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Palladium promotion and deposition on monoclinic zirconia are effective strategies to boost the performance of bulk In

The response of the BAS-TR image plate (IP) was absolutely calibrated using CR-39 track detector for high linear energy transfer (LET) Au ions up to $\sim$1.6 GeV (8.2 MeV/nucleon), accelerated by high-power lasers. The calibration was carried out by employing a high-resolution Thomson parabola spectrometer, which allowed resolving Au ions with closely spaced ionization states up to 58$^+$. A response function was obtained by fitting the photo-stimulated luminescence (PSL) per Au ion for different ion energies, which is broadly in agreement with that expected from ion stopping in the active layer of the IP. This calibration would allow quantifying the ion energy spectra for high energy Au ions, which is important for further investigation of the laser-based acceleration of heavy ion beams., Comment: 6 pages; 4 figures. Submitted to journal for review

In this paper, we report on the acceleration of protons and oxygen ions from tens of micrometer large water droplets by a high-intensity laser in the range of 1020 W/cm2. Proton energies of up to 6 MeV were obtained from a hybrid acceleration regime between classical Coulomb explosion and shocks. Besides the known thermal energy spectrum, a collective acceleration of oxygen ions of different charge states is observed. 3D PIC simulations and analytical models are employed to support the experiential findings and reveal the potential for further applications and studies.

A plethora of metal promoters have been applied to enhance the performance of In2O3 in CO2 hydrogenation to methanol, a prospective energy carrier. However, the lack of systematic catalyst preparation and evaluation precludes a direct comparison of their speciation and promotional effects, and consequently, the design of an optimal system. Herein, flame spray pyrolysis (FSP) is employed as a standardized synthesis method to introduce nine metal promoters (0.5 wt.%) into In2O3. Methanol productivity generally increased on M-In2O3 with selectivity following Pd approximate to Pt > Rh approximate to Ru approximate to Ir > Ni approximate to Co > Ag approximate to In2O3 > Au. In-depth characterization, kinetic analyses, and theoretical calculations reveal a range of metal-dependent speciation which dictate catalyst architecture and degree of promotion. Atomically-dispersed promoters (Pd, Pt, Rh, Ru, and Ir) grant the highest improvement in performance, particularly Pd and Pt, which markedly promote hydrogen activation while hindering undesired CO formation. In contrast, metals in clustered (Ni and Co) and nanoparticle (Ag and Au) forms display moderate and no promotion, respectively. This study provides an atomic-level understanding of In2O3 promotion based on a unified protocol, and highlights the potential of FSP to engineer complex catalytic systems toward more efficient energy transformations., Advanced Energy Materials, 12 (14)

Bulk electron temperatures are calculated for thin Cu targets irradiated by the petawatt class Vulcan laser, from the Kα yield obtained using highly oriented pyrolytic graphite crystals. Cu-Kα emission studies have been used to probe the bulk electron temperature. A 30–80 eV core temperature extends homogeneously over distances up to ten times the laser focal spot size. Energy shifting has been observed due to different ionization states produced for different temperatures in the plasma. Polarization dependencies of plasma temperature are observed through the production of x-rays in different targets. 2D PIC simulations were performed to measure the polarization dependency of bulk electron temperature, which supports our experimental results. This paper could be of importance in understanding the different behavior of laser coupling at different polarizations and their role in x-ray production.

Helical coil accelerators are a recent development in laser-driven ion production, acting on the intrinsically wide divergence and broadband energy spectrum of laser-accelerated protons to deliver ultra-low divergence and quasi-monoenergetic beams. The modularity of helical coil accelerators also provides the attractive prospective of multi-staging. Here we show, on a proof-of-principle basis, a two-stage configuration which allows optical tuning of the energy of the selected proton beamlet. Experimental data, corroborated by particle tracing simulations, highlights the importance of controlling precisely the beam injection. Efficient post-acceleration of the protons with an energy gain up to ∼16 MeV (∼8 MeV per stage, at an average rate of ∼1 GeV m−1) was achieved at an optimal time delay, which allows synchronisation of the selected protons with the accelerating longitudinal electric fields to be maintained through both stages.

At the remote International Chemistry Olympiad 2022 hosted by China, two outstanding students from Switzerland won one bronze medal and one honorable mention. A joint remote participation to the event of the delegations from Germany, Austria, and Switzerland could be realized in Basel with the support of the University of Basel. The International Chemistry Olympiad 2023 will be hosted at ETH Zurich. This itinerary will mark the first time this annual event comes to Switzerland.

Engineered targets are expected to play a key role in future high-power laser experiments calling for joined, extensive knowledge in materials properties, engineering techniques and plasma physics. In this work, we propose a novel patterning procedure of self-supported 10 μm thick Au and Cu foils for obtaining micrometre-sized periodic gratings as targets for high-power laser applications. Accessible techniques were considered, by using cold rolling, electron-beam lithography and the Ar-ion milling process. The developed patterning procedure allows efficient control of the grating and foil surface on large area. Targets consisting of patterned regions of 450 μm × 450 μm, with 2 μm periodic gratings, were prepared on 25 mm × 25 mm Au and Cu free-standing foils, and preliminary investigations of the micro-targets interacting with an ultrashort, relativistic laser pulse were performed. These test experiments demonstrated that, in certain conditions, the micro-gratings show enhanced laser energy absorption and higher efficiency in accelerating charge particle beams compared with planar thin foils of similar thickness.

The shaping of astrophysical outflows into bright, dense, and collimated jets due to magnetic pressure is here investigated using laboratory experiments. Here we look at the impact on jet collimation of a misalignment between the outflow, as it stems from the source, and the magnetic field. For small misalignments, a magnetic nozzle forms and redirects the outflow in a collimated jet. For growing misalignments, this nozzle becomes increasingly asymmetric, disrupting jet formation. Our results thus suggest outflow/magnetic field misalignment to be a plausible key process regulating jet collimation in a variety of objects from our Sun’s outflows to extragalatic jets. Furthermore, they provide a possible interpretation for the observed structuring of astrophysical jets. Jet modulation could be interpreted as the signature of changes over time in the outflow/ambient field angle, and the change in the direction of the jet could be the signature of changes in the direction of the ambient field., Mass outflow is a common process in astrophysical objects. Here the authors investigate in which conditions an astrophysically-scaled laser-produced plasma flow can be collimated and evolves in the presence of a misaligned external magnetic field.

We study the laser-driven acceleration of electrons from overdense hydrogen clusters to energies of up to 13 MeV in laser forward direction and several hundreds of keV in an outer ring-structure. The use of cryogenic hydrogen allows for high repetition-rate operation and examination of the influence of source parameters like temperature and gas flow. The outer ring-structure of accelerated electrons, originating from the interaction, that is robust against the change of laser and target parameters can be observed for low electron densities of ca 3 × 1016 cm−3. For higher electron densities, an additional central spot of electrons in the laser forward direction can be observed. Utilizing 3D particle-in-cell simulations, it is revealed that both electron populations mainly stem from ponderomotive scattering.

Aims. Investigating the process of matter accretion onto forming stars through scaled experiments in the laboratory is important in order to better understand star and planetary system formation and evolution. Such experiments can indeed complement observations by providing access to the processes with spatial and temporal resolution. A previous investigation revealed the existence of a two-component stream: a hot shell surrounding a cooler inner stream. The shell was formed by matter laterally ejected upon impact and refocused by the local magnetic field. That laboratory investigation was limited to normal incidence impacts. However, in young stellar objects, the complex structure of magnetic fields causes variability of the incident angles of the accretion columns. This led us to undertake an investigation, using laboratory plasmas, of the consequence of having a slanted accretion impacting a young star. Methods. Here, we used high power laser interactions and strong magnetic field generation in the laboratory, complemented by numerical simulations, to study the asymmetry induced upon accretion structures when columns of matter impact the surface of young stars with an oblique angle. Results. Compared to the scenario where matter accretes perpendicularly to the star surface, we observe a strongly asymmetric plasma structure, strong lateral ejecta of matter, poor confinement of the accreted material, and reduced heating compared to the normal incidence case. Thus, slanted accretion is a configuration that seems to be capable of inducing perturbations of the chromosphere and hence possibly influencing the level of activity of the corona.

The process of high energy electron acceleration along the surface of grating targets (GTs) that were irradiated by a relativistic, high-contrast laser pulse at an intensity $I=2.5\times 10^{20}~\text{W}/\text{cm}^{2}$ was studied. Our experimental results demonstrate that for a GT with a periodicity twice the laser wavelength, the surface electron flux is more intense for a laser incidence angle that is larger compared to the resonance angle predicted by the linear model. An electron beam with a peak charge of ${\sim}2.7~\text{nC}/\text{sr}$ , for electrons with energies ${>}1.5~\text{MeV}$ , was measured. Numerical simulations carried out with parameters similar to the experimental conditions also show an enhanced electron flux at higher incidence angles depending on the preplasma scale length. A theoretical model that includes ponderomotive effects with more realistic initial preplasma conditions suggests that the laser-driven intensity and preformed plasma scale length are important for the acceleration process. The predictions closely match the experimental and computational results.

We present a study on laser-driven proton acceleration from a hydrogen cluster target. Aiming for the optimisation of the proton source, we performed a detailed parametric scan of the interaction conditions by varying different laser and the target parameters. While the underlying process of a Coulomb-explosion delivers moderate energies, in the range of 100 s of keV, the use of hydrogen as target material comes with the benefit of a debris-free, single-species proton acceleration scheme, enabling high repetition-rate experiments, which are very robust against shot-to-shot fluctuations.

By directing the laser-driven electromagnetic pulses along a helical path, one can achieve a travelling-field accelerator arrangement for simultaneous beam shaping and re-acceleration of laser-accelerated protons. The dynamics of guided acceleration of the transiting protons was studied by varying the length of the helical coil. Experimental data shows that the protons co-moving with the field region exhibit stronger focussing while increasing the coil length, with an increase of kinetic energy due to simultaneous post-acceleration. The net energy gain for a coil of constant pitch however saturates eventually when the post-accelerated protons overtakes the accelerating field region in due course. 3D particle tracing simulation underpins the dynamics of beam transport inside the coil, which highlights the requirement for a variable pitch coil geometry in order to sustain the post-acceleration over an extended coil.

The characteristics of laser driven proton beams can be efficiently controlled and optimised by employing a recently developed helical coil technique, which exploits the transient self-charging of solid targets irradiated by intense laser pulses. Here we demonstrate a well collimated (

The characteristics of laser driven proton beams can be efficiently controlled and optimised by employing a recently developed helical coil technique, which exploits the transient self-charging of solid targets irradiated by intense laser pulses. Here we demonstrate a well collimated (

A new type of proton acceleration stemming from large-scale gradients, low-density targets, irradiated by an intense near-infrared laser is observed. The produced protons are characterized by high-energies (with a broad spectrum), are emitted in a very directional manner, and the process is associated to relaxed laser (no need for high-contrast) and target (no need for ultra-thin or expensive targets) constraints. As such, this process appears quite effective compared to the standard and commonly used Target Normal Sheath Acceleration technique (TNSA), or more exploratory mechanisms like Radiation Pressure Acceleration (RPA). The data are underpinned by 3D numerical simulations which suggest that in these conditions a Low Density Collisionless Shock Acceleration (LDCSA) mechanism is at play, which combines an initial Collisionless Shock Acceleration (CSA) to a boost procured by a TNSA-like sheath field in the downward density ramp of the target, leading to an overall broad spectrum. Experiments performed at a laser intensity of 1020 W/cm2 show that LDCSA can accelerate, from ~1% critical density, mm-scale targets, up to 5 × 109 protons/MeV/sr/J with energies up to 45(±5) MeV in a collimated (~6° half-angle) manner.

Filamentary ionization tracks have been observed via optical probing inside Al-coated glass targets after the interaction of a picosecond 20-TW laser pulse at intensities above 10 19 W/cm 2. The tracks, up to 700 μm in length and between 10 and 20 μm in width, originate from the focal spot region of the laser beam. Simulations performed with 3D particle-in-cell and 2D Fokker-Planck hybrid codes indicate that the observations are consistent with ionization induced in the glass target by magnetized, collimated beams of high-energy electrons produced during the laser interaction.

The spatial and temporal evolution of spontaneous megagauss magnetic fields, generated during the interaction of a picosecond pulse with solid targets at irradiances above $5\ifmmode\times\else\texttimes\fi{}{10}^{18}\mathrm{W}/{\mathrm{cm}}^{2}$ have been measured using Faraday rotation with picosecond resolution. A high density plasma jet has been observed simultaneously with the magnetic fields by interferometry and optical emission. Two-dimensional magnetohydrodynamic simulations reproduced the main features of the experiment and showed that the jet formation is due to pinching by the magnetic fields.

Due to their particular properties, the beams of the multi-MeV protons generated during the interaction of ultraintense (I>10(19) W/cm(2)) short pulses with thin solid targets are most suited for use as a particle probe in laser-plasma experiments. The recently developed proton imaging technique employs the beams in a point-projection imaging scheme as a diagnostic tool for the detection of electric fields in laser-plasma interaction experiments. In recent investigations carried out at the Rutherford Appleton Laboratory (RAL, UK), a wide range of laser-plasma interaction conditions of relevance for inertial confinement fusion (ICF)/fast ignition has been explored. Among the results obtained will be discussed: the electric field distribution in laser-produced long-scale plasmas of ICF interest; the measurement of highly transient electric fields related to the generation and dynamics of hot electron currents following ultra-intense laser irradiation of targets; the observation in underdense plasmas, after the propagation of ultra-intense laser pulses, of structures identified as the remnants of solitons produced in the wake of the pulse.

A series of experiments recently carried out at the Rutherford Appleton Laboratory investigated various aspects of the laser–plasma interaction in the relativistic intensity regime. The propagation of laser pulses through preformed plasmas was studied at intensities exceeding 1019 W/cm2. The transmission of laser energy through long-scale underdense plasmas showed to be inefficient unless a plasma channel is preformed ahead of the main laser pulse. The study of the interaction with overdense plasmas yielded indication of collimated energy transport through the plasma. The production of fast particles during the interaction with solid density targets was also investigated. The measurements revealed the presence of a small-sized directional source of multi-megaelectron volt protons, which was not observed when a plasma was preformed at the back of the solid target. The properties of the source are promising in view of its use in radiographic imaging of dense matter, and preliminary tests were carried out.

Laser imprinting has been studied and, in particular, saturation of areal density perturbations induced by near single mode laser imprinting was observed. Several issues important for the foam buffered direct drive scheme have been investigated. These studies included measurements of the absolute levels of stimulated Brillouin and Raman scattering observed from laser irradiated low density foam targets, either bare or overcoated with a thin layer of gold. A novel scheme is proposed to increase the pressure in indirectly driven targets. By heating a foam supersonically that is attached to a solid target the pressure generated is not only the ablation pressure but also the combined pressure due to ablation at the foam-foil interface and the heated foam material. Planar brominated plastic foil targets overcoated with a low density foam were irradiated by a soft X ray pulse. The pressure was obtained by comparing the rear side trajectory of the driven target observed by soft X ray radiography with one dimensional radiation hydrodynamic simulations. Observations were also carried out of the transition from supersonic to subsonic propagation of an ionization front in low density chlorinated foam targets irradiated by an intense soft X ray pulse. The diagnostic for these measurements was K shell point projection absorption spectroscopy. In the fast ignitor area the channelling and guiding of picosecond laser pulses through underdense plasmas, preformed density channels and microtubes were investigated. It was observed that a large fraction of the incident laser energy can be propagated. Megagauss magnetic fields were measured, with a polarimetric technique, during and after propagation of intense picosecond pulses in preionized plasmas. Two types of toroidal fields, of opposite orientation, were detected. In addition, the production and propagation of an electron beam through solid glass targets irradiated at intensities above 1019W/cm2 were observed using optical probing techniques.

The absorption of subpicosecond uv laser pulses has been measured at intensities above ${10}^{17}{\mathrm{W}/\mathrm{c}\mathrm{m}}^{2}.$ High levels of absorption were observed, up to 55% for s polarization and 65% for p polarization. The behavior with angle of incidence and polarization can be interpreted as due to a combination of resonance and collisional absorption, taking place in a plasma with a scale length of the order of a fraction of the laser wavelength.

Ionization fronts have been observed in low density chlorinated foam targets and low density foams confined in gold tubes using time resolved K-shell absorption spectroscopy. The front was driven by an intense pulse of soft x-rays produced by high power laser irradiation. The density and temperature profiles inferred from the radiographs provided detailed measurement of the conditions. The experimental data were compared to radiation hydrodynamics simulations and reasonable agreement was obtained.

Measurements of self-channeling of picosecond laser pulses due to relativistic and ponderomotive expulsion effects have been obtained in preformed plasmas at laser irradiances between 5–9×1018 Wcm−2. The self-focused channel was surrounded by a multi-megagauss magnetic field. The orientation of the field was consistent with a forward going relativistic electron beam propagating along the laser pulse. Self-channeling and magnetic field generation mechanisms were modeled by multidimensional particle-in-cell (PIC) simulations and good agreement was obtained with the experimental observations. Measurements of the channel expansion after the interaction were obtained and the rate of expansion was consistent with a blast wave solution. The level of transmission of an intense laser pulse through such performed density channels was observed to increase significantly compared to the case without a channel. High levels of transmission of an intense laser pulse through microtubes were also observed. The relevance of...

Transonic ionization fronts have been observed in low-density chlorinated foam targets using time-resolved $K$-shell absorption spectroscopy. The front was driven by an intense pulse of soft x rays produced by high-power laser irradiation of a thin foil. The density and temperature profiles inferred from the radiographs provided detailed measurement of the conditions at a number of times. The experimental data were compared to radiation hydrodynamics simulations and reasonable agreement was obtained.

The fast ignitor scheme consists of three stages and relies on ignition of a part of the compressed fusion fuel of an inertialconfinement fusion capsule by an external trigger. A conventional fusio...

Two spatially separated toroidal magnetic fields in the megagauss range have been detected with Faraday rotation during and after propagation of a relativistically intense laser pulse through preionized plasmas. Besides a field in the outer region of the plasma oriented as a conventional thermoelectric field, a field with the opposite orientation closely surrounding the propagation axis is observed, in conditions under which relativistic channeling occurs. A 3D particle-in-cell code was used to simulate the interaction under the conditions of the experiment.

Efficient guiding of 1-ps infrared laser pulses with power exceeding 10 TW has been demonstrated through hollow capillary tubes with 40- and 100-\ensuremath{\mu}m internal diameters and lengths up to 10 mm, with transmission greater than 80% of the incident energy coupled into the capillary. The beam is guided via multiple reflections off a plasma formed on the walls of the guide by the pulse's rising edge, as inferred from optical probe measurements.

The interaction of short (1−2 ps) laser pulses with solid targets at irradiances of over 1016 Wcm−2, in the presence of a substantial prepulse has been investigated. High absorption of laser energy is found even at high angles of incidence, with evidence for a resonance absorption peak being found for S, P, and circular polarizations. It is considered that this may be a result of refraction and beam filamentation, which causes loss of distinct polarization. Measurements of hard X-ray emission (∼ 100 keV) confirm a resonance absorption type peak at 45−50°, again for all three cases. Typically, 5−15% of the incident light is back-reflected by stimulated Brillouin scatter, with spatially resolved spectra showing evidence of beam hot-spots at high intensity. The possibility that filamentation and refraction of the beam can explain the lack of polarization dependence in the absorption and hard X-ray emission data is discussed.

Recent experiments have shown that low density foam layers can significantly mitigate the perturbing effects of beam nonuniformities affecting the acceleration of thin shells. This problem is studied parametrically with two-dimensional LASNEX [G. B. Zimmerman and W. L. Kruer, Comments Plasma Phys. Controlled Fusion 2, 51 (1975)]. Foam-buffered targets are employed, consisting typically of 250 A of gold, and 50 μm of 50 mg/cm3 C10H8O4 foam attached to a 10 μm foil. In simulation these were characteristically exposed to 1.2 ns, flat-topped green light pulses at 1.4×1014 W/cm2 intensity, bearing 30 μm lateral perturbations of up to 60% variation in intensity. Without the buffer layers the foils were severely disrupted by 1 ns. With buffering only minimal distortion was manifest at 3 ns. The smoothing is shown to derive principally from the high thermal conductivity of the heated foam. The simulation results imply that (1) the foam thickness should exceed the disturbance wavelength; (2) intensities exceeding ...

Creation of a low density, high temperature plasma buffer between the absorption and ablation layers of a directly driven inertial confinement fusion implosion capsule has been proposed as a means to reduce “early time” imprint from laser nonuniformities. This thermal smoothing blanket might be created from a low density foam layer wrapped around the deuterium–tritium filled microballoon. Preliminary spherical implosion tests of this concept using a polystyrene foam layer surrounding a glass microballoon were performed at the Nova laser [Rev. Sci. Instrum. 57, 2101 (1986)], using a 527 nm drive wavelength. Comparison of capsule yield and imploded core symmetry showed promising improvements in overall target performance, relative to one-dimensional undegraded hydrodynamic simulations, when the foam-buffer layer was present.

Laser driven shock waves propagating through foam targets have been diagnosed by side-on time-resolved x-ray absorption spectroscopy. K-shell absorption spectra of chlorine, doped into the foam targets, were matched to a detailed atomic physics model to infer the temperature profile. The density distribution was obtained from the x-ray transmission through the target. 2D radiation-hydrodynamic modeling of the targets reproduced the experimental results. Preheating of material by radiation from the shocked region was shown to have an important contribution to the measured temperature profile.

Relativistic self-channeling of a picosecond laser pulse in a preformed plasma near critical density has been observed both experimentally and in 3D particle-in-cell simulations. Optical probing measurements indicate the formation of a single pulsating propagation channel, typically of about 5{mu}m in diameter. The computational results reveal the importance in the channel formation of relativistic electrons traveling with the light pulse and of the corresponding self-generated magnetic field. {copyright} {ital 1997} {ital The American Physical Society}

A novel x-ray imaging system based on a microchannel-plate combined with a multi-pinhole camera has been employed to study x-ray emission from laser-produced plasmas in the 0.5–3 keV photon energy range. In particular, the interaction of intense laser radiation with such plasmas, under conditions relevant to inertial confinement fusion, was monitored by recording a sequence of consecutive x-ray images with a temporal resolution of 140 ps and a spatial resolution of 10 μm. These images provide valuable information on the main physical mechanisms involved in the interaction process, including collisional absorption of the incident laser energy and electron thermal conduction.

A quantitative study of refractive whole beam defocusing and small scale breakup induced by optical ionization of subpicosecond and picosecond, 0.25 and 1 {mu}m, laser pulses in gas-jet targets at densities above 1{times}10{sup 19} cm{sup {minus}3} has been carried out. A significant reduction of the incident laser intensity was observed due to refraction from ionization-induced density gradients. The level of refraction measured with optical probing correlated well with the fraction of energy transmitted through the plasma. The numerical and analytical models were found to agree well with experimental observations. {copyright} {ital 1996 The American Physical Society.}