Search

The Fusion Evaluated Nuclear Data Library (FENDL) is a comprehensive and validated collection of nuclear cross section data coordinated by the International Atomic Energy Agency (IAEA) Nuclear Data Section (NDS). FENDL assembles the best nuclear data for fusion applications selected from available nuclear data libraries and has been under development for decades. FENDL contains sub-libraries for incident neutron, proton, and deuteron cross sections including general purpose and activation files used for particle transport and nuclide inventory calculations. We describe the history, selection of evaluations for the various sub-libraries (neutron, proton, deuteron) with the focus on transport and reactor dosimetry applications, the processing of the nuclear data for application codes, and the development of the TENDL-2017 library which is the currently recommended activation library for FENDL. We briefly describe the IAEA IRDFF library as the recommended library for dosimetry fusion applications. We also present work on validation of the neutron sub-library using a variety of fusion relevant computational and experimental benchmarks. A variety of cross section libraries are used for the validation work including FENDL-2.1, FENDL-3.1d, FENDL-3.2, ENDF/B-VIII.0, and JEFF-3.2 with the emphasis on the FENDL libraries. The results of the experimental validation showed that the performance of FENDL-3.2b is at least as good and in most cases better than FENDL-2.1. Future work will consider improved evaluations developed by the International Nuclear Data Evaluation Network (INDEN). Additional work will be needed to investigate differences in gas production in structural materials. Covariance matrices need to be updated to support the development of fusion technology. Additional validation work for high-energy neutrons, protons and deuterons, and the activation library will be needed., Comment: 81 pages, 114 figures

It is challenging to distinguish between fusion-fission and quasifission experimentally. To determine the characteristics of quasifission processes associated with dominant phenomena in heavy-ion collisions is important for estimating precisely the fusion cross section, which is relevant to the synthesis of new elements. We classified fusion-fission and quasifission processes theoretically in the past for an accurate assessment of the fusion cross section. However, no detailed analysis focused on each process was performed. In this work, we aimed to analyze the dynamical characteristics of quasifission processes in terms of the Langevin equation model. We specify the quasifission processes, and analyze the scission configuration. Finally, we clarify the origin of several modes included in quasifission. The calculation framework is the multidimensional dynamical model of nucleus-nucleus collisions based on the Langevin equations. It is shown that several quasifission modes exist leading to different fragment deformations. The time scale of the quasifission process differs for several different modes. Each scission configuration and total kinetic energy also differ. The different quasifission modes are caused by the neck relaxation controlling the mass drift toward symmetry. This means that it is possible to discuss the time-dependent functional form of the neck parameter $\epsilon$ for the quasifission process in the framework of the dynamical model based on Langevin equations., Comment: 10 pages, 9 figures. arXiv admin note: text overlap with arXiv:2309.11771, arXiv:2309.15549

In the fusion process, the investigation of the reaction dynamics in the time evolution of the nuclear configuration is necessary. The neck parameter $\epsilon$ which is one of the parameters representing the nuclear configuration in the two center shell model is important in fusion owing to the nucleons transferring through the neck. The time evolution of the neck has not been discussed in detail, but is crucial for fusion cross section in the assessment of new elements synthesis. The dynamical analysis for the fusion hindrance under the neck formation on the nuclear deformation space has been done. The fusion probability $P_\text{CN}$ considering the different denecking motion and the fusion hindrance are discussed. The calculations were performed using the dynamical model of nucleus-nucleus collisions based on the multidimensional Langevin equations.The formation of the neck bridge at the approaching stage is found to be crucial to the fusion hindrance. It is clarified that the inner barrier appears owing to the change in the degree of mass asymmetry $\alpha$ with the relaxation of $\epsilon$.The fusion hindrance occurs because the inner barrier is formed by the early neck formation. The role of the neck parameter $\epsilon$ is critically important for the fusion dynamics., Comment: 9 pages, 9 figures

The very early stage of the coalescence of two nuclei is studied and used to estimate the nuclear viscosity. The time evolution of the neck region has been simulated by the unified Langevin equation method, which is used in the analysis of heavy-ion collisions from the approaching stage to the fusion-fission stage. It is found that the transition from viscous to inertial coalescence that appeared in the neck growth of macroscopic drops can also be seen in the present simulation in nucleus-nucleus collisions. The dynamics of neck growth is analyzed in terms of the hydrodynamical formula and the viscosity coefficient of nuclear matter is estimated using the analogy of macroscopic drops., Comment: 14 pages 6 figures

The capture cross section, the fusion cross section, and the quasi-fission yield producing symmetric fragments ($A_{CN}/2\pm20u$) in the $^{48}$Ca+$^{238}$U reaction are analyzed by the multidimensional Langevin equation taking account of the surface friction effect. From the experimental data, the strength of the tangential friction has been determined. It is presented that tangential friction increases in proportional to the power of the relative velocity of the projectile and the target., Comment: 12 pages, 8 figures

High quality nuclear data is the most fundamental underpinning for all neutron metrology applications. This paper describes the release of version II of the International Reactor Dosimetry and Fusion File (IRDFF-II) that contains a consistent set of nuclear data for fission and fusion neutron metrology applications up to 60~MeV neutron energy. The library is intended to support: a) applications in research reactors; b) safety and regulatory applications in the nuclear power generation in commercial fission reactors; and c) material damage studies in support of the research and development of advanced fusion concepts. The paper describes the contents of the library, documents the thorough verification process used in its preparation, and provides an extensive set of validation data gathered from a wide range of neutron benchmark fields. The new \mbox{IRDFF-II} library includes 119 metrology reactions, four cover material reactions to support self-shielding corrections, five metrology metrics used by the dosimetry community, and cumulative fission products yields for seven fission products in three different neutron energy regions. In support of characterizing the measurement of the residual nuclei from the dosimetry reactions and the fission product decay modes, the present document lists the recommended decay data, particle emission energies and probabilities for 68 activation products. It also includes neutron spectral characterization data for 29 neutron benchmark fields for the validation of the library contents. The IRDFF-II library and comprehensive documentation is available online at https://www-nds.iaea.org/IRDFF/. Evaluated cross sections can be compared with experimental data and other evaluations at https://www-nds.iaea.org/exfor/endf.htm. The new library is expected to become the international reference in neutron metrology for multiple applications., Comment: Submitted to Nuclear Data Sheets, 109 pages, figures revised

The fusion-fission process accompanied by neutron emission is studied in the superheavy-mass region on the basis of the fluctuation-dissipation model combined with a statistical model. The calculation of the trajectory or the shape evolution in the deformation space of the nucleus with neutron emission is performed. Each process (quasi-fission, fusion-fission, and deep quasi-fission processes) has a characteristic travelling time from the point of contact of colliding nuclei to the scission point. These dynamical aspects of the whole process are discussed in terms of the pre-scission neutron multiplicity, which depends on the time spent on each process. We have presented the details of the characteristics of our model calculation in the reactions $^{48}$Ca+$^{208}$Pb and $^{48}$Ca+$^{244}$Pu, and shown how the structure of the distribution of pre-scission neutron multiplicity depends on the incident energy., Comment: 19 pages, 12 figures, Accepted for publication in J. Phys. G

The fusion-fission process in the superheavy mass region is studied systematically by solving the time evolution of nuclear shape in three-dimensional deformation space using the Langevin equation. By analyzing the trajectory in the deformation space, we identify the critical area when the trajectory's destination is determined to be the fusion or the quasi-fission process. It is also clarified that the potential landscape around the critical area is crucial for estimating the fusion probability, and its dependence on the atomic number is presented., Comment: 14 pages, 7 figures, accepted for publication in Nuclear Physics A

Cross sections of the $^{186}$W, $^{187}$Re, $^{188}$Os($\gamma,n$) reactions were measured using quasi-monochromatic photon beams from laser Compton scattering (LCS) with average energies from 7.3 to 10.9 MeV. The results are compared with the predictions of Hauser-Feshbach statistical calculations using four different sets of input parameters. In addition, the inverse neutron capture cross sections were evaluated by constraining the model parameters, especially the $E1$ strength function, on the basis of the experimental data. The present experiment helps to further constrain the correction factor $F_{\sigma}$ for the neutron capture on the 9.75 keV state in $^{187}$Os. Implications of $F_{\sigma}$ to the Re-Os cosmochronology are discussed with a focus on the uncertainty in the estimate of the age of the Galaxy., Comment: 11 pages

We propose an effective method for the precise investigation of the fusion-fission mechanism in the superheavy-mass region, using the fluctuation-dissipation model. The trajectory calculation with friction is performed in the nuclear deformation space using the Langevin equation. In the reaction $^{48}$Ca+$^{244}$Pu, the trajectories are classified into the fusion-fission process, the quasi-fission process and the deep quasi-fission process. By analyzing the time evolution of each trajectory, the mechanism of each process is clearly revealed, i.e., it is explained why a trajectory takes a characteristic path in this model. We discuss, in particular, the condition under which the fusion path is followed, which is crucial in the discussion of the possibility of synthesizing superheavy elements., Comment: 25 pages, 12 figures, accepted for publication in Nuclear Physics A

We analyzed the experimental data of the pre-scission neutron multiplicity in connection with fission fragments in the reaction $^{58}$Ni+$^{208}$Pb at the incident energy corresponding to the excitation energy of compound nucleus $E^{*}$=185.9 MeV, which was performed by D\'{e}MoN group. The relation between the pre-scission neutron multiplicity and each reaction process having different reaction time is investigated. In order to study the fusion-fission process accompanied by neutron emission, the fluctuation-dissipation model combined with a statistical model is employed. It is found that the fusion-fission process and the quasi-fission process are clearly distinguished in correlation with the pre-scission neutron multiplicity., Comment: 11 figures

Dynamical reaction theory is presented for synthesis of superheavy elements. Characteristic features of formation and surviving are discussed, which combinedly determine final residue cross sections of superheavy elements. Preliminary results on Z=114 are also given., Comment: 6 pages, 6 figures

Dynamical reaction theories are reviewed for synthesis of superheavy elements. Characteristic features of formation and surviving are discussed with reference to possible incident channels. Theoretical predictions are presented on favorable incident channels and on optimum energies for synthesis of Z=114., Comment: 4 pages, 5 figures LaTeX file