first time by resonant inelastic light scattering. They are determined to involve two simultaneous spin- flips. At low magnetic fields, the ST energy is below that of the magneto-roton minimum. With increasing in-plane magnetic field these modes energies cross at a critical ratio of the Zeeman and Coulomb energies of eta_c=0.020 +- 0.001. Surprisingly, the intensity of the ST mode grows with temperature in the range in which the magneto-roton modes collapse. The temperature dependence is interpreted in terms of a competition between coexisting phases supporting different excitations. We consider the role of the ST excitations in activated transport at nu=1/3., Comment: 5 pages, 4 color figs

The ground state of the two dimensional electron gas near $\nu$=1 is investigated by inelastic light scattering measurements carried down to very low temperatures. Away from $\nu$=1, the ferromagnetic spin wave collapses and a new low-energy spin wave emerges below the Zeeman gap. The emergent spin wave shows soft behavior as its energy increases with temperature and reaches the Zeeman energy for temperatures above 2 K. The observed softening indicates an instability of the two dimensional electron gas towards a magnetic order that breaks spin rotational symmetry. We discuss our findings in light of the possible existence of a Skyrme crystal., Comment: 4 pages, 4 figures, to appear in Phys. Rev. Lett

Dilute arrays of GaAs/AlGaAs modulation-doped quantum dots (QDs) fabricated by electron-beam lithography and low impact reactive-ion etching exhibit highly homogeneous luminescence. Single quantum dots display spectral emission with peak energies and linewidths linked largely to the geometrical diameter of the dot and to the built-in electron population. Excitonic-like and biexcitonic-like emission intensities have activation energy of about 2 meV. These results highlight the potential of high quality nanofabricated QDs for applications in areas that require fine control of optical emission., Comment: 3 Figures

Composite fermion metal states emerge in quantum Hall bilayers at total Landau level filling factor $\nu_T$=1 when the tunneling gap collapses by application of in-plane components of the external magnetic field. Evidence of this transformation is found in the continua of spin excitations observed by inelastic light scattering below the spin-wave mode at the Zeeman energy. The low-lying spin modes are interpreted as quasiparticle excitations with simultaneous changes in spin orientation and composite fermion Landau level index., Comment: 4 pages 4 figures

We study the absorption spectrum of a two-dimensional electron gas (2DEG) in a magnetic field. We find that that at low temperatures, when the 2DEG is spin polarized, the absorption spectra, which correspond to the creation of spin up or spin down electron, differ in magnitude, linewidth and filling factor dependence. We show that these differences can be explained as resulting from creation of a Mahan exciton in one case, and of a power law Fermi edge singularity in the other., Comment: 4 pages, 4 figures, published in Phys. Rev. Lett

Gate-modulated low-temperature Raman spectra reveal that the electric field effect (EFE), pervasive in contemporary electronics, has marked impacts on long wavelength optical phonons of graphene. The EFE in this two dimensional honeycomb lattice of carbon atoms creates large density modulations of carriers with linear dispersion (known as Dirac fermions). Our EFE Raman spectra display the interactions of lattice vibrations with these unusual carriers. The changes of phonon frequency and line-width demonstrate optically the particle-hole symmetry about the charge-neutral Dirac-point. The linear dependence of the phonon frequency on the EFE-modulated Fermi energy is explained as the electron-phonon coupling of mass-less Dirac fermions., Comment: 4 pages, 4 figures

We present measurements of optical interband absorption in the fractional quantum Hall regime in a GaAs quantum well in the range 0 < nu < 1. We investigate the mechanism of singlet trion absorption, and show that its circular dichroism can be used as a probe of the spin polarization of the ground state of the two-dimensional electron system (2DES). We find that at nu = 1/3 the 2DES is fully spin-polarized. Increasing the filling factor results in a gradual depolarization, with a sharp minimum in the dichroism near nu = 2/3. We find that in the range 0.5 < nu < 0.85 the 2DES remains partially polarized for the broad range of magnetic fields from 2.75 to 11 Tesla. This is consistent with the presence of a mixture of polarized and depolarized regions., Comment: 4 pages, 4 figures (Fig 4 is in color)

Resonant Rayleigh scattering of light from electrons confined in gallium arsenide double quantum wells displays significant changes at temperatures that are below one degree Kelvin. The Rayleigh resonance occurs for photon energies that overlap a quantum well exciton and when electron bilayers condense into a quantum-Hall state. Marked changes in Rayleigh scattering intensities that occur in response to application of an in-plane magnetic field indicate that the unexpected temperature dependence is linked to formation of non-uniform electron fluids in a disordered quantum-Hall phase. These results demonstrate a new realm of study in which resonant Rayleigh scattering methods probe quantum phases of cold electrons in semiconductor heterostructures.

Spin excitations from a partially populated composite fermion level are studied above and below $\nu=1/3$. In the range $2/7<\nu<2/5$ the experiments uncover significant departures from the non-interacting composite fermion picture that demonstrate the increasing impact of interactions as quasiparticle Landau levels are filled. The observed onset of a transition from free to interacting composite fermions could be linked to condensation into the higher order states suggested by transport experiments and numerical evaluations performed in the same filling factor range., Comment: 4 pages, 5 figures, to appear in PRL

We report inelastic light scattering experiments in the fractional quantum Hall regime at filling factors $\nu\lesssim1/3$. A spin mode is observed below the Zeeman energy. The filling factor dependence of the mode energy is consistent with its assignment to spin flip excitations of composite fermions with four attached flux quanta ($\phi$=4). Our findings reveal a composite fermion Landau level structure in the $\phi$=4 sequence., Comment: 7 pages, 4 figures, EP2DS-16 conference, to appear in Physica E

We report inelastic light scattering measurements of spin and charge excitations in nanofabricated AlGaAs/GaAs quantum dots with few electrons. A narrow spin excitation peak is observed and assigned to the intershell triplet-to-singlet monopole mode of dots with four electrons. Configurationinteraction theory provides precise quantitative interpretations that uncover large correlation effects that are comparable to exchange Coulomb interactions., Comment: 4 pages, 4 figures

The Hartree-Fock paradigm of bilayer quantum Hall states with finite tunneling at filling factor $\nu$=1 has full pseudospin ferromagnetic order with all the electrons in the lowest symmetric Landau level. Inelastic light scattering measurements of low energy spin excitations reveal major departures from the paradigm at relatively large tunneling gaps. The results indicate the emergence of a novel correlated quantum Hall state at $\nu$=1 characterized by reduced pseudospin order. Marked anomalies occur in spin excitations when pseudospin polarization collapses by application of in-plane magnetic fields., Comment: ReVTeX4, 4 pages, 3 EPS figures

Resonant inelastic light scattering experiments at $\nu=1/3$ reveal a novel splitting of the long wavelength modes in the low energy spectrum of quasiparticle excitations in the charge degree of freedom. We find a single peak at small wavevectors that splits into two distinct modes at larger wavevectors. The evidence of well-defined dispersive behavior at small wavevectors indicates a coherence of the quantum fluid in the micron length scale. We evaluate interpretations of long wavelength modes of the electron liquid., Comment: 4 pages, 4 figures

Low lying excitations of electron liquids in the fractional quantum Hall (FQH) regime are studied by resonant inelastic light scattering methods. We present here results from charge and spin excitations of FQH states in the lowest spin-split Landau levels that are of current interest. In the range of filling factors $2/5 \geq \nu \geq 1/3$, we find evidence that low energy quasiparticle excitations can be interpreted with spin-split composite fermion quasi-Landau levels. At FQH states around $\nu=3/2$, we find well-defined excitations at 4/3 and 8/5 that are consistent with a spin-unpolarized population of quasi-Landau levels., Comment: 7 pages, 7 figures

Strong resonant enhancements of inelastic light scattering from the long wavelength inter-Landau level magnetoplasmon and the intra-Landau level spin wave excitations are seen for the fractional quantum Hall state at $\nu = 1/3$. The energies of the sharp peaks (FWHM $\lesssim 0.2meV$) in the profiles of resonant enhancement of inelastic light scattering intensities coincide with the energies of photoluminescence bands assigned to negatively charged exciton recombination. To interpret the observed enhancement profiles, we propose three-step light scattering mechanisms in which the intermediate resonant transitions are to states with charged excitonic excitations., Comment: 5 pages, 5 figures

Strongly-correlated two-dimensional electrons in coupled semiconductor bilayers display remarkable broken symmetry many-body states under accessible and controllable experimental conditions. In the cases of continuous quantum phase transitions soft collective modes drive the transformations that link distinct ground states of the electron double layers. In this paper we consider results showing that resonant inelastic light scattering methods detect soft collective modes of the double layers and probe their evolution with temperature and magnetic field. The light scattering experiments offer venues of research of fundamental interactions and continuous quantum phase transitions in low-dimensional electron liquids., Comment: 10 pages, 7 figures

The recent report on the observation of soft magnetorotons in the dispersion of charge-density excitations across the tunneling gap in coupled bilayers at total Landau level filling factor $\nu_T=1$ is reviewed. The inelastic light scattering experiments take advantage of the breakdown of wave-vector conservation that occurs under resonant excitation. The results offer evidence that in the quantum Hall state there is a roton that softens and sharpens markedly when the phase boundary for transitions to highly-correlated compressible states is approached. These findings are interpreted with Hartree-Fock evaluations of the dynamic structure factor. The model includes the effect of disorder in the breakdown of wave-vector conservation and resonance enhancement profiles within a phenomenological approach. These results link the softening of magnetorotons to enhanced excitonic Coulomb interactions in the ferromagnetic bilayers., Comment: 6 pages, 5 figures; conference: EP2DS-15

Resonant inelastic light scattering experiments access the low lying excitations of electron liquids in the fractional quantum Hall regime in the range $2/5 \geq \nu \geq 1/3$. Modes associated with changes in the charge and spin degrees of freedom are measured. Spectra of spin reversed excitations at filling factor $\nu \gtrsim 1/3$ and at $\nu \lesssim 2/5$ identify a structure of lowest spin-split Landau levels of composite fermions that is similar to that of electrons. Observations of spin wave excitations enable determinations of energies required to reverse spin. The spin reversal energies obtained from the spectra illustrate the significant residual interactions of composite fermions. At $\nu = 1/3$ energies of spin reversal modes are larger but relatively close to spin conserving excitations that are linked to activated transport. Predictions of composite fermion theory are in good quantitative agreement with experimental results., Comment: Submitted to special issue of Solid State Comm