Search

Dielectric metasurfaces that combine high-index materials with optical nonlinearities are widely recognized for their potential in various quantum and classical nanophotonic applications. However, the fabrication of high-quality metasurfaces poses significant material-dependent challenges, as their designs are often susceptible to disorder, defects, and scattering losses, which are particularly prone to occur at the edges of nanostructured features. Additionally, the choice of the material platforms featuring second-order optical nonlinearities, $\chi^{(2)}$, is limited to broken-inversion symmetry crystals such as GaAs, GaP, LiNbO$_3$, and various bulk van der Waals materials, including GaSe and NbOCl$_2$. Here, we use a combination of top-down lithography and anisotropic wet etching of a specially stacked van der Waals crystal -- 3R-MoS$_2$, which exhibits both a high refractive index and exceptional $\chi^{(2)}$ nonlinearity, to produce metasurfaces consisting of perfect equilateral triangle nanoholes with atomically precise zigzag edges. Due to the geometry of the triangle, the etching process is accompanied by a transition from an in-plane $C_4$ symmetric structure to a broken-in-plane symmetry configuration, thereby allowing for the realization of the quasi-bound-state-in-the-continuum (q-BIC) concept. The resulting ultrathin metasurface ($\sim$ 20-25 nm) demonstrates a remarkable enhancement in second-harmonic generation (SHG) -- over three orders of magnitude at specific wavelengths and linear polarization directions compared to a host flake.

Recent developments in the registration of histology and micro-computed tomography ({\mu}CT) have broadened the perspective of pathological applications such as virtual histology based on {\mu}CT. This topic remains challenging because of the low image quality of soft tissue CT. Additionally, soft tissue samples usually deform during the histology slide preparation, making it difficult to correlate the structures between histology slide and {\mu}CT. In this work, we propose a novel 2D-3D multi-modal deformable image registration method. The method uses a machine learning (ML) based initialization followed by the registration. The registration is finalized by an analytical out-of-plane deformation refinement. The method is evaluated on datasets acquired from tonsil and tumor tissues. {\mu}CTs of both phase-contrast and conventional absorption modalities are investigated. The registration results from the proposed method are compared with those from intensity- and keypoint-based methods. The comparison is conducted using both visual and fiducial-based evaluations. The proposed method demonstrates superior performance compared to the other two methods., Comment: 12 pages, 4 figures

Nanomechanical resonators with high quality factors ($Q_m$) enable mechanics-based quantum technologies, in particular quantum sensing and quantum transduction. High-$Q_m$ nanomechanical resonators in the kHz to MHz frequency range can be realized in tensile-strained thin films that allow the use of dissipation dilution techniques to drastically increase $Q_m$. In our work, we study the material properties of tensile-strained piezoelectric films made from aluminium nitride (AlN). We characterize crystalline AlN films with a thickness ranging from 45nm to 295nm, which are directly grown on Si(111) by metal-organic vapour-phase epitaxy. We report on the crystal quality and surface roughness, the piezoelectric response, and the residual and released stress of the AlN thin films. Importantly, we determine the intrinsic quality factor of the films at room temperature in high vacuum. We fabricate and characterize AlN nanomechanical resonators that exploit dissipation dilution to enhance the intrinsic quality factor by utilizing the tensile strain in the film. We find that AlN nanomechanical resonators below 200nm thickness exhibit the highest $Q_m\cdot f_m$-product, on the order of $10^{12}$Hz. We discuss possible strategies to optimize the material growth that should lead to devices that reach even higher $Q_m\cdot f_m$-products. This will pave the way for future advancements of optoelectromechanical quantum devices made from tensile-strained piezoelectric AlN., Comment: 14 pages, 12 figures

Superconducting flip-chip interconnects are crucial for the three-dimensional integration of superconducting circuits in sensing and quantum technology applications. We demonstrate a simplified approach for a superconducting flip chip using commercially available indium microspheres and an in-house-built transfer stage for bonding two chips patterned with superconducting thin films. We use a gold-passivated niobium or niobium nitride layer as an under-bump metallization (UBM) layer between an aluminum-based superconducting layer and the indium interconnect. At millikelvin temperatures, our flip-chip assembly can transport a supercurrent with tens of milliamperes, limited by the smallest geometric feature size and critical current density of the UBM layer. We also show that the indium interconnect itself can carry a supercurrent exceeding 1\,A. Our flip-chip assembly does not require patterning and electroplating of indium, nor does it need a flip-chip bonder. Thus, the presented flip-chip devices can be utilized in applications that require few superconducting interconnects carrying large currents at millikelvin temperatures., Comment: 11 pages, 8 figures incl supplemental material

Recent advancements in propagation-based phase-contrast imaging, such as hierarchical imaging, have enabled the visualization of internal structures in large biological specimens and material samples. However, wavefront marker-based techniques, which provide quantitative electron density information, face challenges when imaging larger objects due to stringent beam stability requirements and potential structural changes in objects during longer measurements. Extending the fields-of-view of these methods is crucial for obtaining comparable quantitative results across beamlines and adapting to the smaller beam profiles of fourth-generation synchrotron sources. We introduce a novel technique combining an adapted eigenflat optimization with deformable image registration to address the challenges and enable quantitative high-resolution scans of centimeter-sized objects with micrometre resolution. We demonstrate the potential of the method by obtaining an electron density map of a rat brain sample 15 mm in diameter using speckle-based imaging, despite the limited horizontal field-of-view of 6 mm of the beamline (PETRA III, P05, operated by Hereon at DESY). This showcases the ability of the technique to significantly widen the range of application of wavefront marker-based techniques in both biological and materials science research., Comment: *The authors contributed equally to this work

Canard cascading (CC) is observed in dynamical networks with global adaptive coupling. It is a fast-slow phenomenon characterized by a recurrent sequence of fast transitions between distinct and slowly evolving quasi-stationary states. In this letter, we uncover the dynamical mechanisms behind CC, using an illustrative example of globally and adaptively coupled semiconductor lasers, where CC represents sequential switching on and off the lasers. Firstly, we show that CC is a robust and truly adaptive network effect that is scalable with network size and does not occur without adaptation. Secondly, we uncover multiple saddle slow manifolds (unstable quasi-stationary states) linked by heteroclinic orbits (fast transitions) in the phase space of the system. This allows us to identify CC with a novel heteroclinic canard orbit that organises different unstable quasi-stationary states into an intricate fast-slow limit cycle. Although individual quasi-stationary states are unstable (saddles), the CC cycle as a whole is attractive and robust to parameter changes.

Ground-state cooling of mechanical resonators is a prerequisite for the observation of various quantum effects in optomechanical systems and thus has always been a crucial task in quantum optomechanics. In this paper, we study how to realize ground-state cooling of the mechanical mode in a Fano-mirror optomechanical setup, which allows for enhanced effective optomechanical interaction but typically works in the (deeply) unresolved-sideband regime. We reveal that for such a two-sided cavity geometry with very different decay rates at the two cavity mirrors, it is possible to cool the mechanical mode down to its ground state within a broad range of parameters by using an appropriate single-sided coherent feedback. This is possible even if the total optical loss is more than seven orders of magnitude larger than the mechanical frequency and the feedback efficiency is relatively low. Importantly, we show that a more standard double-sided feedback scheme is not appropriate to cooperate with a Fano-mirror system., Comment: 17 pages, 13 figures. Comments are welcome!

We theoretically investigate the properties of magnetically-levitated superconducting rotors confined in anti-Helmholtz traps, for application in magnetomechanical experiments. We study both the translational modes and a librational mode. The librational mode gives an additional degree of freedom that levitated spheres do not have access to. We compare rotors of different shapes: ellipsoids, cylinders and cuboids. We find that the stable orientations of the rotors depend on the rotors' aspect ratios., Comment: 17 pages, 6 figures

High-\Qm{} mechanical resonators are crucial for applications where low noise and long coherence time are required, as mirror suspensions, quantum cavity optomechanical devices, or nanomechanical sensors. Tensile strain in the material enables the use of dissipation dilution and strain engineering techniques, which increase the mechanical quality factor. These techniques have been employed for high-\Qm{} mechanical resonators made from amorphous materials and, recently, from crystalline materials such as InGaP, SiC, and Si. A strained crystalline film exhibiting substantial piezoelectricity expands the capability of high-\Qm{} nanomechanical resonators to directly utilize electronic degrees of freedom. In this work we realize nanomechanical resonators with \Qm{} up to $2.9\times 10^{7}$ made from tensile-strained \SI{290}{\nano\meter}-thick AlN, which is an epitaxially-grown crystalline material offering strong piezoelectricity. We demonstrate nanomechanical resonators that exploit dissipation dilution and strain engineering to reach a \Qf-product approaching $10^{13}$\,\SI{}{\hertz} at room temperature. We realize a novel resonator geometry, triangline, whose shape follows the Al-N bonds and offers a central pad that we pattern with a photonic crystal. This allows us to reach an optical reflectivity above 80\% for efficient coupling to out-of-plane light. The presented results pave the way for quantum optoelectromechanical devices at room temperature based on tensile-strained AlN.

An optomechanical microcavity can considerably enhance the interaction between light and mechanical motion by confining light to a sub-wavelength volume. However, this comes at the cost of an increased optical loss rate. Therefore, microcavity-based optomechanical systems are placed in the unresolved-sideband regime, preventing sideband-based ground-state cooling. A pathway to reduce optical loss in such systems is to engineer the cavity mirrors, i.e., the optical modes that interact with the mechanical resonator. In our work, we analyze such an optomechanical system, whereby one of the mirrors is strongly frequency-dependent, i.e., a suspended Fano mirror. This optomechanical system consists of two optical modes that couple to the motion of the suspended Fano mirror. We formulate a quantum-coupled-mode description that includes both the standard dispersive optomechanical coupling as well as dissipative coupling. We solve the Langevin equations of the system dynamics in the linear regime showing that ground-state cooling from room temperature can be achieved even if the cavity is per se not in the resolved-sideband regime, but achieves effective sideband resolution through strong optical mode coupling. Importantly, we find that the cavity output spectrum needs to be properly analyzed with respect to the effective laser detuning to infer the phonon occupation of the mechanical resonator. Our work also predicts how to reach the regime of nonlinear quantum optomechanics in a Fano-based microcavity by engineering the properties of the Fano mirror., Comment: 20 pages, 13 figures. Minor revision: clarify some assumptions, check energy equipartition (new fig. 13). Code to plot the article's figures available at https://gitlab.com/juliette.monsel/fano-mirror-cavity-optomechanics

To optimize materials' stability, automated high-throughput workflows are of increasing interest. However, many of those workflows use processes not suitable for large-area depositions which limits the transferability of results. While combinatorial approaches based on vapour-based depositions are inherently scalable, their potential for controlled stability assessments has yet to be exploited. Based on MAPbI3 thin-films as a prototypical system, we demonstrate a combinatorial inert-gas workflow to study materials degradation based on intrinsic factors only, closely resembling conditions in encapsulated de-vices. Through a comprehensive set of automated X-Ray fluorescence (XRF), X-Ray diffraction (XRD) and UV-Vis characterizations, we aim to obtain a holistic understanding of thin-film properties of pristine and aged thin-films. From phase changes derived from XRD characterizations before and after aging, we observe simi-lar aging behaviours for MAPbI3 thin-films with varying PbI2 residuals. Using a custom-designed in-situ UV-Vis aging setup, the combinatorial libraries are exposed to relevant aging conditions, such as heat or light-bias exposure. Simultaneously, UV-Vis photospectroscopy is performed to gain kinetic insights into the aging process which can be linked to intrinsic degradation processes such as autocatalytic decomposition. Despite scattering effects, which complicate the conventional interpretation of in-situ UV-Vis results, we demonstrate how a machine learning model trained on the comprehensive characterization data before and after the aging process can link optical changes to phase changes during aging. Consequently, this approach does not only enable semi-quantitative comparisons of materials' stability but also provides detailed insights into the underlying degradation processes which are otherwise mostly reported for investigations on single samples.

Transition metal dichalcogenide (TMD) heterobilayers provide a versatile platform to explore unique excitonic physics via properties of the constituent TMDs and external stimuli. Interlayer excitons (IXs) can form in TMD heterobilayers as delocalized or localized states. However, the localization of IX in different types of potential traps, the emergence of biexcitons in the high-excitation regime, and the impact of potential traps on biexciton formation have remained elusive. In our work, we observe two types of potential traps in a MoSe$_2$/WSe$_2$ heterobilayer, which result in significantly different emission behavior of IXs at different temperatures. We identify the origin of these traps as localized defect states and the moir{\'e} potential of the TMD heterobilayer. Furthermore, with strong excitation intensity, a superlinear emission behavior indicates the emergence of interlayer biexcitons, whose formation peaks at a specific temperature. Our work elucidates the different excitation and temperature regimes required for the formation of both localized and delocalized IX and biexcitons, and, thus, contributes to a better understanding and application of the rich exciton physics in TMD heterostructures., Comment: 18 pages, 15 figures incl supplemental material

We present a detailed study of mechanically compliant, photonic-crystal-based microcavities featuring a quasi-bound state in the continuum. Such systems have recently been predicted to reduce the optical loss in Fabry-Perot-type optomechanical cavities. However, they require two identical photonic-crystal slabs facing each other, which poses a considerable challenge for experimental implementation. We investigate how such an ideal system can be simplified and still exhibit a quasi-bound state in the continuum. We find that a suspended photonic-crystal slab facing a distributed Bragg reflector realizes an optomechanical system with a quasi-bound state in the continuum. In this system, the radiative cavity loss can be eliminated to the extent that the cavity loss is dominated by dissipative loss originating from material absorption only. These proposed optomechanical cavity designs are predicted to feature optical quality factors in excess of 10^5., Comment: 11 pages, 14 figures

Comparing and evaluating small area estimation (SAE) models for a given application is inherently difficult. Typically, many areas lack enough data to check unit-level modeling assumptions or to assess unit-level predictions empirically; and no ground truth is available for checking area-level estimates. Design-based simulation from artificial populations can help with each of these issues, but only if the artificial populations realistically represent the application at hand and are not built using assumptions that inherently favor one SAE model over another. In this paper, we borrow ideas from random hot deck, approximate Bayesian bootstrap (ABB), and k Nearest Neighbor (kNN) imputation methods to propose a kNN-based approximation to ABB (KBAABB), for generating an artificial population when rich unit-level auxiliary data is available. We introduce diagnostic checks on the process of building the artificial population, and we demonstrate how to use such an artificial population for design-based simulation studies to compare and evaluate SAE models, using real data from the Forest Inventory and Analysis (FIA) program of the US Forest Service.