1. Carbon-14 emission from the pressurized heavy water reactor nuclear power plant at Kaiga, India.
- Author
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Bharath, Arya Krishnan K, D'Souza RS, Rashmi Nayak S, Dileep BN, Ravi PM, Mangavi SS, Salunke GS, Veerendra D, and Karunakara N
- Subjects
- Nuclear Power Plants, Carbon Radioisotopes analysis, Deuterium Oxide, India, Gases, Radiation Monitoring, Air Pollutants, Radioactive analysis
- Abstract
This is a detailed study on oxide (CO
2 ) and reduced (hydrocarbons, Cn Hm ) forms of14 C releases through gaseous effluents from the Kaiga nuclear power plant (NPP), on the West Coast of India, where 4 × 220 MW(e) pressurized heavy water reactors (PHWRs) are operating. The gaseous effluent from the common stack of reactor units 3 and 4 (each of 220 MW(e)) was sampled from 2017 to 2020 for14 C activity monitoring and analysed for14 C activity by liquid scintillation counting. The normalized release rate corresponding to the four-year monitoring period had a geometric mean value of 0.12 TBq GW(e)-1 a-1 (geometric standard deviation = 7.4), and the arithmetic mean with associated standard deviation was 0.75 ± 1.47 TBq GW(e)-1 a-1 . The relative percentage contribution of reduced form (CH4 ) of14 C species was less than 1.27% of the total release. The normalized release rate from Kaiga NPP was similar to those reported for the other PHWR NPPs of the world. The14 C specific activity in the ambient air in the vicinity of the NPP was monitored at four locations. The maximum excess14 C activity values in the ambient air in the vicinity of the NPP, evaluated by comparing the specific activity recorded for the clean air region at ∼300 km from the NPP, were 65.1 Bq kg-1 C (28.76 pMC) and 222.4 Bq kg-1 C (98.23 pMC) for the years 2019 and 2020 respectively. In addition, the release rates were calculated from the Gaussian plume model using site-specific atmospheric dilution factors and the excess14 C specific activity measured at four off-site monitoring stations. The calculated values of release rates were in agreement (within a factor of ∼3) with the measured values., Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper., (Copyright © 2022 Elsevier Ltd. All rights reserved.)- Published
- 2022
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