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Benefiting from improved stability due to stronger interlayer van der Waals interactions, few-layer fullerene networks are experimentally more accessible compared to monolayer polymeric C$_{60}$. However, there is a lack of systematic theoretical studies on the material properties of few-layer C$_{60}$ networks. Here, we compare the structural, electronic and optical properties of bilayer and monolayer fullerene networks. The band gap and band-edge positions remain mostly unchanged after stacking two layers into a bilayer, enabling the bilayer to be almost as efficient a photocatalyst as the monolayer. The effective mass ratio along different directions is varied for conduction band states due to interlayer interactions,leading to enhanced anisotropy in carrier transport. Additionally, stronger exciton absorption is found in the bilayer than that in the monolayer over the entire visible light range, rendering the bilayer a more promising candidate for photovoltaics. Moreoever, the polarisation dependence of optical absorption in the bilayer is increased in the red-yellow light range, offering unique opportunities in photonics and display technologies with tailored optical properties over specific directions. Our study provides strategies to tune electronic and optical properties of 2D polymeric C$_{60}$ via the introduction of stacking degrees of freedom., Comment: 7 pages, 4 figures

Leveraging multimodal data to drive breakthroughs in e-commerce applications through Multimodal Foundation Models (MFMs) is gaining increasing attention from the research community. However, there are significant challenges that hinder the optimal use of multimodal e-commerce data by foundation models: (1) the scarcity of large-scale, high-quality multimodal benchmark datasets; and (2) the lack of effective multimodal information integration methods. To address these challenges, in this paper, we introduce MMECInstruct, the first-ever, large-scale, and high-quality multimodal instruction dataset for e-commerce. We also develop CASLIE, a simple, lightweight, yet effective framework for integrating multimodal information for e-commerce. Leveraging MMECInstruct, we fine-tune a series of e-commerce MFMs within CASLIE, denoted as CASLIE models. Our comprehensive evaluation demonstrates that CASLIE models substantially outperform 5 categories of advanced baseline models in the in-domain evaluation. Moreover, CASLIE models show strong generalizability to out-of-domain settings. MMECInstruct and CASLIE models are publicly accessible through https://ninglab.github.io/CASLIE/., Comment: Xinyi Ling and Bo Peng contributed equally to this paper

Although the circumgalactic medium (CGM) plays a vital role in galaxy evolution, studying the emission from CGM is challenging due to its low surface brightness and the complexities involved in interpreting resonant lines like Ly$\alpha$. The near-infrared coverage, unprecedented sensitivity, and high spatial resolution of the JWST enable us to study the optical strong lines associated with the extended Ly$\alpha$ "nebulae" at redshift 2-3. These lines serve as diagnostic tools to infer the physical conditions in the massive CGM gas reservoir of these systems. In deep medium-band images taken by the JWST, we serendipitously discover the [O III] emission from the CGM surrounding a massive interacting galaxy system at redshift z ~ 2.8, known to be embedded in a bright extended (100 kpc) Ly$\alpha$ "nebula". This is the first time that the [O III] lines are detected from a Ly$\alpha$ "nebula", and the JWST images reveal that the CGM gas actually resides in narrow (~ 2.5 kpc) filamentary structures with strong [O III] emission, tracing the same extent as the Ly$\alpha$ emission. Analysis of the [O III] suggests that the emitting CGM is fully ionized and is energetically dominated by mechanical heating. We also find that the inferred density and pressure are higher than those commonly predicted by simulations of the CGM. We conclude that the observed CGM emission originates from the gas expelled by the episodic feedback processes, cooling down and enriching the CGM, while travelling to a distance of at least 60 kpc. These observations demonstrate how fierce feedback processes shape gas distribution and properties in the CGM around massive halos. While the deep high-resolution imaging opens up a new discovery space for investigating the CGM, it also challenges numerical simulations to explain and reproduce the exquisitely complex structures revealed by the observations., Comment: 13 pages, 6 figures, 1 table, submitted to A&A Letter

Conversational Recommender Systems (CRS) proactively engage users in interactive dialogues to elicit user preferences and provide personalized recommendations. Existing methods train Reinforcement Learning (RL)-based agent with greedy action selection or sampling strategy, and may suffer from suboptimal conversational planning. To address this, we present a novel Monte Carlo Tree Search (MCTS)-based CRS framework SAPIENT. SAPIENT consists of a conversational agent (S-agent) and a conversational planner (S-planner). S-planner builds a conversational search tree with MCTS based on the initial actions proposed by S-agent to find conversation plans. The best conversation plans from S-planner are used to guide the training of S-agent, creating a self-training loop where S-agent can iteratively improve its capability for conversational planning. Furthermore, we propose an efficient variant SAPIENT-e for trade-off between training efficiency and performance. Extensive experiments on four benchmark datasets validate the effectiveness of our approach, showing that SAPIENT outperforms the state-of-the-art baselines.

Dissipation is usually considered a negative factor for observing quantum effects and for harnessing them for quantum technologies. Here we propose a scheme for speeding up the generation of quantum entanglement between two coupled qubits by introducing a strong dissipation channel to one of these qubits. The maximal entanglement is conditionally established by evenly distributing a single excitation between these two qubits. When the excitation is initially held by the dissipative qubit, the dissipation accelerates the excitation re-distribution process for the quantum state trajectory without quantum jumps. Our results show that the time needed to conditionally attain the maximal entanglement is monotonously decreased as the dissipative rate is increased. We further show that this scheme can be generalized to accelerate the production of the W state for the three-qubit system, where one NH qubit is symmetrically coupled to two Hermitian qubits., Comment: 2 figures

Text-to-image diffusion models have been demonstrated with unsafe generation due to unfiltered large-scale training data, such as violent, sexual, and shocking images, necessitating the erasure of unsafe concepts. Most existing methods focus on modifying the generation probabilities conditioned on the texts containing unsafe descriptions. However, they fail to guarantee safe generation for unseen texts in the training phase, especially for the prompts from adversarial attacks. In this paper, we re-analyze the erasure task and point out that existing methods cannot guarantee the minimization of the total probabilities of unsafe generation. To tackle this problem, we propose Dark Miner. It entails a recurring three-stage process that comprises mining, verifying, and circumventing. It greedily mines embeddings with maximum generation probabilities of unsafe concepts and reduces unsafe generation more effectively. In the experiments, we evaluate its performance on two inappropriate concepts, two objects, and two styles. Compared with 6 previous state-of-the-art methods, our method achieves better erasure and defense results in most cases, especially under 4 state-of-the-art attacks, while preserving the model's native generation capability. Our code will be available on GitHub.

The assembly of molecules with covalent networks can form varied lattice structures with distinct physical and chemical properties from conventional atomic lattices. Using the smallest stable [5,6]fullerene units as building blocks, various 2D C$_{24}$ networks can be formed with superior stability and strength compared to the recently synthesised monolayer polymeric C$_{60}$. Monolayer C$_{24}$ harnesses the properties of both carbon crystals and fullerene molecules, such as stable chemical bonds, suitable band gaps and large surface area, facilitating photocatalytic water splitting. The electronic band gaps of C$_{24}$ are comparable to TiO$_2$, providing appropriate band edges with sufficient external potential for overall water splitting over the acidic and neutral pH range. Upon photoexcitation, strong solar absorption enabled by strongly bound bright excitons can generate carriers effectively, while the type-II band alignment between C$_{24}$ and other 2D monolayers can separate electrons and holes in individual layers simultaneously. Additionally, the number of surface active sites of C$_{24}$ monolayers are three times more than that of their C$_{60}$ counterparts in a much wider pH range, providing spontaneous reaction pathways for hydrogen evolution reaction. Our work provides insights into materials design using tunable building blocks of fullerene units with tailored functions for energy generation, conversion and storage., Comment: 15 pages, 8 figures, 2 tables

Wheeled-legged robots offer significant mobility and versatility but face substantial challenges when operating on slippery terrains. Traditional model-based controllers for these robots assume no slipping. While reinforcement learning (RL) helps quadruped robots adapt to different surfaces, recovering from slips remains challenging, especially for systems with few contact points. Estimating the ground friction coefficient is another open challenge. In this paper, we propose a novel friction-aware safety locomotion framework that integrates Large Vision Language Models (LVLMs) with a RL policy. Our approach explicitly incorporates the estimated friction coefficient into the RL policy, enabling the robot to adapt its behavior in advance based on the surface type before reaching it. We introduce a Friction-From-Vision (FFV) module, which leverages LVLMs to estimate ground friction coefficients, eliminating the need for large datasets and extensive training. The framework was validated on a customized wheeled inverted pendulum, and experimental results demonstrate that our framework increases the success rate in completing driving tasks by adjusting speed according to terrain type, while achieving better tracking performance compared to baseline methods. Our framework can be simply integrated with any other RL policies., Comment: submitted to icra2025

The prosperity of social media platforms has raised the urgent demand for semantic-rich services, e.g., event and storyline attribution. However, most existing research focuses on clip-level event understanding, primarily through basic captioning tasks, without analyzing the causes of events across an entire movie. This is a significant challenge, as even advanced multimodal large language models (MLLMs) struggle with extensive multimodal information due to limited context length. To address this issue, we propose a Two-Stage Prefix-Enhanced MLLM (TSPE) approach for event attribution, i.e., connecting associated events with their causal semantics, in movie videos. In the local stage, we introduce an interaction-aware prefix that guides the model to focus on the relevant multimodal information within a single clip, briefly summarizing the single event. Correspondingly, in the global stage, we strengthen the connections between associated events using an inferential knowledge graph, and design an event-aware prefix that directs the model to focus on associated events rather than all preceding clips, resulting in accurate event attribution. Comprehensive evaluations of two real-world datasets demonstrate that our framework outperforms state-of-the-art methods.

Recently, methods like Zero-1-2-3 have focused on single-view based 3D reconstruction and have achieved remarkable success. However, their predictions for unseen areas heavily rely on the inductive bias of large-scale pretrained diffusion models. Although subsequent work, such as DreamComposer, attempts to make predictions more controllable by incorporating additional views, the results remain unrealistic due to feature entanglement in the vanilla latent space, including factors such as lighting, material, and structure. To address these issues, we introduce the Visual Isotropy 3D Reconstruction Model (VI3DRM), a diffusion-based sparse views 3D reconstruction model that operates within an ID consistent and perspective-disentangled 3D latent space. By facilitating the disentanglement of semantic information, color, material properties and lighting, VI3DRM is capable of generating highly realistic images that are indistinguishable from real photographs. By leveraging both real and synthesized images, our approach enables the accurate construction of pointmaps, ultimately producing finely textured meshes or point clouds. On the NVS task, tested on the GSO dataset, VI3DRM significantly outperforms state-of-the-art method DreamComposer, achieving a PSNR of 38.61, an SSIM of 0.929, and an LPIPS of 0.027. Code will be made available upon publication.

We have used the Five-hundred-meter Aperture Spherical radio Telescope (FAST) to make a blind ultra-deep survey for neutral hydrogen (HI). We present the complete results from the first of six fields (FUDS0). This observation of 95 hours allowed us to achieve a high sensitivity ($\sim 50~\mu$Jy beam$^{-1}$) and a high frequency resolution (22.9 kHz) over an area of 0.72 deg$^2$. We detected 128 galaxies in HI distributed over the redshift range of $0 0.38$, where no unlensed HI emission has previously been directly detected. Estimates of completeness and reliability are presented for the catalog. Consistency of continuum and HI flux estimates with NVSS and AUDS, respectively, confirms the accuracy of calibration method and data reduction pipeline developed for the full FUDS survey., Comment: 14 pages, 14 figures

Observable estimation is a core primitive in NISQ-era algorithms targeting quantum chemistry applications. To reduce the state preparation overhead required for accurate estimation, recent works have proposed various simultaneous measurement schemes to lower estimator variance. Two primary grouping schemes have been proposed: fully commutativity (FC) and qubit-wise commutativity (QWC), with no compelling means of interpolation. In this work we propose a generalized framework for designing and analyzing context-aware hybrid FC/QWC commutativity relations. We use our framework to propose a noise-and-connectivity aware grouping strategy: Generalized backend-Aware pauLI Commutation (GALIC). We demonstrate how GALIC interpolates between FC and QWC, maintaining estimator accuracy in Hamiltonian estimation while lowering variance by an average of 20% compared to QWC. We also explore the design space of near-term quantum devices using the GALIC framework, specifically comparing device noise levels and connectivity. We find that error suppression has a more than $13\times$ larger impact on device-aware estimator variance than qubit connectivity with even larger correlation differences in estimator biases., Comment: 33 pages, 4 figures

With the rapid development of generative technologies, AI-Generated Images (AIGIs) have been widely applied in various aspects of daily life. However, due to the immaturity of the technology, the quality of the generated images varies, so it is important to develop quality assessment techniques for the generated images. Although some models have been proposed to assess the quality of generated images, they are inadequate when faced with the ever-increasing and diverse categories of generated images. Consequently, the development of more advanced and effective models for evaluating the quality of generated images is urgently needed. Recent research has explored the significant potential of the visual language model CLIP in image quality assessment, finding that it performs well in evaluating the quality of natural images. However, its application to generated images has not been thoroughly investigated. In this paper, we build on this idea and further explore the potential of CLIP in evaluating the quality of generated images. We design CLIP-AGIQA, a CLIP-based regression model for quality assessment of generated images, leveraging rich visual and textual knowledge encapsulated in CLIP. Particularly, we implement multi-category learnable prompts to fully utilize the textual knowledge in CLIP for quality assessment. Extensive experiments on several generated image quality assessment benchmarks, including AGIQA-3K and AIGCIQA2023, demonstrate that CLIP-AGIQA outperforms existing IQA models, achieving excellent results in evaluating the quality of generated images., Comment: accepted by ICPR2024

Talking head synthesis is a practical technique with wide applications. Current Neural Radiance Field (NeRF) based approaches have shown their superiority on driving one-shot talking heads with videos or signals regressed from audio. However, most of them failed to take the audio as driven information directly, unable to enjoy the flexibility and availability of speech. Since mapping audio signals to face deformation is non-trivial, we design a Single-Shot Speech-Driven Neural Radiance Field (S^3D-NeRF) method in this paper to tackle the following three difficulties: learning a representative appearance feature for each identity, modeling motion of different face regions with audio, and keeping the temporal consistency of the lip area. To this end, we introduce a Hierarchical Facial Appearance Encoder to learn multi-scale representations for catching the appearance of different speakers, and elaborate a Cross-modal Facial Deformation Field to perform speech animation according to the relationship between the audio signal and different face regions. Moreover, to enhance the temporal consistency of the important lip area, we introduce a lip-sync discriminator to penalize the out-of-sync audio-visual sequences. Extensive experiments have shown that our S^3D-NeRF surpasses previous arts on both video fidelity and audio-lip synchronization., Comment: ECCV 2024

The significance of estimating video watch time has been highlighted by the rising importance of (short) video recommendation, which has become a core product of mainstream social media platforms. Modeling video watch time, however, has been challenged by the complexity of user-video interaction, such as different user behavior modes in watching the recommended videos and varying watching probabilities over the video horizon. Despite the importance and challenges, existing literature on modeling video watch time mostly focuses on relatively black-box mechanical enhancement of the classical regression/classification losses, without factoring in user behavior in a principled manner. In this paper, we for the first time take on a user-centric perspective to model video watch time, from which we propose a white-box statistical framework that directly translates various user behavior assumptions in watching (short) videos into statistical watch time models. These behavior assumptions are portrayed by our domain knowledge on users' behavior modes in video watching. We further employ bucketization to cope with user's non-stationary watching probability over the video horizon, which additionally helps to respect the constraint of video length and facilitate the practical compatibility between the continuous regression event of watch time and other binary classification events. We test our models extensively on two public datasets, a large-scale offline industrial dataset, and an online A/B test on a short video platform with hundreds of millions of daily-active users. On all experiments, our models perform competitively against strong relevant baselines, demonstrating the efficacy of our user-centric perspective and proposed framework.

In this work, we propose TextIM, a novel framework for synthesizing TEXT-driven human Interactive Motions, with a focus on the precise alignment of part-level semantics. Existing methods often overlook the critical roles of interactive body parts and fail to adequately capture and align part-level semantics, resulting in inaccuracies and even erroneous movement outcomes. To address these issues, TextIM utilizes a decoupled conditional diffusion framework to enhance the detailed alignment between interactive movements and corresponding semantic intents from textual descriptions. Our approach leverages large language models, functioning as a human brain, to identify interacting human body parts and to comprehend interaction semantics to generate complicated and subtle interactive motion. Guided by the refined movements of the interacting parts, TextIM further extends these movements into a coherent whole-body motion. We design a spatial coherence module to complement the entire body movements while maintaining consistency and harmony across body parts using a part graph convolutional network. For training and evaluation, we carefully selected and re-labeled interactive motions from HUMANML3D to develop a specialized dataset. Experimental results demonstrate that TextIM produces semantically accurate human interactive motions, significantly enhancing the realism and applicability of synthesized interactive motions in diverse scenarios, even including interactions with deformable and dynamically changing objects.

Neutral hydrogen (HI) is the primary component of the cool interstellar medium (ISM) and is the reservoir of fuel for star formation. Owing to the sensitivity of existing radio telescopes, our understanding of the evolution of the ISM in galaxies remains limited, as it is based on only a few hundred galaxies detected in HI beyond the local Universe. With the high sensitivity of the Five-hundred-meter Aperture Spherical radio Telescope (FAST), we carried out a blind HI search, the FAST Ultra-Deep Survey (FUDS), which extends to redshifts up to 0.42 and a sensitivity of 50 $\rm \mu Jy \cdot beam^{-1}$. Here, we report the first discovery of six galaxies in HI at $z>0.38$. For these galaxies, the FAST angular resolution of $\sim\,4'$ corresponds to a mean linear size of $\sim1.3\,h_{70}^{-1}\,$Mpc. These galaxies are among the most distant HI emission detections known, with one having the most massive HI content ($10^{10.93 \pm 0.04}~h_{70}^{-2}\, \rm M_\odot$). Using recent data from the DESI survey, and new observations with the Hale, BTA, and Keck telescopes, optical counterparts are detected for all galaxies within the 3-$\sigma$ positional uncertainty ($0.5\,h_{70}^{-1}\,$Mpc) and $\rm 200\,km \cdot s^{-1}$ in recession velocity. Assuming that the dominant source of HI is the identified optical counterpart, we find an evidence of evolution in the HI content of galaxies over the last 4.2 Gyr. Our new high-redshift HI galaxy sample provides the opportunity to better investigate the evolution of cool gas in galaxies. A larger sample size in the future will allow us to refine our knowledge of the formation and evolution of galaxies., Comment: 14 pages, 6 figures, 3 tables

Multiple object tracking (MOT) from unmanned aerial vehicle (UAV) platforms requires efficient motion modeling. This is because UAV-MOT faces both local object motion and global camera motion. Motion blur also increases the difficulty of detecting large moving objects. Previous UAV motion modeling approaches either focus only on local motion or ignore motion blurring effects, thus limiting their tracking performance and speed. To address these issues, we propose the Motion Mamba Module, which explores both local and global motion features through cross-correlation and bi-directional Mamba Modules for better motion modeling. To address the detection difficulties caused by motion blur, we also design motion margin loss to effectively improve the detection accuracy of motion blurred objects. Based on the Motion Mamba module and motion margin loss, our proposed MM-Tracker surpasses the state-of-the-art in two widely open-source UAV-MOT datasets. Code will be available., Comment: arXiv admin note: text overlap with arXiv:2308.07207

We introduce PICA, a novel representation for high-fidelity animatable clothed human avatars with physics-accurate dynamics, even for loose clothing. Previous neural rendering-based representations of animatable clothed humans typically employ a single model to represent both the clothing and the underlying body. While efficient, these approaches often fail to accurately represent complex garment dynamics, leading to incorrect deformations and noticeable rendering artifacts, especially for sliding or loose garments. Furthermore, previous works represent garment dynamics as pose-dependent deformations and facilitate novel pose animations in a data-driven manner. This often results in outcomes that do not faithfully represent the mechanics of motion and are prone to generating artifacts in out-of-distribution poses. To address these issues, we adopt two individual 3D Gaussian Splatting (3DGS) models with different deformation characteristics, modeling the human body and clothing separately. This distinction allows for better handling of their respective motion characteristics. With this representation, we integrate a graph neural network (GNN)-based clothed body physics simulation module to ensure an accurate representation of clothing dynamics. Our method, through its carefully designed features, achieves high-fidelity rendering of clothed human bodies in complex and novel driving poses, significantly outperforming previous methods under the same settings., Comment: Project page: https://ustc3dv.github.io/PICA/

Causal reasoning is fundamental to human intelligence and crucial for effective decision-making in real-world environments. Despite recent advancements in large vision-language models (LVLMs), their ability to comprehend causality remains unclear. Previous work typically focuses on commonsense causality between events and/or actions, which is insufficient for applications like embodied agents and lacks the explicitly defined causal graphs required for formal causal reasoning. To overcome these limitations, we introduce a fine-grained and unified definition of causality involving interactions between humans and/or objects. Building on the definition, we construct a novel dataset, CELLO, consisting of 14,094 causal questions across all four levels of causality: discovery, association, intervention, and counterfactual. This dataset surpasses traditional commonsense causality by including explicit causal graphs that detail the interactions between humans and objects. Extensive experiments on CELLO reveal that current LVLMs still struggle with causal reasoning tasks, but they can benefit significantly from our proposed CELLO-CoT, a causally inspired chain-of-thought prompting strategy. Both quantitative and qualitative analyses from this study provide valuable insights for future research. Our project page is at https://github.com/OpenCausaLab/CELLO.

Current medical image classification efforts mainly aim for higher average performance, often neglecting the balance between different classes. This can lead to significant differences in recognition accuracy between classes and obvious recognition weaknesses. Without the support of massive data, deep learning faces challenges in fine-grained classification of fatty liver. In this paper, we propose an innovative deep learning framework that combines feature decoupling and adaptive adversarial training. Firstly, we employ two iteratively compressed decouplers to supervised decouple common features and specific features related to fatty liver in abdominal ultrasound images. Subsequently, the decoupled features are concatenated with the original image after transforming the color space and are fed into the classifier. During adversarial training, we adaptively adjust the perturbation and balance the adversarial strength by the accuracy of each class. The model will eliminate recognition weaknesses by correctly classifying adversarial samples, thus improving recognition robustness. Finally, the accuracy of our method improved by 4.16%, achieving 82.95%. As demonstrated by extensive experiments, our method is a generalized learning framework that can be directly used to eliminate the recognition weaknesses of any classifier while improving its average performance. Code is available at https://github.com/HP-ML/MICCAI2024., Comment: MICCAI 2024

We consider the robust contract design problem when the principal only has limited information about the actions the agent can take. The principal evaluates a contract according to its worst-case performance caused by the uncertain action space. Carroll (AER 2015) showed that a linear contract is optimal among deterministic contracts. Recently, Kambhampati (JET 2023) showed that the principal's payoff can be strictly increased via randomization over linear contracts. In this paper, we characterize the optimal randomized contract, which remains linear and admits a closed form of its cumulative density function. The advantage of randomized contracts over deterministic contracts can be arbitrarily large even when the principal knows only one non-trivial action of the agent. Furthermore, our result generalizes to the model of contracting with teams, by Dai and Toikka (Econometrica 2022)., Comment: Full version of EC 2024 paper

Energy- and resource-efficient electrocatalytic water splitting is of paramount importance to enable sustainable hydrogen production. The best bulk catalyst for the hydrogen evolution reaction (HER), i.e., platinum, is one of the scarcest elements on Earth. The use of raw material for HER can be dramatically reduced by utilizing nanoclusters. In addition, nanoalloying can further improve the performance of these nanoclusters. In this paper, we present results for HER on nanometer-sized ligand-free AuPt nanoclusters grafted on carbon nanotubes. These results demonstrate excellent monodispersity and a significant reduction of the overpotential for the electrocatalytic HER. We utilize atomistic machine learning techniques to elucidate the atomic-scale origin of the synergistic effect between Pt and Au. We show that the presence of surface Au atoms, known to be poor HER catalysts, in a Pt(core)/AuPt(shell) nanocluster structure, drives an anomalous enhancement of the inherently high catalytic activity of Pt atoms.

6D Object Pose Estimation is a crucial yet challenging task in computer vision, suffering from a significant lack of large-scale datasets. This scarcity impedes comprehensive evaluation of model performance, limiting research advancements. Furthermore, the restricted number of available instances or categories curtails its applications. To address these issues, this paper introduces Omni6DPose, a substantial dataset characterized by its diversity in object categories, large scale, and variety in object materials. Omni6DPose is divided into three main components: ROPE (Real 6D Object Pose Estimation Dataset), which includes 332K images annotated with over 1.5M annotations across 581 instances in 149 categories; SOPE(Simulated 6D Object Pose Estimation Dataset), consisting of 475K images created in a mixed reality setting with depth simulation, annotated with over 5M annotations across 4162 instances in the same 149 categories; and the manually aligned real scanned objects used in both ROPE and SOPE. Omni6DPose is inherently challenging due to the substantial variations and ambiguities. To address this challenge, we introduce GenPose++, an enhanced version of the SOTA category-level pose estimation framework, incorporating two pivotal improvements: Semantic-aware feature extraction and Clustering-based aggregation. Moreover, we provide a comprehensive benchmarking analysis to evaluate the performance of previous methods on this large-scale dataset in the realms of 6D object pose estimation and pose tracking.

The Standard Quadratic optimization Problem (StQP), arguably the simplest among all classes of NP-hard optimization problems, consists of extremizing a quadratic form (the simplest nonlinear polynomial) over the standard simplex (the simplest polytope/compact feasible set). As a problem class, StQPs may be nonconvex with an exponential number of inefficient local solutions. StQPs arise in a multitude of applications, among them mathematical finance, machine learning (clustering), and modeling in biosciences (e.g., selection and ecology). This paper deals with such StQPs under an additional sparsity or cardinality constraint, which, even for convex objectives, renders NP-hard problems. One motivation to study StQPs under such sparsity restrictions is the high-dimensional portfolio selection problem with too many assets to handle, in particular, in the presence of transaction costs. Here, relying on modern conic optimization techniques, we present tractable convex relaxations for this relevant but difficult problem. We propose novel equivalent reformulations of these relaxations with significant dimensional reduction, which is essential for the tractability of these relaxations when the problem size grows. Moreover, we propose an instance generation procedure which systematically avoids too easy instances. Our extensive computational results illustrate the high quality of the relaxation bounds in a significant number of instances. Furthermore, in contrast with exact mixed-integer quadratic programming models, the solution time of the relaxations is very robust to the choices of the problem parameters. In particular, the reduced formulations achieve significant improvements in terms of the solution time over their counterparts., Comment: Technical Report, School of Mathematics, The University of Edinburgh, Edinburgh, EH9 3FD, Scotland, United Kingdom

In this paper, we analyze the properties of the recently proposed real-time equation-of-motion coupled-cluster (RT-EOM-CC) cumulant Green's function approach [J. Chem. Phys. 2020, 152, 174113]. We specifically focus on identifying the limitations of the original time-dependent coupled cluster (TDCC) ansatz and propose an enhanced double TDCC ansatz ensuring the exactness in the expansion limit. Additionally, we introduce a practical cluster-analysis-based approach for characterizing the peaks in the computed spectral function from the RT-EOM-CC cumulant Green's function approach, which is particularly useful for the assignments of satellite peaks when many-body effects dominate the spectra. Our preliminary numerical tests focus on reproducing, approximating, and characterizing the exact impurity Green's function of the three-site and four-site single impurity Anderson models using the RT-EOM-CC cumulant Green's function approach. The numerical tests allow us to have a direct comparison between the RT-EOM-CC cumulant Green's function approach and other Green's function approaches in the numerical exact limit.

Syngas conversion into higher alcohols represents a promising avenue for transforming coal or biomass into liquid fuels. However, the commercialization of this process has been hindered by the high cost, low activity, and inadequate C$_{2+}$OH selectivity of catalysts. Herein, we have developed Cu/Co carbon wood catalysts, offering a cost-effective and stable alternative with exceptional selectivity for catalytic conversion. The formation of Cu/Co nanoparticles was found, influenced by water-1,2-propylene glycol ratios in the solution, resulting in bidisperse nanoparticles. The catalyst exhibited a remarkable CO conversion rate of 74.8% and a selectivity of 58.7% for C$_{2+}$OH, primarily comprising linear primary alcohols. This catalyst demonstrated enduring stability and selectivity under industrial conditions, maintaining its efficacy for up to 350 h of operation. We also employed density functional theory (DFT) to analyze selectivity, particularly focusing on the binding strength of CO, a crucial precursor for subsequent reactions leading to the formation of CH$_3$OH. DFT identified the pathway of CH$_x$ and CO coupling, ultimately yielding C$_2$H$_5$OH. This computational understanding, coupled with high performance of the Cu/Co-carbon wood catalyst, paves ways for the development of catalytically selective materials tailored for higher alcohols production, thereby ushering in new possibility in this field.

The recent advancements in exoplanet observations enable the potential detection of exo-Venuses, rocky planets with carbon-rich atmospheres. How extended these atmospheres can be, given high carbon abundances, has not been studied. To answer this, we present a model for a theoretical class of exoplanets - puffy Venuses - characterized by thick, carbon-dominated atmospheres in equilibrium with global magma oceans. Our model accounts for carbon and hydrogen partition between the atmosphere and the magma ocean, as well as the C-H-O equilibrium chemistry throughout a semi-grey, radiative-convective atmosphere. We find that radius inflation by puffy Venus atmospheres is significant on small and irradiated planets: carbon content of 1200 ppm (or that of ordinary chondrites) can generate an atmosphere of ~0.16 - 0.3 $R_{\oplus}$ for an Earth-mass planet with equilibrium temperatures of 1500 to 2000 K. We identify TOI-561 b as an especially promising puffy Venus candidate, whose under-density could be attributed to a thick C-rich atmosphere. We also advocate for a puffy Venus interpretation of 55 Cancri e, where recent JWST observation indicates the presence of a CO/CO2 atmosphere. Puffy Venuses may thus constitute a testable alternative interpretation for the interior structure of underdense low-mass exoplanets., Comment: Accepted by ApJ on Aug. 12th, 2024