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The accurate determination of the electronic structure of strongly correlated materials using first principle methods is of paramount importance in condensed matter physics, computational chemistry, and material science. However, due to the exponential scaling of computational resources, incorporating such materials into classical computation frameworks becomes prohibitively expensive. In 2016, Bauer et al. proposed a hybrid quantum-classical approach to correlated materials Phys. Rev. X 6, 031045 (2016)}] that can efficiently tackle the electronic structure of complex correlated materials. Here, we experimentally demonstrate that approach to tackle the computational challenges associated with strongly correlated materials. By seamlessly integrating quantum computation into classical computers, we address the most computationally demanding aspect of the calculation, namely the computation of the Green's function, using a spin quantum processor. Furthermore, we realize a self-consistent determination of the single impurity Anderson model through a feedback loop between quantum and classical computations. A quantum phase transition in the Hubbard model from the metallic phase to the Mott insulator is observed as the strength of electron correlation increases. As the number of qubits with high control fidelity continues to grow, our experimental findings pave the way for solving even more complex models, such as strongly correlated crystalline materials or intricate molecules., Comment: 6 pages + appendices

A fundamental challenge in quantum thermodynamics is the exploration of inherent dimensional constraints in thermodynamic machines. In the context of two-level systems, the most compact refrigerator necessitates the involvement of three entities, operating under self-contained conditions that preclude the use of external work sources. Here, we build such a smallest refrigerator using a nuclear spin system, where three distinct two-level carbon-13 nuclei in the same molecule are involved to facilitate the refrigeration process. The self-contained feature enables it to operate without relying on net external work, and the unique mechanism sets this refrigerator apart from its classical counterparts. We evaluate its performance under varying conditions and systematically scrutinize the cooling constraints across a spectrum of scenarios, which sheds light on the interplay between quantum information and thermodynamics., Comment: 6 pages + appendices

Quantum control plays a crucial role in enhancing precision scaling for quantum sensing. However, most existing protocols require perfect control, even though real-world devices inevitably have control imperfections. Here, we consider a fundamental setting of quantum sensing with imperfect clocks, where the duration of control pulses and the interrogation time are all subject to uncertainty. Under this scenario, we investigate the task of frequency estimation in the presence of a non-Markovian environment. We design a control strategy and prove that it outperforms any control-free strategies, recovering the optimal Heisenberg scaling up to a small error term that is intrinsic to this model. We further demonstrate the advantage of our control strategy via experiments on a nuclear magnetic resonance (NMR) platform. Our finding confirms that the advantage of quantum control in quantum sensing persists even in the presence of imperfections., Comment: 18 pages, 7 figures

We experimentally probe the interplay of the quantum switch with the laws of thermodynamics. The quantum switch places two channels in a superposition of orders and may be applied to thermalizing channels. Quantum-switching thermal channels has been shown to give apparent violations of the second law. Central to these apparent violations is how quantum switching channels can increase the capacity to communicate information. We experimentally show this increase and how it is consistent with the laws of thermodynamics, demonstrating how thermodynamic resources are consumed. We use a nuclear magnetic resonance approach with coherently controlled interactions of nuclear spin qubits. We verify an analytical upper bound on the increase in capacity for channels that preserve energy and thermal states, and demonstrate that the bound can be exceeded for an energy-altering channel. We show that the switch can be used to take a thermal state to a state that is not thermal, whilst consuming free energy associated with the coherence of a control system. The results show how the switch can be incorporated into quantum thermodynamics experiments as an additional resource., Comment: 6 pages, 4 figures. Comments are welcome!

Quantum metrology is supposed to significantly improve the precision of parameter estimation by utilizing suitable quantum resources. However, the predicted precision can be severely distorted by realistic noises. Here, we propose a control-enhanced quantum metrology scheme to defend against these noises for improving the metrology performance. Our scheme can automatically alter the parameter encoding dynamics with adjustable controls, thus leading to optimal resultant states that are less sensitive to the noises under consideration. As a demonstration, we numerically apply it to the problem of frequency estimation under several typical Markovian noise channels. Through comparing our control-enhanced scheme with the standard scheme and the ancilla-assisted scheme, we show that our scheme performs better and can improve the estimation precision up to around one order of magnitude. Furthermore, we conduct a proof-of-principle experiment in nuclear magnetic resonance system to verify the effectiveness of the proposed scheme. The research here is helpful for current quantum platforms to harness the power of quantum metrology in realistic noise environments., Comment: 9 pages, 5 figures

Topological quantum computation (TQC) is one of the most striking architectures that can realize fault-tolerant quantum computers. In TQC, the logical space and the quantum gates are topologically protected, i.e., robust against local disturbances. The topological protection, however, requires rather complicated lattice models and hard-to-manipulate dynamics; even the simplest system that can realize universal TQC--the Fibonacci anyon system--lacks a physical realization, let alone braiding the non-Abelian anyons. Here, we propose a disk model that can realize the Fibonacci anyon system, and construct the topologically protected logical spaces with the Fibonacci anyons. Via braiding the Fibonacci anyons, we can implement universal quantum gates on the logical space. Our proposal is platform-independent. As a demonstration, we implement a topological Hadamard gate on a logical qubit through a sequence of $15$ braiding operations of three Fibonacci anyons with merely $2$ nuclear spin qubits. The gate fidelity reaches 97.18% by randomized benchmarking. We further prove by experiment that the logical space and Hadamard gate are topologically protected: local disturbances due to thermal fluctuations result in a global phase only. Our work is a proof of principle of TQC and paves the way towards fault-tolerant quantum computation., Comment: 8 pages, 4 figures

In open quantum systems, the precision of metrology inevitably suffers from the noise. {In Markovian open quantum dynamics, the precision can not be improved by using entangled probes although the measurement time is effectively shortened.} However, it was predicted over one decade ago that in a non-Markovian one, the error can be significantly reduced by the quantum Zeno effect (QZE) [Chin, Huelga, and Plenio, Phys. Rev. Lett. \textbf{109}, 233601 (2012)]. In this work, we apply a recently-developed quantum simulation approach to experimentally verify that entangled probes can improve the precision of metrology by the QZE. Up to $n=7$ qubits, we demonstrate that the precision has been improved by a factor of $n^{1/4}$, which is consistent with the theoretical prediction. Our quantum simulation approach may provide an intriguing platform for experimental verification of various quantum metrology schemes., Comment: 6 pages, 4 figures

Noise is ubiquitous in real quantum systems, leading to non-Hermitian quantum dynamics, and may affect the fundamental states of matter. Here we report in experiment a quantum simulation of the two-dimensional non-Hermitian quantum anomalous Hall (QAH) model using the nuclear magnetic resonance processor. Unlike the usual experiments using auxiliary qubits, we develop a stochastic average approach based on the stochastic Schr\"odinger equation to realize the non-Hermitian dissipative quantum dynamics, which has advantages in saving the quantum simulation sources and simplifies implementation of quantum gates. We demonstrate the stability of dynamical topology against weak noise, and observe two types of dynamical topological transitions driven by strong noise. Moreover, a region that the emergent topology is always robust regardless of the noise strength is observed. Our work shows a feasible quantum simulation approach for dissipative quantum dynamics with stochastic Schr\"odinger equation and opens a route to investigate non-Hermitian dynamical topological physics.

Indefinite causal order (ICO) is playing a key role in recent quantum technologies. Here, we experimentally study quantum thermodynamics driven by ICO on nuclear spins using the nuclear magnetic resonance system. We realize the ICO of two thermalizing channels to exhibit how the mechanism works, and show that the working substance can be cooled or heated albeit it undergoes thermal contacts with reservoirs of the same temperature. Moreover, we construct a single cycle of the ICO refrigerator based on the Maxwell's demon mechanism, and evaluate its performance by measuring the work consumption and the heat energy extracted from the low-temperature reservoir. Unlike classical refrigerators in which the coefficient of performance (COP) is perversely higher the closer the temperature of the high-temperature and low-temperature reservoirs are to each other, the ICO refrigerator's COP is always bounded to small values due to the non-unit success probability in projecting the ancillary qubit to the preferable subspace. To enhance the COP, we propose and experimentally demonstrate a general framework based on the density matrix exponentiation (DME) approach, as an extension to the ICO refrigeration. The COP is observed to be enhanced by more than three times with the DME approach. Our work demonstrates a new way for non-classical heat exchange, and paves the way towards construction of quantum refrigerators on a quantum system., Comment: 5 pages, 4 figures