1. Integration of polydopamine-coated Nb2CTx MXene nanosheets into PLA membranes for enhanced antifouling performance and efficient SARS-CoV-2 removal from raw wastewater.
- Author
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Pandey, Ravi P., Ankitha, Menon, Daou, Mariane, Ouda, Mariam, Abdul Rasheed, P., Tizani, Lina, and Hasan, Shadi W.
- Subjects
POLYLACTIC acid ,NANOSTRUCTURED materials ,SARS-CoV-2 ,SEWAGE ,ULTRAFILTRATION ,POROSITY - Abstract
[Display omitted] • PDA@Nb 2 CT x was prepared by in-situ polymerization of dopamine hydrochloride. • PDA@Nb 2 CT x /PLA membrane was successfully designed for SARS-CoV-2 removal. • Incorporation of PDA@Nb 2 CT x into PLA improved antifouling and separation properties. • 6% PDA@Nb 2 CT x /PLA offered higher flux recovery ratio compared to PLA membrane. In this study, we synthesised a two-dimensional (2D) Nb 2 CT x MXene coated with polydopamine (PDA) (PDA@Nb 2 CT x) nanosheets as a promising nanofiller. The biocompatible and biodegradable polylactic acid (PLA) (PDA@Nb 2 CT x /PLA)-based ultrafiltration (UF) membranes were fabricated by incorporation of PDA@Nb 2 CT x nanosheets into PLA polymer matrix via phase inversion. The physicochemical properties, and separation performance of developed PDA@Nb 2 CT x /PLA membranes were studied. The 6 wt% PDA@Nb 2 CT x /PLA membrane showed highest porosity and mean pore size of 78.60 % and 52.95 nm; respectively. The 6 wt% PDA@Nb 2 CT x /PLA membrane reported ∼4-fold higher pure water permeability (PWP) (493.82 L m
−2 h−1 bar−1 ) compared to the pristine PLA membrane. The 6 wt% PDA@Nb 2 CT x /PLA membrane offered 2.6-fold and 1.64-fold higher flux recovery ratio (FRR; %) compared to the PLA and 6 wt% PLA/Nb 2 CT x membranes; respectively. The reported 6 wt% PDA@Nb 2 CT x /PLA membrane shows a great potential in wastewater and biomedical related applications. [ABSTRACT FROM AUTHOR]- Published
- 2024
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