1. A trajectory-based estimate of the tropospheric ozone column using the residual method
- Author
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Hennie Kelder, S. Chandra, Pieternel F. Levelt, Holger Vömel, E. Joseph, Esko Kyrö, S. J. Oltmans, Valery Dorokhov, Anne M. Thompson, Lucien Froidevaux, David J. Moore, Signe B. Andersen, John T. Merrill, Gérard Ancellet, René Stübi, Susan E. Strahan, P. Viatte, Jonathan Davies, Georg Hansen, Masatomo Fujiwara, B. Bojkov, Nathaniel J. Livesey, P. von der Gathen, Gert J. R. Coetzee, H. De Backer, G. Koenig-Langlo, Bryan N. Duncan, P. Skrivankova, Hans Claude, David W. Tarasick, Pawan K. Bhartia, Greg Bodeker, Gary A. Morris, Sophie Godin-Beekmann, Margarita Yela, Jacquelyn C. Witte, H. Dier, Beverly J. Johnson, Marc Allaart, M. C. Parrondos, Bertrand Calpini, Emilio Cuevas, G. Zablocki, Susan S. Kulawik, Françoise Posny, Mark R. Schoeberl, Michael J. Newchurch, F. J. Schmidlin, Alberto Redondas, C. P. Leong, Jerald R. Ziemke, Valérie Thouret, NASA Goddard Space Flight Center (GSFC), Goddard Earth Sciences and Technology Center (GEST), University of Maryland [Baltimore County] (UMBC), University of Maryland System-University of Maryland System, Jet Propulsion Laboratory (JPL), NASA-California Institute of Technology (CALTECH), Royal Netherlands Meteorological Institute (KNMI), Science Systems and Applications, Inc. [Lanham] (SSAI), PennState Meteorology Department, Pennsylvania State University (Penn State), Penn State System-Penn State System, Izaña Atmospheric Research Center (IARC), Agencia Estatal de Meteorología (AEMet), Environment Canada (Downsview), National Institute of Water and Atmospheric Research [Lauder] (NIWA), Norwegian Institute for Air Research (NILU), NOAA Earth System Research Laboratory (ESRL), National Oceanic and Atmospheric Administration (NOAA), Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado [Boulder]-National Oceanic and Atmospheric Administration (NOAA), Department of Atmospheric Science [Huntsville], University of Alabama in Huntsville (UAH), Service d'aéronomie (SA), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Meteorologisches Observatorium Hohenpeißenberg (MOHp), Deutscher Wetterdienst [Offenbach] (DWD), Danish Meteorological Institute (DMI), Arctic Research Centre of Finnish Meteorological Institute, Finnish Meteorological Institute (FMI), Laboratorio de Atmosfera [Madrid], Spanish Space Agency, Centre of Aerology [Poland], Institute of Meteorology and Water Management - National Research Institute (IMGW - PIB), United Kingdom Met Office [Exeter], Lindenberg Meteorological Observatory - Richard Assmann Observatory (MOL-RAO), Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung (AWI), Payerne Aerological Station, Federal Office of Meteorology and Climatology MeteoSwiss, Czech Hydrometeorological Institute (CHMI), Central Aerological Observatory (CAO), Russian Federal Service for Hydrometeorology and Environmental Monitoring (Roshydromet), Institut Royal Météorologique de Belgique [Bruxelles] - Royal Meteorological Institute (IRM), Department of Environmental Affairs and Tourism, Marine and Coastal Management, South African Government, Graduate School of Environmental Science [Sapporo], Hokkaido University [Sapporo, Japan], Laboratoire d'aérologie (LAERO), Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Laboratoire de physique de l'atmosphère (LPA), Institut national des sciences de l'Univers (INSU - CNRS)-Université de La Réunion (UR)-Centre National de la Recherche Scientifique (CNRS), Department of Physics and Astronomy [Valparaiso], Valparaiso University, Graduate School of Oceanography [Narragansett], University of Rhode Island (URI), Malaysian Meteorological Department (MetMalaysia), Ministry of Science, Technology and Innovation [Malaysia] (MOSTI), Howard University, Institut Royal Météorologique de Belgique [Bruxelles] (IRM), Centre National de la Recherche Scientifique (CNRS)-Observatoire Midi-Pyrénées (OMP), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées, and Fluids and Flows
- Subjects
Atmospheric Science ,Residual method ,010504 meteorology & atmospheric sciences ,Microwave Limb Sounder ,Soil Science ,010501 environmental sciences ,Aquatic Science ,Oceanography ,Atmospheric sciences ,01 natural sciences ,Troposphere ,chemistry.chemical_compound ,Geochemistry and Petrology ,Earth and Planetary Sciences (miscellaneous) ,pollution ,Tropospheric ozone ,Stratosphere ,0105 earth and related environmental sciences ,Earth-Surface Processes ,Water Science and Technology ,Ozone Monitoring Instrument ,tropospheric ozone ,[PHYS.PHYS.PHYS-AO-PH]Physics [physics]/Physics [physics]/Atmospheric and Oceanic Physics [physics.ao-ph] ,Ecology ,Paleontology ,Forestry ,air quality ,Geophysics ,Tropospheric Emission Spectrometer ,chemistry ,13. Climate action ,Space and Planetary Science ,Climatology ,Middle latitudes ,Environmental science ,Tropospheric column ozone ,Tropopause - Abstract
We estimate the tropospheric column ozone using a forward trajectory model to increase the horizontal resolution of the Aura Microwave Limb Sounder (MLS) derived stratospheric column ozone. Subtracting the MLS stratospheric column from Ozone Monitoring Instrument total column measurements gives the trajectory enhanced tropospheric ozone residual (TTOR). Because of different tropopause definitions, we validate the basic residual technique by computing the 200-hPa-to-surface column and comparing it to the same product from ozonesondes and Tropospheric Emission Spectrometer measurements. Comparisons show good agreement in the tropics and reasonable agreement at middle latitudes, but there is a persistent low bias in the TTOR that may be due to a slight high bias in MLS stratospheric column. With the improved stratospheric column resolution, we note a strong correlation of extratropical tropospheric ozone column anomalies with probable troposphere-stratosphere exchange events or folds. The folds can be identified by their colocation with strong horizontal tropopause gradients. TTOR anomalies due to folds may be mistaken for pollution events since folds often occur in the Atlantic and Pacific pollution corridors. We also compare the 200-hPa-to-surface column with Global Modeling Initiative chemical model estimates of the same quantity. While the tropical comparisons are good, we note that chemical model variations in 200-hPa-to-surface column at middle latitudes are much smaller than seen in the TTOR.
- Published
- 2007