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The discovery of live 60Fe in a deep-sea crust with proposed interstellar origin followed by evidence for elevated interplanetary 3He in the same crust raised the question on how to unambiguously identify the true production site of the identified 60Fe. Here, we show the implementation of the dyadic radionuclide system 60Fe / 53Mn to serve as a tool for the identification of surplus interstellar 60Fe over interplanetary production. The recent updates in experimental 60Fe and 53Mn data from iron meteorites as well as in production rate models confirm the validity and robustness of this dyadic system for future applications.

We explore the spatial and temporal variations in denudation rates in the northern Pamir—Tian Shan region using 10Be‐derived denudation rates from modern (n = 110) and buried sediment (2.0–2.7 Ma; n = 3), and long‐term exhumation rates from published apatite fission track (AFT; n = 705) and apatite (U‐Th‐Sm)/He (AHe; n = 211) thermochronology. We found moderate correlations between denudation rates and topographic metrics and weak correlations between denudation rates and annual rainfall, highlighting complex linkages among tectonics, climate, and surface processes that vary locally. The 10Be data show a spatial trend of decreasing modern denudation rates from west to east, suggesting that deformation and precipitation control denudation in the northern Pamir and western Tian Shan. Farther east, the denudational response of the landscape to Quaternary glaciations is more pronounced and reflected in our data. Modern 10Be denudation rates are generally higher than the long‐term AFT and AHe exhumation rates across the studied area. In the Kyrgyz Tian Shan, on average, the highest 10Be denudation rates are recorded in the Terskey range, south of Lake Issyk‐Kul. Here, modern denudation rates are higher than 10Be‐derived paleo‐denudation rates, which are comparable in magnitude with the long‐term exhumation rates inferred from AFT and AHe. We propose that denudation in the region, particularly in the Terskey range, remained relatively steady during the Neogene and early Pleistocene. Denudation increased due to glacial‐interglacial cycles in the Quaternary, but this occurred after the onset and intensification of the Northern Hemisphere glaciations at 2.7 Ma. Plain Language Summary: Tectonic forces create mountains, while climatically modulated erosion breaks them down into sediment that rivers carry to the final depositional basin. This cycle affects global climate over long periods, but it's unclear whether mountain uplift causes climate change or if climate cooling leads to faster erosion and mountain uplift. To tackle these questions, we explore temporal and spatial changes in rates of denudation in the northern Pamir—Tian Shan region and find that rates remained steady during the Neogene and early Pleistocene but increased due to glacial‐interglacial cycles in the Quaternary. We also find that modern denudation rates decrease from west to east. This suggests that tectonic deformation controls denudation in the northern Pamir and western Tian Shan, while further east the denudational response of the landscape to Quaternary glaciations is more pronounced and reflected in our data. Dominant controls on modern denudation rates vary across the mountain range and reflect local factors. Our results highlight how the evolution of mountain belts strongly depends on denudation, which reflects complex interactions between tectonics, climatic changes, and surface processes, and show how in the northern Pamir—Tian Shan region, climate cooling during the Quaternary period resulted in faster erosion rates. Key Points: Modern denudation rates are higher than paleo‐denudation rates from 2.0 to 2.7 Ma and exhumation rates inferred from thermochronologyDenudation in the Terskey range remained steady during the Neogene and early Pleistocene and then increased in the Quaternary after 2.0 MaThe denudational response to Quaternary glaciations is detectable in the Kyrgyz and Chinese portions of the Tian Shan [ABSTRACT FROM AUTHOR]

The long-lived radioisotope 182Hf (T1/2 = 8.9 Ma) is of high astrophysical interest as its potential abundance in environmental archives would provide insight into recent r-process nucleosynthesis in the vicinity of our solar system. Despite substantial efforts, it could not be measured at natural abundances with conventional AMS so far due to strong isobaric interference from stable 182W. Equally important is an increase in ion source efficiency for the anions of interest. The new Ion Laser InterAction Mass Spectrometry (ILIAMS) technique at VERA tackles the problem of elemental selectivity in AMS with a novel approach. It achieves near-complete suppression of isobar contaminants via selective laser photodetachment of decelerated anion beams in a gas-filled radio-frequency quadrupole (RFQ) ion cooler. The technique exploits differences in electron affinities (EA) within elemental or molecular isobaric systems neutralizing anions with EAs smaller than the photon energy. Alternatively, these differences in EA can also facilitate anion separation via chemical reactions with the buffer gas. We present first results with this approach on AMS-detection of 182Hf. With He +O2 mixtures as buffer gas in the RFQ, suppression of 182WF5− vs 180HfF 5− by >105 has been demonstrated. Mass analysis of the ejected anion beam identified the formation of oxyfluorides as an important reaction channel. The overall Hf-detection efficiency at VERA presently is 1.4% and the W-corrected blank value is 182Hf/180Hf = (3.4 ± 2.1)×10−14. In addition, a survey of different sample materials for highest negative ion yields of HfF 5− with Cs-sputtering has been conducted.

Activations with neutrons in the keV energy range were routinely performed at the Karlsruhe Institute of Technology (KIT) in Germany in order to simulate stellar conditions for neutron-capture cross sections. A quasi-Maxwell-Boltzmann neutron spectrum of kT = 25 keV, being of interest for the astrophysical s-process, was produced by the 7Li(p,n) reaction utilizing a 1912 keV proton beam at the Karlsruhe Van de Graaff accelerator. Activated samples resulting in long-lived nuclear reaction products with half-lives in the order of yr 100 Myr were analyzed by Accelerator Mass Spectrometry (AMS). Comparison of the obtained reaction cross sections to literature data from previous Time-of-Flight (ToF) measurements showed that the selected AMS data are systematically lower than the ToF data. To investigate this discrepancy, 54Fe(n,γ)55Fe and 35Cl(n,γ)36Cl reaction cross sections were newly measured at the Frankfurt Neutron Source (FRANZ) in Germany. To complement the existing data, an additional neutron activation of 54Fe and 35Cl at a proton energy of 2 MeV was performed. The results will give implications for the stellar environment at kT = 90 keV, reaching the not yet experimentally explored high-energy s-process range. AMS measurements of the activated samples are scheduled.