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The interaction of relativistically intense lasers with opaque targets represents a highly non-linear, multi-dimensional parameter space. This limits the utility of sequential 1D scanning of experimental parameters for the optimisation of secondary radiation, although to-date this has been the accepted methodology due to low data acquisition rates. High repetition-rate (HRR) lasers augmented by machine learning present a valuable opportunity for efficient source optimisation. Here, an automated, HRR-compatible system produced high fidelity parameter scans, revealing the influence of laser intensity on target pre-heating and proton generation. A closed-loop Bayesian optimisation of maximum proton energy, through control of the laser wavefront and target position, produced proton beams with equivalent maximum energy to manually-optimized laser pulses but using only 60% of the laser energy. This demonstration of automated optimisation of laser-driven proton beams is a crucial step towards deeper physical insight and the construction of future radiation sources., Comment: 11 pages

We report on experimental investigations of proton acceleration from solid foils irradiated with PW-class laser-pulses, where highest proton cut-off energies were achieved for temporal pulse parameters that varied significantly from those of an ideally Fourier transform limited (FTL) pulse. Controlled spectral phase modulation of the driver laser by means of an acousto-optic programmable dispersive filter enabled us to manipulate the temporal shape of the last picoseconds around the main pulse and to study the effect on proton acceleration from thin foil targets. The results show that applying positive third order dispersion values to short pulses is favourable for proton acceleration and can lead to maximum energies of 70 MeV in target normal direction at 18 J laser energy for thin plastic foils, significantly enhancing the maximum energy compared to ideally compressed FTL pulses. The paper further proves the robustness and applicability of this enhancement effect for the use of different target materials and thicknesses as well as laser energy and temporal intensity contrast settings. We demonstrate that application relevant proton beam quality was reliably achieved over many months of operation with appropriate control of spectral phase and temporal contrast conditions using a state-of-the-art high-repetition rate PW laser system.

We report on reproducible shock acceleration from irradiation of a $\lambda = 10$ $\mu$m CO$_2$ laser on optically shaped H$_2$ and He gas targets. A low energy laser prepulse ($I\lesssim10^{14}\, {\rm Wcm^{-2}}$) was used to drive a blast wave inside the gas target, creating a steepened, variable density gradient. This was followed, after 25 ns, by a high intensity laser pulse ($I>10^{16}\, {\rm Wcm^{-2}}$) that produces an electrostatic collisionless shock. Upstream ions were accelerated for a narrow range of prepulse energies ($> 110$ mJ & $< 220$mJ). For long density gradients ($\gtrsim 40 \mu$m), broadband beams of He$^+$ and H$^+$ were routinely produced, whilst for shorter gradients ($\lesssim 20 \mu$m), quasimonoenergetic acceleration of proton was observed. These measurements indicate that the properties of the accelerating shock and the resultant ion energy distribution, in particular the production of narrow energy spread beams, is highly dependent on the plasma density profile. These findings are corroborated by 2D PIC simulations.

Spectrally-peaked proton beams ($E_{p}\approx 8$ MeV, $\Delta E\approx 4$ MeV) have been observed from the interaction of an intense laser ($> 10^{19 }$ Wcm$^{-2}$) with ultrathin CH foils, as measured by spectrally-resolved full beam profiles. These beams are reproducibly generated for foil thicknesses (5-100 nm), and exhibit narrowing divergence with decreasing target thickness down to $\approx 8^\circ$ for 5 nm. Simulations demonstrate that the narrow energy spread feature is a result of buffered acceleration of protons. Due to their higher charge-to-mass ratio, the protons outrun a carbon plasma driven in the relativistic transparency regime.

Observations of the interaction of an intense {\lambda}0 \approx 10 {\mu}m laser pulse with near-critical overdense plasmas (ne = 1.8 - 3 nc) are presented. For the first time, transverse optical probing is used to show a recession of the front surface caused by radiation pressure driven hole-boring by the laser pulse with an initial velocity > 10^6 ms-1, and the resulting collisionless shocks. The collisionless shock propagates through the plasma, dissipates into an ion-acoustic solitary wave, and eventually becomes collisional as it slows further. These conclusions are supported by PIC simulations which show that the initial evolution is dominated by collisionless mechanisms.

High energy ion beams (> MeV) generated by intense laser pulses promise to be viable alternatives to conventional ion beam sources due to their unique properties such as high charge, low emittance, compactness and ease of beam delivery. Typically the acceleration is due to the rapid expansion of a laser heated solid foil, but this usually leads to ion beams with large energy spread. Until now, control of the energy spread has only been achieved at the expense of reduced charge and increased complexity. Radiation pressure acceleration (RPA) provides an alternative route to producing laser-driven monoenergetic ion beams. In this paper, we show the interaction of an intense infrared laser with a gaseous hydrogen target can produce proton spectra of small energy spread (~ 4%), and low background. The scaling of proton energy with the ratio of intensity over density (I/n) indicates that the acceleration is due to the shock generated by radiation-pressure driven hole-boring of the critical surface. These are the first high contrast mononenergetic beams that have been theorised from RPA, and makes them highly desirable for numerous ion beam applications.

By tailoring the wavefront of the laser pulse used in a laser-wakefield accelerator, we show that the properties of the x-rays produced due to the electron beam's betatron oscillations in the plasma can be controlled. By creating a wavefront with coma, we find that the critical energy of the synchrotron-like x-ray spectrum can be significantly increased. The coma does not substantially change the energy of the electron beam, but does increase its divergence and produces an energy-dependent exit angle, indicating that changes in the x-ray spectrum are due to an increase in the electron beam's oscillation amplitude within the wakefield., Comment: 7 pages, 2 figures, submitted to Appl. Phys. Lett