Search

Isomeric states and associated collective structures have been studied up to high spin in Hg198,200,202 using multinucleon transfer reactions and the Gammasphere array. A coupled rotational band, with possible four-quasiparticle character, is established in Hg198. Sequences built on two-quasiparticle, positive-and negative-parity levels are assigned to Hg202. New isomers in Hg202 with Iπ=(7-) and (9-), and T1/2 = 10.4(4) ns and 1.4(3) ns, respectively, have been identified. A half-life of 1.0(3) ns is established for the Iπ=12+ state in Hg200. B(E2) values deduced from isomeric transitions in Hg isotopes indicate that, while collectivity near the ground state gradually diminishes from N = 112 to N = 124, it is found to increase for the 12+ and 9-states up to N = 118, followed by a reduction for higher neutron numbers. Calculations using the ultimate cranker code provide insight into the variation of deformation with spin and allow for an understanding of observed band crossings. The evolution of collectivity with spin, and along the isotopic chain, is described.

International audience; Nonyrast, excited states in neutron-rich W186 were populated via inelastic-scattering reactions using beams of Xe136 nuclei accelerated to 725 and 800 MeV. Levels populated in the reactions were investigated via particle-γ coincidence techniques using the Gammasphere array of high-purity germanium detectors and the compact heavy-ion counter, CHICO2. The Kπ=2+ (γ), Kπ=0+ and Kπ=2− (octupole) rotational side bands were extended to spins 14ℏ, 12ℏ, and 13ℏ, respectively. A staggering pattern observed in the energies of levels in the Kπ=2+ band was found to be consistent with a potential that gets softer to vibration in the γ degree of freedom with increasing spin. The odd-even staggering of states in the Kπ=2− band was found to exhibit a phase opposite to that seen in the γ band; an effect most probably associated with Coriolis coupling to other, unobserved octupole vibrational bands in W186.

Nonyrast, excited states in neutron-rich 186W were populated via inelastic-scattering reactions using beams of 136Xe nuclei accelerated to 725 and 800 MeV. Levels populated in the reactions were investigated via particleγ coincidence techniques using the Gammasphere array of high-purity germanium detectors and the compact heavy-ion counter, CHICO2. The Kπ = 2+ (γ), Kπ = 0+ and Kπ = 2− (octupole) rotational side bands were extended to spins 14¯h,12¯ h, and 13¯h, respectively. A staggering pattern observed in the energies of levels in the Kπ = 2+ band was found to be consistent with a potential that gets softer to vibration in the γ degree of freedom with increasing spin. The odd-even staggering of states in the Kπ = 2− band was found to exhibit a phase opposite to that seen in the γ band; an effect most probably associated with Coriolis coupling to other, unobserved octupole vibrational bands in 186W.

The ground-state properties of neutron-rich Nb106 and its β decay into Mo106 have been studied using the CARIBU radioactive-ion-beam facility at Argonne National Laboratory. Niobium-106 ions were extracted from a Cf252 fission source and mass separated before being delivered as low-energy beams to the Canadian Penning Trap, as well as the X-Array and SATURN β-decay-spectroscopy station. The measured Nb106 ground-state mass excess of -66202.0(13) keV is consistent with a recent measurement but has three times better precision; this work also rules out the existence of a second long-lived, β-decaying state in Nb106 above 5 keV in excitation energy. The decay half-life of Nb106 was measured to be 1.097(21) s, which is 8% longer than the adopted value. The level scheme of the decay progeny, Mo106, has been expanded up to ≈4MeV. The distribution of decay strength and considerable population of excited states in Mo106 of J≥3 emphasizes the need to revise the adopted Jπ=1- ground-state spin-parity assignment of Nb106; it is more likely to be J≥3.

The excited level structures of Tl202 and Pb203, above the 7+ and 29/2- isomers, respectively, have been studied. An isomer with Iπ=20+ and T1/2=215(10)μs has been established in Tl202, and the level scheme extended from I=10 to 20ℏ with the placement of fifteen new transitions. In Pb203, the Iπ=37/2+ state is established to be metastable, with T1/2=2.5(3)ns. Levels in both nuclei arise from intrinsic excitations, with likely particle-hole character for the higher-lying states in Pb203. The 20+ isomer in Tl202 is most likely associated with a πh11/2-1 - ν(i13/2-2,f5/2-1) configuration, while the 37/2+ state in Pb203 results from the excitation of five neutrons. Calculations, using both an empirical approach and the oxbash code, have been performed to aid in the description of the excited level structure.

The neutron-rich dysprosium isotopes $^{168}$Dy$_{102}$ and $^{169}$Dy$_{103}$ have been investigated using the EURICA γ-ray spectrometer, following production via in-flight fission of a high-intensity uranium beam in conjunction with isotope separation through the BigRIPS separator at RIBF in RIKEN Nishina Center. For $^{168}$Dy, a previously unreported isomer with a half-life of 0.57(7) μs has been identified at an excitation energy of 1378 keV, and its presence affirmed independently using γ-γ-γ coincidence data taken with Gammasphere via two-proton transfer from an enriched $^{170}$Er target performed at Argonne National Laboratory. This isomer is assigned Jπ=Kπ=(4−) based on the measured transition strengths, decay patterns, and the energy systematics for two-quasiparticle states in N=102 isotones. The underlying mechanism of two-quasiparticle excitations in the doubly midshell region is discussed in comparison with the deformed QRPA and multi-quasiparticle calculations. In $^{169}$Dy, the B(E2) value for the transition de-exciting the previously unreported Kπ=(1/2−) isomeric state at 166 keV to the Kπ=(5/2−) ground state is approximately two orders of magnitude larger than the E2 strength for the corresponding isomeric-decay transition in the N=103 isotone $^{173}$Yb, suggesting the presence of a significant γ-vibrational admixture with a dominant neutron one-quasiparticle component in the isomeric state.

The neutron-rich dysprosium isotopes ¹⁶⁸Dy₁₀₂ and ¹⁶⁹Dy₁₀₃ have been investigated using the EURICA γ-ray spectrometer, following production via in-flight fission of a high-intensity uranium beam in conjunction with isotope separation through the BigRIPS separator at RIBF in RIKEN Nishina Center. For ¹⁶⁸Dy, a previously unreported isomer with a half-life of 0.57(7) μs has been identified at an excitation energy of 1378 keV, and its presence affirmed independently using γ-γ-γ coincidence data taken with Gammasphere via two-proton transfer from an enriched ¹⁷⁰Er target performed at Argonne National Laboratory. This isomer is assigned Jπ = Kπ = (4⁻) based on the measured transition strengths, decay patterns, and the energy systematics for two-quasiparticle states in N = 102 isotones. The underlying mechanism of two-quasiparticle excitations in the doubly midshell region is discussed in comparison with the deformed QRPA and multi-quasiparticle calculations. In ¹⁶⁹Dy, the B(E2) value for the transition de-exciting the previously unreported Kπ = (1/2⁻) isomeric state at 166 keV to the Kπ = (5/2⁻) ground state is approximately two orders of magnitude larger than the E2 strength for the corresponding isomeric-decay transition in the N = 103 isotone ¹⁷³Yb, suggesting the presence of a significant γ-vibrational admixture with a dominant neutron one-quasiparticle component in the isomeric state.

The structure of decoupled positive-parity and semidecoupled negative-parity bands up to high spin in Hg197,199 has been studied using multinucleon transfer reactions with the Gammasphere array. A positive-parity band in Hg199 with the (νi13/2)3 decoupled configuration that deexcites to levels in the negative-parity sequences is newly established. The semidecoupled sequences in both isotopes are extended to higher spin. Rotation-aligned angular momenta and crossing frequencies determined from experiment are in fair agreement with those from cranking calculations. A transition from oblate collective rotation at low spin to triaxial noncollective shapes at high spin is indicated.

A six-quasiparticle isomer with T1/2 = 57(2) ns has been established in the doubly-odd isotope Tl200 and its level scheme is significantly extended. Half-lives of previously reported isomers in Tl200 and Pb201,202 have been determined and revised values are reported in a few cases, with T1/2 = 397(17) ns and 7.0(5) ns for the Iπ=5+ and 7- states in Tl200, 52(2) ns for the 41/2+ level in Pb201, and 93(4) ns for the 16+ state in Pb202. Configurations for the isomers have been assigned and these predominantly involve intrinsic excitations of neutrons from the i13/2 subshell. The inferred transition rates for the decay of these isomers compare well with single-particle estimates attesting to their intrinsic character.

The structure of the odd-A isotopes Pt193,195,197, which lie along the line of stability, has been studied up to high spin through multinucleon transfer reactions. Positive- and negative-parity sequences in Pt193,195 have been considerably extended and multiple band crossings established. An isomer with T1/2=5.0(5) ns and Iπ=25/2- is present in Pt195. The isotopes Pt193,195 are characterized by moderate oblate deformation, and angular momentum generation at high spin in the yrast, positive-parity sequences is attributed to the rotation alignment of i13/2 neutrons and h11/2 protons. A detailed understanding of the observed features is presented using calculations based on tilted axis cranking covariant density functional theory as well as others with the ultimate cranker code.

Electromagnetic quadrupole transition strength is a sensitive probe of the evolution of the structure of nuclei, particularly the competition between collectivity and magicity. We have performed a new lifetime measurement of the 21+ state of 12Be to study the interplay of these phenomena. The lifetime was measured with the Doppler Shift Attenuation Method using the γ-ray detector GRETINA. Excited states of 12Be were produced via inelastic scattering at 55 MeV/nucleon, using several different targets to control for systematic uncertainties in the stopping powers. The lifetime is determined to be τ=1.38±0.10(stat)±0.19(sys) ps, which is about half the previously reported value at twice the precision. The reduced transition strength deduced from this result is B(E2;21+→01+)=14.2±1.0(stat)±2.0(sys) e2fm4, which supports the quenching of the N=8 shell gap in 12Be.

Fast-rotating N=151 isotones 245Pu, 247Cm and 249Cf have been studied through inelastic excitation and transfer reactions with radioactive targets. While all have a ground-state band built on a νj15/2[734]9/2− Nilsson configuration, new excited bands have also been observed in each isotone. These odd-N excited bands allow a comparison of the alignment behavior for two different configurations, where the νj15/2 alignment is either blocked or allowed. The effect of higher order deformations is explored through cranking calculations, which help clarify the elusive nature of νj15/2 alignments. Keywords: Superheavy, Neutron-rich, Inelastic and transfer reactions, Rotational alignments, Higher-order deformations

States in Tl209 were populated using a multinucleon transfer reaction with a Xe136 beam impinging on a thick Pb208 target at E=785 MeV. The beam was pulsed at 825-ns intervals in order to perform isomer decay spectroscopy. The known Jπ=17/2+ isomer in Tl209 was located at 1228(4) keV and measured to have a half-life of T1/2=146(10) ns. A second isomer with Jπ=13/2+ was found to have T1/2=14(5) ns. The previously suggested low-energy X and Y transitions were found to have energies 57(2) and 47(2) keV respectively, while the measurement of conversion coefficients and a new decay path make the spin assignments below the isomers experimentally firm. Correlating the delayed γ transitions with the prompt beam flash allowed the decay of states above the isomer to be found. The longer-lived isomer represents full alignment of the simplest two-particle, one-hole configuration and illuminates the remarkably weak coupling of the proton hole to the Pb210 core.

States in Tl209 were populated using a multinucleon transfer reaction with a Xe136 beam impinging on a thick Pb208 target at E=785 MeV. The beam was pulsed at 825-ns intervals in order to perform isomer decay spectroscopy. The known Jπ=17/2+ isomer in Tl209 was located at 1228(4) keV and measured to have a half-life of T1/2=146(10) ns. A second isomer with Jπ=13/2+ was found to have T1/2=14(5) ns. The previously suggested low-energy X and Y transitions were found to have energies 57(2) and 47(2) keV respectively, while the measurement of conversion coefficients and a new decay path make the spin assignments below the isomers experimentally firm. Correlating the delayed γ transitions with the prompt beam flash allowed the decay of states above the isomer to be found. The longer-lived isomer represents full alignment of the simplest two-particle, one-hole configuration and illuminates the remarkably weak coupling of the proton hole to the Pb210 core.