1. Terahertz stimulated parametric downconversion of a magnon mode in an antiferromagnet
- Author
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Zhang, Zhuquan, Chien, Yu-Che, Wong, Man Tou, Gao, Frank Y., Liu, Zi-Jie, Ma, Xiaoxuan, Cao, Shixun, Baldini, Edoardo, and Nelson, Keith A.
- Subjects
Condensed Matter - Materials Science - Abstract
In condensed matter systems, interactions between collective modes offer avenues for nonlinear coherent manipulation of coupled excitations and quantum phases. Antiferromagnets, with their inherently coupled magnon modes, provide a promising platform for nonlinear control of microscopic spin waves and macroscopic magnetization. However, nonlinear magnon-magnon interactions have been only partially elaborated, leaving key gaps in the prospects for potential ultrahigh-bandwidth magnonic signal processing. Here, we use a pair of intense terahertz pulses to sequentially excite two distinct coherent magnon modes in an antiferromagnet and find that the magnon mode with a lower frequency undergoes amplification when the higher-frequency mode is driven. We unveil the nonlinear excitation pathways of this stimulated parametric downconversion process by using polarization-selective two-dimensional terahertz spectroscopy. Our work provides fundamental insights into nonlinear magnonics in antiferromagnets, laying the groundwork for forthcoming spintronic and magnonic devices based on nonlinear magnon-magnon interactions.
- Published
- 2024