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Entanglement plays a crucial role in the development of quantum-enabled devices. One significant objective is the deterministic creation and distribution of entangled states, achieved, for example, through a mechanical oscillator interacting with confined electromagnetic fields. In this study, we explore a cavity resonator containing a two-sided perfect mirror. Although the mirror separates the cavity modes into two independent confined electromagnetic fields, the radiation pressure interaction gives rise to high-order effective interactions across all subsystems. Depending on the chosen resonant conditions, which are also related to the position of the mirror, we study $2n$-photon entanglement generation and bilateral photon pair emission. Demonstrating the non-classical nature of the mechanical oscillator, we provide a pathway to control these phenomena, opening potential applications in quantum technologies. Looking ahead, similar integrated devices could be used to entangle subsystems across vastly different energy scales, such as microwave and optical photons.

The dynamical Casimir effect is the physical phenomenon where the mechanical energy of a movable wall of a cavity confining a quantum field can be converted into quanta of the field itself. This effect has been recognized as one of the most astonishing predictions of quantum field theory. At the quantum scale, the energy conversion can also occur incoherently, namely without an physical motion of the wall. We employ quantum thermodynamics to show that this phenomenon can be employed as a tool to cool down the wall when there is a non-vanishing temperature gradient between the wall and the cavity. At the same time, the process of heat-transfer enables to share the coherence from one cavity mode, driven by a laser, to the wall, thereby forcing its coherent oscillation. Finally, we show how to employ one laser drive to cool the entire system including the case when it is composed of other subsystems.

We present a quantum heat engine based on a cavity with two oscillating mirrors that confine a quantum field as the working substance. The engine performs an Otto cycle during which the walls and a field mode interact via a nonlinear Hamiltonian. Resonances between the frequencies of the cavity mode and the walls allow to transfer heat from the hot and the cold bath by exploiting the conversion between phononic and photonic excitations. We study the time evolution of the system and show that net work can be extracted after a full cycle. We evaluate the efficiency of the process.

The hopping mechanism plays a key role in collective phenomena emerging in many-body physics. The ability to create and control systems that display this feature is important for next generation quantum technologies. Here we study two cavities separated by a vibrating two-sided perfect mirror and show that, within currently available experimental parameters, this system displays photon-pair hopping between the two electromagnetic resonators. In particular, the two-photon hopping is not due to tunneling, but rather to higher order resonant processes. Starting from the classical problem, where the vibrating mirror perfectly separates the two sides of the cavity, we quantize the system and then the two sides can interact. This opens the possibility to investigate a new mechanism of photon-pair propagation in optomechanical lattices., Comment: 9 pages, 4 figures

We show that spontaneous Raman scattering of incident radiation can be observed in cavity-QED systems without external enhancement or coupling to any vibrational degree of freedom. Raman scattering processes can be evidenced as resonances in the emission spectrum, which become clearly visible as the cavity-QED system approaches the ultrastrong coupling regime. We provide a quantum mechanical description of the effect, and show that ultrastrong light-matter coupling is a necessary condition for the observation of Raman scattering. This effect, and its strong sensitivity to the system parameters, opens new avenues for the characterization of cavity QED setups and the generation of quantum states of light.

Pure dephasing originates from the non-dissipative information exchange between quantum systems and environments, and plays a key-role in both spectroscopy and quantum information technology. Often pure dephasing constitutes the main mechanism of decay of quantum correlations. Here we investigate how pure dephasing of one of the components of a hybrid quantum system affects the dephasing rate of the system transitions. We find that, in turn, the interaction, in the case of a light-matter system, can significantly affect the form of the stochastic perturbation describing the dephasing of a subsystem, depending on the adopted gauge. Neglecting this issue can lead to wrong and unphysical results when the interaction becomes comparable to the bare resonance frequencies of subsystems, which correspond to the ultrastrong and deep-strong coupling regimes. We present results for two prototypical models of cavity quantun electrodynamics: the quantum Rabi and the Hopfield model.

We show that an atom can be coupled to a mechanical oscillator via quantum vacuum fluctuations of a cavity field enabling energy transfer processes between them. In a hybrid quantum system consisting of a cavity resonator with a movable mirror and an atom, these processes are dominated by two pair-creation mechanisms: the counterrotating (atom-cavity system) and dynamical Casimir interaction terms (optomechanical system). Because of these two pair-creation mechanisms, the resonant atom-mirror coupling is the result of high-order virtual processes with different transition paths well described in our theoretical framework. We perform a unitary transformation to the atom-mirror system Hamiltonian, exhibiting two kinds of multiple-order transitions of the pair creation. By tuning the frequency of the atom, we show that photon frequency conversion can be realized within a cavity of multiple modes. Furthermore, when involving two atoms coupled to the same mechanical mode, a single vibrating excitation of the mechanical oscillator can be simultaneously absorbed by the two atoms. Considering recent advances in strong and ultrastrong coupling for cavity optomechanics and other systems, we believe our proposals can be implemented using available technology., Comment: 22 pages, 16 figure

The prototypical system constituted by a two-level atom interacting with a quantized single-mode electromagnetic field is described by the quantum Rabi model (QRM). The QRM is potentially valid at any light-matter interaction regime, ranging from the weak (where the decay rates exceeds the coupling rate) to the deep strong coupling (where the interaction rate exceeds the bare transition frequencies of the subsystems). However, when reaching the ultrastrong coupling regime, several theoretical issues may prevent the correct description of the observable dynamics of such a system: (i) the standard quantum optics master equation fails to correctly describe the interaction of this system with the reservoirs; (ii) the correct output photon rate is no longer proportional to the intracavity photon number; and (iii) the appears to violate gauge invariance. Here, we study the photon flux emission rate of this system under the incoherent excitation of the two-level atom for any light-matter interaction strength, and consider different effective temperatures. The dependence of the emission spectra on the coupling strength is the result of the interplay between energy levels, matrix elements of the observables, and the density of states of the reservoirs. Within this approach, we also study the occurence of light-matter decoupling in the deep strong coupling regime, and show how all of the obtained results are gauge invariant., Comment: 25 pages, 21 figures

We introduce a protocol to transfer excitations between two noninteracting qubits via purely dissipative processes (i.e., in the Lindblad master equation there is no coherent interaction between the qubits). The fundamental ingredients are the presence of collective (i.e. nonlocal) dissipation and unbalanced local dissipation rates (the qubits dissipate at different rates). The resulting quantum trajectories show that the measurement backaction changes the system wave function and induces a passage of the excitation from one qubit to the other. While similar phenomena have been witnessed for a non-Markovian environment, here the dissipative quantum state transfer is induced by an update of the observer knowledge of the wave function in the presence of a Markovian (memoryless) environment -- this is a single quantum trajectory effect. Beyond single quantum trajectories and postselection, such an effect can be observed by histogramming the quantum jumps along several realizations at different times. By investigating the effect of the temperature in the presence of unbalanced local dissipation, we demonstrate that, if appropriately switched on and off, the collective dissipator can act as a Maxwell's demon. These effects are a generalized measure equivalent to the standard projective measure description of quantum teleportation and Maxwell's demon. They can be witnessed in state-of-the-art setups given the extreme experimental control in, e.g., superconducting qubits or Rydberg atoms., Comment: 11 pages, 5 figures

We show that the dynamical Casimir effect in an optomechanical system can be achieved under incoherent mechanical pumping. We adopt a fully quantum-mechanical approach for both the cavity field and the oscillating mirror. The dynamics is then evaluated using a recently-developed master equation approach in the dressed picture, including both zero and finite temperature photonic reservoirs. This analysis shows that the dynamical Casimir effect can be observed even when the mean value of the mechanical displacement is zero. This opens up new possibilities for the experimental observation of this effect. We also calculate cavity emission spectra both in the resonant and the dispersive regimes, providing useful information on the emission process., Comment: 10 pages, 6 figures

It has been shown elsewhere that two spatially separated atoms can jointly absorb one photon, whose frequency is equal to the sum of the transition frequencies of the two atoms. We describe this process in the presence of an ensemble of many two-level atoms, and show that it can be used to generate spin squeezing and entanglement. This resonant collective process allows to create a sizeable squeezing already at the single-photon limit. It represents a novel way for generating manybody spin-spin interactions, yielding a two-axis twisting-like interaction among the spins, which is very effcient for the generation of spin squeezing. We perform explicit calculations for ensembles of magnetic molecules coupled to a superconducting coplanar cavities. This system represents an attractive on-chip architecture for the realization of improved sensing., Comment: 14 pages, 8 figures

To observe the dynamical Casimir effect (DCE) induced by a moving mirror is a long-standing challenge because the mirror velocity needs to approach the speed of light. Here, we present an experimentally feasible method for observing this mechanical DCE in an optomechanical system. It employs a detuned, parametric driving to squeeze a cavity mode, so that the mechanical mode, with a typical resonance frequency, can parametrically and resonantly couple to the squeezed cavity mode, thus leading to a resonantly amplified DCE in the squeezed frame. The DCE process can be interpreted as {\it mechanically-induced two-photon hyper-Raman scattering} in the laboratory frame. Specifically, {\it a photon pair} of the parametric driving absorbs a single phonon and then is scattered into an anti-Stokes sideband. We also find that the squeezing, which additionally induces and amplifies the DCE, can be extremely small. Our method requires neither an ultra-high mechanical-oscillation frequency (i.e., a mirror moving at nearly the speed of light) nor an ultrastrong single-photon optomechanical coupling and, thus, could be implemented in a wide range of physical systems., Comment: 19 pages, 17 figures

The ability to entangle quantum systems is crucial for many applications in quantum technology, including quantum communication and quantum computing. Here, we propose a new, simple, and versatile setup for deterministically creating Bell and Greenberger-Horne-Zeilinger (GHZ) states between photons of different frequencies in a two-step protocol. The setup consists of a quantum bit (qubit) coupled ultrastrongly to three photonic resonator modes. The only operations needed in our protocol are to put the qubit in a superposition state, and then tune its frequency in and out of resonance with sums of the resonator-mode frequencies. By choosing which frequency we tune the qubit to, we select which entangled state we create. We show that our protocol can be implemented with high fidelity using feasible experimental parameters in state-of-the-art circuit quantum electrodynamics. One possible application of our setup is as a node distributing entanglement in a quantum network., Comment: 15 pages, 7 figures

The interaction among the components of a hybrid quantum system is often neglected when considering the coupling of these components to an environment. However, if the interaction strength is large, this approximation leads to unphysical predictions, as has been shown for cavity-QED and optomechanical systems in the ultrastrong-coupling regime. To deal with these cases, master equations with dissipators retaining the interaction between these components have been derived for the quantum Rabi model and for the standard optomechanical Hamiltonian. In this article, we go beyond these previous derivations and present a general master equation approach for arbitrary hybrid quantum systems interacting with thermal reservoirs. Specifically, our approach can be applied to describe the dynamics of open hybrid systems with harmonic, quasi-harmonic, and anharmonic transitions. We apply our approach to study the influence of temperature on multiphoton vacuum Rabi oscillations in circuit QED. We also analyze the influence of temperature on the conversion of mechanical energy into photon pairs in an optomechanical system, which has been recently described at zero temperature. We compare our results with previous approaches, finding that these sometimes overestimate decoherence rates and understimate excited-state populations.

Two close parallel mirrors attract due to a small force (Casimir effect) originating from the electromagnetic quantum vacuum uctuations of the electromagnetic field. These vacuum uctuations can also induce motional forces exerted upon one mirror when the other one moves. Here we consider an optomechanical system consisting of two vibrating mirrors coupled to an optical resonator. We find that motional forces can determine noticeable coupling rates between the two spatially separated vibrating mirrors. We show that, by tuning the two mechanical oscillators into resonance, energy is exchanged between them at the quantum level. This coherent motional coupling is enabled by the exchange of virtual photon pairs, originating from the dynamical Casimir effect. The process proposed here shows that the electromagnetic quantum vacuum is able to transfer mechanical energy somewhat like an ordinary uid. We show that this system can also operate as a mechanical parametric down-converter even at very weak excitations. These results demonstrate that vacuuminduced motional forces open up new possibilities for the development of optomechanical quantum technologies., Comment: 15 pages, 12 Figures

We study the dynamical Casimir effect using a fully quantum-mechanical description of both the cavity field and the oscillating mirror. We do not linearize the dynamics, nor do we adopt any parametric or perturbative approximation. By numerically diagonalizing the full optomechanical Hamiltonian, we show that the resonant generation of photons from the vacuum is determined by a ladder of mirror-field {\em vacuum Rabi splittings}. We find that vacuum emission can originate from the free evolution of an initial pure mechanical excited state, in analogy with the spontaneous emission from excited atoms. By considering a coherent drive of the mirror, using a master-equation approach to take losses into account, we are able to study the dynamical Casimir effect for optomechanical coupling strengths ranging from weak to ultrastrong. We find that a resonant production of photons out of the vacuum can be observed even for mechanical frequencies lower than the cavity-mode frequency. Since high mechanical frequencies, which are hard to achieve experimentally, were thought to be imperative for realizing the dynamical Casimir effect, this result removes one of the major obstacles for the observation of this long-sought effect. We also find that the dynamical Casimir effect can create entanglement between the oscillating mirror and the radiation produced by its motion in the vacuum field, and that vacuum Casimir-Rabi oscillations can occur., Comment: 30 pages, 8 figures

Spontaneous parametric down-conversion is a well-known process in quantum nonlinear optics in which a photon incident on a nonlinear crystal spontaneously splits into two photons. Here we propose an analogous physical process where one excited atom directly transfers its excitation to a pair of spatially-separated atoms with probability approaching one. The interaction is mediated by the exchange of virtual rather than real photons. This nonlinear atomic process is coherent and reversible, so the pair of excited atoms can transfer the excitation back to the first one: the atomic analogue of sum-frequency generation of light. The parameters used to investigate this process correspond to experimentally-demonstrated values in ultrastrong circuit quantum electrodynamics. This approach can be extended to realize other nonlinear inter-atomic processes, such as four-atom mixing, and is an attractive architecture for the realization of quantum devices on a chip. We show that four-qubit mixing can efficiently implement quantum repetition codes and, thus, can be used for error-correction codes.

We propose a new method for frequency conversion of photons which is both versatile and deterministic. We show that a system with two resonators ultrastrongly coupled to a single qubit can be used to realize both single- and multiphoton frequency-conversion processes. The conversion can be exquisitely controlled by tuning the qubit frequency to bring the desired frequency-conversion transitions on or off resonance. Considering recent experimental advances in ultrastrong coupling for circuit QED and other systems, we believe that our scheme can be implemented using available technology., Comment: 16 pages, 10 figures

We show how analogues of a large number of well-known nonlinear-optics phenomena can be realized with one or more two-level atoms coupled to one or more resonator modes. Through higher-order processes, where virtual photons are created and annihilated, an effective deterministic coupling between two states of such a system can be created. In this way, analogues of three-wave mixing, four-wave mixing, higher-harmonic and -subharmonic generation (i.e., up- and downconversion), multiphoton absorption, parametric amplification, Raman and hyper-Raman scattering, the Kerr effect, and other nonlinear processes can be realized. The effective coupling becomes weaker the more intermediate transition steps are needed. However, given the recent experimental progress in ultrastrong light-matter coupling, especially in the field of circuit quantum electrodynamics, we estimate that many of these nonlinear-optics analogues can be realized with currently available technology., Comment: 23 pages, 10 figures, 2 tables

We consider two separate atoms interacting with a single-mode optical resonator. When the frequency of the resonator field is twice the atomic transition frequency, we show that there exists a resonant coupling between \textit{one} photon and \textit{two} atoms, via intermediate virtual states connected by counter-rotating processes. If the resonator is prepared in its one-photon state, the photon can be jointly absorbed by the two atoms in their ground state which will both reach their excited state with probability close to one. Like ordinary quantum Rabi oscillations, this process is coherent and reversible, so that two atoms in their excited state will undergo a downward transition jointly emitting a single cavity photon. This joint absorption and emission processes can also occur with three atoms. The parameters used to investigate this process correspond to experimentally demonstrated values in circuit quantum electrodynamics systems., Comment: 16 pages, 5 figures

When an atom is strongly coupled to a cavity, the two systems can exchange a single photon through a coherent Rabi oscillation. This process enables precise quantum-state engineering and manipulation of atoms and photons in a cavity, which play a central role in quantum information and measurement. Recently, a new regime of cavity QED has been reached experimentally where the strength of the interaction between light and artificial atoms (qubits) becomes comparable to the atomic transition frequency or the resonance frequency of the cavity mode. Here we show that this regime can strongly modify the concept of vacuum Rabi oscillations, enabling multiphoton exchanges between the qubit and the resonator. We find that experimental state-of-the-art circuit- QED systems can undergo two- and three-photon vacuum Rabi oscillations. These anomalous Rabi oscillations can be exploited for the realization of efficient Fock-state sources of light and complex entangled states of qubits., Comment: 25 pages,7 figures