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A high percentage of the world's population lives in areas where air pollutant concentrations exceed the World Health Organization guidelines. This work aims to develop and test, a high-resolution multi-scale air pollution modelling system by integrating a set of adequate tools. This system is able to provide detailed air pollutant concentrations in urban areas and support air quality management strategies through a better identification of different atmospheric processes. It also allows furthering the design and assessment of air pollution control measures for a specific area. To evaluate its performance and suitability, the system was applied to the Macau Special Administrative Region (SAR), China, one of the most densely populated areas on earth, during a winter period when this area is affected by high levels of Particulate Matter (PM). Although the developed system tends to underestimate the PM concentrations, it revealed a good performance in reproducing the temporal and spatial air pollution patterns. Several exceedances of the Chinese air quality standards were calculated and high population exposure to PM pollution was estimated. The tested urban atmospheric emission reduction scenarios have shown air quality improvements, indicating that emission reduction measures at urban level should focus on the domestic sector. However, it is crucial to implement joint pollution prevention strategies with neighbouring regions to improve the air quality in Macau SAR. The approach developed in this work can support policymakers in defining new strategies to reduce atmospheric pollution in urban areas., Competing Interests: Declaration of Competing Interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper., (Copyright © 2023. Published by Elsevier B.V.)

Within the scope of the Aveiro STEAM City project, an air quality monitoring network was installed in the city of Aveiro (Portugal), to evaluate the potential of sensors to characterize spatial and temporal patterns of air quality in the city. The network consists of nine sensors stations with air quality sensors (PM10, PM2.5, NO 2 , O 3 and CO) and two meteorological stations, distributed within selected locations in the city of Aveiro. The analysis of the data was done for a one-year measurement period, from June 2020 to May 2021, using temporal profiles, statistical comparisons with reference stations and Air Quality Indexes (AQI). The analysis of sensors data indicated that air quality variability exists for all pollutants and stations. The majority of the study area is characterized by good air quality, but specific areas-associated with hotspot traffic zones-exhibit medium, poor and bad air quality more frequently. The daily patterns registered are significantly different between the affected and non-affected road traffic sites, mainly for PM and NO 2 pollutants. The weekly profile, significative deltas are found between week and weekend: NO 2 is reduced on the weekends at traffic sites, but PM10 is higher in specific areas during winter weekends, which is explained by residential combustion sources.

People spend most of their time in indoor environments without knowing about the air quality in these spaces. In this study, indoor low-cost sensors were used (for 5 months) to assess the comfort and air quality patterns in two indoor households. To strengthen the robustness of the considered approach and build confidence in the obtained comfort and indoor air quality (IAQ) levels, the sensor measurements were also compared against information from reference monitoring equipment; in which, high correlation coefficients were obtained (> 0.85) and also low errors (on average 22%). The IAQ results were strongly influenced by the residents' activity and behaviour, the outdoor weather conditions, and indoor/outdoor air pollution sources. Overall, the recommended values of temperature and relative humidity for the occupant's comfort in indoor environments were not fulfilled. The highest particulate matter (PM) levels were recorded at the weekend (on average +14% higher), while maximum CO 2 and CO levels were obtained on the weekdays (on average +9% higher). PM daily profiles followed the outdoor concentrations with the maximum levels at the end of the night and the lowest values in the early morning/mid-afternoon. The highest and lowest CO 2 concentrations were registered in the early morning (< 1536 ppm) and mid-afternoon (< 627 ppm), respectively, while the CO daily profiles showed a high impact of outdoor emissions, with the minimum concentrations up to 0.81 mg m -3 (at 10 a.m. or 6 p.m.), and a maximum concentration of 1.87 mg m -3 (at 10 p.m.). Real-time comfort conditions and IAQ levels are a powerful approach to providing fast decisions to minimise human exposure and prevent negative health impacts., (© 2022. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.)

Autonomous vehicles (AVs) are pointed out as the technology that will reshape the concept of mobility, with significant implications for the economy, the environment, and society. This fact will bring new challenge to cities urban planning. Research to anticipate the AVs impacts, maximizing their benefits and reduce trade-offs are currently crucial. This work investigates the potential challenges and benefits of gradually replace internal combustion engine human driven vehicles with different penetration rates of AVs - 10%, 30%, 50%, 70%, 90%, and 100% - in urban roads of different characteristics, either in terms of traffic singularities or volumes, and its related implications on air quality. For that purpose, two urban areas with distinct features, Porto and Aveiro, were selected as case studies, and a modelling setup composed of a traffic model, an emission model, and a local air quality model was applied. The results revealed that the AVs benefits are directly linked with the urban design and the road characteristics. In the Aveiro case study, the AVs promoted positive changes with average reductions in daily NOx emissions (compared with the baseline scenario, without AVs) ranging between -2.1% (for C10%) and -7.7% (for C100%). In line with the emissions impacts, positive effects were found on air quality, with average reductions of NO 2 concentrations up to -4% (for C100%). In Porto urban area, slight differences in NOx emissions were obtained (<2%), which implied no changes in the air quality levels. The distinct impact of AVs in the study areas is mostly explained by the traffic light coordination system and directional split distributions in the main roads. These results provide valuable insights to support decision-makers in the definition of strategies that allow the integration of these new emerging technologies in the road infrastructure, considering the features of the urban design, traffic profile and road characteristics., (Copyright © 2022 Elsevier Ltd. All rights reserved.)

Air pollution is a global challenge, and especially urban areas are particularly affected by acute episodes. Traditional approaches used to mitigate air pollution primarily consider the technical aspects of the problem but not the role of citizen behaviour and day-to-day practices. ClairCity, a Horizon 2020 funded project, created an impact assessment framework considering the role of citizen behaviour to create future scenarios, aiming to improve urban environments and the wellbeing and health of its inhabitants. This framework was applied to six pilot cases: Bristol, Amsterdam, Ljubljana, Sosnowiec, Aveiro Region and Liguria Region, considering three-time horizons: 2025, 2035 and 2050. The scenarios approach includes the Business As Usual (BAU) scenario and a Final Unified Policy Scenarios (FUPS) established by citizens, decision-makers, local planners and stakeholders based on data collected through a citizen and stakeholder co-creation process. Therefore, this paper aims to present the ClairCity outcomes, analysing the quantified impacts of selected measures in terms of emissions, air quality, population exposure, and health. Each case study has established a particular set of measures with different levels of ambition, therefore different levels of success were achieved towards the control and mitigation of their specific air pollution problems. The transport sector was the most addressed by the measures showing substantial improvements for NO 2 , already with the BAU scenarios, and overall, even better results when applying the citizen-led FUPS scenarios. In some cases, due to a lack of ambition for the residential and commercial sector, the results were not sufficient to fulfil the WHO guidelines. Overall, it was found in all cities that the co-created scenarios would lead to environmental improvements in terms of air quality and citizens' health compared to the baseline year of 2015. However, in some cases, the health impacts were lower than air quality due to the implementation of the measures not affecting the most densely populated areas. Benefits from the FUPS comparing to the BAU scenario were found to be highest in Amsterdam and Bristol, with further NO 2 and PM10 emission reductions around 10%-16% by 2025 and 19%-28% by 2050, compared to BAU., (Copyright © 2021 Elsevier Ltd. All rights reserved.)

Green roofs, as part of urban green structures, have been pointed out as the solution to pursuit the goal of healthy cities. This study aims to investigate the direct, focused on meteorological changes, and indirect, related to both meteorological and emissions changes, impacts of green roofs on air quality (PM10, NO 2 and O 3 ). For that, the numerical modelling system composed by the WRF-SLUCM-CHIMERE models was applied to a 1-year period (2017), having as case study the Porto urban area. The EnergyPlus model was also applied to estimate the green roofs impacts on the building's energy needs and related impacts on air quality and atmospheric emissions. The analysis of the direct impacts showed that green roofs promote a temperature increase during the autumn and winter seasons and a temperature decrease during the spring and summer seasons. Both negative - concentrations increase - and positive - concentrations decrease - impacts were obtained for the primary, PM10 and NO 2 , and secondary, O 3 , air pollutants, respectively, due to changes in the dynamical structure of the urban boundary layer. The indirect effects of green roofs showed their potential to enhance the buildings energy efficiency, reducing the cooling and heating needs. These changes in energy consumption promoted an overall decrease of the environmental and economic indicators. Regarding air quality, the impact was negligible. The obtained results highlight the need for a multipurpose evaluation of the impacts of green roofs, with the different effects having to be traded off against each other to better support the decision-making process., Competing Interests: Declaration of competing interest The authors Sandra Rafael, Luís P. Correia, Ana Ascenso, Bruno Augusto, Diogo Lopes, and Ana Isabel Miranda would like to declare that there is no conflict of interests., (Copyright © 2021 Elsevier B.V. All rights reserved.)

Atmospheric particles are a major environmental health risk. Assessments of air pollution related health burden are often based on outdoor concentrations estimated at residential locations, ignoring spatial mobility, time-activity patterns, and indoor exposures. The aim of this work is to quantify impacts of these factors on outdoor-originated fine particle exposures of school children. We apply nested WRF-CAMx modelling of PM 2.5 concentrations, gridded population, and school location data. Infiltration and enrichment factors were collected and applied to Athens, Kuopio, Lisbon, Porto, and Treviso. Exposures of school children were calculated for residential and school outdoor and indoor, other indoor, and traffic microenvironments. Combined with time-activity patterns six exposure models were created. Model complexity was increased incrementally starting from residential and school outdoor exposures. Even though levels in traffic and outdoors were considerably higher, 80-84% of the exposure to outdoor particles occurred in indoor environments. The simplest and also commonly used approach of using residential outdoor concentrations as population exposure descriptor (model 1), led on average to 26% higher estimates (15.7 μg/m 3 ) compared with the most complex model (# 6) including home and school outdoor and indoor, other indoor and traffic microenvironments (12.5 μg/m 3 ). These results emphasize the importance of including spatial mobility, time-activity and infiltration to reduce bias in exposure estimates., Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper., (Copyright © 2021 The Authors. Published by Elsevier B.V. All rights reserved.)

The Pearl River Delta (PRD) region is located on the southeast coast of mainland China and it is an important economic hub. The high levels of particulate matter (PM) in the atmosphere, however, and poor visibility have become a complex environmental problem for the region. Air quality modeling systems are useful to understand the temporal and spatial distribution of air pollution, making use of atmospheric emission data as inputs. Over the years, several atmospheric emission inventories have been developed for the Asia region. The main purpose of this work is to evaluate the performance of the air quality modeling system for simulating PM concentrations over the PRD using three atmospheric emission inventories (i.e., EDGAR, REAS and MIX) during a winter and a summer period. In general, there is a tendency to underestimate PM levels, but results based on the EDGAR emission inventory show slightly better accuracy. However, improvements in the spatial and temporal disaggregation of emissions are still needed to properly represent PRD air quality. This study's comparison of the three emission inventories' data, as well as their PM simulating outcomes, generates recommendations for future improvements to atmospheric emission inventories and our understanding of air pollution problems in the PRD region.

Air pollution is a global threat leading to large impacts on human health and ecosystems. In Europe, air quality remains poor in many areas, despite reductions in emissions and ambient concentrations. Air pollution and climate change are the biggest environmental concerns for Europeans, implying concerted and integrated actions to tackle them. The revised 2016 European National Emission Ceilings Directive (NECD) enforces Member States to implement strategies, based on emission reduction measures, aimed to comply with targets by 2030 and achieve European Union (EU) and World Health Organization air quality objectives for environment and health protection. Despite those strategies are designed for 2030, the influence of climate change on air quality is not accounted for. In this sense, the purpose of this paper is the evaluation of the climate change impact on future air quality, taking into consideration emission reduction measures. The WRF-CAMx air quality modelling system was applied over Europe for one year selected as representative of a short-term changing climate (around 2030), and compared to a base case year, to estimate to what extent the climate variables by themselves could positively or negatively influence air quality. Results indicate that meteorological conditions may be decisive for the air quality state in the future. Differences between future and present simulations pointed to a global decrease of ozone levels in the future; increases and decreases in particulate matter and nitrogen dioxide concentrations over different seasons and European regions. This work is intended to contribute to a better understanding of the influence of climate variables on air quality improvement strategies as an additional support to European environmental authorities in developing the National Air Pollution Control Programmes in the scope of NECD., Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper., (Copyright © 2020 Elsevier B.V. All rights reserved.)

Smoke inhalation poses a serious health threat to firefighters (FFs), with potential effects including respiratory and cardiac disorders. In this work, environmental and physiological data were collected from FFs, during experimental fires performed in 2015 and 2019. Extending a previous work, which allowed us to conclude that changes in heart rate (HR) were associated with alterations in the inhalation of carbon monoxide (CO), we performed a HR analysis according to different levels of CO exposure during firefighting based on data collected from three FFs. Based on HR collected and on CO occupational exposure standards (OES), we propose a classifier to identify CO exposure levels through the HR measured values. An ensemble of 100 bagged classification trees was used and the classification of CO levels obtained an overall accuracy of 91.9%. The classification can be performed in real-time and can be embedded in a decision fire-fighting support system. This classification of FF' exposure to critical CO levels, through minimally-invasive monitored HR, opens the possibility to identify hazardous situations, preventing and avoiding possible severe problems in FF' health due to inhaled pollutants. The obtained results also show the importance of future studies on the relevance and influence of the exposure and inhalation of pollutants on the FF' health, especially in what refers to hazardous levels of toxic air pollutants.

Toxic metals as arsenic (As), cadmium (Cd), nickel (Ni), and lead (Pb) exist in the atmosphere as particulate matter components. Their concentration levels in the European Union (EU) are regulated by European legislation, which sets target and limit values as annual means, and by the World Health Organization (WHO) that defines guidelines and reference values for those metal elements. Modelling tools are recommended to support air quality assessment regarding the toxic metals; however, few studies have been performed and those assessments rely on discrete measurements or field campaigns. This study aims to evaluate the capability of air quality modelling tools to verify the legislation compliance concerning the atmospheric levels of toxic elements and to identify the main challenges and limitations of using a modelling assessment approach for regulatory purposes, as a complement to monitoring. The CAMx air quality model was adapted and applied over Porto and Lisbon urban regions in Portugal at 5 × 5-km 2 and 1 × 1-km 2 horizontal resolution for the year 2015, and the results were analysed and compared with the few measurements available in three locations. The comparison between modelled and measured data revealed an overestimation of the model, although annual averages are much lower than the regulated standards. The comparison of the 5-km and 1-km resolutions' results indicates that a higher resolution does not necessarily imply a better performance, pointing out uncertainties in emissions and the need to better describe the magnitude and spatial allocation of toxic metal emissions. This work highlighted that an increase of the spatial and temporal coverage of monitoring sites would allow to improve the model design, contribute to a better knowledge on toxic metals atmospheric emission sources and to increase the capacity of models to simulate atmospheric particulate species of health concern.

Climate change is increasingly exerting pressure with intensified impacts in the short-, medium-, and long-term. Cities are highly vulnerable to the impacts of climate change, and it is recognized that they play a significant role in the European Strategy on adaptation to climate change. This study intends to develop a climate adaptation framework to identify effective measures that will be evaluated using a multi-urban area located in the north of Portugal, as a case study. The climate adaptation framework was developed following the Urban Adaptation Support Tool (AST), adapted to the Portuguese reality. The Weather Research and Forecasting (WRF) model was used to provide future projections with a high level of spatial resolution over the study area, increasing the accuracy of the identification of future climatic vulnerabilities. The results show a tendency for an increase of extreme weather events associated with the increase of both temperature and annual accumulated precipitation variables. A set of both urban and rural measures to promote a sustainable development path to climate adaptability and increase cities resilience to climate change are presented and discussed.

Understanding air pollution in urban areas is crucial to identify mitigation actions that may improve air quality and, consequently, minimize human exposure to air pollutants and their impact. This study aimed to assess the temporal evolution of the air quality in the city of Setúbal (Portugal) during a time period of 10 years (2003-2012), by evaluating seasonal trends of air pollutants (PM 10 , PM 2.5 , O 3 , NO, NO 2 and NO x ) measured in nine monitoring stations. In order to identify emission sources of particulate matter, PM 2.5 and PM 2.5-10 were characterized in two different areas (urban traffic and industrial) in winter and summer and, afterwards, source apportionment was performed by means of Positive Matrix Factorization. Overall, the air quality has been improving over the years with a decreasing trend of air pollutant concentration, with the exception of O 3 . Despite this improvement, levels of PM 10 , O 3 and nitrogen oxides still do not fully comply with the requirements of European legislation, as well as with the guideline values of the World Health Organization (WHO). The main anthropogenic sources contributing to local PM levels were traffic, industry and wood burning, which should be addressed by specific mitigation measures in order to minimize their impact on the local air quality.

The impacts of autonomous vehicles (AV) on safety, energy and atmospheric emissions have been recognised to be important issues, but an air quality impact assessment is missing. In this study, by using a numerical modelling approach, the impact of AV on the air quality of a medium-sized Portuguese urban area was evaluated. For that, the air pollutants nitrogen oxides (NOx) and carbon dioxide (CO 2 ) were considered and three scenarios were developed: i) a baseline scenario; ii) an autonomous scenario, assuming an AV market penetration rate of 30%; and iii) an electric autonomous scenario, taking into account that those 30% of AV are pure battery electric cars. A modelling system composed by a road traffic model, a road transport emission model and a Computational Fluid Dynamics air quality model was used. The autonomous scenario promoted an increase of both NOx (+1.8%) and CO 2 (+0.7%) emissions, while the electric autonomous scenario resulted in emission reductions of about 30% for both air pollutants. In terms of air quality, distinct patterns were found: i) the autonomous scenario promoted both increases and decreases of NOx concentrations; and ii) the electric autonomous scenario promoted a widespread reduction of NOx concentrations (with an average value of -4%). Overall the results showed that AV have the potential to improve urban air quality, but, further research is needed to enrich the findings of this work., Competing Interests: Declaration of competing interest The authors Sandra Rafael, Luís P. Correia, Diogo Lopes, Jorge Bandeira, Margarida Coelho, Mário Andrade, Carlos Borrego and Ana Isabel Miranda, would like to declare that there is no conflict of interests., (Copyright © 2020 Elsevier B.V. All rights reserved.)

With rapid economic growth, road transport is contributing substantial adverse effects on urban air quality, especially in densely populated cities with high growth rate of GDP per capita, such as Macau. A high spatial-temporal resolution road traffic emission inventory is essential for assessment of environmental stresses imposed by local vehicle movements. To improve the accuracy and temporal-spatial resolution for emission inventory, through a bottom-up approach, link-based road traffic emission inventory with a spatial resolution of 0.1 km ∗ 0.1 km and a temporal resolution of 1 h for Macau in 2014 was developed by using a traffic model (VISUM), a road traffic emission model (TREM), the Geographic Information System (GIS), and the most up-to-date information available. Results show that the total annual emissions of CO, CO 2 , PM, NO X , and VOC in 2014 were 14,770, 413,099, 69, 1151, and 2945 tons, respectively. The estimated fuel consumption agreed well also with the statistical fuel consumption in Macau. Meanwhile, analysis of 3 scenarios on changes of road traffic emissions due to the operation of a light railway transit (LRT) system, variation on share of diesel, electric, and gasoline within the vehicle fleet, and replacement of vehicles with ones of Euro 5 and Euro 6 emission standards was carried out. This study provides a solid framework for developing high spatial-temporal resolution emission inventories for other densely populated cities of small area.

Timor-Leste's Maternal Mortality Ratio remains one of the highest in Asia. There is ample evidence that maternal deaths may be reduced substantially through the provision of good-quality modern methods of contraception. Many Timorese women wish to stop or delay having children. However, even when health services make contraception available, it does not mean that people will use it. Collaborating with Marie Stopes Timor-Leste, this qualitative research project used decolonising methodology to explore perceived influences contributing to contraceptive choices, and gain insight into how women's decisions to access contraception in Timor-Leste occur. Over two fieldwork periods (2013 and 2015), we used focus group discussions and structured interviews to speak with 68 women and 80 men, aged 18-49 years, across four districts of Timor-Leste. Findings demonstrate that the decision to access contraception is often contentious and complicated. These tensions echo concerns and ambiguities contained within global and national reproductive health policy. Overwhelmingly, participants emphasised that despite her wishes, a woman can only rarely exercise her right to access contraception freely and independently. She is most often constrained by family, cultural, traditional and educational influences.

Background: While global maternal deaths have decreased significantly, hundreds of thousands of women still die from pregnancy and birth complications. Interventions such as skilled birth attendants, emergency transportation to health facilities and birth preparedness have been successful at reducing such deaths, however barriers to seeking, reaching, and receiving respectful care persist., Objective: This study aimed to identify what influences people's decisions to seek antenatal care and care during labour and birth in Timor-Leste, a low-middle income newly independent nation in South East Asia with a high maternal death rate. The study aimed to provide emic/local insights to help midwives and maternal health providers tailor care and resources appropriately, thus improving maternal health., Design: This qualitative study with a decolonising methodology, was designed to explore the perceptions of reproductive aged Timorese women and men, situating Timorese worldviews in the centre of the research process. Data collection occurred in four municipalities of Timor-Leste in October 2015 and included 9 focus group discussions with 80 men, and 17 individual reproductive history interviews with women., Findings: An expanded 'Three Delays' model was used to frame the findings. The study found multiple factors impacting on decisions to seek antenatal care and care during labour and birth. Husbands, history, minimal birth preparedness, ethno-physiological beliefs (personal perceptions of how the body works), infrastructure limitations, geographical location, hospital policies and staff attitudes influenced and potentially delayed the decision to seek or reach care., Key Conclusion and Implications for Practice and Policy: Policies and programs that increase accessibility of midwives and encourage birth preparedness are vital. Given the current locus of power in families in Timor-Leste, it is imperative that men are educated regarding the importance of care from skilled providers, and supported to access such care with their partners. Culturally respectful, inclusive and quality care needs to be emphasised so that trust is established between health providers and communities., (Copyright © 2018 Elsevier Ltd. All rights reserved.)

Maternal mortality remains a significant public health challenge for Timor-Leste. Although access to quality family planning measures may greatly reduce such deaths, consideration of indigenous perceptions, and how they influence reproductive health decision-making and behavior, is crucial if health services are to provide initiatives that are accepted and helpful in improving reproductive health outcomes. We aimed to demonstrate that body mapping is an effective method to traverse language and culture to gain emic insights and indigenous worldviews. The authors' two qualitative research projects (2013 and 2015) used a decolonizing methodology in four districts of Timor-Leste, body mapping with 67 men and 40 women to illuminate ethno-physiology and indigenous beliefs about conception, reproduction, and contraception. Body mapping provided a beneficial conduit for identifying established indigenous reproductive perceptions, understandings, and vocabulary, plus fears surrounding contraception. This may inform health service provision and engagement, ultimately improving the reproductive health of community members.

The use of modelling tools to support decision-makers to plan air quality policies is now quite widespread in Europe. In this paper, the Regional Integrated Assessment Tool (RIAT+), which was designed to support policy-maker decision on optimal emission reduction measures to improve air quality at minimum costs, is applied to the Porto Urban Area (Portugal). In addition to technological measures, some local measures were included in the optimization process. Case study results are presented for a multi-objective approach focused on both NO 2 and PM10 control measures, assuming equivalent importance in the optimization process. The optimal set of air quality measures is capable to reduce simultaneously the annual average concentrations values of PM10 and NO 2 in 1.7 and 1.0 μg/m 3 , respectively. This paper illustrates how the tool could be used to prioritize policy objectives and help making informed decisions about reducing air pollution and improving public health.

Air pollution is, increasingly, a concern to our society given the threats to human health and the environment. Concerted actions to improve air quality have been taken at different levels, such as through the development of Air Quality Plans (AQPs). However, air quality impacts associated with the implementation of abatement measures included in AQPs are often neglected. In order to identify the major gaps and strengths in current knowledge, a literature review has been performed on existing methodologies to estimate air pollution-related health impacts and subsequent external costs. Based on this review, the Impact Pathway Approach was adopted and applied within the context of the MAPLIA research project to assess the health impacts and benefits (or avoided external costs) derived from improvements in air quality. Seven emission abatement scenarios, based on individual and combined abatement measures, were tested for the major activity sectors (traffic, residential and industrial combustion and production processes) of a Portuguese urban area (Grande Porto) with severe particular matter (PM10) air pollution problems. Results revealed a strong positive correlation between population density and health benefits obtained from the assessed reduction scenarios. As a consequence, potential health benefits from reduction scenarios are largest in densely populated areas with high anthropic activity and, thus, where air pollution problems are most alarming. Implementation of all measures resulted in a reduction in PM10 emissions by almost 8%, improving air quality by about 1% and contributing to a benefit of 8.8 million €/year for the entire study domain. The introduction of PM10 reduction technologies in industrial units was the most beneficial abatement measure. This study intends to contribute to policy support for decision-making on air quality management., (Copyright © 2016 Elsevier Ltd. All rights reserved.)

When ambient air quality standards established in the EU Directive 2008/50/EC are exceeded, Member States are obliged to develop and implement Air Quality Plans (AQP) to improve air quality and health. Notwithstanding the achievements in emission reductions and air quality improvement, additional efforts need to be undertaken to improve air quality in a sustainable way - i.e. through a cost-efficiency approach. This work was developed in the scope of the recently concluded MAPLIA project "Moving from Air Pollution to Local Integrated Assessment", and focuses on the definition and assessment of emission abatement measures and their associated costs, air quality and health impacts and benefits by means of air quality modelling tools, health impact functions and cost-efficiency analysis. The MAPLIA system was applied to the Grande Porto urban area (Portugal), addressing PM10 and NOx as the most important pollutants in the region. Four different measures to reduce PM10 and NOx emissions were defined and characterized in terms of emissions and implementation costs, and combined into 15 emission scenarios, simulated by the TAPM air quality modelling tool. Air pollutant concentration fields were then used to estimate health benefits in terms of avoided costs (external costs), using dose-response health impact functions. Results revealed that, among the 15 scenarios analysed, the scenario including all 4 measures lead to a total net benefit of 0.3M€·y(-1). The largest net benefit is obtained for the scenario considering the conversion of 50% of open fire places into heat recovery wood stoves. Although the implementation costs of this measure are high, the benefits outweigh the costs. Research outcomes confirm that the MAPLIA system is useful for policy decision support on air quality improvement strategies, and could be applied to other urban areas where AQP need to be implemented and monitored., (Copyright © 2016. Published by Elsevier B.V.)

The increase of the share of renewable energy in Portugal can be met from different sources, of which forest biomass residues (FBR) can play a main role. Taking into account the demand for information about the strategy of FBR to energy, and its implications on the Portuguese climate policy, the impact of energy conversion of FBR on air quality is evaluated. Three emission scenarios were defined and a numerical air quality model was selected to perform this evaluation. The results reveal that the biomass thermal plants contribute to an increment of the pollutant concentrations in the atmosphere, however restricted to the surrounding areas of the thermal plants, and most significant for NO₂ and O₃., (Copyright © 2014 Elsevier B.V. All rights reserved.)

Quantifying the impact of air pollution on the public's health has become an increasingly critical component in policy discussion. Recent data indicate that more than 70% of the world population lives in cities. Several studies reported that current levels of air pollutants in urban areas are associated with adverse health risks, namely, cardiovascular diseases and lung cancer. IARC recently classified outdoor air pollution and related particulate matter (PM) as carcinogenic to humans. Despite the air quality improvements observed over the last few years, there is still continued widespread exceedance within Europe, particularly regarding PM and nitrogen oxides (NOx). The European Air Quality Directive 2008/50/EC requires Member States to design appropriate air quality plans for zones where air quality does not comply with established limit values. However, in most cases, air quality is only quantified using a combination of monitored and modeled data and no health impact assessment is carried out. An integrated approach combining the effects of several emission abatement measures on air quality, impacts on human health, and associated implementation costs enables an effective cost-benefit analysis and an added value to the decision-making process. Hence, this review describes the basic steps and tools for integrating health into air quality assessment (health indicators, exposure-response functions). In addition, consideration is given to two major outdoor pollutants: PM and NO2. A summary of the health metrics used to assess the health impact of PM and NO2 and recent epidemiologic data are also described.

In summer, high levels of ozone (O3) are frequently measured at both Galicia and Northern Portugal air quality monitoring stations, even exceeding the limit values imposed by legislation. This work aims to investigate the origin of these high O3 concentrations by the application of a chemical transport modelling system over the northwestern area of the Iberian Peninsula. The WRF-CHIMERE modelling system was applied with high resolution to simulate the selected air pollution episodes that occurred simultaneously in Galicia and North Portugal and in order to study both the contribution of local emission sources and the influence of transboundary pollution. Emission inputs have been prepared based on the development of the Portuguese and Galician emission inventories. The obtained results for O3 have been evaluated and validated against observations. Modelling results show possible contribution of the transboundary transport over the border of two neighbour regions/countries, indicating that the O3 episode starts over the urban and industrialised area of North coast of Portugal, reaching the maximum peaks over this region; at the same time, O3 levels increased over Galicia region, where lower concentrations, but still high, were observed. These results pointed out that air quality management should not be driven by political boundaries and highlight the importance of joining efforts between neighbouring countries.

A very high ozone episode with observed hourly values above 350 μg m(-3) occurred in July 2005 at the Lamas d'Olo air quality monitoring station, located in a mountainous area in the north of Portugal. Aiming to identify the origin and formation of this ozone-rich episode, a statistical analysis and a modelling approach were applied. A cross-spectrum analysis in the frequency domain and a synoptic analysis of the meteorological and air quality time series were performed. In order to go further in this analysis, a numerical modelling approach was applied. The results indicate that the transport of ozone and its precursors is the main responsible for the high ozone concentrations. Together with the local mountain breeze and subsidence conditions, the sea-breeze circulation transporting pollutants from the coastal urban and industrialized areas that reach the site during late afternoon turn out to be the driving forces for the ozone peaks., (Copyright © 2011 Elsevier Ltd. All rights reserved.)

The potential impacts of climate-induced changes in air pollution levels and its impacts on population health were investigated. The IPCC scenario (SRES A2) was used to analyse the effects of climate on future PM10 concentrations over Portugal and their impact on short-term population exposure and mortality. The air quality modelling system has been applied with high spatial resolution looking on climate changes at regional scale. To quantify health impacts related to air pollution changes, the WHO methodology for health impact assessment was implemented. The results point to 8% increase of premature mortality attributed to future PM10 levels in Portugal. The pollution episodes with daily average PM10 concentration above the current legislated value (50 μg·m⁻³) would be responsible for 81% of attributable cases. The absolute number of deaths attributable to PM10 under future climate emphasizes the importance of indirect effects of climate change on human health.

Smoke from forest fires contains significant amounts of gaseous and particulate pollutants. Firefighters exposed to wildland fire smoke can suffer from several acute and chronic adverse health effects. Consequently, exposure data are of vital importance for the establishment of cause/effect relationships between exposure to smoke and firefighter health effects. The aims of this study were to (1) characterize the relationship between wildland smoke exposure and medical parameters and (2) identify health effects pertinent to wildland forest fire smoke exposure. In this study, firefighter exposure levels of carbon monoxide (CO), nitrogen dioxide (NO₂), and volatile organic compounds (VOC) were measured in wildfires during three fire seasons in Portugal. Personal monitoring devices were used to measure exposure. Firefighters were also tested for exhaled nitric oxide (eNO) and CO before and after their firefighting activities. Data indicated that exposure levels during firefighting activities were beyond limits recommended by the Occupational Exposure Standard (OES) values. Medical tests conducted on the firefighters also indicated a considerable effect on measured medical parameters, with a significant increase in CO and decrease in NO in exhaled air of majority of the firefighters.

The main purpose of this work is to estimate the impact of forest fires on air pollution applying the LOTOS-EUROS air quality modeling system in Portugal for three consecutive years, 2003-2005. Forest fire emissions have been included in the modeling system through the development of a numerical module, which takes into account the most suitable parameters for Portuguese forest fire characteristics and the burnt area by large forest fires. To better evaluate the influence of forest fires on air quality the LOTOS-EUROS system has been applied with and without forest fire emissions. Hourly concentration results have been compared to measure data at several monitoring locations with better modeling quality parameters when forest fire emissions were considered. Moreover, hourly estimates, with and without fire emissions, can reach differences in the order of 20%, showing the importance and the influence of this type of emissions on air quality., (Copyright © 2011 Elsevier B.V. All rights reserved.)

Forest fires represent a serious threat to public security in Europe due to the large burned area. Moreover, smoke pollution due to forest fire events is an important public health issue for the communities directly affected, and particularly for the personnel involved in firefighting operations. Aiming to contribute to the scientific knowledge concerning firefighters exposure to forest fires smoke, data of individual exposure to carbon monoxide, nitrogen dioxide, volatile organic compounds, and particulate matter were obtained during experimental field fires for a group of 10 firefighters equipped with portable "in continuum" measuring devices. Measured values are very high exceeding the Occupational Exposure Standard limits, in particular for peak limit thresholds. These are the first measurements and analysis of firefighter's individual exposure to toxic gases and particles in fire smoke experiments in Europe. However, they already indicate that urgent measures to avoid these levels of exposure are needed., (Copyright 2010 Elsevier Ltd. All rights reserved.)

The main objectives of this work focus, firstly, on a review of the current existent methodologies to estimate air quality modelling uncertainty, and, secondly, in the preparation of guidelines for modelling uncertainty estimation, which can be used by local and regional authorities responsible for air quality management. From the application exercise, it was concluded that it is possible to define a subset of statistical parameters able to reproduce the general uncertainties estimation. Concerning the quality indicators defined by EU directives, the results show that the legislated uncertainty estimation measures are ambiguous and inadequate in several aspects, mainly in what concerns the error measures for hourly and daily indicators based on the highest observed concentration. A relative error at the percentile correspondent to the allowed number of exceedances of the limit value was suggested and tested, showing that is a more robust and appropriate parameter for model performance evaluation.

According to the Air Quality Framework Directive, air pollutant concentration levels have to be assessed and reported annually by each European Union member state, taking into consideration European air quality standards. Plans and programmes should be implemented in zones and agglomerations where pollutant concentrations exceed the limit and target values. The main objective of this study is to perform a long-term air quality simulation for Portugal, using the CHIMERE chemistry-transport model, applied over Portugal, for the year 2001. The model performance was evaluated by comparing its results to air quality data from the regional monitoring networks and to data from a diffusive sampling experimental campaign. The results obtained show a modelling system able to reproduce the pollutant concentrations' temporal evolution and spatial distribution observed at the regional networks of air quality monitoring. As far as the fulfilment of the air quality targets is concerned, there are excessive values for nitrogen and sulfur dioxides, ozone also being a critical gaseous pollutant in what concerns hourly concentrations and AOT40 (Accumulated Over Threshold 40 ppb) values.

The Framework Directive (FWD) and the proposed Daughter Directives are the newest legislative instruments concerning a new political strategy and air quality management approach for Europe. Additionally, the member countries of the United Nations Economic Commission for Europe have included the concepts of critical load and level for planning air pollution abatement strategies and as a base of international agreements concerning limitation of the emissions of air pollutants. These concepts imply an accurate knowledge about pollutants deposition fluxes. The paper describes the main needs and the tools available to define a strategy of air quality management in Portugal. Two study cases are presented: (1) extensive monitoring plan to assess the impact of an urban incinerator plant; and (2) contribution to a methodology to estimate critical levels for a coastal region in Portugal. These different approaches allowed illustrating the complexity of the implementation of an air pollution management strategy.

Volatile organic compounds (VOCs) are the main precursors of tropospheric ozone production, playing an important role in photochemical pollution of the atmosphere and, consequently, in the degradation of air quality. Air quality photochemical models require a specific VOC profile for each different main source, based on the most important group compounds. Chromatographic techniques have been used to identify and measure VOC in Portugal. These measured values were used to simulate photochemical pollution, and modelling results were compared with those from another simulation using VOC class distributions from the literature. Ozone concentration values estimated via both simulations indicate the importance of using VOC data from Portugal instead of those obtained in different conditions.

A forecast of expected evolution of carbon dioxide (CO(2)) emissions in Portugal between 1988 and 2010 is presented. Predictions show that CO(2) emissions will almost double in the next twenty years. The equivalent potential CO(2) emissions from nitrogen oxides (NO(x)) and volatile organic compounds (VOC), for a time horizon of 20 years, is also presented. NO(x) and VOC emissions seem to make a significant contribution to the global warming potential of Portuguese emissions. Estimates of CO(2) emissions due to forest fires have been made, oriented towards the study of the Portuguese contribution to the global warming. If the burned area exceeds 100 000 ha this contribution could reach 7% of the total Portuguese CO(2) emissions. The global warming potential of Portuguese forest emissions were also calculated. The climate change predicted to Portugal could be responsible for an increase in the forest fires and consequently for a greater contribution of its emissions to the total values. It was concluded that it is important to quantify emissions of the greenhouse gases, including the contribution of forest fire emissions, not only in Portugal, but in all the Southern European countries.