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We observe the dissipative dynamics of a dense, strongly interacting gas of bosonic atom pairs in an optical lattice, controlling the strength of the two-body interactions over a wide parameter regime. We study how three-body losses contribute to the lattice dynamics, addressing a number of open questions related to the effects of strong dissipation in a many-body system, including the relationship to the continuous quantum Zeno effect. We observe rapid break-up of bound pairs for weak interactions, and for stronger interactions we see doublon decay rates that are asymmetric when changing from attractive and repulsive interactions, and which strongly depend on the interactions and on-site loss rates. By comparing our experimental data with a theoretical analysis of few-body dynamics, we show that these features originate from a non-trivial combination of dissipative dynamics described by a lattice model beyond a standard Bose-Hubbard Hamiltonian, and the modification of three-atom dynamics on a single site, which is generated alongside strong three-body loss. Our results open new possibilities for investigating bosonic atoms with strong three-body loss features, and allow for the better understanding of the parameter regimes that are required to realize strong effective three-body interactions., Comment: 8 pages, 4 figures

A model for determining the hyperfine structure of the excited electronic states of diatomic bialkali heteronuclear molecules is formulated from the atomic hyperfine interactions, and is applied to the case of bosonic $^{39}$KCs and fermionic $^{40}$KCs molecules. The hyperfine structure of the potential energy curves of the states correlated to the K($4s\,^2S_{1/2}$)+Cs($6p\,^2P_{1/2,3/2}$) dissociation limits is described in terms of different coupling schemes depending on the internuclear distance $R$. These results provide the first step in the calculation of the hyperfine structure of rovibrational levels of these excited molecular states in the perspective of the identification of efficient paths for creating ultracold ground-state KCs molecules., Comment: 12 pages, 15 figures

We combine theory and experiment to investigate five-body recombination in an ultracold gas of atomic cesium at negative scattering length. A refined theoretical model, in combination with extensive laboratory tunability of the interatomic interactions, enables the five-body resonant recombination rate to be calculated and measured. The position of the new observed recombination feature agrees with a recent theoretical prediction and supports the prediction of a family of universal cluster states at negative $a$ that are tied to an Efimov trimer., Comment: 14 pages, 5 figures

Ultracold atomic gases have developed into prime systems for experimental studies of Efimov three-body physics and related few-body phenomena, which occur in the universal regime of resonant interactions. In the last few years, many important breakthroughs have been achieved, confirming basic predictions of universal few-body theory and deepening our understanding of such systems. We review the basic ideas along with the fast experimental developments of the field, focussing on ultracold cesium gases as a well-investigated model system. Triatomic Efimov resonances, atom-dimer Efimov resonances, and related four-body resonances are discussed as central observables. We also present some new observations of such resonances, supporting and complementing the set of available data., Comment: 23 pages, 13 figures

We perform precision measurements on a Mott-insulator quantum state of ultracold atoms with tunable interactions. We probe the dependence of the superfluid-to-Mott-insulator transition on the interaction strength and explore the limits of the standard Bose-Hubbard model description. By tuning the on-site interaction energies to values comparable to the interband separation, we are able to quantitatively measure number-dependent shifts in the excitation spectrum caused by effective multi-body interactions., Comment: 4 pages, 4 figures

We report on the observation of triatomic Efimov resonances in an ultracold gas of cesium atoms. Exploiting the wide tunability of interactions resulting from three broad Feshbach resonances in the same spin channel, we measure magnetic-field dependent three-body recombination loss. The positions of the loss resonances yield corresponding values for the three-body parameter, which in universal few-body physics is required to describe three-body phenomena and in particular to fix the spectrum of Efimov states. Our observations show a robust universal behavior with a three-body parameter that stays essentially constant., Comment: 4 pages, 3 figures

We present experimentally derived potential curves and spin-orbit interaction functions for the strongly perturbed $A^{1}\Sigma_{u}^{+}$ and $b^{3}\Pi_{u}$ states of the cesium dimer. The results are based on data from several sources. Laser-induced fluorescence Fourier transform spectroscopy (LIF FTS) was used some time ago in the Laboratoire Aim\'{e} Cotton primarily to study the $X ^{1}\Sigma_{g}^{+}$ state. More recent work at Tsinghua University provides information from moderate resolution spectroscopy on the lowest levels of the $b^{3}\Pi_{0u}^{\pm}$ states as well as additional high resolution data. From Innsbruck University, we have precision data obtained with cold Cs$_{2}$ molecules. Recent data from Temple University was obtained using the optical-optical double resonance polarization spectroscopy technique, and finally, a group at the University of Latvia has added additional LIF FTS data. In the Hamiltonian matrix, we have used analytic potentials (the Expanded Morse Oscillator form) with both finite-difference (FD) coupled-channels and discrete variable representation (DVR) calculations of the term values. Fitted diagonal and off-diagonal spin-orbit functions are obtained and compared with {\it ab initio} results from Temple and Moscow State universities.

We report the simultaneous production of Bose-Einstein condensates (BECs) of $^{87}$Rb and $^{133}$Cs atoms in separate optical traps. The two samples are mixed during laser cooling and loading but are separated by $400 \mu$m for the final stage of evaporative cooling. This is done to avoid considerable interspecies three-body recombination, which causes heating and evaporative loss. We characterize the BEC production process, discuss limitations, and outline the use of the dual-species BEC in future experiments to produce rovibronic ground state molecules, including a scheme facilitated by the superfluid-to-Mott-insulator (SF-MI) phase transition.

We report on the observation of an elementary exchange process in an optically trapped ultracold sample of atoms and Feshbach molecules. We can magnetically control the energetic nature of the process and tune it from endoergic to exoergic, enabling the observation of a pronounced threshold behavior. In contrast to relaxation to more deeply bound molecular states, the exchange process does not lead to trap loss. We find excellent agreement between our experimental observations and calculations based on the solutions of three-body Schr\"odinger equation in the adiabatic hyperspherical representation. The high efficiency of the exchange process is explained by the halo character of both the initial and final molecular states., Comment: 4 pages, 4 figures

We discuss our recent observation of an atom-dimer Efimov resonance in an ultracold mixture of Cs atoms and Cs_2 Feshbach molecules [Nature Phys. 5, 227 (2009)]. We review our experimental procedure and present additional data involving a non-universal g-wave dimer state, to contrast our previous results on the universal s-wave dimer. We resolve a seeming discrepancy when quantitatively comparing our experimental findings with theoretical results from effective field theory., Comment: Conference Proceeding ICPEAC 2009 Kalamazoo, to appear in Journal of Physics: Conference Series

We study collisions in an optically trapped, pure sample of ultracold Cs$_2$ molecules in various internal states. The molecular gas is created by Feshbach association from a near-degenerate atomic gas, with adjustable temperatures in the nanokelvin range. We identify several narrow loss resonances, which point to the coupling to more complex molecular states and may be interpreted as Feshbach resonances in dimer-dimer interactions. Moreover, in some molecular states we observe a surprising temperature dependence in collisional loss. This shows that the situation cannot be understood in terms of the usual simple threshold behavior for inelastic two-body collisions. We interpret this observation as further evidence for a more complex molecular structure beyond the well-understood dimer physics., Comment: To appear in Laser Physics, special issue in memoriam Prof. Vladilen S. Letokhov

We report on the measurement of four-body recombination rate coefficients in an atomic gas. Our results obtained with an ultracold sample of cesium atoms at negative scattering lengths show a resonant enhancement of losses and provide strong evidence for the existence of a pair of four-body states, which is strictly connected to Efimov trimers via universal relations. Our findings confirm recent theoretical predictions and demonstrate the enrichment of the Efimov scenario when a fourth particle is added to the generic three-body problem., Comment: 4 pages, 4 figures

We report on the observation of interspecies Feshbach resonances in an ultracold, optically trapped mixture of Rb and Cs atoms. In a magnetic field range up to 300 G we find 23 interspecies Feshbach resonances in the lowest spin channel and 2 resonances in a higher channel of the mixture. The extraordinarily rich Feshbach spectrum suggests the importance of different partial waves in both the open and closed channels of the scattering problem along with higher-order coupling mechanisms. Our results provide, on one hand, fundamental experimental input to characterize the Rb-Cs scattering properties and, on the other hand, identify possible starting points for the association of ultracold heteronuclear RbCs molecules., Comment: 7 pages, 3 figures, 1 table

We present an analytic model to calculate the atomic scattering length near a Feshbach resonance from data on the molecular binding energy. Our approach considers finite-range square-well potentials and can be applied near broad, narrow, or even overlapping Feshbach resonances. We test our model on Cs$_2$ Feshbach molecules. We measure the binding energy using magnetic-field modulation spectroscopy in a range where one broad and two narrow Feshbach resonances overlap. From the data we accurately determine the Cs atomic scattering length and the positions and widths of two particular resonances., Comment: 6 pages, 4 figures

The field of few-body physics has originally been motivated by understanding nuclear matter. New model systems to experimentally explore few-body quantum systems can now be realized in ultracold gases with tunable interactions. Albeit the vastly different energy regimes of ultracold and nuclear matter (peV as compared to MeV), few-body phenomena are universal for near-resonant two-body interactions. Efimov states represent a paradigm for universal three-body states, and evidence for their existence has been obtained in measurements of three-body recombination in an ultracold gas of caesium atoms. Interacting samples of halo dimers can provide further information on universal few-body phenomena. Here we study interactions in an optically trapped mixture of such halo dimers with atoms, realized in a caesium gas at nanokelvin temperatures. We observe an atom-dimer scattering resonance, which we interpret as being due to a trimer state hitting the atom-dimer threshold. We discuss the close relation of this observation to Efimov's scenario, and in particular to atom-dimer Efimov resonances., Comment: 12 pages, 3 figures

We study inelastic collisions in a pure, trapped sample of Feshbach molecules made of bosonic cesium atoms in the quantum halo regime. We measure the relaxation rate coefficient for decay to lower-lying molecular states and study the dependence on scattering length and temperature. We identify a pronounced loss minimum with varying scattering length along with a further suppression of loss with decreasing temperature. Our observations provide insight into the physics of a few-body quantum system that consists of four identical bosons at large values of the two-body scattering length., Comment: 4 pages, 4 figures

We report on the control of interaction-induced dephasing of Bloch oscillations for an atomic Bose-Einstein condensate in an optical lattice under the influence of gravity. When tuning the strength of the interaction towards zero by means of a Feshbach resonance, the dephasing time is increased from a few to more than twenty thousand Bloch oscillation periods. We quantify the dephasing in terms of the width of the quasi-momentum distribution and measure its dependence on time for different values of the scattering length. Minimizing the dephasing allows us to realize a BEC-based atom interferometer in the non-interacting limit. We use it for a precise determination of a zero-crossing for the atomic scattering length and to observe collapse and revivals of Bloch oscillations when the atomic sample is subject to a spatial force gradient., Comment: 4 pages, 5 figures

We experimentally demonstrate Cs2 Feshbach molecules well above the dissociation threshold, which are stable against spontaneous decay on the timescale of one second. An optically trapped sample of ultracold dimers is prepared in an l-wave state and magnetically tuned into a region with negative binding energy. The metastable character of these molecules arises from the large centrifugal barrier in combination with negligible coupling to states with low rotational angular momentum. A sharp onset of dissociation with increasing magnetic field is mediated by a crossing with a g-wave dimer state and facilitates dissociation on demand with a well defined energy., Comment: 4 pages, 5 figures

We explore the rich internal structure of Cs_2 Feshbach molecules. Pure ultracold molecular samples are prepared in a CO_2-laser trap, and a multitude of weakly bound states is populated by elaborate magnetic-field ramping techniques. Our methods use different Feshbach resonances as input ports and various internal level crossings for controlled state transfer. We populate higher partial-wave states of up to eight units of rotational angular momentum (l-wave states). We investigate the molecular structure by measurements of the magnetic moments for various states. Avoided level crossings between different molecular states are characterized through the changes in magnetic moment and by a Landau-Zener tunneling method. Based on microwave spectroscopy, we present a precise measurement of the magnetic-field dependent binding energy of the weakly bound s-wave state that is responsible for the large background scattering length of Cs. This state is of particular interest because of its quantum-halo character., Comment: 15 pages, 12 figures, 4 tables

We report on the realization of a time-domain `St\"uckelberg interferometer', which is based on the internal state structure of ultracold Feshbach molecules. Two subsequent passages through a weak avoided crossing between two different orbital angular momentum states in combination with a variable hold time lead to high-contrast population oscillations. This allows for a precise determination of the energy difference between the two molecular states. We demonstrate a high degree of control over the interferometer dynamics. The interferometric scheme provides new possibilities for precision measurements with ultracold molecules., Comment: 4 pages, 5 figures

Three interacting particles form a system which is well known for its complex physical behavior. A landmark theoretical result in few-body quantum physics is Efimov's prediction of a universal set of weakly bound trimer states appearing for three identical bosons with a resonant two-body interaction. Surprisingly, these states even exist in the absence of a corresponding two-body bound state and their precise nature is largely independent of the particular type of the two-body interaction potential. Efimov's scenario has attracted great interest in many areas of physics; an experimental test however has not been achieved. We report the observation of an Efimov resonance in an ultracold thermal gas of cesium atoms. The resonance occurs in the range of large negative two-body scattering lengths and arises from the coupling of three free atoms to an Efimov trimer. We observe its signature as a giant three-body recombination loss when the strength of the two-body interaction is varied near a Feshbach resonance. This resonance develops into a continuum resonance at non-zero collision energies, and we observe a shift of the resonance position as a function of temperature. We also report on a minimum in the recombination loss for positive scattering lengths, indicating destructive interference of decay pathways. Our results confirm central theoretical predictions of Efimov physics and represent a starting point from which to explore the universal properties of resonantly interacting few-body systems., Comment: 8 pages, 4 figures, Proceedings of ICAP-2006 (Innsbruck)

Systems of three interacting particles are notorious for their complex physical behavior. A landmark theoretical result in few-body quantum physics is Efimov's prediction of a universal set of bound trimer states appearing for three identical bosons with a resonant two-body interaction. Counterintuitively, these states even exist in the absence of a corresponding two-body bound state. Since the formulation of Efimov's problem in the context of nuclear physics 35 years ago, it has attracted great interest in many areas of physics. However, the observation of Efimov quantum states has remained an elusive goal. Here we report the observation of an Efimov resonance in an ultracold gas of cesium atoms. The resonance occurs in the range of large negative two-body scattering lengths, arising from the coupling of three free atoms to an Efimov trimer. Experimentally, we observe its signature as a giant three-body recombination loss when the strength of the two-body interaction is varied. We also detect a minimum in the recombination loss for positive scattering lengths, indicating destructive interference of decay pathways. Our results confirm central theoretical predictions of Efimov physics and represent a starting point with which to explore the universal properties of resonantly interacting few-body systems. While Feshbach resonances have provided the key to control quantum-mechanical interactions on the two-body level, Efimov resonances connect ultracold matter to the world of few-body quantum phenomena., Comment: 18 pages, 3 figures

We observe magnetically tuned collision resonances for ultracold Cs2 molecules stored in a CO2-laser trap. By magnetically levitating the molecules against gravity, we precisely measure their magnetic moment. We find an avoided level crossing which allows us to transfer the molecules into another state. In the new state, two Feshbach-like collision resonances show up as strong inelastic loss features. We interpret these resonances as being induced by Cs4 bound states near the molecular scattering continuum. The tunability of the interactions between molecules opens up novel applications such as controlled chemical reactions and synthesis of ultracold complex molecules.

We report a new scheme to create weakly bound Cs$_2$ molecules from an atomic Bose-Einstein condensate. The method is based on switching the magnetic field to a narrow Feshbach resonance and yields a high atom-molecule conversion efficiency of more than 30%, a factor of three higher than obtained with conventional magnetic-field ramps. The Cs$_2$ molecules are created in a single $g$-wave rotational quantum state. The observed dependence of the conversion efficiency on the magnetic field and atom density shows scattering processes beyond two-body coupling to occur in the vicinity of the Feshbach resonance., Comment: 7 pages, 4 figures, submitted to Europhysics Letters

We report on the creation of a two-dimensional Bose-Einstein condensate of cesium atoms in a gravito-optical surface trap. The condensate is produced a few micrometer above a dielectric surface on an evanescent-wave atom mirror. After evaporative cooling by all-optical means, expansion measurements for the tightly confined vertical motion show energies well below the vibrational energy quantum. The presence of a condensate is observed in two independent ways by a magnetically induced collapse at negative scattering length and by measurements of the horizontal expansion.

Single Cesium atoms are cooled and trapped inside a small optical cavity by way of a novel far-off-resonance dipole-force trap (FORT), with observed lifetimes of 2 to 3 seconds. Trapped atoms are observed continuously via transmission of a strongly coupled probe beam, with individual events lasting ~ 1 s. The loss of successive atoms from the trap N = 3 -> 2 -> 1 -> 0 is thereby monitored in real time. Trapping, cooling, and interactions with strong coupling are enabled by the FORT potential, for which the center-of-mass motion is only weakly dependent on the atom's internal state., Comment: 5 pages, 4 figures Revised version to appear in Phys. Rev. Lett

A dense gas of cesium atoms at the crossover to two-dimensionality is prepared in a highly anisotropic surface trap that is realized with two evanescent light waves. Temperatures as low as 100nK are reached with 20.000 atoms at a phase-space density close to 0.1. The lowest quantum state in the tightly confined direction is populated by more than 60%. The system offers intriguing prospects for future experiments on degenerate quantum gases in two dimensions.

An optical microtrap is realized on a dielectric surface by crossing a tightly focused laser beam with an horizontal evanescent-wave atom mirror. The nondissipative trap is loaded with $\sim$$10^5$ cesium atoms through elastic collisions from a cold reservoir provided by a large-volume optical surface trap. With an observed 300-fold local increase of the atomic number density approaching $10^{14}{\rm cm}^{-3}$, unprecedented conditions of cold atoms close to a surface are realized.

We investigate single ions of $^{40}Ca^+$ in Paul traps for quantum information processing. Superpositions of the S$_{1/2}$ electronic ground state and the metastable D$_{5/2}$ state are used to implement a qubit. Laser light on the S$_{1/2} \leftrightarrow$ D$_{5/2}$ transition is used for the manipulation of the ion's quantum state. We apply sideband cooling to the ion and reach the ground state of vibration with up to 99.9% probability. Starting from this Fock state $|n=0>$, we demonstrate coherent quantum state manipulation. A large number of Rabi oscillations and a ms-coherence time is observed. Motional heating is measured to be as low as one vibrational quantum in 190 ms. We also report on ground state cooling of two ions., Comment: 12 pages, 6 figures. submitted to Journal of Modern Optics, Special Issue on Quantum Optics: Kuehtai 2000

A single Ca+ ion in a Paul trap has been cooled to the ground state of vibration with up to 99.9% probability. Starting from this Fock state |n=0> we have demonstrated coherent quantum state manipulation on an optical transition. Up to 30 Rabi oscillations within 1.4 ms have been observed. We find a similar number of Rabi oscillations after preparation of the ion in the |n=1> Fock state. The coherence of optical state manipulation is only limited by laser and ambient magnetic field fluctuations. Motional heating has been measured to be as low as one vibrational quantum in 190 ms., Comment: 4 pages, 5 figures