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Analysis of bulk meteorite compositions has revealed small isotopic variations due to the presence of material (e.g., stardust) that preserved the signature of nuclear reactions occurring in specific stellar sites. The interpretation of such anomalies provides evidence for the environment of the birth of the Sun, its accretion process, the evolution of the solar proto-planetary disk, and the formation of the planets. A crucial element of such interpretation is the comparison of the observed anomalies to predictions from models of stellar nucleosynthesis. To date, however, this comparison has been limited to a handful of model predictions. This is mostly because the calculated stellar abundances need to be transformed into a specific representation, which nuclear astrophysicists and stellar nucleosynthesis researchers are not familiar with. Here, we show in detail that this representation is needed to account for mass fractionation effects in meteorite data that can be generated both in nature and during instrumental analysis. We explain the required internal normalisation to a selected isotopic ratio, describe the motivations behind such representation more widely, and provide the tools to perform the calculations. Then, we present some examples considering two elements produced by the $slow$ neutron-capture ($s$) process: Sr and Mo. We show which specific representations for the Sr isotopic composition calculated by $s$-process models better disentangle the nucleosynthetic signatures from stars of different metallicity. For Mo, the comparison between data and models is improved due to a recent re-analysis of the $^{95}$Mo neutron-capture cross section., Comment: Accepted for publication in the EPJA Special Issue on: 'From reactors to stars' in honor of Franz K\"appeler

While modelling the galactic chemical evolution (GCE) of stable elements provides insights to the formation history of the Galaxy and the relative contributions of nucleosynthesis sites, modelling the evolution of short-lived radioisotopes (SLRs) can provide supplementary timing information on recent nucleosynthesis. To study the evolution of SLRs, we need to understand their spatial distribution. Using a 3-dimensional GCE model, we investigated the evolution of four SLRs: Mn-53, Fe-60, Hf-182, and Pu-244 with the aim of explaining detections of recent (within the last $\approx$1-20 Myr) deposition of live Mn-53, Fe-60, and Pu-244 of extrasolar origin into deep-sea reservoirs. We find that core-collapse supernovae (CCSNe) are the dominant propagation mechanism of SLRs in the Galaxy. This results in the simultaneously arrival of these four SLRs on Earth, although they could have been produced in different astrophysical sites, which can explain why live extrasolar Mn-53, Fe-60, and Pu-244 are found within the same, or similar, layers of deep-sea sediments. We predict that Hf-182 should also be found in such sediments at similar depths., Comment: 22 pages, 11 figures

We investigate the origin in the early Solar System of the short-lived radionuclide 244Pu (with a half life of 80 Myr) produced by the rapid (r) neutron-capture process. We consider two large sets of r-process nucleosynthesis models and analyse if the origin of 244Pu in the ESS is consistent with that of the other r and slow (s) neutron-capture process radioactive nuclei. Uncertainties on the r-process models come from both the nuclear physics input and the astrophysical site. The former strongly affects the ratios of isotopes of close mass (129I/127I, 244Pu/238U, and 247Pu/235U). The 129I/247Cm ratio, instead, which involves isotopes of a very different mass, is much more variable than those listed above and is more affected by the physics of the astrophysical site. We consider possible scenarios for the evolution of the abundances of these radioactive nuclei in the galactic interstellar medium and verify under which scenarios and conditions solutions can be found for the origin of 244Pu that are consistent with the origin of the other isotopes. Solutions are generally found for all the possible different regimes controlled by the interval ($\delta$) between additions from the source to the parcel of interstellar medium gas that ended up in the Solar System, relative to decay timescales. If r-process ejecta in interstellar medium are mixed within a relatively small area (leading to a long $\delta$), we derive that the last event that explains the 129I and 247Cm abundances in the early Solar System can also account for the abundance of 244Pu. Due to its longer half life, however, 244Pu may have originated from a few events instead of one only. If r-process ejecta in interstellar medium are mixed within a relatively large area (leading to a short $\delta$), we derive that the time elapsed from the formation of the molecular cloud to the formation of the Sun was 9-16 Myr., Comment: 17 pages, 3 figures, published on Universe as part of the Special Issue "Nuclear Astrophysics in the Era of High Precision Astronomy"

Radioactive nuclei are the key to understanding the circumstances of the birth of our Sun because meteoritic analysis has proven that many of them were present at that time. Their origin, however, has been so far elusive. The ERC-CoG-2016 RADIOSTAR project is dedicated to investigating the production of radioactive nuclei by nuclear reactions inside stars, their evolution in the Milky Way Galaxy, and their presence in molecular clouds. So far, we have discovered that: (i) radioactive nuclei produced by slow ($^{107}$Pd and $^{182}$Hf) and rapid ($^{129}$I and $^{247}$Cm) neutron captures originated from stellar sources - asymptotic giant branch (AGB) stars and compact binary mergers, respectively - within the galactic environment that predated the formation of the molecular cloud where the Sun was born; (ii) the time that elapsed from the birth of the cloud to the birth of the Sun was of the order of 10$^7$ years, and (iii) the abundances of the very short-lived nuclei $^{26}$Al, $^{36}$Cl, and $^{41}$Ca can be explained by massive star winds in single or binary systems, if these winds directly polluted the early Solar System. Our current and future work, as required to finalise the picture of the origin of radioactive nuclei in the Solar System, involves studying the possible origin of radioactive nuclei in the early Solar System from core-collapse supernovae, investigating the production of $^{107}$Pd in massive star winds, modelling the transport and mixing of radioactive nuclei in the galactic and molecular cloud medium, and calculating the galactic chemical evolution of $^{53}$Mn and $^{60}$Fe and of the p-process isotopes $^{92}$Nb and $^{146}$Sm., Comment: accepted for publication on Universe Special Issue AGB Stars - In Honor of Professor Maurizio Busso on the Occasion of His 70th Birthday

The composition of the early Solar System can be inferred from meteorites. Many elements heavier than iron were formed by the rapid neutron-capture process (r process), but the astrophysical sources where this occurred remain poorly understood. We demonstrate that the near-identical half-lives ($\simeq$ 15.6 Myr) of the radioactive r-process nuclei 129I and 247Cm preserve their ratio, irrespective of the time between production and incorporation into the Solar System. We constrain the last r-process source by comparing the measured meteoritic 129I / 247Cm = 438 $\pm$ 184 to nucleosynthesis calculations based on neutron star merger and magneto-rotational supernova simulations. Moderately neutron-rich conditions, often found in merger disk ejecta simulations, are most consistent with the meteoritic value. Uncertain nuclear physics data limit our confidence in this conclusion., Comment: 36 pages, 7 figures, 7 tables

Solar system materials are variably depleted in moderately volatile elements (MVEs) relative to the proto-solar composition. To address the origin of this MVE depletion, we conducted a systematic study of high-precision K isotopic composition on 16 carbonaceous chondrites (CCs) of types CM1-2, CO3, CV3, CR2, CK4-5 and CH3 and 28 ordinary chondrites (OCs) covering petrological types 3 to 6 and chemical groups H, L, and LL. We observed significant overall K isotope (delta41K) variations (-1.54 to 0.70 permil). The K isotope compositions of CCs are largely higher than the Bulk Silicate Earth (BSE) value, whereas OCs show typically lower values than BSE. Neither CCs nor OCs show resolvable correlations between K isotopes and chemical groups, petrological types, shock levels, exposure ages, fall or find occurrence, or terrestrial weathering. The lack of a clear trend between K isotopes and K content indicates that the K isotope fractionations were decoupled from the relative elemental K depletions. The range of K isotope variations in the CCs is consistent with a four-component (chondrule, refractory inclusion, matrix and water) mixing model that is able to explain the bulk elemental and isotopic compositions of the main CC groups, but requires a fractionation in K isotopic compositions in chondrules. We propose that the major control of the isotopic compositions of group averages is condensation or vaporization in nebular environments that is preserved in the compositional variation of chondrules. Parent-body processes (aqueous alteration, thermal metamorphism, and metasomatism) can mobilize K and affect the K isotopes in individual samples. In the case of the OCs, the full range of K isotopic variations can only be explained by the combined effects of the size and relative abundances of chondrules, parent-body aqueous and thermal alteration., Comment: 71 pages, 2 tables, 9 figures

Enstatite chondrites and aubrites are meteorites that show the closest similarities to the Earth in many isotope systems that undergo mass-independent and mass-dependent isotope fractionations. Due to the analytical challenges to obtain high-precision K isotopic compositions in the past, potential differences in K isotopic compositions between enstatite meteorites and the Earth remained uncertain. We report the first high-precision K isotopic compositions of eight enstatite chondrites and four aubrites and find that there is a significant variation of K isotopic compositions among enstatite meteorites (from -2.34 permil to -0.18 permil). However, K isotopic compositions of nearly all enstatite meteorites scatter around the Bulk Silicate Earth (BSE) value. The average K isotopic composition of the eight enstatite chondrites (-0.47 +/- 0.57 permil) is indistinguishable from the BSE value (-0.48 +/- 0.03 permil), thus further corroborating the isotopic similarity between Earth' building blocks and enstatite meteorite precursors. We found no correlation of K isotopic compositions with the chemical groups, petrological types, shock degrees, and terrestrial weathering conditions; however, the variation of K isotopes among enstatite meteorite can be attributed to the parent body processing. Our sample of the main group aubrite MIL 13004 is exceptional and has an extremely light K isotopic composition (delta 41K= -2.34 +/- 0.12 permil). We attribute this unique K isotopic feature to the presence of abundant djerfisherite inclusions in our sample because this K-bearing sulfide mineral is predicted to be enriched in 39K during equilibrium exchange with silicates., Comment: 46 pages, 7 figures, 2 tables, published in Meteoritics & Planetary Science