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Fallout from atmospheric nuclear tests, especially from those conducted at the Pacific Proving Grounds between 1946 and 1958, contaminated areas of the Northern Marshall Islands. A radiological survey at some Northern Marshall Islands was conducted from September through November 1978 to evaluate the extent of residual radioactive contamination. The atolls included in the Northern Marshall Islands RadiologicalSurvey (NMIRS) were Likiep, Ailuk, Utirik, Wotho, Ujelang, Taka, Rongelap, Rongerik, Bikar, Ailinginae, and Mejit and Jemo Islands. The original test sites, Bikini and Enewetak Atolls, were also visited on the survey. An aerial survey was conducted to determine the external gamma exposure rate. Terrestrial (soil, food crops, animals, and native vegetation), cistern and well water samples, and marine (sediment,seawater, fish and clams) samples were collected to evaluate radionuclide concentrations in the atoll environment. Samples were processedand analyzed for 137Cs, 90Sr, 239+240Pu and 241Am. The dose from the ingestion pathway was calculated using the radionuclide concentration data and a diet model for local food, marine, and water consumption. The ingestion pathway contributes 70% to 90% of the estimated dose. Approximately 95% of thedose is from 137Cs. 90Sr is the second most significant radionuclide via ingestion. External gamma exposure from 137Cs accounts for about 10% to 30% of the dose.239+240Pu and 241Am are the major contributors to dose via the inhalation pathway; however, inhalation accounts for only about 1% of the total estimated dose, based on surface soil levels and resuspension studies. All doses are computed for concentrations decay corrected to 1996. The maximum annual effective dose from manmade radionuclides at these atolls ranges from.02 mSv y-1 to 2.1 mSv y-1. The background dose in the Marshall Islands is estimated t [ABSTRACT FROM AUTHOR]

Between June 1946 and October 1958, Enewetak and Bikini Atolls were used by the US as testing grounds for 66 nuclear devices. The combined explosive yield from these tests was 107 million t (million t TNT equivalents). This testing produced close-in fallout debris that was contaminated with quantities of radioactive fission and particle activated products, and unspent radioactive nuclear fuel that entered the aquatic environment of the atolls. Today, the sediments in the lagoons are reservoirs for tens of TBq of the transuranics and some long-lived fission and activation products. The larger amounts of contamination are associated with fine and coarse sediment material adjacent to the locations of the high yield explosions. Radionuclides are also distributed vertically in the sediment column to various depths in all regions of the lagoons. Concentrations greater than fallout background levels are found in filtered water sampled over several decades from all locations and depths in the lagoons. This is a direct indication that the radionuclides are continuously mobilized to solution from the solid phases. Of particular importance is the fact that the long-lived radionuclides are accumulated to different levels by indigenous aquatic plants and organisms that are used as food by resident people. One might anticipate finding continuous high contamination levels in many of the edible marine organisms from the lagoons, since the radionuclides associated with the sediments are not contained and are available to the different organisms in a relatively shallow water environment. This is not the case. We estimate that the radiological dose from consumption of the edible parts of marine foods at Enewetak and Bikini is presently approximately 0.05% of the total 50-year integral effective dose from all other exposure pathways that include ingestion of terrestrial foods and drinking water, external exposure and inhalation. The total radiological dose from the marine pathway is dominated by the natural radionuclides, 210Po and 210Pb. Man-made radionuclides presently contribute < 0.3% of the dose from these natural radionuclides in the marine food chain and within approximately 90 years only 0.15%.

The 43 nuclear tests conducted at Enewetak Atoll by the United States between 1948 and 1958 produced close-in fallout that contaminated the islands and lagoon of the atoll with radioactive fission and activation products, and unfissioned nuclear fuel. In 1972, the U.S. government announced that it would conduct a cleanup and restoration operation to return the atoll to the Enewetak people. The radiological cleanup began in 1977 and lasted to 1980 and focused on reducing the concentration of the transuranium elements (238,239,240Pu and 241Am = TRU) in soils on some of the islands that might eventually be used for residence or for subsistence agricultural. The cleanup plan called for relocating soil and some other contaminated debris to Runit Island on the eastern perimeter of the Atoll. Some of the contaminated soil was mixed with cement and the mixture placed below the water level in the Cactus Crater that was formed by a nuclear explosion in 1958. The remainder of the contaminated material was mixed with concrete and placed above ground over the crater in the shape of a dome. A concrete cap was constructed over the dome of soil. Concern has been expressed by the people of Enewetak and by others over the possible aquatic impacts from the radionuclides entombed in the crater. A National Academy of Sciences committee examined the dome and concluded that the containment structure and its contents present no credible health hazard to the people of Enewetak, either now or in the future. The committee suggested that "at least part of the radioactivity contained in the structure is available for transport to the groundwater and subsequently to the lagoon and it is important to determine whether this pathway may be a significant one." Therefore, a surveillance program was started in 1980, in conjunction with other research efforts, to study the radionuclides in samples of fish, groundwater, and lagoon seawater. Our data and conclusions support the findings suggested by the National Academy committee over a decade ago in that any assumption of rapid remobilization of all or any of the dome's transuranics or other radionuclides is an extreme one. Any fear that this structure contains amounts of activity whose release would cause damage to the environment that will result in greater effect on human health is unfounded.

The concentrations of 210Po and 210Pb have been determined in many local foods consumed by societies residing on different atolls in the Marshall Islands. The average daily intake of these two naturally occurring radionuclides from local and imported food is estimated to be 2.18 and 0.36 Bq, respectively. Local foods contribute 87% of the 210Po and 47% of the 210Pb associated with the diet. The items contributing the majority of the activity to the diet are derived from the marine environment and include parts of fish, invertebrates, seabirds and eggs of seabirds. The committed effective dose from ingestion of 210Po and 210Pb is approximately 2 mSv/year (200 mrem/year). This pathway now contributes 83% of the natural background irradiation received by residents in the Marshall Islands. Because the naturally occurring radionuclides are omnipresent in terrestrial and marine foods at all atolls, the annual intake and computed dose can be considered as typical values for individuals with comparable diets and inhabiting other islands in the Pacific.

The elution first of calcium and then of strontium by complex formation with cyclohexanediaminetetra-acetic acid (CyDTA) after sorption on ion-exchange columns, is shown to require careful control of pH and the concentrations of CyDTA and NH(4)(+). A procedure is described for volumetric analysis of calcium and strontium, and for use of this separation procedure before determination of (90)Sr in sea-water. Careful choice of reagents and materials is shown to be necessary for use of such a method in determination of trace amounts of radiostrontium.