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YbCu4Au is a unique material exhibiting multiple quantum fluctuations simultaneously. In this study, we investigated the field-induced criticality in YbCu4Au, based on comprehensive micro and macro measurements, including powder X-ray diffraction (XRD), neutron powder diffraction (NPD), nuclear magnetic resonance, magnetization, resistivity, specific heat, muon spin rotation relaxation (muSR), and X-ray absorption spectroscopy (XAS). Single crystals of YbCu4Au were grown, and their crystal structure was determined using XRD, and NPD measurements. Magnetic successive transitions were observed below 1 T by specific heat, resistivity, NPD, and muSR measurements. XAS measurements further indicate that the valence of Yb ions (+2.93) remained unchanged above 2 T. Moreover, the change in quadrupole frequency observed in the previous study is attributable to the electric quadrupole, as the expected value of the electric quadrupole was finite under magnetic fields [S. Wada et al., Journal of Physics: Condensed Matter, 20, 175201 (2008).]. These experimental results suggest that YbCu4Au exhibited bicritical behavior near 1 T, arising from the competition between RKKY interaction, accounting for the magnetic phases, and the Zeeman effect., Comment: 9 pages, 8 figures

Magnetic structures of the noncentrosymmetric magnet Sr$_2$MnSi$_2$O$_7$ were examined through neutron diffraction for powder and single-crystalline samples, as well as magnetometry measurements. All allowed magnetic structures under the space group $P\bar{4}2_1 m$ with the magnetic wavevector $\vec{q}_{\rm m}=(0,0,1/2)$~r.l.u., were analysed via irreducible representation and magnetic space group approaches. The compound is refined to have in-plane magnetic moments within the magnetic space group $Cmc2_1.1^{\prime}_c$ (\#36.177) under zero field, which can be altered to $P2_1 2_1 2_1.1^{\prime}_c$ (\#19.28) above $\mu_0 H=0.067(5)$~T to align induced weak-ferromagnetic components within one layer on the $ab$-plane. All refined parameters are provided following the recent framework based upon the magnetic space group, which better conveys when exchanging crystallographic information for commensurate magnetic structures., Comment: 7 pages, 4 figures

Lattice formation of swirling textures is ubiquitous in solid-state materials, such as a magnetic skyrmion lattice in chiral magnets. In the magnetic skyrmion lattices, their moving states and dynamics under external perturbations are still unrevealed, although a detailed understanding of the dynamics is crucial to realizing spintronic applications, such as magnetic domain-wall racetrack memory. Here, we report in detail on the transient state of a moving magnetic skyrmion lattice in bulk single-crystalline MnSi under alternating current (AC) using small-angle neutron scattering. A rotation and concomitant broadening of the spot width in the azimuthal direction of the magnetic skyrmion reflections originating from the plastic deformation of the magnetic skyrmion lattice were found only at low AC frequencies, whereas above the threshold AC frequency (ft ~ 0.12 Hz) the rotation was not observed, and the spot width becomes sharper. The observed complex response of the magnetic skyrmion reflections can be explained by the change in dislocation density in the magnetic skyrmion lattice. At frequencies higher than ft, the magnetic skyrmions oscillate removing the dislocations, indicating that the dislocation density is controlled by the AC frequency., Comment: 13 pages, 10 figures

Magnon spin currents in the ferrimagnetic garnet Tb3Fe5O12 with 4f electrons were examined through the spin-Seebeck effect and neutron scattering measurements. The compound shows a magnetic compensation, where the spin-Seebeck signal reverses above and below Tcomp = 249.5(4) K. Unpolarized neutron scattering unveils two major magnon branches with finite energy gaps, which are well-explained in the framework of spin-wave theory. Their temperature dependencies and the direction of the precession motion of magnetic moments, i.e. magnon polarization, defined using polarized neutrons, explain the reversal at Tcomp and decay of the spin-Seebeck signals at low temperatures. We illustrate an example that momentum- and energy-resolved microscopic information is a prerequisite to understanding the magnon spin current., Comment: 7 pages, 5 figures

We demonstrate field-induced single-ion magnetic anisotropy resulting from the multiorbital Kondo effect on the diluted ytterbium alloy $(\mathrm{Lu}_{1-x}\mathrm{Yb}_x)\mathrm{Rh}_2\mathrm{Zn}_{20}$. Single-ion anisotropic metamagnetic behavior is revealed in low-temperature regions where the local Fermi-liquid state is formed. Specific hea, low-field magnetic susceptibility, and resistivity indicate reproduction of the ground-state properties by the $\mathrm{SU}(N = 8)$ Kondo model with a relatively large $c$-$f$ hybridization of $T_{\mathrm{K}} = 60.9 \ \mathrm{K}$. Dynamical susceptibility measurements on $\mathrm{Yb}\mathrm{Rh}_2\mathrm{Zn}_{20}$ support realizing the multiorbital Kondo ground state in $(\mathrm{Lu}_{1-x}\mathrm{Yb}_x)\mathrm{Rh}_2\mathrm{Zn}_{20}$. The single-ion magnetic anisotropy becomes evident above $\sim5 \ \mathrm{T}$, which is lower than the isotropic Kondo crossover field of 22.7 T, verifying blurred low-lying crystal field states through the multiorbital Kondo effect., Comment: 14 pages, 12 figures, 6 pages of supplementary material

Spin dynamics of the spin-1/2 kagome lattice antiferromagnet Cs$_2$Cu$_3$SnF$_{12}$ was studied using high-resolution, time-of-flight inelastic neutron scattering. The flat mode, a characteristic of the frustrated kagome antiferromagnet, and the low-energy dispersive mode, which is dominated by magnons, can be well described by the linear spin-wave theory. However, the theory fails to describe three weakly dispersive modes between 9 and 14 meV. These modes could be attributed to two-spinon bound states, which decay into free spinons away from the zone center and at a high temperature, giving rise to continuum scattering., Comment: 4 figures and Supplementary Information

Quest for new states of matter near an ordered phase is a promising route for making modern physics forward. By probing thermal properties of a ferroelectric (FE) crystal Ba1-xSrxAl2O4, we have clarified that low-energy excitation of acoustic phonons is remarkably enhanced with critical behavior at the border of the FE phase. The phonon spectrum is significantly damped toward the FE phase boundary and transforms into glasslike phonon excitation which is reminiscent of a boson peak. This system thus links long-standing issues of amorphous solids and structural instability in crystals to pave the way to controlling lattice fluctuation as a new tuning parameter., Comment: 6 pages, 4 figures

We measure the mode-resolved direction of the precessional motion of the magnetic order, i.e., magnon polarization, via the chiral term of inelastic polarized neutron scattering spectra. The magnon polarisation is important in spintronics, affecting thermodynamic properties such as the magnitude and sign of the spin Seebeck effect. The observation of both signs of magnon polarization in Y3Fe5O12 also gives direct proof of its ferrimagnetic nature. The experiments agree very well with atomistic simulations of the scattering cross section., Comment: 6 pages, 4 figures

High-resolution time-of-flight powder neutron diffraction and high-field magnetization were measured to investigate the magnetic structure and existence of a field-induced magnetic phase transition in the distorted kagome antiferromagnet Cs$_2$Cu$_3$SnF$_{12}$. Upon cooling from room temperature, the compound undergoes a structural phase transition at $T_\textrm{t}=185$ K from the rhombohedral space group $R\bar{3}m$ with the perfect kagome spin network to the monoclinic space group $P2_1/n$ with the distorted kagome planes. The distortion results in three inequivalent exchange interactions among the $S=1/2$ Cu$^{2+}$ spins that magnetically order below $T_\textrm{N}=20.2$ K. Magnetization measured with a magnetic field applied within the kagome plane reveals small in-plane ferromagnetism resulting from spin canting. On the other hand, the out-of-plane magnetization does not show a clear hysteresis loop of the ferromagnetic component nor a prominent anomaly up to 170 T, with the exception of the subtle knee-like bend around 90 T, which could indicate the 1/3 magnetization plateau. The combined analysis using the irreducible representations of the magnetic space groups and magnetic structure refinement on the neutron powder diffraction data suggests that the magnetic moments order in the magnetic space group $P2_1'/n'$ with the all-in-all-out spin structure, which by symmetry allows for the in-plane canting, consistent with the in-plane ferromagnetism observed in the magnetization., Comment: 14 pages, 9 figures, published version with typos corrected

Using small-angle neutron scattering (SANS), we investigate the deformation of the magnetic skyrmion lattice in bulk single-crystalline MnSi under electric current flow. A significant broadening of the skyrmion-lattice-reflection peaks was observed in the SANS pattern for current densities greater than a threshold value j_t ~ 1 MA/m^2 (10^6 A/m^2). We show this peak broadening to originate from a spatially inhomogeneous rotation of the skyrmion lattice, with an inverse rotation sense observed for opposite sample edges aligned with the direction of current flow. The peak broadening (and the corresponding skyrmion lattice rotations) remain finite even after switching off the electric current. These results indicate that skyrmion lattices under current flow experience significant friction near the sample edges, and plastic deformation due to pinning effects, these being important factors that must be considered for the anticipated skyrmion-based applications in chiral magnets at the nanoscale.

Antiferromagnetic spin fluctuations were investigated in the normal states of the parent ($x = 0$), under-doped ($x = 0.04$) and optimally-doped ($x = 0.06$) Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ single crystals using inelastic neutron scattering technique. For all the doping levels, quasi-two-dimensional antiferromagnetic fluctuations were observed as a broad peak localized at ${\it Q} = (1/2, 1/2, l)$. At lower energies, the peak shows an apparent anisotropy in the $hk0$ plane; longitudinal peak widths are considerably smaller than transverse widths. The anisotropy is larger for the higher doping level. These results are consistent with the random phase approximation (RPA) calculations taking account of the orbital character of the electronic bands, confirming that the anisotropic nature of the spin fluctuations in the normal states is mostly dominated by the nesting of Fermi surfaces. On the other hand, the quasi-two-dimensional spin correlations grow much rapidly for decreasing temperature in the $x = 0$ parent compound, compared to that expected for nearly antiferromagnetic metals. This may be another sign of the unconventional nature of the antiferromagnetic transition in BaFe$_2$As$_2$., Comment: 9 pages, 6 figures

Magnetic excitations in the spin-$\frac{1}{2}$ distorted kagome lattice antiferromagnet Cs$_2$Cu$_3$SnF$_{12}$, which has an ordered ground state owing to the strong Dzyaloshinskii-Moriya interaction, were studied using inelastic neutron scattering. Although the spin-wave dispersion can be qualitatively understood in terms of linear spin-wave theory (LSWT), the excitation energies are renormalized by a factor of approximately 0.6 from those calculated by LSWT, almost irrespective of the momentum transfer. This inadequacy of LSWT, which is attributed to quantum fluctuations, provides evidence of negative quantum renormalization in the spin-$\frac{1}{2}$ kagome lattice antiferromagnet., Comment: 8 pages, 6 figures, including Supplemental Materials

High intensity pulsed neutron scattering reveals a new set of magnetic excitations in the pinwheel valence bond solid state of the distorted kagome lattice antiferromagnet Rb$_2$Cu$_3$SnF$_{12}$. The polarization of the dominant dispersive modes (2 meV $<\hbar\omega< $7 meV) is determined and found consistent with a dimer series expansion with strong Dzyaloshinskii-Moriya interactions ($D/J=0.18$). A weakly dispersive mode near 5 meV and shifted "ghosts" of the main modes are attributed to the enlarged unit cell below a $T=215$ K structural transition. Continuum scattering between 8 meV and 10 meV might be interpreted as a remnant of the kagome spinon continuum [T.-H. Han et al., Nature 492, 406 (2012)], Comment: 7 pages, 5 figures

We report a comprehensive study of dc susceptibility, specific heat, neutron diffraction, and inelastic neutron scattering measurements on polycrystalline Ba3(Cr1-xVx)2O8 samples, where x=0, 0.06, 0.15, and 0.53. A Jahn-Teller structure transition occurs for x=0, 0.06, and 0.15 samples and the transition temperature is reduced upon vanadium substitution from 70(2) K at x=0 to 60(2) K at x=0.06 and 0.15. The structure becomes less distorted as x increases and such transition disappears at x=0.53. The observed magnetic excitation spectrum indicates that the singlet ground state remains unaltered and spin gap energy \Delta=1.3(1) meV is identical within the instrument resolution for all x. In addition, the dispersion bandwidth W decreases with increase of x. At x=0.53, W is reduced to 1.4(1) meV from 2.0(1) meV at x=0., Comment: 11 pages, 7 figures, some typos are corrected

Magnetic susceptibility and muon spin relaxation (muSR) experiments have been carried out on the quasi-2D triangular-lattice spin S = 2 antiferromagnet FeGa2S4. The muSR data indicate a sharp onset of a frozen or nearly-frozen spin state at T* = 31(2) K, twice the spin-glass-like freezing temperature T_f = 16(1) K. The susceptibility becomes field dependent below T*, but no sharp anomaly is observed in any bulk property. A similar transition is observed in muSR data from the spin-1 isomorph NiGa2S4. In both compounds the dynamic muon spin relaxation rate lambda_d(T) above T* agrees well with a calculation of spin-lattice relaxation by Chubukov, Sachdev, and Senthil in the renormalized classical regime of a 2D frustrated quantum antiferromagnet. There is no firm evidence for other mechanisms. At low temperatures lambda_d(T) becomes temperature independent in both compounds, indicating persistence of spin dynamics. Scaling of lambda_d(T) between the two compounds is observed from ~T_f to ~1.5T*. Although the muSR data by themselves cannot exclude a truly static spin component below T*, together with the susceptibility data they are consistent with a slowly-fluctuating "spin gel" regime between T_f and T*. Such a regime and the absence of a divergence in lambda_d(T) at T* are features of two unconventional mechanisms: (1) binding/unbinding of Z_2 vortex excitations, and (2) impurity spins in a nonmagnetic spin-nematic ground state. The absence of a sharp anomaly or history dependence at T* in the susceptibility of FeGa2S4, and the weakness of such phenomena in NiGa2S4, strongly suggest transitions to low-temperature phases with unconventional dynamics., Comment: 13 pages, 6 figures, accepted for publication in Physical Review B

We report positive muon spin relaxation measurements on the triangular lattice magnetic system FeGa2S4. A magnetic transition not previously detected by specific heat and magnetic susceptibility measurements is found in zero field at T^* \simeq 30 K. It is observed through the temperature dependencies of the signal amplitude and the spin-lattice relaxation rate. This transition is therefore not a conventional magnetic phase transition. Since persistent spin dynamics is observed down to 0.1 K, the ground state cannot be of the canonical spin-glass type, which could be suggested from hysteresis effects in the bulk susceptibility below T_f \simeq 16 K. These results are compared to those found for the isomorph NiGa2S4. It is argued that the fate of the transition, which has been interpreted in terms of the Z_2 topological transition in this latter system, is probably different in FeGa2S4., Comment: 5 pages, 3 figures

A novel secure communication network with quantum key distribution in a metropolitan area is reported. Different QKD schemes are integrated to demonstrate secure TV conferencing over a distance of 45km, stable long-term operation, and application to secure mobile phones., Comment: 21 pages, 19 figures

Neutron scattering is used to investigate spin correlations in ultra pure single crystals of the S=1 triangular lattice NiGa2S4. Despite a Curie-Weiss temperature of Theta_CW=-80(2) K, static (tau > 1 ns) short range (xi_ab=26(3) \AA) incommensurate order prevails for T>1.5 K. The incommensurate modulation Q_0=(0.155(3),0.155(3),0), Theta_CW, and the spin wave velocity (c=4400 m/s) can be accounted for by antiferromagnetic third-nearest neighbor interactions J_3=2.8(6) meV and ferromagnetic nearest neighbor coupling J_1=-0.35(9) J_3. Inter-plane correlations are limited to nearest neighbors and weakened by an in-plane field. These observations show that the short range ordered glassy phase that has been observed in a number of highly degenerate systems, can persist near the clean limit., Comment: 4 pages, 4 figures, to be published in Physical Review Letters

We report on the experimental demonstration of a source of hybrid entanglement pairs between two different degrees of freedom, a 1550 nm time-bin qubit and an 810 nm polarization qubit. The polarization qubit at 810 nm is transformed by an asymmetric Mach-Zehnder interferometer consisted of a Glan laser prism and a polarization-maintaining fiber. We obtained visibilities of 95.8% and 88% along Z-Z and X-X axes on the Poincare sphere, respectively with a coincidence count rate of more than 800 c/s after entanglement format transformation. These values are well above the threshold of 70.7% needed to violate a Bell inequality and allow distilling a secure key in the quantum key distribution., Comment: 11pages, 4 figures

Muon spin rotation (muSR) experiments reveal unconventional spin freezing and dynamics in the two-dimensional (2D) triangular lattice antiferromagnet NiGa2S4. Long-lived disordered Ni-spin freezing (correlation time > 10-6 s at 2 K) sets in below T_f = 8.5 +- 0.5 K with a mean-field-like temperature dependence. The observed exponential temperature dependence of the muon spin relaxation above T_f is strong evidence for 2D critical spin fluctuations. Slow Ni spin fluctuations coexist with quasistatic magnetism at low temperatures but are rapidly suppressed for fields > 10 mT, in marked contrast with the field-independent specific heat. The muSR and bulk susceptibility data indicate a well-defined 2D phase transition at T_f, below which NiGa2S4 is neither a conventional magnet nor a singlet spin liquid., Comment: 5 pages, 4 figures, to be published in Phys. Rev. B

In this Letter, we report the results of ESR measurements in high magnetic fields up to about 53 T on single crystals of NiGa2S4 to clarify the spin dynamics in more detail. We have found that the dynamics of Z2 vortices affects the temperature dependence of the ESR absorption linewidth and the frequency dependence of the ESR resonance fields at 1.3 K is well explained by a conventional spin wave theory. These results suggest an occurrence of Z2 vortex-induced topological transition., Comment: 5 pages, 3 figures

We have performed $^{69,71}$Ga nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) and muon spin rotation/resonance on the quasi two-dimensional antiferromagnet (AFM) NiGa$_2$S$_4$, in order to investigate its spin dynamics and magnetic state at low temperatures. Although there exists only one crystallographic site for Ga in NiGa$_2$S$_4$, we found two distinct Ga signals by NMR and NQR. The origin of the two Ga signals is not fully understood, but possibly due to stacking faults along the c axis which induce additional broad Ga NMR and NQR signals with different local symmetries. We found the novel spin freezing occurring at $T_{\rm f}$, at which the specific heat shows a maximum, from a clear divergent behavior of the nuclear spin-lattice relaxation rate $1/T_{1}$ and nuclear spin-spin relaxation rate $1/T_{2}$ measured by Ga-NQR as well as the muon spin relaxation rate $\lambda$. The main sharp NQR peaks exhibit a stronger tendency of divergence, compared with the weak broader spectral peaks, indicating that the spin freezing is intrinsic in NiGa$_2$S$_4$. The behavior of these relaxation rates strongly suggests that the Ni spin fluctuations slow down towards $T_{\rm f}$, and the temperature range of the divergence is anomalously wider than that in a conventional magnetic ordering. A broad structureless spectrum and multi-component $T_1$ were observed below 2 K, indicating that a static magnetic state with incommensurate magnetic correlations or inhomogeneously distributed moments is realized at low temperatures. However, the wide temperature region between 2 K and $T_{\rm f}$, where the NQR signal was not observed, suggests that the Ni spins do not freeze immediately below $T_{\rm f}$, but keep fluctuating down to 2 K with the MHz frequency range., Comment: 14 pages, 14 figures. To appear in Phys. Rev. B

We have studied the electronic structure of the Ni triangular lattice in NiGa$_2$S$_4$ using photoemission spectroscopy and subsequent model calculations. The cluster-model analysis of the Ni 2$p$ core-level spectrum shows that the S 3$p$ to Ni 3$d$ charge-transfer energy is $\sim$ -1 eV and the ground state is dominated by the $d^9L$ configuration ($L$ is a S 3$p$ hole). Cell perturbation analysis for the NiS$_2$ triangular lattice indicates that the strong S 3$p$ hole character of the ground state provides the enhanced superexchange interaction between the third nearest neighbor sites., Comment: 10 pages, 5 figures, accepted to PRL

A numerical simulation of fluid flows in a Laval nozzle is performed to observe formations of acoustic black holes and the classical counterpart to Hawking radiation under a realistic setting of the laboratory experiment. We determined the Hawking temperature of the acoustic black hole from obtained numerical data. Some noteworthy points in analyzing the experimental data are clarified through our numerical simulation., Comment: 26 pages, published version

We report the generation of polarization-entangled photons by femtosecond-pulse-pumped spontaneous parametric down-conversion in a cascade of two type-I crystals. Highly entangled pulsed states were obtained by introducing a temporal delay between the two orthogonal polarization components of the pump field. They exhibited high-visibility quantum interference and a large concurrence value, without the need of post-selection using narrow-bandwidth-spectral filters. The results are well explained by the theory which incorporates the space-time dependence of interfering two-photon amplitudes if dispersion and birefringence in the crystals are appropriately taken into account. Such a pulsed entangled photon well localized in time domain is useful for various quantum communication experiments, such as quantum cryptography and quantum teleportation., Comment: 12 pages, 11 figures, REVTEX

We experimentally demonstrate that entanglement of bi-photon polarization state can be restored by spectral filters. This restoration procedure can be viewed as a new class of quantum eraser, which retrieves entanglement rather than just interference by manipulating an ancillary degree of freedom., Comment: 4 pages, 4 figures

Quantum mechanical complementarity ensures the security of the key-distribution scheme reported by Brassard and Bennet in 1984 (BB84), but does not prohibit use of multi-photons as a signal carrier. We describe a novel BB84 scheme in which two nearly orthogonal coherent states carry the key, and the superposition of these states (cat states) protects the communication channel from eavesdropping. Information leakage to eavesdroppers can be determined from the visibility of the interferential fringes in the distribution of the outcome when a certain quadrature component is measured through homodyne detection. The effect of channel loss and detector inefficiency is discussed., Comment: 20 pages, 4 figures, RevTeX, submitted to PRA, Revised 2000/2/23

We investigate the cosmological perturbation of two-scalar field model during the reheating phase after inflation. Using the exact solution of the perturbation in long-wavelength limit, which is expressed in terms of the background quantities, we analyze the behavior of the metric perturbation. The oscillating inflaton field gives rise to the parametric resonance of the massless scalar field and this leads to the amplification of the iso-curvature mode of the metric perturbations., Comment: 13 pages, 2 Encapsulated Postscript figures, revtex, references are added and type miss is corrected