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For the deep reduction of nitrogen, the microbial fuel cell-constructed wetland (MFC-CW) was conducted for treating carbon constraint wastewater. Results indicated that nitrogen removal decreased from 94.96% to 24.96% with influent COD/TN (chemical oxygen demand/total nitrogen) from 4 to 0. MFC-CW was seriously affected by low organic wastewater. Wetland plants contributed to denitrification, with TN removal increasing from 46.13% to 64.87%. The bioenergy output showed a linear relationship with influent COD, and the maximum power density of 1.17 mW/m

To solve wetland plant litter disposal and improve the nitrogen removal of carbon-limited wastewater, the integration of microbial fuel cell (MFC) and recycled utilization of ryegrass litter planted in constructed wetland (CW) may be effective. CW and MFC-CW with periodical ryegrass litter addition (10 days one cycle) were constructed to study the effects of ryegrass litter on nitrogen removal, electricity production and microorganism community. The results showed that total nitrogen removal of CW and MFC-CW after ryegrass litter addition reached 80.54 ± 10.99% and 81.94 ± 7.30%, increased by 22.19% and 17.50%, respectively. Three-dimensional excitation emission matrix fluorescence spectroscopy results revealed that the soluble organic matters produced by the hydrolyzed ryegrass litter were mainly tryptophan, tyrosine and fulvic acid, which promoted the growth of microorganisms and denitrification. The dosage of 200 g m

Advanced processing of low C/N sewage faces the carbon sources shortage, while quantities of agricultural biomass wastes need to be disposed. This study investigated the potential of quantitative modified biomass addition in constructed wetlands (CWs) filled with polyethylene fillers. Results showed that the lignin in NaOH-heating pretreated corn stalks (NH-CSs) was destroyed, and the wrinkles on the stalks increased and became more soft after pretreatment, which was more conducive to the utilization of carbon sources and attachment of microorganisms. Compared with glucose and sodium acetate, the denitrification with mixed carbon source (glucose and NH-CSs) had the highest effective utilization percentage (61.37%) and NH-CSs were expected to become stable and fast-release carbon sources. After adding 30 g NH-CSs to the rear unit of CW with polyethylene fillers (CW-A), TN removal efficiency was increased by 18.21%, and the average removal efficiency of COD, NH4+-N, TN, and TP reached 54.83%, 89.95%, 64.11%, and 45.04%, respectively. Compared with the traditional CW (CW-B), CW-A had a significant denitrification advantage (P

Stormwater runoff is identified as a major source of pollution in water bodies, and to limit the impact of these pollutants on groundwater quality, permeable asphalt pavement systems (PAPS) have been built worldwide. But so far, few have considered zeolite or regulated zeolite as a post-treatment in reservoirs in PAPS. This study aimed at investigating the efficiencies of modified zeolites in removing NH4+-N and TP from stormwater runoff and providing a novel insight into the research on the reuse of stormwater runoff by PAPS. The effect of PAPS with a zeolite-regulated reservoir on removing nutrient in stormwater was explored by artificial rainfall experiments and temporary storage experiments. Results showed that the removal rate of NH4+-N and TP in PAPS with a regulated-zeolite reservoir increased by 23.7% and 37.2%, respectively, during simulated rainfall events when compared to those without a regulated-zeolite reservoir. TP was mainly removed by the form of phosphorus precipitation such as Zr(H2PO4)2. Ion exchange and adsorption during the temporary storage period were considered as the main approaches for removal of NH4+-N and TP. This study can help develop an optimal strategy for the operation of PAPS in treating stormwater runoff from urban roads.

This study was aimed to investigate the removal processes of nitrogen (TN), NH4+-N and phosphorus (TP) from surface runoff by performing experiments on the filter layers in porous asphalt pavement (PAP). Experiments were conducted to compare the differences of the filter layer placed at the top, the middle or the bottom of PAP. The effects of retention time on the removal of the pollutants and the adsorption capacity of PAP materials were also investigated. Results indicated that the filter layer placed under the bed course improved the removal rates of pollutants compared to the other two cases on the whole. The concentration of TP in the effluent decreased by 80% after the 48 h retention time. In conclusion, this study demonstrated that the positions of filter layers and the temporary retention time of surface runoff within the bed course of PAP were critical parameters for determining the removal processes of pollutants. Thus, a certain retention time for surface runoff in bed course is of great importance for PAP to serve as an effective low impact development technology for stormwater management.

Bioretention has great potential in managing and purifying urban stormwater runoff. However, information regarding the removal of nutrients in bioretention systems with the use of media, plants, and saturated areas is still limited. In this study, three devices of control, conventional bioretention (DS), and strengthened bioretention (SZ) were investigated to enhance the simultaneous removal of nitrogen and phosphorus. The experimental column SZ showed the best performance for total phosphorus (TP), ammonia (NH4+-N) and total nitrogen (TN) removal (85.6&ndash, 92.4%, 83.1&ndash, 92.7%, 57.1&ndash, 74.1%, respectively), whereas DS columns performed poorly for NH4+-N removal (43.6&ndash, 81.2%) under different conditions. For the removal of nitrate, the columns of Control and DS exhibited negative performance (&minus, 14.3% and &minus, 8.2%) in a typical event. Further evaluation of water quality revealed that in the early stages of rainfall, the effluent of the SZ column was able to reach quality standards of Grade IV for surface water in China. Moreover, although the ion-exchange and phosphate precipitation occurred on the surface of the media, which were placed in the saturation zone, it did not change the surface crystal structure.

A microbial fuel cell–constructed wetland (MFC-CW) with water hyacinth is established to remove the nitrogen and organics from municipal wastewater treatment plants (WWTPs) effluents. Because insufficient carbon sources in influent might decrease pollutants removal efficiency and electricity generation, this research aimed to select high-quality and low-cost biomass as additional carbon source to improve the performance of MFC-CW. Cellulose and hemicellulose (xylan) were chosen as the biomass. Results indicated that xylan displayed a higher nitrate removal (above 92%) compared with cellulose (10.9%). With xylan as carbon source, the anode packing removed nitrate above 80%, while the cathode packing only removed around 50%. With glucose as sole carbon source, the maximum total nitrogen (TN) removal of MFC-CW was 87.66 ± 4.23%, which was higher than that of MFC (85.58 ± 4.14%). The chemical oxygen demand (COD) and TN in the effluent of MFC-CW were maintained below 25 mg/L and 1.5 mg/L, respectively, with the COD/TN ratio around 5.4 and hydraulic retention time (HRT) at 48 h. The TN removal reached the maximum efficiency of 88.78 ± 3.98% when glucose and xylan ratio was in 40%:60% as composite carbon sources, and COD and TN in the effluent were below 20 mg/L and 1.5 mg/L, respectively. In addition, xylan as the additional carbon source significantly promoted the power density compared with sole glucose. Microbial community diversity in the MFC-CW was significantly higher than that in the single MFC or CW. Proteobacteria and Cyanobacteria_norank were relatively more dominant in the MFC-CW than those in the single MFC or CW, which accounted for high nitrogen removal and power generation. Findings in this study proved that MFC-CW with biomass addition enhanced nitrogen removal and power generation.

Nitrogen residues in effluent from municipal wastewater treatment deteriorate aquatic ecosystem, and the common method is to add external carbon sources. Considering the low cost and easy availability, agricultural biomasses are often applied as the external carbon sources for carbon-limited wastewater treatment. This research estimated the feasibility of adding agricultural wastes to simultaneously enhance nitrogen removal and bioelectricity generation in microbial fuel cell-constructed wetland (MFC-CW), and the results were compared to those in MFC. Different agricultural wastes (corncob, straw, rice husk) were compared, and corncob showed a higher carbon release ability. The results revealed that the carbon release of corncob was a diffusion process, and fitted the second-order kinetics with the highest released chemical oxygen demand (COD) of 47.6 mg·(g·L)−1. Corncob addition significantly enhanced the nutrients removal in MFC-CW with original influent COD of 22 mg L−1, and the maximum total nitrogen (TN), nitrate nitrogen (NO3−-N), ammonia nitrogen (NH4+-N) removals were 86.6 ± 1.6%, 97.2 ± 0.3%, 73.1 ± 2.8%, respectively. Besides, the bioelectricity generation performance was also promoted with the maximum voltage and power density of 340 mV and 23.5 mW/m3, whereas the internal resistance slightly increased. The findings provide an economic way for nitrogen removal, energy recovery and agricultural wastes management by MFC-CW when treating carbon-limited wastewater.