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Combining a precise sputter etching method with subsequent AlO$_x$ growth within an atomic layer deposition chamber enables fabrication of atomically flat lateral patterns of SiO$_2$ and AlO$_x$. The transfer of MoSe$_2$ monolayers onto these dielectrically modulated substrates results in formation of lateral heterojunctions, with the flat substrate topography leading to minimal strain across the junction. Kelvin probe force microscopy (KPFM) measurements show significant variations in the contact potential difference (CPD) across the interface, with AlO$_x$ regions inducing a 230~mV increase in CPD. Spatially resolved photoluminescence spectroscopy reveals shifts in spectral weight of neutral and charged exciton species across the different dielectric regions. On the AlO$_x$ side, the Fermi energy moves closer to the conduction band, leading to a higher trion-to-exciton ratio, indicating a bandgap shift consistent with CPD changes. In addition, transient reflection spectroscopy highlights the influence of the dielectric environment on carrier dynamics, with the SiO$_2$ side exhibiting rapid carrier decay typical of neutral exciton recombination. In contrast, the AlO$_x$ side shows slower, mixed decay behavior consistent with conversion of trions back into excitons. These results demonstrate how dielectric substrate engineering can tune the electronic and optical characteristics of proximal two-dimensional materials, allowing scalable fabrication of advanced junctions for novel (opto)electronics applications., Comment: 24 pages, 5 figures. SI: 2 pages, 3 figures. We welcome your feedback!

Spin-photon interfaces based on group-IV colour centres in diamond offer a promising platform for quantum networks. A key challenge in the field is realizing precise single-defect positioning and activation, which is crucial for scalable device fabrication. Here we address this problem by demonstrating a two-step fabrication method for tin vacancy (SnV-) centres that uses site-controlled ion implantation followed by local femtosecond laser annealing with in-situ spectral monitoring. The ion implantation is performed with sub-50 nm resolution and a dosage that is controlled from hundreds of ions down to single ions per site, limited by Poissonian statistics. Using this approach, we successfully demonstrate site-selective creation and modification of single SnV- centres. The technique opens a window onto materials tuning at the single defect level, and provides new insight into defect structures and dynamics during the annealing process. While demonstrated for SnV- centres, this versatile approach can be readily generalised to other implanted colour centres in diamond and wide-bandgap materials., Comment: 10 pages, 4 figures, methods, and supplementary information

Inspired by the program of discrete holography, we show that Jackiw-Teitelboim (JT) gravity on a hyperbolic tiling of Euclidean AdS$_2$ gives rise to an Ising model on the dual lattice, subject to a topological constraint. The Ising model involves an asymptotic boundary condition with spins pointing opposite to the magnetic field. The topological constraint enforces a single domain wall between the spins of opposite direction, with the topology of a circle. The resolvent of JT gravity is related to the free energy of this Ising model, and the classical limit of JT gravity corresponds to the Ising low-temperature limit. We study this Ising model through a Monte Carlo approach and a mean-field approximation. For finite truncations of the infinite hyperbolic lattice, the map between both theories is only valid in a regime in which the domain wall has a finite size. For the extremal cases of large positive or negative coupling, the domain wall either shrinks to zero or touches the boundary of the lattice. This behavior is confirmed by the mean-field analysis. We expect that our results may be used as a starting point for establishing a holographic matrix model duality for discretized gravity., Comment: 33 pages, 7 figures

An important challenge in machine learning is to predict the initial conditions under which a given neural network will be trainable. We present a method for predicting the trainable regime in parameter space for deep feedforward neural networks, based on reconstructing the input from subsequent activation layers via a cascade of single-layer auxiliary networks. For both the MNIST and CIFAR10 datasets, we show that a single epoch of training of the shallow cascade networks is sufficient to predict the trainability of the deep feedforward network, thereby providing a significant reduction in overall training time. We achieve this by computing the relative entropy between reconstructed images and the original inputs, and show that this probe of information loss is sensitive to the phase behaviour of the network. Moreover, our approach illustrates the network's decision making process by displaying the changes performed on the input data at each layer. Our results provide a concrete link between the flow of information and the trainability of deep neural networks, further explaining the role of criticality in these systems., Comment: 21 pages, 5 figures, 1 table Minor changes to presentation, typos corrected

HYPERTILING is a high-performance Python library for the generation and visualization of regular hyperbolic lattices embedded in the Poincar\'e disk model. Using highly optimized, efficient algorithms, hyperbolic tilings with millions of vertices can be created in a matter of minutes on a single workstation computer. Facilities including computation of adjacent vertices, dynamic lattice manipulation, refinements, as well as powerful plotting and animation capabilities are provided to support advanced uses of hyperbolic graphs. In this manuscript, we present a comprehensive exploration of the package, encompassing its mathematical foundations, usage examples, applications, and a detailed description of its implementation., Comment: 54 pages, 21 figures

PbCuTe$_2$O$_6$ is considered as one of the rare candidate materials for a three-dimensional quantum spin liquid (QSL). This assessment was based on the results of various magnetic experiments, performed mainly on polycrystalline material. More recent measurements on single crystals revealed an even more exotic behavior, yielding ferroelectric order below $T_{\text{FE}}\approx 1\,\text{K}$, accompanied by distinct lattice distortions, and a somewhat modified magnetic response which is still consistent with a QSL. Here we report on low-temperature measurements of various thermodynamic, magnetic and dielectric properties of single crystalline PbCuTe$_2$O$_6$ in magnetic fields $B\leq 14.5\,\text{T}$. The combination of these various probes allows us to construct a detailed $B$-$T$ phase diagram including a ferroelectric phase for $B \leq$ $8\,\text{T}$ and a $B$-induced magnetic phase at $B \geq$ $11\,\text{T}$. These phases are preceded by or coincide with a structural transition from a cubic high-temperature phase into a distorted non-cubic low-temperature state. The phase diagram discloses two quantum critical points (QCPs) in the accessible field range, a ferroelectric QCP at $B_{c1}$ = $7.9\,\text{T}$ and a magnetic QCP at $B_{c2}$ = $11\,\text{T}$. Field-induced lattice distortions, observed in the state at $T>$ $1\,\text{K}$ and which are assigned to the effect of spin-orbit interaction of the Cu$^{2+}$-ions, are considered as the key mechanism by which the magnetic field couples to the dielectric degrees of freedom in this material.

We report the measurement of sub-MeV solar neutrinos through the use of their associated Cherenkov radiation, performed with the Borexino detector at the Laboratori Nazionali del Gran Sasso. The measurement is achieved using a novel technique that correlates individual photon hits of events to the known position of the Sun. In an energy window between 0.54 MeV to 0.74 MeV, selected using the dominant scintillation light, we have measured 10887$^{+2386}_{-2103} (\mathrm{stat.})\pm 947 (\mathrm{syst.})$ ($68\%$ confidence interval) solar neutrinos out of 19904 total events. This corresponds to a $^{7}$Be neutrino interaction rate of 51.6$^{+13.9}_{-12.5}$ counts/(day$\cdot$ 100 ton), which is in agreement with the Standard Solar Model predictions and the previous spectroscopic results of Borexino. The no-neutrino hypothesis can be excluded with $>$5$\sigma$ confidence level. For the first time, we have demonstrated the possibility of utilizing the directional Cherenkov information for sub-MeV solar neutrinos, in a large-scale, high light yield liquid scintillator detector. This measurement provides an experimental proof of principle for future hybrid event reconstruction using both Cherenkov and scintillation signatures simultaneously., Comment: 6 pages, 4 figures, short letter of arXiv:2109.04770

Liquid scintillator detectors play a central role in the detection of neutrinos from various sources. In particular, it is the only technique used so far for the precision spectroscopy of sub-MeV solar neutrinos, as demonstrated by the Borexino experiment at the Gran Sasso National Laboratory in Italy. The benefit of a high light yield, and thus a low energy threshold and a good energy resolution, comes at the cost of the directional information featured by water Cherenkov detectors, measuring $^8$B solar neutrinos above a few MeV. In this paper we provide the first directionality measurement of sub-MeV solar neutrinos which exploits the correlation between the first few detected photons in each event and the known position of the Sun for each event. This is also the first signature of directionality in neutrinos elastically scattering off electrons in a liquid scintillator target. This measurement exploits the sub-dominant, fast Cherenkov light emission that precedes the dominant yet slower scintillation light signal. Through this measurement, we have also been able to extract the rate of $^{7}$Be solar neutrinos in Borexino. The demonstration of directional sensitivity in a traditional liquid scintillator target paves the way for the possible exploitation of the Cherenkov light signal in future kton-scale experiments using liquid scintillator targets. Directionality is important for background suppression as well as the disentanglement of signals from various sources., Comment: 19 pages, 15 Figures, revised version after comments from PRD Referees, shorter letter submitted with the title: "First Directional Measurement of sub-MeV Solar Neutrinos with Borexino"

Nanowire lasers can be monolithically and site-selectively integrated onto silicon photonic circuits. To assess their full potential for ultrafast opto-electronic devices, a detailed understanding of their lasing dynamics is crucial. However, the roles played by their resonator geometry and the microscopic processes that mediate energy exchange between the photonic, electronic, and phononic subsystems are largely unexplored. Here, we study the dynamics of GaAs-AlGaAs core-shell nanowire lasers at cryogenic temperatures using a combined experimental and theoretical approach. Our results indicate that these NW lasers exhibit sustained intensity oscillations with frequencies ranging from 160 GHz to 260 GHz. As the underlying physical mechanism, we identified self-induced electron-hole plasma temperature oscillations resulting from a dynamic competition between photoinduced carrier heating and cooling via phonon scattering. These dynamics are intimately linked to the strong interaction between the lasing mode and the gain material, which arises from the wavelength-scale dimensions of these lasers. We anticipate that our results could lead to new approaches for ultrafast intensity and phase modulation of chip-integrated nanoscale semiconductor lasers., Comment: Revised manuscript

Cosmogenic radio-nuclei are an important source of background for low-energy neutrino experiments. In Borexino, cosmogenic $^{11}$C decays outnumber solar $pep$ and CNO neutrino events by about ten to one. Highly efficient identification of this background is mandatory for these neutrino analyses. We present here the details of the most consolidated strategy, used throughout Borexino solar neutrino measurements. It hinges upon finding the space-time correlations between $^{11}$C decays, the preceding parent muons and the accompanying neutrons. This article describes the working principles and evaluates the performance of this Three-Fold Coincidence (TFC) technique in its two current implementations: a hard-cut and a likelihood-based approach. Both show stable performances throughout Borexino Phases II (2012-2016) and III (2016-2020) data sets, with a $^{11}$C tagging efficiency of $\sim$90 % and $\sim$63-66 % of the exposure surviving the tagging. We present also a novel technique that targets specifically $^{11}$C produced in high-multiplicity during major spallation events. Such $^{11}$C appear as a burst of events, whose space-time correlation can be exploited. Burst identification can be combined with the TFC to obtain about the same tagging efficiency of $\sim$90 % but with a higher fraction of the exposure surviving, in the range of $\sim$66-68 %., Comment: 21 pages, 14 figures (but 15 files, one figure being made of 2 images), 3 tables

Borexino is a liquid scintillator detector located at the Laboratori Nazionale del Gran Sasso, Italy with the main goal to measure solar neutrinos. The experiment recently provided the first direct experimental evidence of CNO-cycle neutrinos in the Sun, rejecting the no-CNO signal hypothesis with a significance greater than 5$\sigma$ at 99\%C.L. The intrinsic $^{210}$Bi is an important background for this analysis due to its similar spectral shape to that of CNO neutrinos. $^{210}$Bi can be measured through its daughter $^{210}$Po which can be distinguished through an event-by-event basis via pulse shape discrimination. However, this required reducing the convective motions in the scintillator that brought additional $^{210}$Po from peripheral sources. This was made possible through the thermal insulation and stabilization campaign performed between 2015 and 2016. This article will explain the strategy and the different methods performed to extract the $^{210}$Bi upper limit in Phase-III (Jul 2016- Feb 2020) of the experiment through the analysis of $^{210}$Po in the cleanest region of the detector called the Low Polonium Field., Comment: Contribution to the 2021 Neutrinos session of the 55th Rencontres de Moriond

Neutrinos are elementary particles which are known since many years as fundamental messengers from the interior of the Sun. The Standard Solar Model, which gives a theoretical description of all nuclear processes which happen in our star, predicts that roughly 99% of the energy produced is coming from a series of processes known as the "pp chain". Such processes have been studied in detail over the last years by means of neutrinos, thanks also to the important measurements provided by the Borexino experiment. The remaining 1% is instead predicted to come from a separate loop-process, known as the "CNO cycle". This sub-dominant process is theoretically well understood, but has so far escaped any direct observation. Another fundamental aspect is that the CNO cycle is indeed the main nuclear engine in stars more massive than the Sun. In 2020, thanks to the unprecedented radio-purity and temperature control achieved by the Borexino detector over recent years, the first ever detection of neutrinos from the CNO cycle has been finally announced. The milestone result confirms the existence of this nuclear fusion process in our Universe. Here, the details of the detector stabilization and the analysis techniques adopted are reported., Comment: 7 pages, 3 figures. Contribution to the 2021 Neutrinos session of the 55th Rencontres de Moriond

Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin liquid candidate systems were identified in quasi-two-dimensional (quasi-2D) systems. For 3D, however, the situation is less favourable as quantum fluctuations are reduced and competing states become more relevant. Here we report a comprehensive study of thermodynamic, magnetic and dielectric properties on single crystalline and pressed-powder samples of PbCuTe$_2$O$_6$, a candidate material for a 3D frustrated quantum spin liquid featuring a hyperkagome lattice. Whereas the low-temperature properties of the powder samples are consistent with the recently proposed quantum spin liquid state, an even more exotic behaviour is revealed for the single crystals. These crystals show ferroelectric order at $T_{\text{FE}} \approx 1\,\text{K}$, accompanied by strong lattice distortions, and a modified magnetic response -- still consistent with a quantum spin liquid -- but with clear indications for quantum critical behaviour., Comment: 59 pages, 15 figures, This version of the article has been accepted for publication, after peer review but is not the Version of Record and does not reflect post-acceptance improvements, or any corrections. The Version of Record is available online

For most of their existence stars are fueled by the fusion of hydrogen into helium proceeding via two theoretically well understood processes, namely the $pp$ chain and the CNO cycle. Neutrinos emitted along such fusion processes in the solar core are the only direct probe of the deep interior of the star. A complete spectroscopy of neutrinos from the {\it pp} chain, producing about 99\% of the solar energy, has already been performed \cite{bib:Nature-2018}. Here, we report the direct observation, with a high statistical significance, of neutrinos produced in the CNO cycle in the Sun. This is the first experimental evidence of this process obtained with the unprecedentedly radio-pure large-volume liquid-scintillator Borexino detector located at the underground Laboratori Nazionali del Gran Sasso in Italy. The main difficulty of this experimental effort is to identify the excess of the few counts per day per 100 tonnes of target due to CNO neutrino interactions above the backgrounds. A novel method to constrain the rate of \bi contaminating the scintillator relies on the thermal stabilisation of the detector achieved over the past 5 years. In the CNO cycle, the hydrogen fusion is catalyzed by the carbon (C) - nitrogen (N) - oxygen (O) and thus its rate, as well as the flux of emitted CNO neutrinos, directly depends on the abundance of these elements in solar core. Therefore, this result paves the way to a direct measurement of the solar metallicity by CNO neutrinos. While this result quantifies the relative contribution of the CNO fusion in the Sun to be of the order of 1\%, this process is dominant in the energy production of massive stars. The occurrence of the primary mechanism for the stellar conversion of hydrogen into helium in the Universe has been proven., Comment: 43 pages, 14 figures

Neutrinos emitted in the carbon, nitrogen, oxygen (CNO) fusion cycle in the Sun are a sub-dominant, yet crucial component of solar neutrinos whose flux has not been measured yet. The Borexino experiment at the Laboratori Nazionali del Gran Sasso (Italy) has a unique opportunity to detect them directly thanks to the detector's radiopurity and the precise understanding of the detector backgrounds. We discuss the sensitivity of Borexino to CNO neutrinos, which is based on the strategies we adopted to constrain the rates of the two most relevant background sources, pep neutrinos from the solar pp-chain and Bi-210 beta decays originating in the intrinsic contamination of the liquid scintillator with Pb-210. Assuming the CNO flux predicted by the high-metallicity Standard Solar Model and an exposure of 1000 daysx71.3 t, Borexino has a median sensitivity to CNO neutrino higher than 3 sigma. With the same hypothesis the expected experimental uncertainty on the CNO neutrino flux is 23%, provided the uncertainty on the independent estimate of the Bi-210 interaction rate is 1.5 cpd/100t. Finally, we evaluated the expected uncertainty of the C and N abundances and the expected discrimination significance between the high and low metallicity Standard Solar Models (HZ and LZ) with future more precise measurement of the CNO solar neutrino flux., Comment: 16 pages, 12 figures

We report on searches for neutrinos and antineutrinos from astrophysical sources performed with the Borexino detector at the Laboratori Nazionali del Gran Sasso in Italy. Electron antineutrinos ($\bar{\nu}_e$) are detected in an organic liquid scintillator through the inverse $\beta$-decay reaction. In the present work we set model-independent upper limits in the energy range 1.8-16.8 MeV on neutrino fluxes from unknown sources that improve our previous results, on average, by a factor 2.5. Using the same data set, we first obtain experimental constraints on the diffuse supernova $\bar{\nu}_e$ fluxes in the previously unexplored region below 8 MeV. A search for $\bar{\nu}_e$ in the solar neutrino flux is also presented: the presence of $\bar{\nu}_e$ would be a manifestation of a non-zero anomalous magnetic moment of the neutrino, making possible its conversion to antineutrinos in the strong magnetic field of the Sun. We obtain a limit for a solar $\bar{\nu}_e$ flux of 384 cm$^{-2}$s$^{-1}$ (90% C.L.), assuming an undistorted solar $^{8}$B neutrinos energy spectrum, that corresponds to a transition probability $p_{ \nu_e \rightarrow \bar\nu_{e}}<$ 7.2$\times$10$^{-5}$ (90% C.L.) for E$_{\bar {\nu}_e}$ $>$ 1.8 MeV. At lower energies, by investigating the spectral shape of elastic scattering events, we obtain a new limit on solar $^{7}$Be-$\nu_e$ conversion into $\bar{\nu}_e$ of $p_{ \nu_e \rightarrow \bar \nu_{e}}<$ 0.14 (90% C.L.) at 0.862 keV. Last, we investigate solar flares as possible neutrino sources and obtain the strongest up-to-date limits on the fluence of neutrinos of all flavor neutrino below 3-7 ,MeV. Assuming the neutrino flux to be proportional to the flare's intensity, we exclude an intense solar flare as the cause of the observed excess of events in run 117 of the Cl-Ar Homestake experiment., Comment: 18 pages, 8 figures, 4 tables, 73 references

This paper presents a geoneutrino measurement using 3262.74 days of data taken with the Borexino detector at LNGS in Italy. By observing $52.6 ^{+9.4}_{-8.6} ({\rm stat}) ^{+2.7}_{-2.1}({\rm sys})$ geoneutrinos (68% interval) from $^{238}$U and $^{232}$Th, a signal of $47.0^{+8.4}_{-7.7}\,({\rm stat)}^{+2.4}_{-1.9}\,({\rm sys})$ TNU with $^{+18.3}_{-17.2}$% total precision was obtained. This result assumes the same Th/U mass ratio found in chondritic CI meteorites but compatible results were found when contributions from $^{238}$U and $^{232}$Th were fit as free parameters. Antineutrino background from reactors is fit unconstrained and found compatible with the expectations. The null-hypothesis of observing a signal from the mantle is excluded at a 99.0% C.L. when exploiting the knowledge of the local crust. Measured mantle signal of $21.2 ^{+9.6}_{-9.0} ({\rm stat})^{+1.1}_{-0.9} ({\rm sys})$ TNU corresponds to the production of a radiogenic heat of $24.6 ^{+11.1}_{-10.4}$ TW (68% interval) from $^{238}$U and $^{232}$Th in the mantle. Assuming 18% contribution of $^{40}$K in the mantle and $8.1^{+1.9}_{-1.4}$ TW of radiogenic heat of the lithosphere, the Borexino estimate of the total Earth radiogenic heat is $38.2 ^{+13.6}_{-12.7}$ TW, corresponding to a convective Urey ratio of 0.78$^{+0.41}_{-0.28}$. These values are compatible with different geological models, however there is a 2.4$\sigma$ tension with those which predict the lowest concentration of heat-producing elements. By fitting the data with a constraint on the reactor antineutrino background, the existence of a hypothetical georeactor at the center of the Earth having power greater than 2.4 TW at 95% C.L. is excluded. Particular attention is given to all analysis details, which should be of interest for the next generation geoneutrino measurements., Comment: 69 pages, 56 Figures (some composed of multiple files), 17 Tables, 135 References

The Borexino detector measures solar neutrino fluxes via neutrino-electron elastic scattering. Observed spectra are determined by the solar-$\nu_{e}$ survival probability $P_{ee}(E)$, and the chiral couplings of the neutrino and electron. Some theories of physics beyond the Standard Model postulate the existence of Non-Standard Interactions (NSI's) which modify the chiral couplings and $P_{ee}(E)$. In this paper, we search for such NSI's, in particular, flavor-diagonal neutral current interactions that modify the $\nu_e e$ and $\nu_\tau e$ couplings using Borexino Phase II data. Standard Solar Model predictions of the solar neutrino fluxes for both high- and low-metallicity assumptions are considered. No indication of new physics is found at the level of sensitivity of the detector and constraints on the parameters of the NSI's are placed. In addition, with the same dataset the value of $\sin^2\theta_W$ is obtained with a precision comparable to that achieved in reactor antineutrino experiments., Comment: 28 pages, 7 figures. Slight modifications in the title, abstract, and conclusion. Few references added. Text expanded for clarity. Accepted in JHEP

We have measured the flux of cosmic muons in the Laboratori Nazionali del Gran Sasso at 3800\,m\,w.e. to be $(3.432 \pm 0.003)\cdot 10^{-4}\,\mathrm{{m^{-2}s^{-1}}}$ based on ten years of Borexino data acquired between May 2007 and May 2017. A seasonal modulation with a period of $(366.3 \pm 0.6)\,\mathrm{d}$ and a relative amplitude of $(1.36 \pm0.04)\%$ is observed. The phase is measured to be $(181.7 \pm 0.4)\,\mathrm{d}$, corresponding to a maximum at the 1$^\mathrm{st}$ of July. Using data inferred from global atmospheric models, we show the muon flux to be positively correlated with the atmospheric temperature and measure the effective temperature coefficient $\alpha_\mathrm{T} = 0.90 \pm 0.02$. The origin of cosmic muons from pion and kaon decays in the atmosphere allows to interpret the effective temperature coefficient as an indirect measurement of the atmospheric kaon-to-pion production ratio $r_{\mathrm{K}/\pi} = 0.11^{+0.11}_{-0.07}$ for primary energies above $18\,\mathrm{TeV}$. We find evidence for a long-term modulation of the muon flux with a period of $\sim 3000\,\mathrm{d}$ and a maximum in June 2012 that is not present in the atmospheric temperature data. A possible correlation between this modulation and the solar activity is investigated. The cosmogenic neutron production rate is found to show a seasonal modulation in phase with the cosmic muon flux but with an increased amplitude of $(2.6 \pm 0.4)\%$., Comment: 30 pages, 16 figures, proofreading for publication in JCAP

A spectral fitter based on the graphics processor unit (GPU) has been developed for Borexino solar neutrino analysis. It is able to shorten the fitting time to a superior level compared to the CPU fitting procedure. In Borexino solar neutrino spectral analysis, fitting usually requires around one hour to converge since it includes time-consuming convolutions in order to account for the detector response and pile-up effects. Moreover, the convergence time increases to more than two days when including extra computations for the discrimination of $^{11}$C and external $\gamma$s. In sharp contrast, with the GPU-based fitter it takes less than 10 seconds and less than four minutes, respectively. This fitter is developed utilizing the GooFit project with customized likelihoods, pdfs and infrastructures supporting certain analysis methods. In this proceeding the design of the package, developed features and the comparison with the original CPU fitter are presented., Comment: 5 pages, 2 figures, proceeding for TAUP 2017 XV International Conference on Topics in Astroparticle and Underground Physics

We have investigated PLLA crystallization in lamellae-forming PS-b-PLLA confined to straight cylindrical nanopores under weak confinement (nanopore diameter D / equilibrium PS-b-PLLA period L0 larger than 4.8). Molten PS-b-PLLA predominantly forms concentric lamellae along the nanopores, but intertwined helices occur even for D/L0 = 7.3. Quenching PS-b-PLLA melts below TG(PS) results in PLLA cold crystallization strictly confined by the vitrified PS domains. Above TG(PS), PLLA crystallization is templated by the PS-b-PLLA melt domain structure in the nanopore centers, while adsorption on the nanopore walls stabilizes the outermost cylindrical PS-b-PLLA shell. In between, the nanoscopic PS-b-PLLA melt domain structure apparently ripens to reduce frustrations transmitted from the outermost immobilized PS-b-PLLA layer. The onset of PLLA crystallization catalyzes the ripening while transient ripening states are arrested by advancing PLLA crystallization. Certain helical structure motifs persist PLLA crystallization even if PS is soft. The direction of fastest PLLA crystal growth is preferentially aligned with the nanopore axes to the same degree as for PLLA homopolymer, independent of whether PS is vitreous or soft.

We report on an improved measurement of the $^8$B solar neutrino interaction rate with the Borexino experiment at the Laboratori Nazionali del Gran Sasso. Neutrinos are detected via their elastic scattering on electrons in a large volume of liquid scintillator. The measured rate of scattered electrons above 3 MeV of energy is $0.223\substack{+0.015 \\ -0.016}\,(stat)\,\substack{+0.006 \\ -0.006}\,(syst)$ cpd/100 t, which corresponds to an observed solar neutrino flux assuming no neutrino flavor conversion of $\Phi\substack{\rm ES \\ ^8\rm B}=2.57\substack{+0.17 \\ -0.18}(stat)\substack{+0.07\\ -0.07}(syst)\times$10$^6$ cm$^{-2}\,$s$^{-1}$. This measurement exploits the active volume of the detector in almost its entirety for the first time, and takes advantage of a reduced radioactive background following the 2011 scintillator purification campaign and of novel analysis tools providing a more precise modeling of the background. Additionally, we set a new limit on the interaction rate of solar $hep$ neutrinos, searched via their elastic scattering on electrons as well as their neutral current-mediated inelastic scattering on carbon, $^{12}$C($\nu,\nu'$)$^{12}$C* ($E_{\gamma}$= 15.1 MeV)., Comment: 14 pages, 13 figures, 4 tables

Because final properties of nanoscale polymeric structures are largely determined by the solid-state microstructure of the confined polymer, it is imperative not only to understand how the microstructure of polymers develops under nanoscale confinement but also to establish means to manipulate it. Here we present a series of processing strategies, adapted from methods used in bulk polymer processing, that allow to control the solidification of polymer nanostructures. Firstly, we show that supramolecular nucleating agents can be readily used to modify the crystallization kinetics of confined poly(vinylidene fluoride) (PVDF). In addition, we demonstrate that microstructural features that are not traditionally affected by nucleating agents, such as the orientation of crystals, can be tuned with the crystallization temperature applied. Interestingly, we also show that high crystallization temperatures and long annealing periods induce the formation of the modification of PVDF, hence enabling the simple production of ferro/piezoelectric nanostructures. We anticipate that the approaches presented here can open up a plethora of new possibilities for the processing of polymer-based nanostructures with tailored properties and functionalities.

We present the first simultaneous measurement of the interaction rates of $pp$, $^7$Be, and $pep$ solar neutrinos performed with a global fit to the Borexino data in an extended energy range (0.19-2.93)$\,$MeV. This result was obtained by analyzing 1291.51$\,$days of Borexino Phase-II data, collected between December 2011 and May 2016 after an extensive scintillator purification campaign. We find: rate($pp$)$\,$=$\,$$134$$\,$$\pm$$\,$$10$$\,$($stat$)$\,$$^{\rm +6}_{\rm -10}$$\,$($sys$)$\,$cpd/100$\,$t, rate($^7$Be)$\,$=$\,$$48.3$$\,$$\pm$$\,$$1.1$$\,$($stat$)$\,$$^{\rm +0.4}_{\rm -0.7}$$\,$($sys$)$\,$cpd/100$\,$t, and rate($pep$)$\,$=$\,$$2.43$$\pm$$\,$$0.36$$\,$($stat$)$^{+0.15}_{-0.22}$$\,$($sys$)$\,$cpd/100$\,$t. These numbers are in agreement with and improve the precision of our previous measurements. In particular, the interaction rate of $^7$Be $\nu$'s is measured with an unprecedented precision of 2.7%, showing that discriminating between the high and low metallicity solar models is now largely dominated by theoretical uncertainties. The absence of $pep$ neutrinos is rejected for the first time at more than 5$\,$$\sigma$. An upper limit of $8.1$$\,$cpd/100$\,$t (95%$\,$C.L.) on the CNO neutrino rate is obtained by setting an additional constraint on the ratio between the $pp$ and $pep$ neutrino rates in the fit. This limit has the same significance as that obtained by the Borexino Phase-I (currently providing the tightest bound on this component), but is obtained by applying a less stringent constraint on the $pep$ $\nu$ flux., Comment: 8 pages, 7 figures

A search for the solar neutrino effective magnetic moment has been performed using data from 1291.5 days exposure during the second phase of the Borexino experiment. No significant deviations from the expected shape of the electron recoil spectrum from solar neutrinos have been found, and a new upper limit on the effective neutrino magnetic moment of $\mu_{\nu}^{eff}$ $<$ 2.8$\cdot$10$^{-11}$ $\mu_{B}$ at 90\% c.l. has been set using constraints on the sum of the solar neutrino fluxes implied by the radiochemical gallium experiments.Using the limit for the effective neutrino moment, new limits for the magnetic moments of the neutrino flavor states, and for the elements of the neutrino magnetic moments matrix for Dirac and Majorana neutrinos, are derived., Comment: 7 pages, 2 figures

Free-space optical communication links are promising channels for establishing secure quantum communication. Here we study the transmission of nonclassical light through a turbulent atmospheric link under diverse weather conditions, including rain or haze. To include these effects, the theory of light transmission through atmospheric links in the elliptic-beam approximation presented by Vasylyev et al. [D. Vasylyev et al., Phys. Rev. Lett. 117, 090501 (2016); arXiv:1604.01373] is further generalized.It is demonstrated, with good agreement between theory and experiment, that low-intensity rain merely contributes additional deterministic losses, whereas haze also introduces additional beam deformations of the transmitted light. Based on these results, we study theoretically the transmission of quadrature squeezing and Gaussian entanglement under these weather conditions., Comment: 14 pages, 8 figures

We present the results of a low-energy neutrino search using the Borexino detector in coincidence with the gravitational wave (GW) events GW150914, GW151226 and GW170104. We searched for correlated neutrino events with energies greater than 250 keV within a time window of $\pm500$ s centered around the GW detection time. A total of five candidates were found for all three GW150914, GW151226 and GW170104. This is consistent with the number of expected solar neutrino and background events. As a result, we have obtained the best current upper limits on the GW event neutrino fluence of all flavors ($\nu_e, \nu_{\mu}, \nu_{\tau}$) in the energy range $(0.5 - 5.0)$ MeV., Comment: 8 pages, 5 figures

We describe the Monte Carlo (MC) simulation package of the Borexino detector and discuss the agreement of its output with data. The Borexino MC 'ab initio' simulates the energy loss of particles in all detector components and generates the resulting scintillation photons and their propagation within the liquid scintillator volume. The simulation accounts for absorption, reemission, and scattering of the optical photons and tracks them until they either are absorbed or reach the photocathode of one of the photomultiplier tubes. Photon detection is followed by a comprehensive simulation of the readout electronics response. The algorithm proceeds with a detailed simulation of the electronics chain. The MC is tuned using data collected with radioactive calibration sources deployed inside and around the scintillator volume. The simulation reproduces the energy response of the detector, its uniformity within the fiducial scintillator volume relevant to neutrino physics, and the time distribution of detected photons to better than 1% between 100 keV and several MeV. The techniques developed to simulate the Borexino detector and their level of refinement are of possible interest to the neutrino community, especially for current and future large-volume liquid scintillator experiments such as Kamland-Zen, SNO+, and Juno.

We detected the seasonal modulation of the $^7$Be neutrino interaction rate with the Borexino detector at the Laboratori Nazionali del Gran Sasso in Italy. The period, amplitude, and phase of the observed time evolution of the signal are consistent with its solar origin, and the absence of an annual modulation is rejected at 99.99\% C.L. The data are analyzed using three methods: the sinusoidal fit, the Lomb-Scargle and the Empirical Mode Decomposition techniques, which all yield results in excellent agreement., Comment: 11 palese, 13 figures