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We have measured black carbon (BC) concentrations at Syowa Station, Antarctica, since February 2005. The measured BC concentrations in 2005–2016 were corrected to equivalent BC (EBC) concentrations using Weingartner's method. Seasonal features of EBC concentrations, long-range transport from mid-latitudes to the Antarctic coast, and their origins were characterized. Results show that daily median EBC concentrations were below the detection limit (0.2 ng m−3) to 63.8 ng m−3 at Syowa Station (median, 1.8 ng m−3; mean, 2.7 ng m−3 during the measurement period of February 2005–December 2016). Although seasonal features and year-to-year variations in EBC concentrations were observed, no long-term trend of EBC concentrations was clear during our measurement period. Seasonal features of EBC concentrations showed a spring maximum during September–October at Syowa Station. To elucidate EBC transport processes, origins, and the potential source area (PSA), we compared EBC data to backward trajectory analysis and chemical transport model simulation. From comparison with backward trajectory, high EBC concentrations were found in air masses from the marine boundary layer. This finding implies that transport via the marine boundary layer was the most important transport pathway to EBC concentrations at Antarctic coasts. Some EBC was supplied to the Antarctic region by transport via the upper free troposphere. Chemical transport model simulation demonstrated that the most important origins and PSA of EBC at Syowa Station were biomass burning in South America and southern Africa. Fossil fuel combustion in South America and southern Africa also have important contributions. The absorption Ångström exponent (AAE) showed clear seasonal features with 0.5–1.0 during April–October and maximum (1.0–1.5) in December–February. The AAE features might be associated with organic aerosols and mixing states of EBC.

The majority of aerosol data are obtained from daytime measurements, and there are few datasets available for studying nighttime aerosol characteristics. In order to estimate the aerosol optical depth (AOD) and the precipitable water vapor (PWV) during the nighttime using the moon as a light source, a sky radiometer (POM-02, Prede Ltd., Japan) was modified. The amplifier was adjusted so that POM-02 could measure lower levels of input irradiance. In order to track the moon based on the calculated values, a simplified formula was incorporated into the firmware. A new position sensor with a four-quadrant detector to adjust the tracking of the Sun and moon was also developed. The calibration constant, which is the sensor output for the extraterrestrial solar and lunar irradiance at the mean Earth–Sun distance, was determined by using the Langley method. The measurements for the Langley calibration were conducted at the National Oceanic and Atmospheric Administration/Mauna Loa Observatory (NOAA/MLO) from 28 September 2017 to 7 November 2017. By assuming that the correct reflectance is proportional to the reflectance estimated by the Robotic Lunar Observatory (ROLO) irradiance model, the calibration constant for the lunar direct irradiance was successfully determined using the Langley method. The ratio of the calibration constant for the moon to that of the Sun was often greater than 1; the value of the ratio was 0.95 to 1.18 in the visible and near-infrared wavelength regions. This indicates that the ROLO model often underestimates the reflectance. In addition, this ratio depended on the phase angle. In this study, this ratio was approximated by a quadratic equation of the phase angle. By using this approximation, the reflectance of the moon can be calculated to within an accuracy of 1 % or less. In order to validate the estimates of the AOD and PWV, continuous measurements with POM-02 were conducted at the Japan Meteorological Agency/Meteorological Research Institute (JMA/MRI) from January 2018 to May 2018, and the AOD and PWV were estimated. The results were compared with the AOD and PWV obtained by independent methods. The AOD was compared with that estimated by the National Institute for Environmental Studies (NIES) High Spectral Resolution Lidar measurements (wavelength: 532 nm), and the PWV was compared with the PWV obtained from a radiosonde and the Global Positioning System. In addition, the continuity of the AOD (PWV) before and after sunrise and sunset in Tsukuba was examined, and the AOD (PWV) of AERONET and that of POM-02 at MLO were compared. In the results, the daytime and nighttime AOD (PWV) measurements are shown to be statistically almost equivalent. The AODs (PWVs) during the daytime and nighttime for POM-02 are presumed to have the same degree of precision and accuracy within the measurement uncertainty.

We measured equivalent black carbon (EBC) concentrations at Syowa Station, Antarctica from February 2005 to characterize seasonal features of EBC concentrations and their origins, and to monitor long-range transport of aerosols from mid-latitudes to the Antarctic coast. Results show that EBC concentrations were below the detection limit (0.2 ng m−3) to 63.8 ng m−3 at Syowa Station (median, 1.8 ng m−3; mean, 2.7 ng m−3 during the measurement period). Although seasonal features and year-to-year variations of EBC concentrations were observed, no long-term trend of EBC concentrations was clear during our measurement period. Seasonal features of EBC concentrations showed a spring maximum during September–October at Syowa Station. The absorption Ångström exponent (AAE) was 0.5–1.0 during April–October; it reached its maximum values (1.0–1.5) during summer. The AAE features imply that EBC was mixed internally in the Antarctic troposphere and that organic aerosols engendered high AAE in the summer. To elucidate EBC transport processes, origins, and the potential source area (PSA), we compared EBC data to backward trajectory analysis and model simulation. Results show that EBC might be transported directly to Syowa Station from mid-latitudes mainly via the boundary layer and the lower free troposphere. Some BC was transported to Antarctic regions via the upper free troposphere. Biomass burning in South America and southern Africa is the most dominant PSA for BC transported to Syowa Station. Fossil fuel combustion in South America and southern Africa also have important contributions.

The Ninth Symposium on Polar Science/Ordinary sessions: [OM] Polar meteorology and glaciology, Wed. 5 Dec. / Entrance Hall (1st floor), National Institute of Polar Research

The Ninth Symposium on Polar Science/Ordinary sessions: [OM] Polar meteorology and glaciology, Wed. 5 Dec. / Entrance Hall (1st floor), National Institute of Polar Research

The Ninth Symposium on Polar Science/Ordinary sessions: [OM] Polar meteorology and glaciology, Wed. 5 Dec. / Entrance Hall (1st floor), National Institute of Polar Research

The Ninth Symposium on Polar Science/Ordinary sessions: [OM] Polar meteorology and glaciology, Wed. 5 Dec. / Entrance Hall (1st floor), National Institute of Polar Research

A method is proposed for detecting clouds from whole-sky color images obtained with an all-sky camera (ASC) system. In polar regions, cloud detection using whole-sky images usually suffers from large uncertainties in fractional cloud cover retrievals because of large solar zenith angles (SZAs) and high surface albedo, which cause “whitening” in the images. These problems are addressed by using differences between real images and virtual clear-sky images for a particular observation time with the same SZA. The method is applied to ASC images obtained at Ny-Alesund, Svalbard in May of 2005–2007, and the results are compared with Micro-Pulse Lidar (MPL) measurements. When no clouds were detected by MPL, the false cloud detection rate from ASC classification was 2.1% in total hours. Conversely, when clouds were detected by MPL, the ASC classification underestimated the clouds by 11.6%. In most cases, this occurred when MPL detected very optically thin clouds. Furthermore, the variability of cloud fractions estimated by MPL and ASC was roughly constant regardless of the SZA. Thus, it is confirmed that the method developed in this study is valid for cloud detection from whole-sky color images.

動揺する船上においても太陽直達光を観測できるように，船舶用スカイラジオメータの太陽追尾性能を改良した．改良点は，太陽追尾精度の向上，測器視野角の拡大，太陽追尾速度の迅速化および測定手法の改良である．改良後の装置を用いて，第51次および第52次日本南極地域観測隊の本観測時に，南極観測船「しらせ」船上において太陽直達光および天空輝度分布を測定し，動揺した船上での直達光観測に成功した．直達光から算出された波長500nm における大気エアロゾルの光学的厚さは0.01-0.34であり，東南アジアおよび春季の西太平洋上で高い値を示した．オングストローム指数は－0.06～2.00の範囲であり，東南アジアおよびシドニー付近で最大を示した．今後，船舶用スカイラジオメータが，海洋上の大気エアロゾルに関する知見を深めると期待される．, The sun-tracking performance of a shipborne sky radiometer was improved to attain accurate aerosol optical thickness (AOT) from direct solar measurements on a pitching and rolling vessel. Improvements were made in the accuracy of sun-pointing measurements, field-of-view expansion, sun-tracking speed, and measurement method. Radiometric measurements of direct solar and sky brightness distribution were performed using the shipborne sky radiometer onboard the Antarctic research vessel (R/V) Shirase during JARE-51 (2009-2010) and JARE-52 (2010-2011). The temporal variation of signal intensity measured by the radiometer under cloudless conditions was smooth, demonstrating that the radiometer could measure direct sunlight onboard the R/V. AOT at 500 nm ranged from 0.01 to 0.34, and values over Southeast Asia and over the western Pacific Ocean in spring were higher than those over other regions. The Angstrom exponent ranged from －0.06 to 2.00, and values over Southeast Asia and off the coast near Sydney were the highest. The improved shipborne sky radiometer will contribute to a good understanding of the nature of aerosols over the ocean.

Unusual aerosol enhancement is often observed at Syowa Station, Antarctica, during winter and spring. Simultaneous aerosol measurements near the surface and in the upper atmosphere were conducted twice using a ground-based optical particle counter, a balloon-borne optical particle counter, and micropulse lidar (MPL) in August and September 2012. During 13–15 August, aerosol enhancement occurred immediately after a storm condition. A high backscatter ratio and high aerosol concentrations were observed from the surface to ca. 2.5 km over Syowa Station. Clouds appeared occasionally at the top of the aerosol-enhanced layer during the episode. Aerosol enhancement was terminated on 15 August by strong winds from a cyclone's approach. In the second case, on 5–7 September, aerosol number concentrations in Dp > 0.3 μm near the surface reached > 104 L−1 at about 15:00 UT (Universal Time) on 5 September despite calm wind conditions, whereas MPL measurement exhibited aerosols were enhanced at about 04:00 UT at 1000–1500 m above Syowa Station. The aerosol enhancement occurred near the surface to ca. 4 km. In both cases, air masses with high aerosol enhancement below 2.5–3 km were transported mostly from the boundary layer over the sea-ice area. In addition, air masses at 3–4 km in the second case came from the boundary layer over the open-sea area. This air mass history strongly suggests that dispersion of sea-salt particles from the sea-ice surface contributes considerably to aerosol enhancement in the lower free troposphere (about 3 km) and that the release of sea-salt particles from the ocean surface engenders high aerosol concentrations in the free troposphere (3–4 km). Continuous MPL measurements indicate that high aerosol enhancement occurred mostly in surface–lower free troposphere (3 km) during the period July–September.

Cloud observations over the past decade from six Arctic atmospheric observatories are investigated to derive estimates of cloud occurrence fraction, vertical distribution, persistence in time, diurnal cycle, and boundary statistics. Each observatory has some combination of cloud lidar, radar, ceilometer, and/or interferometer for identifying and characterizing clouds. By optimally combining measurements from these instruments, it is found that annual cloud occurrence fractions are 58%–83% at the Arctic observatories. There is a clear annual cycle wherein clouds are least frequent in the winter and most frequent in the late summer and autumn. Only in Eureka, Nunavut, Canada, is the annual cycle shifted such that the annual minimum is in the spring with the maximum in the winter. Intersite monthly variability is typically within 10%–15% of the all-site average. Interannual variability at specific sites is less than 13% for any given month and, typically, is less than 3% for annual total cloud fractions. Low-level clouds are most persistent at the observatories. The median cloud persistence for all observatories is 3–5 h; however, 5% of cloud systems at far western Arctic sites are observed to occur for longer than 100 consecutive hours. Weak diurnal variability in cloudiness is observed at some sites, with a daily minimum in cloud occurrence near solar noon for those seasons for which the sun is above the horizon for at least part of the day.

東京海洋大学「海鷹丸」の南極海研究航海において,大気エアロゾルの光学的厚さ(AOT)の観測を実施した.南極海インド洋セクターでの500 nmでのAOTは,0.02-0.12の範囲であった.南極大陸沿岸域でのAOTは比較的低く,0.02前後であった.40-60゜Sの海域では,0.1以上の値を示すことがあった.インド洋低中緯度帯でのAOTは,0.05-0.15の範囲であった.風速とAOTとに正の相関がみられたことから,南極海では光学的に海塩粒子が卓越し,風速がAOTに影響を及ぼしていると考えられる.AOTが高くなるにつれ,オングストローム指数は減少した.AOTの波長スペクトルにおいて,380 nmと870 nmのAOTはべき関数からずれる傾向がみられた.レイリーの光学的厚さの算出方法を比較したところ,ずれが大幅に改善される可能性が示された.今後,より観測精度を高めていくためには,機器定数の精度を把握するとともに,レイリーの光学的厚さの算出方法の見直しなどが必要である., Aerosol optical thickness (AOT) was measured during Antarctic research cruises of R V Umitaka-Maru. The measured AOTs at 500 nm in the Indian sector of the Antarctic Ocean ranged from 0.02 to 0.12. In Antarctic coastal waters, the AOTs were as low as around 0.05. On the other hand, the some AOTs were higher than 0.1 from 40゜S to 60゜S. In middle and low latitude regions of the Indian Ocean, the AOTs ranged from 0.05 to 0.15. The AOTs were correlated with wind speed. It is indicated that sea-salt particles, generated by wind, dominated optically and wind speed affected the AOT in the Antarctic Ocean. Angstro¨m exponent decreased with increasing AOT. In the AOT wavelength spectra, some AOTs in 380 nm and 870 nm tended to deviate from the power function. Comparing calculation methods of Rayleigh optical thickness suggested a possibility of reducing the deviations of these AOTs. In the future, accuracy check of the instrument constant and review of the calculation method of Rayleigh optical thickness are recommended to enhance the accuracy of maritime AOT measurement.

Ten-year (2004–2013) observations of cloud and surface shortwave (SW) and longwave (LW) fluxes at Ny-Ålesund were analysed to investigate monthly variations in cloudiness and their impacts on the surface LW radiation budget and near-surface temperature (Ts). The cloud fraction (CF) showed distinct monthly variations, high in summer (0.90) and lower in winter (0.79). The downward SW flux increased from March and showed a peak (~200 W m−2) in June. In contrast, the downward LW (LWD) flux increased from ~200 W m−2 in February to ~300 W m−2 in July. Both LWD and upward LW (LWU) fluxes and their difference increased during winter as lowest cloud base height (LCBH) decreased and CF increased. Ts difference and both LW fluxes difference (ΔLWD and ΔLWU), calculated as the difference in monthly mean Ts and LW between all-sky and cloud-free conditions, were highly correlated (R2 = 0.68 for LWD and R2 = 0.92 for LWU). Dramatic changes in Ts, CF and LW fluxes at Ny-Ålesund were closely associated with cold and warm air mass advection on a multi-day time scale. The average Ts under low-level clouds (LCBH ≤ 2 km) was estimated as −7.4 ± 6.1 °C due to warm air masses advected from the North Atlantic Ocean and Barents Sea, whereas the average Ts on cloud-free days was −14.5 ± 5.7 °C because of cold air mass advection from the pole. However, the duration of low-level clouds may not be long enough to drive such large Ts variations. 75-percentile of low-level cloud conditions at Ny-Ålesund persisted up to 2.3 days, whereas cloud-free and high-altitude cloud (LCBH > 2 km) conditions lasted for approximately 0.8 and 0.5 days, respectively. This implies that cloud LW effects on several warm days may be larger than the monthly average, but may not be accumulated enough to induce surface warming due to abrupt Ts drop associated with cold air mass advection.

During the Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR) in March and April 2007, measurements obtained at the AWIPEV Arctic Research Base in Ny-Ålesund, Spitsbergen at 78.9° N, 11.9° E (operated by the Alfred Wegener Institute for Polar and Marine Research – AWI and the Institut polaire français Paul-Emile Victor – IPEV), supported the airborne campaign. This included lidar data from the Koldewey Aerosol Raman Lidar (KARL) and the Micro Pulse Lidar (MPL), located in the atmospheric observatory as well as photometer data and the daily launched radiosonde. The MPL features nearly continuous measurements; the KARL was switched on whenever weather conditions allowed observations (145 h in 61 days). From 1 March to 30 April, 71 meteorological balloon soundings were performed and compared with the concurrent MPL measurements; photometer measurements are available from 18 March. For the KARL data, a statistical overview of particle detection based on their optical properties backscatter ratio and volume depolarization can be given. The altitudes of the occurrence of the named features (subvisible and visible ice and water as well as mixed-phase clouds, aerosol layers) as well as their dependence on different air mass origins are analyzed. Although the spring 2007 was characterized by rather clean conditions, diverse case studies of cloud and aerosol occurrence during March and April 2007 are presented in more detail, including temporal development and main optical properties as depolarization, backscatter and extinction coefficients. Links between air mass origins and optical properties can be presumed but need further evidence.

During the period of scientific campaign "Arctic Study of Tropospheric Aerosols, Clouds and Radiation 2004" (ASTAR2004), precipitation samples were collected in late spring at Ny-Alesund, Svalbard and their ionic components were analyzed in parallel with the measurement of properties of atmospheric aerosol particles at the same place. Backward trajectory analyses indicated that the air mass above the observatory initially dominated by air masses from the Arctic Ocean, then those from western Siberia and later those from Greenland and the Arctic Ocean. In the measurement period, six precipitation samples were obtained and five of them were analyzed their ionic components by ionchromatography. The concentrations of nss-sulphate in precipitations were between 1.8 and 24.6 ppm from which the scavenging ratio and scavenging coefficients were calculated using the data such as the concentrations of nss-sulphate in aerosol particles, amounts of precipitations, and the heights of precipitations obtained from radar echo data. The scavenging ratio ranged from 1.0×106 to 17×106 which are comparable values reported in other areas. A detailed comparison between precipitation events and the number concentration of aerosol particles obtained from optical particle counters suggests that the type of precipitations, i.e. rain or snow, significantly affects the number concentrations of aerosol particles.

The dynamic seeding and glaciation of a mixed-phase cloud by ice crystals injected from above at Ny Alesund, Svalbard, Norway is described using continuous lidar measurements and thermodynamic data. Glaciation of this cloud was caused by ice crystal growth and sedimentation due to the preferential differences in saturation vapor pressure over ice versus liquid water and riming. The lidar data suggest that precipitation reached the ground for nearly 4 h as a result. The symbiosis between ice and liquid water hydrometeor presence in the polar troposphere is unique. Thermal perturbations and airmass fluctuations influence microphysical cloud characteristics and radiative balance, which makes the otherwise pristine region sensitive to lower-latitude anthropogenic and biogenic influences and a focal point for observing indirect effects and their influence on climate change. The development of lidar technologies capable of continuous and autonomous measurements is yielding important datasets to study unique atmospheric phenomena.

In spring 2006, the European Arctic was abnormally warm, setting new historical temperature records. During this warm period, smoke from agricultural fires in Eastern Europe intruded into the European Arctic and caused the most severe air pollution episodes ever recorded there. This paper confirms that biomass burning (BB) was indeed the source of the observed air pollution, studies the transport of the smoke into the Arctic, and presents an overview of the observations taken during the episode. Fire detections from the MODIS instruments aboard the Aqua and Terra satellites were used to estimate the BB emissions. The FLEXPART particle dispersion model was used to show that the smoke was transported to Spitsbergen and Iceland, which was confirmed by MODIS retrievals of the aerosol optical depth (AOD) and AIRS retrievals of carbon monoxide (CO) total columns. Concentrations of halocarbons, carbon dioxide and CO, as well as levoglucosan and potassium, measured at Zeppelin mountain near Ny Ålesund, were used to further corroborate the BB source of the smoke at Spitsbergen. The ozone (O3) and CO concentrations were the highest ever observed at the Zeppelin station, and gaseous elemental mercury was also elevated. A new O3 record was also set at a station on Iceland. The smoke was strongly absorbing – black carbon concentrations were the highest ever recorded at Zeppelin – and strongly perturbed the radiation transmission in the atmosphere: aerosol optical depths were the highest ever measured at Ny Ålesund. We furthermore discuss the aerosol chemical composition, obtained from filter samples, as well as the aerosol size distribution during the smoke event. Photographs show that the snow at a glacier on Spitsbergen became discolored during the episode and, thus, the snow albedo was reduced. Samples of this polluted snow contained strongly elevated levels of potassium, sulphate, nitrate and ammonium ions, thus relating the discoloration to the deposition of the smoke aerosols. This paper shows that, to date, BB has been underestimated as a source of aerosol and air pollution for the Arctic, relative to emissions from fossil fuel combustion. Given its significant impact on air quality over large spatial scales and on radiative processes, the practice of agricultural waste burning should be banned in the future.

第6回極域科学シンポジウム分野横断セッション：[IA] 急変する北極気候システム及びその全球的な影響の総合的解明―GRENE北極気候変動研究事業研究成果報告2015―11月19日（木） 国立極地研究所 2階 大会議室

第6回極域科学シンポジウム[OM] 極域気水圏11月16日（月） 統計数理研究所 セミナー室2（D304）

New shipborne aureolemeter was developed to improve the sun-tracking performance for accurate measurements of not only direct but also circumsolar radiation, even on a vessel weltering. Sun position is determined by a real-time image processing system with a CCD camera. The accuracy of the sun position determination is finer than 0.01°. The radiometer is tracked the sun under a feedback control with the derived sun position. For a sky radiance distribution measurement, the control target position on the CCD camera image is shifted a pixel corresponding to a measuring scattering angle. In the case of a scattering angle larger than 7°, the radiometer’s tracking is conducted under feed forward control on the basis of the angle of roll and pitch monitored with a gyroscope. The instrument constants were determined from a Langley plot method. Test observation was conducted onboard the Antarctic research vessel (R/V) Shirase during the 56th Japanese Antarctic Research Expedition (JARE-56; 2014-2015). Aerosol optical thickness (AOT) was measured. The measurement of the sky radiance distribution is being analyzed to derive the aerosol optical properties.

A Micro-Pulse Lidar (MPL) has been operated in Ny-Alesund, Svalbard (78°55'N, 11°56'E, 0.010 km msl) to collect zenith scattering profiles of aerosols and clouds since 1998. The Ice, Cloud, and land Elevation Satellite (ICESat) was launched by NASA in January 2003 with a single payload instrument, the Geoscience Laser Altimeter System (GLAS), designed for active remote sensing of the atmosphere as well as ice sheet height change in the cryosphere. Overpass experiments for ground validation of the ICESat/GLAS atmospheric measurements were performed in 2003 and 2004. Two case-studies comparing lidar measurements from space-borne GLAS and ground-based MPL in the Arctic are described here for a geometrically thick but optically thin cloud and a geometrically thin but optically thick cloud. The result validates the basic procedure for cloud signal processing and attenuation correction of the GLAS data.

The technological advancements of the past two to three decades enabled the establishment of space-borne observational systems to measure worldwide clouds and related radiation fields at the top of the atmosphere. This data when combined with further information on the thermodynamic state of the atmosphere and ground allows for estimates of the radiation budget at ground and within the atmosphere. This information is urgently required to calibrate the output of climate models and to understand current changes in the climate system. Results of the International Satellite Cloud Climatology Project (ISCCP) are here presented and compared with another but similar data set of the Global Energy and Water Cycle Experiment (GEWEX-SRB) and with ground-based measurements. This data describes details in space and time of the variability of radiation budget parameters at the surface and at the top of the atmosphere over the entire globe. Over the Arctic ice fields-our studies concern areas poleward of about 60°N-considerable uncertainties of more than 20Wm^(-2) still exist in both the long-wave and short-wave budget components at ground.