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Ozone is expected to fully recover from the chlorofluorocarbon (CFC) era by the end of the 21st century. Furthermore, because of anthropogenic climate change, a cooler stratosphere decelerates ozone loss reactions and is projected to lead to a super recovery of ozone. We investigate the ozone distribution over the 21st century with four different future scenarios using simulations of the Whole Atmosphere Community Climate Model (WACCM). At the end of the 21st century, the equatorial upper stratosphere has roughly 0.5 to 1.0 ppm more ozone in the scenario with the highest greenhouse gas emissions compared to the conservative scenario. Polar ozone levels exceed those in the pre-CFC era in scenarios that have the highest greenhouse gas emissions. This is true in the Arctic stratosphere and the Antarctic lower stratosphere. The Antarctic upper stratosphere is an exception, where different scenarios all have similar levels of ozone during winter, which do not exceed pre-CFC levels. Our results show that this is due to excess nitrogen oxides (NOx) descending faster from above in the stronger scenarios of greenhouse gas emissions. NOx in the polar thermosphere and upper mesosphere is mainly produced by energetic electron precipitation (EEP) and partly by solar UV via transport from low latitudes. Our results indicate that the thermospheric/upper mesospheric NOx will be important factor for the future Antarctic ozone evolution and could potentially prevent a super recovery of ozone in the upper stratosphere. publishedVersion

Energetic electron precipitation (EEP) affects the high‐latitude middle atmosphere by producing NOₓ compounds that destroy ozone. Earlier studies have shown that in the wintertime polar stratosphere, increased EEP enhances the westerly wind surrounding the pole, the polar vortex. This EEP effect has been found to depend on the quasi‐biennial oscillation (QBO) of equatorial winds, but the mechanism behind this modulation has so far remained unresolved. In this study we examine the atmospheric effect of EEP and its modulation by QBO using the corrected electron flux measurements by NOAA/POES satellites and the ERA‐Interim reanalysis data of zonal wind, temperature, and ozone in winter months of 1980–2016. We verify the EEP‐related strengthening of the polar vortex, warming (cooling) in the upper (lower) stratosphere and a reduction of ozone mass mixing ratio in the polar stratosphere. We also verify that the EEP effect is stronger and more significant especially in late winter, when the QBO at 30 hPa is easterly. We find here that the difference in the EEP effect between the two QBO phases is largest using a roughly 6‐month lag for QBO. We demonstrate that ozone mass mixing ratio in the lower polar stratosphere, a proxy for the strength of Brewer‐Dobson circulation, is also larger during QBO‐E than QBO‐W, with the difference maximizing when the QBO is lagged by 6 months. Our findings indicate that the modulation of the Brewer‐Dobson circulation by QBO controls how the EEP affects the polar vortex.

Northern Hemisphere winter circulation is affected by both solar and terrestrial forcings. El-Niño events and volcanic eruptions have been shown to produce a negative and a positive North Atlantic Oscillation (NAO) signature, respectively. Recent studies show a positive NAO signature related to both geomagnetic activity (proxy for solar wind driven particle precipitation) and sunspot activity (proxy for solar irradiance). Here the relative role of these four different drivers on the Northern Hemisphere wintertime circulation is studied using a statistical analysis of observational and reanalysis data during 1868–2014. The phase of the Quasi-Biennial Oscillation (QBO) is used to study driver signals in different stratospheric conditions. Moreover, the effects are separated for early/mid- and late winter. Our findings suggest a stratospheric mediation of the ENSO signal to the Atlantic side, which is delayed and modulated by the QBO unlike the signal in the Pacific side. The positive NAO by volcanic activity is preferentially obtained in the westerly QBO. We also find a substantial QBO modulation for geomagnetic activity and late winter sunspot activity, which favours a stratospheric pathway and the top-down mechanisms. However, signal in the North Pacific produced by early/mid-winter sunspot activity remain rather similar in different QBO phases and supports a direct forcing from the troposphere by the bottom-up sunspot mechanism.

This thesis studies the long-term relation between the solar wind driven energetic particle forcing into the atmosphere and the tropospheric circulation in the Northern Hemisphere winter. The work covers the period of more than one hundred years since the turn of the 20th century to present. The thesis makes a statistical analysis of satellite measurements of precipitating energetic electrons, sunspot number data and geomagnetic activity, and compares them with temperature and pressure measurements made at the Earth’s surface. Recent results, both observational and from chemistry climate models, have indicated significant effects in the Earth’s middle atmosphere due to the energetic electrons precipitating from the magnetosphere. These effects include the formation of reactive hydrogen and nitrogen oxides in the high latitude mesosphere and the depletion of ozone caused by them. Ozone is a radiatively active and important gas, which affects the thermal structure and dynamics of the middle atmosphere. Accordingly, the depletion of ozone can intensify the large scale stratospheric circulation pattern called the polar vortex. Winter weather conditions on the surface have been shown to be dependent on the polar vortex strength. This thesis shows that there is a significant relation between the average fluxes of medium energy (ten to hundred keVs) precipitating electrons and surface temperatures in parts of the Northern Hemisphere in winter time. Temperatures are positively correlated with electron fluxes in North Eurasia and negatively correlated in Greenland during the period 1980–2010 which is covered by direct satellite observations of precipitating particles. This difference is especially notable when major sudden stratospheric warmings and the quasi-biennial oscillation (QBO), which both are known to affect the polar vortex strength, are taken into account. When extended to the late 19th century, the analysis shows that a similar temperature pattern is predominated during the declining phase of the sunspot cycle. The high speed solar wind streams and energetic particle precipitation typically maximize also at the declining phase of the solar cycle. This specific temperature pattern is related to the variability of the northern annular mode (NAM), which is the most significant circulation pattern in the Northern Hemisphere winter. Before the space era, geomagnetic activity measured by ground observations can be used as a proxy for energetic particle precipitation. Earlier studies have found a significant positive correlation between geomagnetic activity and NAM since the 1960s. We find that, when the QBO measured at 30 hPa height is in the easterly phase, a positive correlation is extended to the beginning of 1900s. We also show that high geomagnetic activity causes a stronger effect in the Northern Hemisphere winter than high sunspot activity, especially in the Atlantic and Eurasia. A comprehensive knowledge of the Earth’s climate system and all its drivers is crucial for the future projection of climate. Solar variability effects have been estimated to produce only a small factor to the global climate change. However, there is increasing evidence, including the results presented in this thesis, that the different forms of solar variability can have a substantial effect to regional and seasonal climate variability. With this new evidence, the solar wind related particle effects in the atmosphere are now gaining increasing attention. These effects will soon be included in the next coupled model inter comparison project (CMIP6) as an additional solar related climate effect. This emphasizes the relevance of this thesis.