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In 1927, during the fifth Solvay Conference, Einstein and Bohr described a double-slit interferometer with a "movable slit" that can detect the momentum recoil of one photon. Here, we report a faithful realization of the Einstein-Bohr interferometer using a single atom in an optical tweezer, cooled to the motional ground state in three dimensions. The single atom has an intrinsic momentum uncertainty comparable to a single photon, which serves as a movable slit obeying the minimum Heisenberg uncertainty principle. The atom's momentum wavefunction is dynamically tunable by the tweezer laser power, which enables observation of an interferometric visibility reduction at a shallower trap, demonstrating the quantum nature of this interferometer. We further identify classical noise due to atom heating and precession, illustrating a quantum-to-classical transition., Comment: 18 pages, 4 figures

Topological phases at quantum criticality attract much attention recently. Here we numerically study the interaction-induced phase transitions at around the topological quantum critical points of an extended Su-Schrieffer-Heeger (SSH) chain with next-nearest-neighbor hopping. This extended SSH model shows topological phase transitions between the topologically trivial and nontrivial critical phases when interaction is absent. So long as the interaction terms are turned on, the topologically nontrivial (trivial) critical phases are driven into topologically nontrivial (trivial) insulator phases with finite energy gaps. Particularly, we find the trivial insulator phase is further driven to the nontrivial insulator phase, through interaction-induced topological phase transition, although interaction generally is harmful to nontrivial topology. The stability of trivial insulator phase against interaction tends to vanish at the multicritical point that separates the trivial and nontrivial critical phases. Our work provides a concrete example for manifesting the impact of interaction on topological quantum criticality., Comment: 6 pages, 4 figures

Quantum money is the first invention in quantum information science, promising advantages over classical money by simultaneously achieving unforgeability, user privacy, and instant validation. However, standard quantum money relies on quantum memories and long-distance quantum communication, which are technologically extremely challenging. Quantum "S-money" tokens eliminate these technological requirements while preserving unforgeability, user privacy, and instant validation. Here, we report the first full experimental demonstration of quantum S-tokens, proven secure despite errors, losses and experimental imperfections. The heralded single-photon source with a high system efficiency of 88.24% protects against arbitrary multi-photon attacks arising from losses in the quantum token generation. Following short-range quantum communication, the token is stored, transacted, and verified using classical bits. We demonstrate a transaction time advantage over intra-city 2.77 km and inter-city 60.54 km optical fibre networks, compared with optimal classical cross-checking schemes. Our implementation demonstrates the practicality of quantum S-tokens for applications requiring high security, privacy and minimal transaction times, like financial trading and network control. It is also the first demonstration of a quantitative quantum time advantage in relativistic cryptography, showing the enhanced cryptographic power of simultaneously considering quantum and relativistic physics., Comment: 74 pages, 6 figures

A quantum network provides an infrastructure connecting quantum devices with revolutionary computing, sensing, and communication capabilities. As the best-known application of a quantum network, quantum key distribution (QKD) shares secure keys guaranteed by the laws of quantum mechanics. A quantum satellite constellation offers a solution to facilitate the quantum network on a global scale. The Micius satellite has verified the feasibility of satellite quantum communications, however, scaling up quantum satellite constellations is challenging, requiring small lightweight satellites, portable ground stations and real-time secure key exchange. Here we tackle these challenges and report the development of a quantum microsatellite capable of performing space-to-ground QKD using portable ground stations. The quantum microsatellite features a payload weighing approximately 23 kg, while the portable ground station weighs about 100 kg. These weights represent reductions by more than an order and two orders of magnitude, respectively, compared to the Micius satellite. Additionally, we multiplex bidirectional satellite-ground optical communication with quantum communication, enabling key distillation and secure communication in real-time. Using the microsatellite and the portable ground stations, we demonstrate satellite-based QKD with multiple ground stations and achieve the sharing of up to 0.59 million bits of secure keys during a single satellite pass. The compact quantum payload can be readily assembled on existing space stations or small satellites, paving the way for a satellite-constellation-based quantum and classical network for widespread real-life applications., Comment: 40 pages, 8 figures

Nonlocality, evidenced by the violation of Bell inequalities, not only signifies entanglement but also highlights measurement incompatibility in quantum systems. Utilizing the generalized Clauser-Horne-Shimony-Holt (CHSH) Bell inequality, our high-efficiency optical setup achieves a loophole-free violation of $2.0132$. This result provides a device-independent lower bound on entanglement, quantified as the entanglement of formation at $0.0159$. Moreover, by tuning the parameters of the generalized Bell inequality, we enhance the estimation of measurement incompatibility, which is quantified by an effective overlap of $4.3883 \times 10^{-5}$. To explore the intricate interplay among nonlocality, entanglement, and measurement incompatibility, we generate mixed states, allowing for flexible modulation of entanglement via fast switching among the four Bell states using Pockels cells, achieving a fidelity above $99.10\%$. Intriguingly, our results reveal a counterintuitive relationship where increasing incompatibility initially boosts nonlocality but eventually leads to its reduction. Typically, maximal nonlocality does not coincide with maximal incompatibility. This experimental study sheds light on the optimal management of quantum resources for Bell-inequality-based quantum information processing., Comment: 15 pages, 9 figures

The entangled photons are crucial resources for quantum communications and networking. Here, we present an ultra-bright polarization-entangled photon source based on a periodically poled lithium niobate waveguide designed for practical quantum communication networks. Using a 780 nm pump laser, the source achieves a pair generation rate of 2.4 $\times 10^{10}$ pairs/s/mW. This work has achieved a directly measured power of 17.9 nW in entangled photon generation with a 3.2 mW pump power. Based on this, we demonstrate the practicality of the source by conducting quantum key distribution experiments over long-distance fiber links, achieving the applicable secure key rates of up to 440.80 bits/s over 200 km with 62 dB loss and reaching a maximum secure key generation distance of 404 km. These results demonstrate the potential of wavelength-multiplexed polarization-entangled photon sources for high-speed, long-distance quantum communication, positioning them as key components for future large-scale quantum networks., Comment: 18 pages, 6 figures

The emergence of quantum mechanics and general relativity has transformed our understanding of the natural world significantly. However, integrating these two theories presents immense challenges, and their interplay remains untested. Recent theoretical studies suggest that the single-photon interference covering huge space can effectively probe the interface between quantum mechanics and general relativity. We developed an alternative design using unbalanced Michelson interferometers to address this and validated its feasibility over an 8.4 km free-space channel. Using a high-brightness single-photon source based on quantum dots, we demonstrated single-photon interference along this long-distance baseline. We achieved a phase measurement precision of 16.2 mrad, which satisfied the measurement requirements for a gravitational redshift at the geosynchronous orbit by five times the standard deviation. Our results confirm the feasibility of the single-photon version of the Colella-Overhauser-Werner experiment for testing the quantum effects in curved spacetime., Comment: 22 pages, 6 figures

Frequency tunable qubit plays a significant role for scalable superconducting quantum processors. The state-of-the-art room-temperature electronics for tuning qubit frequency suffers from unscalable limit, such as heating problem, linear growth of control cables, etc. Here we propose a scalable scheme to tune the qubit frequency by using in situ superconducting circuit, which is based on radio frequency superconducting quantum interference device (rf-SQUID). We demonstrate both theoretically and experimentally that the qubit frequency could be modulated by inputting several single pulses into rf-SQUID. Compared with the traditional scheme, our scheme not only solves the heating problem, but also provides the potential to exponentially reduce the number of cables inside the dilute refrigerator and the room-temperature electronics resource for tuning qubit frequency, which is achieved by a time-division-multiplex (TDM) scheme combining rf-SQUID with switch arrays. With such TDM scheme, the number of cables could be reduced from the usual $\sim 3n$ to $\sim \log_2{(3n)} + 1$ for two-dimensional quantum processors comprising $n$ qubits and $\sim 2n$ couplers. Our work paves the way for large-scale control of superconducting quantum processor., Comment: 9 pages, 6 figures

Quantum Computational Superiority boasts rapid computation and high energy efficiency. Despite recent advances in classical algorithms aimed at refuting the milestone claim of Google's sycamore, challenges remain in generating uncorrelated samples of random quantum circuits. In this paper, we present a groundbreaking large-scale system technology that leverages optimization on global, node, and device levels to achieve unprecedented scalability for tensor networks. This enables the handling of large-scale tensor networks with memory capacities reaching tens of terabytes, surpassing memory space constraints on a single node. Our techniques enable accommodating large-scale tensor networks with up to tens of terabytes of memory, reaching up to 2304 GPUs with a peak computing power of 561 PFLOPS half-precision. Notably, we have achieved a time-to-solution of 14.22 seconds with energy consumption of 2.39 kWh which achieved fidelity of 0.002 and our most remarkable result is a time-to-solution of 17.18 seconds, with energy consumption of only 0.29 kWh which achieved a XEB of 0.002 after post-processing, outperforming Google's quantum processor Sycamore in both speed and energy efficiency, which recorded 600 seconds and 4.3 kWh, respectively.

Random quantum circuit sampling serves as a benchmark to demonstrate quantum computational advantage. Recent progress in classical algorithms, especially those based on tensor network methods, has significantly reduced the classical simulation time and challenged the claim of the first-generation quantum advantage experiments. However, in terms of generating uncorrelated samples, time-to-solution, and energy consumption, previous classical simulation experiments still underperform the \textit{Sycamore} processor. Here we report an energy-efficient classical simulation algorithm, using 1432 GPUs to simulate quantum random circuit sampling which generates uncorrelated samples with higher linear cross entropy score and is 7 times faster than \textit{Sycamore} 53 qubits experiment. We propose a post-processing algorithm to reduce the overall complexity, and integrated state-of-the-art high-performance general-purpose GPU to achieve two orders of lower energy consumption compared to previous works. Our work provides the first unambiguous experimental evidence to refute \textit{Sycamore}'s claim of quantum advantage, and redefines the boundary of quantum computational advantage using random circuit sampling., Comment: This work was completed on August 2023. A further 50x improvement has been achieved and will be posted on arXiv shortly

Single-photon sources are essential for quantum networks, enabling applications ranging from quantum key distribution (QKD) to the burgeoning quantum internet. Despite the remarkable advancements, the current reliance of QKD on attenuated coherent (laser) light sources has imposed a fundamental limit on the secret key rate (SKR). This constraint is primarily attributable to the scarcity of single-photon components within coherent light, confined by an inherent upper bound of 1/e. Here, we report high-rate QKD using a high-efficiency single-photon source, enabling an SKR transcending the fundamental rate limit of coherent light. We developed an on-demand, bright semiconductor quantum-dot single-photon source with an efficiency of 0.71(2), exceeding the inherent bound of coherent light by approximately 2.87 dB. Implementing narrow-bandwidth filtering and random polarization modulation, we conducted a field QKD trial over a 14.6(1.1)-dB-loss free-space urban channel, achieving an SKR of 0.00108 bits per pulse. This surpasses the practical limit of coherent-light-based QKD by 2.53 dB. Our findings conclusively demonstrate the superior performance of nanotechnology-based single-photon sources over coherent light for QKD applications, marking a pivotal stride towards the realization of a global quantum internet., Comment: 22 pages, 5 figures, 1 Table

Finding accurate ground state energy of a many-body system has been a major challenge in quantum chemistry. The integration of classic and quantum computers has shed new light on resolving this outstanding problem. Here we propose QiankunNet-VQE, a transformer based language models enforced with quantum computing to learn and generate quantum states. It has been implemented using up to 12 qubits and attaining an accuracy level competitive with state-of-the-art classical methods. By leveraging both quantum and classical resources, this scheme overcomes the limitations of variational quantum eigensolver(VQE) without the need for cumbersome error mitigation. Moreover, QiankunNet-VQE provides a different route to achieve a practical quantum advantage for solving many-electron Schr\"odinger equation without requiring extremely precise preparation and measurement of the ground-state wavefunction on quantum computer.

To make practical quantum algorithms work, large-scale quantum processors protected by error-correcting codes are required to resist noise and ensure reliable computational outcomes. However, a major challenge arises from defects in processor fabrication, as well as occasional losses or cosmic rays during the computing process, all of which can lead to qubit malfunctions and disrupt error-correcting codes' normal operations. In this context, we introduce an automatic adapter to implement the surface code on defective lattices. Unlike previous approaches, this adapter leverages newly proposed bandage-like super-stabilizers to save more qubits when defects are clustered, thus enhancing the code distance and reducing super-stabilizer weight. For instance, in comparison with earlier methods, with a code size of 27 and a random defect rate of 2\%, the disabled qubits decrease by $1/3$, and the average preserved code distance increases by 63\%. This demonstrates a significant reduction in overhead when handling defects using our approach, and this advantage amplifies with increasing processor size and defect rates. Our work presents a low-overhead, automated solution to the challenge of adapting the surface code to defects, an essential step towards scaling up the construction of large-scale quantum computers for practical applications.

Long baseline diffraction-limited optical aperture synthesis technology by interferometry plays an important role in scientific study and practical application. In contrast to amplitude (phase) interferometry, intensity interferometry -- which exploits the quantum nature of light to measure the photon bunching effect in thermal light -- is robust against atmospheric turbulence and optical defects. However, a thermal light source typically has a significant divergence angle and a low average photon number per mode, forestalling the applicability over long ranges. Here, we propose and demonstrate active intensity interferometry for super-resolution imaging over the kilometer range. Our scheme exploits phase-independent multiple laser emitters to produce the thermal illumination and uses an elaborate computational algorithm to reconstruct the image. In outdoor environments, we image two-dimension millimeter-level targets over 1.36 kilometers at a resolution of 14 times the diffraction limit of a single telescope. High-resolution optical imaging and sensing are anticipated by applying long-baseline active intensity interferometry in general branches of physics and metrology., Comment: 42 pages, 11 figures

In this work, we give a hybrid quantum-classical algorithm for solving electronic structure problems of molecules using only linear quantum optical systems. The variational ansatz we proposed is a hybrid of non-interacting Boson dynamics and classical computational chemistry methods, specifically, the Hartree-Fock method and the Configuration Interaction method. The Boson part is built by a linear optical interferometer which is easier to realize compared with the well-known Unitary Coupled Cluster (UCC) ansatz composed of quantum gates in conventional VQE and the classical part is merely classical processing acting on the Hamiltonian. We called such ansatzes Boson Sampling-Classic (BS-C). The appearance of permanents in the Boson part has its physical intuition to provide different kinds of resources from commonly used single-, double-, and higher-excitations in classical methods and the UCC ansatz to exploring chemical quantum states. Such resources can help enhance the accuracy of methods used in the classical parts. We give a scalable hybrid homodyne and photon number measurement procedure for evaluating the energy value which has intrinsic abilities to mitigate photon loss errors and discuss the extra measurement cost induced by the no Pauli exclusion principle for Bosons with its solutions. To demonstrate our proposal, we run numerical experiments on several molecules and obtain their potential energy curves reaching chemical accuracy., Comment: 15 pages, 5 figures

Quantum randomness relies heavily on the accurate characterization of the generator implementation, where the device imperfection or inaccurate characterization can lead to incorrect entropy estimation and practical bias, significantly affecting the reliability of the generated randomness. Measurement-device-independent (MDI) quantum random number generation (QRNG) endeavors to produce certified randomness, utilizing uncharacterized and untrusted measurement devices that are vulnerable to numerous attack schemes targeting measurement loopholes. However, existing implementations have shown insufficient performance thus far. Here, we propose a high-speed MDI-QRNG scheme based on a robust measurement tomography approach against the imperfection of single-photon sources. Compared with the conventional approach, the decoy-state method is introduced to obtain more accurate tomography results and a tighter lower bound of randomness. Finally, by using a high-speed time-bin encoding system, we experimentally demonstrated the scheme and obtained a reliable min-entropy lower bound of $7.37 \times 10^{-2}$ bits per pulse, corresponding to a generation rate over 23 Mbps, which substantially outperforms the existing realizations and makes a record in discrete-variable semi-device-independent QRNGs., Comment: 20 pages, 9 figures, including appendixes. Accepted for publication in Quantum Science and Technology

Quantum key distribution is a cornerstone of quantum technology, offering information-theoretical secure keys for remote parties. With many quantum communication networks established globally, the mode-pairing protocol stands out for its efficacy over inter-city distances using simple setups, emerging as a promising solution. In this study, we employ the mode-pairing scheme into existing inter-city fiber links, conducting field tests across distances ranging from tens to about a hundred kilometers. Our system achieves a key rate of $1.217$ kbit/s in a $195.85$ km symmetric link and $3.089$ kbit/s in a $127.92$ km asymmetric link without global phase locking. The results demonstrate that the mode-pairing protocol can achieve key rates comparable to those of a single quantum link between two trusted nodes on the Beijing-Shanghai backbone line, effectively reducing the need for half of the trusted nodes. These field tests confirm the mode-pairing scheme's adaptability, efficiency, and practicality, positioning it as a highly suitable protocol for quantum networks., Comment: 15 pages, 5 figures, 6 tables

We report on an experimental simulation of the spin-1 Heisenberg model with composite bosons in a one-dimensional chain based on the two-component Bose-Hubbard model. Exploiting our site-and spin-resolved quantum gas microscope, we observed faster superexchange dynamics of the spin-1 system compared to its spin-1/2 counterpart, which is attributed to the enhancement effect of multi-bosons. We further probed the non-equilibrium spin dynamics driven by the superexchange and single-ion anisotropy terms, unveiling the linear expansion of the spin-spin correlations, which is limited by the Lieb-Robinson bound. Based on the superexchange process, we prepared and verified the entangled qutrits pairs with these composite spin-1 bosons, potentially being applied in qutrit-based quantum information processing.

The counterflow superfluidity (CSF) was predicted two decades ago. Counterintuitively, while both components in the CSF have fluidity, their correlated counterflow currents cancel out leading the overall system to an incompressible Mott insulator. However, realizing and identifying the CSF remain challenging due to the request on extreme experimental capabilities in a single setup. Here, we observe the CSF in a binary Bose mixture in optical lattices. We prepare a low-entropy spin-Mott state by conveying and merging two spin-1/2 bosonic atoms at every site and drive it adiabatically to the CSF at $\sim$ 1 nK. Antipair correlations of the CSF are probed though a site- and spin-resolved quantum gas microscope in both real and momentum spaces. These techniques and observations provide accessibility to the symmetry-protected topological quantum matters., Comment: 13 pages, 10 figures

The fermionic Hubbard model (FHM)[1], despite its simple form, captures essential features of strongly correlated electron physics. Ultracold fermions in optical lattices[2, 3] provide a clean and well-controlled platform for simulating FHM. Doping its antiferromagnetic ground state at half filling, various exotic phases are expected to arise in the FHM simulator, including stripe order[4], pseudogap[5], and d-wave superconductors[6], offering valuable insights into high-temperature superconductivity[7{9]. Although notable progress, such as the observation of antiferromagnetic correlations over short[10] and extended distances[11], has been obtained, the antiferromagnetic phase has yet to be realized due to the significant challenges of achieving low temperatures in a large and uniform quantum simulator. Here, we report the observation of the antiferromagnetic phase transition in a three-dimensional fermionic Hubbard system comprising lithium-6 atoms in a uniform optical lattice with approximately 800,000 sites. When the interaction strength, temperature, and doping concentration are finely tuned to approach their respective critical values, sharp increases in the spin structure factor (SSF) are observed. These observations can be well described by a power-law divergence, with a critical exponent of 1.396 from the Heisenberg universality class[12]. At half filling and with optimal interaction strength, the measured SSF reaches 123(8), signifying the establishment of an antiferromagnetic phase. Our results set the stage for exploring the low-temperature phase diagram of FHM.

Fractional quantum Hall (FQH) states, known for their robust topological order and the emergence of non-Abelian anyons, have captured significant interest due to the appealing applications in fault-tolerant quantum computing. Bottom-up approach on an engineered quantum platform will provide opportunities to operate FQH states without external magnetic field and enhance local and coherent manipulation of these exotic states. Here we demonstrate a lattice version of photon FQH state using a programmable on-chip platform based on photon blockade and engineering gauge fields on a novel two-dimensional circuit quantum electrodynamics (QED) system. We first observe the effective photon Lorentz force and butterfly spectrum in the artificial gauge field, a prerequisite for FQH states. After adiabatic assembly of Laughlin FQH wavefunction of 1/2 filling factor from localized photons, we observe strong density correlation and chiral topological flow among the FQH photons. We then verify the unique features of FQH states in response to external fields, including the incompressibility of generating quasiparticles and the smoking-gun signature of fractional quantum Hall conductivity. Our work represents a significant advance in the bottom-up creation and manipulation of novel strongly correlated topological quantum matter composed of photons and opens up possibilities for fault-tolerant quantum information devices., Comment: 8 pages, 6 figures

In this work, we give a quantum algorithm for solving the ground states of a class of Hamiltonians. The mechanism of the exponential speedup that appeared in our algorithm comes from dissipation in open quantum systems. To utilize the dissipation, the central idea is to treat $n$-qubit density matrices $\rho$ as $2n$-qubit pure states $|\rho\rangle$ by vectorization and normalization. By doing so, the Lindblad master equation (LME) becomes a Schr\"odinger equation with non-Hermitian Hamiltonian $L$. The steady-state $\rho_{ss}$ of the LME, therefore, corresponds to the ground states $|\rho_{ss}\rangle$ of Hamiltonians with the form $L^\dag L$. The runtime of the LME has no dependence on $\zeta$ the overlap between the initial state and the ground state compared with the Heisenberg scaling $\mathcal{O}(\zeta^{-1})$ in other algorithms. For the input part, given a Hamiltonian $H$, under plausible assumptions, we give a polynomial-time classical procedure to judge and solve whether there exists $L$ such that $H-E_0=L^\dag L$. For the output part, we define the mission as estimating expectation values of arbitrary operators with respect to the ground state $|\rho_{ss}\rangle$, which can be done surprisingly by an efficient measurement protocol on $\rho_{ss}$ with no need to prepare $|\rho_{ss}\rangle$. We give several pieces of evidence on the quantum hardness of really preparing $|\rho_{ss}\rangle$, which indicates a potential complexity separation between our algorithm and those projection-based quantum algorithms such as quantum phase estimation. Further, we show that the Hamiltonians that can be efficiently solved by our algorithms contain classically hard instances assuming $\text{P}\neq \text{BQP}$. Later, we discuss and analyze several important aspects of the algorithm including generalizing to other types of Hamiltonians and the "non-linear`` dynamics in the algorithm., Comment: 19 pages, 4 figures

Solid-state qubits with a photonic interface is very promising for quantum networks. Color centers in silicon carbide have shown excellent optical and spin coherence, even when integrated with membranes and nano-structures. Additionally, nuclear spins coupled with electron spins can serve as long-lived quantum memories. Pioneering work in previous has realized the initialization of a single nuclear spin and demonstrated its entanglement with an electron spin. In this paper, we report the first realization of single-shot readout for a nuclear spin in SiC. We obtain a deterministic readout fidelity of 98.2% with a measurement duration of 1.13 ms. With a dual-step readout scheme, we obtain a readout fidelity as high as 99.5% with a success efficiency of 89.8%. Our work complements the experimental toolbox of harnessing both electron and nuclear spins in SiC for future quantum networks., Comment: 5 pages, 4 figures

Surface currents emerge in superconductors exposed to magnetic fields, and are a key signature of the Meissner effect. Analogously, chiral dynamics were observed in quantum simulators under synthetic Abelian gauge fields. The flexible control of these simulators also facilitates the engineering of non-Abelian gauge fields, but their impact on the chiral dynamics remains elusive. Here, by employing the cutting-edge momentum-lattice technique, we implement a synthetic SU(2) gauge field in a spinful 1D ladder and study the rich chiral dynamics therein. We confirm the non-Abelian nature of the synthetic potential by observing the non-Abelian Aharonov-Bohm effect on a single plaquette. More importantly, the chiral current along the two legs of the ladder is observed to be spin-dependent and highly tunable through the parameters of the gauge potential. We experimentally map out different dynamic regimes of the chiral current, and reveal the underlying competition between overlaying flux ladders with distinct spin compositions. Our experiment demonstrates the dramatic impact of non-Abelian gauge fields on the system dynamics, paving the way for future studies of exotic synthetic gauge fields on the versatile platform of momentum lattices., Comment: 6 pages, 4 figures

The manipulation of particle transport in synthetic quantum matter is an active research frontier for its theoretical importance and potential applications. Here we experimentally demonstrate an engineered topological transport in a synthetic flat-band lattice of ultracold $^{87}$Rb atoms. We implement a quasi-one-dimensional rhombic chain with staggered flux in the momentum space of the atomic condensate and observe biased local oscillations that originate from the interplay of the staggered flux and flat-band localization under the mechanism of Aharonov-Bohm caging. Based on these features, we design and experimentally confirm a state-dependent chiral transport under the periodic modulation of the synthetic flux. We show that the phenomenon is topologically protected by the winding of the Floquet Bloch bands of a coarse-grained effective Hamiltonian. The observed chiral transport offers a strategy for efficient quantum device design where topological robustness is ensured by fast Floquet driving and flat-band localization., Comment: 5 pages, 3 figures

Bell's theorem states that quantum mechanical description on physical quantity cannot be fully explained by local realistic theories, and lays solid basis for various quantum information applications. Hardy's paradox is celebrated to be the simplest form of Bell's theorem concerning its "All versus Nothing" way to test local realism. However, due to experimental imperfections, existing tests of Hardy's paradox require additional assumptions of experimental systems, which constitute potential loopholes for faithfully testing local realistic theories. Here, we experimentally demonstrate Hardy's nonlocality through a photonic entanglement source. By achieving a detection efficiency of $82.2\%$, a quantum state fidelity of $99.10\%$ and applying high speed quantum random number generators for measurement setting switching, the experiment is implemented in a loophole-free manner. During $6$ hours of running, a strong violation of $P_{\text{Hardy}}=4.646\times 10^{-4}$ up to $5$ standard deviations is observed with $4.32\times 10^{9}$ trials. A null hypothesis test shows that the results can be explained by local realistic theories with an upper bound probability of $10^{-16348}$. These testing results present affirmative evidence against local realism, and provide an advancing benchmark for quantum information applications based on Hardy's paradox.

Quantum key distribution (QKD) holds the potential to establish secure keys over long distances. The distance of point-to-point QKD secure key distribution is primarily impeded by the transmission loss inherent to the channel. In the quest to realize a large-scale quantum network, increasing the QKD distance under current technology is of great research interest. Here we adopt the 3-intensity sending-or-not-sending twin-field QKD (TF-QKD) protocol with the actively-odd-parity-pairing method. The experiment demonstrates the feasibility of secure QKD over a 1002 km fibre channel considering the finite size effect. The secure key rate is $3.11\times10^{-12}$ per pulse at this distance. Furthermore, by optimizing parameters for shorter fiber distances, we conducted performance tests on key distribution for fiber lengths ranging from 202 km to 505 km. Notably, the secure key rate for the 202 km, the normal distance between major cities, reached 111.74 kbps., Comment: 18 pages, 3 figures

Photon loss is the biggest enemy for scalable photonic quantum information processing. This problem can be tackled by using quantum error correction, provided that the overall photon loss is below a threshold of 1/3. However, all reported on-demand and indistinguishable single-photon sources still fall short of this threshold. Here, by using tailor shaped laser pulse excitation on a high-quantum efficiency single quantum dot deterministically coupled to a tunable open microcavity, we demonstrate a high-performance source with a single-photon purity of 0.9795(6), photon indistinguishability of 0.986(16), and an overall system efficiency of 0.717(20), simultaneously. This source for the first time reaches the efficiency threshold for scalable photonic quantum computing. With this source, we further demonstrate 1.87(13) dB intensity squeezing, and consecutive 40-photon events with 1.67 mHz count rate.

Satellite-based greenhouse gases (GHG) sensing technologies play a critical role in the study of global carbon emissions and climate change. However, none of the existing satellite-based GHG sensing technologies can achieve the measurement of broad bandwidth, high temporal-spatial resolution, and high sensitivity at the same time. Recently, dual-comb spectroscopy (DCS) has been proposed as a superior candidate technology for GHG sensing because it can measure broadband spectra with high temporal-spatial resolution and high sensitivity. The main barrier to DCS's display on satellites is its short measurement distance in open air achieved thus far. Prior research has not been able to implement DCS over 20 km of open-air path. Here, by developing a bistatic setup using time-frequency dissemination and high-power optical frequency combs, we have implemented DCS over a 113 km turbulent horizontal open-air path. Our experiment successfully measured GHG with 7 nm spectral bandwidth and a 10 kHz frequency and achieved a CO2 sensing precision of <2 ppm in 5 minutes and <0.6 ppm in 36 minutes. Our results represent a significant step towards advancing the implementation of DCS as a satellite-based technology and improving technologies for GHG monitoring, Comment: 24 pages, 6 figures

Twin-field quantum key distribution (TF-QKD) overcomes the linear rate-loss limit, which promises a boost of secure key rate over long distance. However, the complexity of eliminating the frequency differences between the independent laser sources hinders its practical application. Here, taking the saturated absorption spectroscopy of acetylene as an absolute reference, we propose and demonstrate a simple and practical approach to realize TF-QKD without requiring relative frequency control of the independent laser sources. Adopting the 4-intensity sending-or-not-sending TF-QKD protocol, we experimentally demonstrate the TF-QKD over 502 km, 301 km and 201 km ultra-low loss optical fiber respectively. We expect this high-performance scheme will find widespread usage in future intercity and free-space quantum communication networks., Comment: 13 pages, 5 figures, 7 tables

Free-running InGaAs/InP single-photon detectors (SPDs) based on negative-feedback avalanche diodes (NFADs) are the key components for applications requiring asynchronous single-photon detection in the near-infrared region. From the perspective of practical applications, the features of SPDs in terms of high photon detection efficiency (PDE), low noise, large sensitive area, and compactness are highly desired for system integration and performance enhancement. Here, we present the implementation of a compact four-channel multimode fiber coupling free-running InGaAs/InP SPD, with the best overall performance to date. On the one hand, we design and fabricate structure-optimized InGaAs/InP NFAD devices with 25 $\mu$m diameter active area and integrated thin film resistors to enhance the maximum achievable PDE. On the other hand, we apply a compact thermoacoustic cryocooler to regulate the operating temperature of NFADs within a large range, and design a dedicated readout circuit with minimized parasitic parameters and tunable settings of hold-off time to suppress the afterpulsing effect. The SPD is then characterized to achieve remarkable overall performance simultaneously at 1550 nm, i.e., 40% PDE, 2.3 kcps dark count rate, 8% afterpulse probability and 49 ps timing jitter (full width at half maximum) under the conditions of 5.9 V excess bias voltage, 10 $\mu$s hold-off time and 213 K operation temperature. Such performance and the results of the long-term stability tests indicate that the SPD could be a favorable solution for practical applications., Comment: 7 pages, 7 figures. Accepted for publication in the IEEE Journal of Selected Topics in Quantum Electronics

The nature of pseudogap lies at the heart of strongly-interacting superconductivity and superfluidity. With known pairing interactions, unitary Fermi gases provide an ideal testbed to verify whether a pseudogap can arise from many-body pairing. Here we report the observation of the long-sought pair-fluctuation-driven pseudogap in homogeneous unitary Fermi gases of lithium-6 atoms, by precisely measuring the spectral function through momentum-resolved microwave spectroscopy without the serious effects of final-state effect. We find a large pseudogap above the superfluid transition. The inverse pair lifetime exhibits a thermally-activated exponential behavior, uncovering the microscopic virtual pair breaking and recombination mechanism. The obtained large, T-independent single-particle scattering rate is comparable with that set by the Planckian limit. Our findings quantitatively characterize the pseudogap in strongly-interacting Fermi gases, highlighting the role of preformed pairing as a precursor to superfluidity.

Berry curvature is a fundamental element to characterize topological quantum physics, while a full measurement of Berry curvature in momentum space was not reported for topological states. Here we achieve two-dimensional Berry curvature reconstruction in a photonic quantum anomalous Hall system via Hall transport measurement of a momentum-resolved wave packet. Integrating measured Berry curvature over the two-dimensional Brillouin zone, we obtain Chern numbers corresponding to -1 and 0. Further, we identify bulk-boundary correspondence by measuring topology-linked chiral edge states at the boundary. The full topological characterization of photonic Chern bands from Berry curvature, Chern number, and edge transport measurements enables our photonic system to serve as a versatile platform for further in-depth study of novel topological physics.

Towards realizing the future quantum internet, a pivotal milestone entails the transition from two-node proof-of-principle experiments conducted in laboratories to comprehensive, multi-node setups on large scales. Here, we report on the debut implementation of a multi-node entanglement-based quantum network over a metropolitan area. We equipped three quantum nodes with atomic quantum memories and their telecom interfaces, and combined them into a scalable phase-stabilized architecture through a server node. We demonstrated heralded entanglement generation between two quantum nodes situated 12.5 km apart, and the storage of entanglement exceeding the round-trip communication time. We also showed the concurrent entanglement generation on three links. Our work provides a metropolitan-scale testbed for the evaluation and exploration of multi-node quantum network protocols and starts a new stage of quantum internet research., Comment: 21 pages in total, 4 figures and 1 table in the main text, 5 figures and 8 tables in the supplementary material

Photoassociation of ultracold atoms is a resonant light-assisted collision process, in which two colliding atoms absorb a photon and form an excited molecule. Since the first observation about three decades ago, the photoassociation of ultracold atoms has made a significant impact on the study of ultracold atoms and molecules. Extending the photoassociation of atoms to the photoassociation of atom-molecule pairs or molecule-molecule pairs will offer many new opportunities in the study of precision polyatomic molecular spectroscopy, formation of ultracold polyatomic molecules, and quantum control of molecular collisions and reactions. However, the high density of states and the photoexcitation of the collision complex by the trapping laser make photoassociation into well-defined quantum states of polyatomic molecules extremely difficult. Here we report on the observation of photoassociation resonances in ultracold collisions between $^{23}$Na$^{40}$K molecules and $^{40}$K atoms. We perform photoassociation in a long-wavelength optical dipole trap to form deeply bound triatomic molecules in the electronically excited states. The atom-molecule Feshbach resonance is used to enhance the free-bound Franck-Condon overlap. The photoassociation into well-defined quantum states of excited triatomic molecules is identified by observing resonantly enhanced loss features. These loss features depend on the polarization of the photoassociation lasers, allowing us to assign the rotational quantum numbers. The observation of ultracold atom-molecule photoassociation resonances paves the way toward preparing ground-state triatomic molecules, provides a new high-resolution spectroscopy technique for polyatomic molecules, and is also important to atom-molecule Feshbach resonances., Comment: 8 pages, 4 figures