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The inverse design of tailored organic molecules for specific optoelectronic devices of high complexity holds an enormous potential, but has not yet been realized1,2. The complexity and literally infinite diversity of conjugated molecular structures present both, an unprecedented opportunity for technological breakthroughs as well as an unseen optimization challenge. Current models rely on big data which do not exist for specialized research films. However, a hybrid computational and high throughput experimental screening workflow allowed us to train predictive models with as little as 149 molecules. We demonstrate a unique closed-loop workflow combining high throughput synthesis and Bayesian optimization that discovers new hole transporting materials with tailored properties for solar cell applications. A series of high-performance molecules were identified from minimal suggestions, achieving up to 26.23% (certified 25.88%) power conversion efficiency in perovskite solar cells. Our work paves the way for rapid, informed discovery in vast molecular libraries, revolutionizing material selection for complex devices. We believe that our approach can be generalized to other emerging fields and indeed accelerate the development of optoelectronic semiconductor devices in general., Comment: 21 pages, 5 figures

The Conformer has become the most popular encoder model for automatic speech recognition (ASR). It adds convolution modules to a transformer to learn both local and global dependencies. In this work we describe a faster, more memory-efficient, and better-performing transformer, called Zipformer. Modeling changes include: 1) a U-Net-like encoder structure where middle stacks operate at lower frame rates; 2) reorganized block structure with more modules, within which we re-use attention weights for efficiency; 3) a modified form of LayerNorm called BiasNorm allows us to retain some length information; 4) new activation functions SwooshR and SwooshL work better than Swish. We also propose a new optimizer, called ScaledAdam, which scales the update by each tensor's current scale to keep the relative change about the same, and also explictly learns the parameter scale. It achieves faster convergence and better performance than Adam. Extensive experiments on LibriSpeech, Aishell-1, and WenetSpeech datasets demonstrate the effectiveness of our proposed Zipformer over other state-of-the-art ASR models. Our code is publicly available at https://github.com/k2-fsa/icefall., Comment: Published as a conference paper at ICLR 2024

In this paper, we introduce Libriheavy, a large-scale ASR corpus consisting of 50,000 hours of read English speech derived from LibriVox. To the best of our knowledge, Libriheavy is the largest freely-available corpus of speech with supervisions. Different from other open-sourced datasets that only provide normalized transcriptions, Libriheavy contains richer information such as punctuation, casing and text context, which brings more flexibility for system building. Specifically, we propose a general and efficient pipeline to locate, align and segment the audios in previously published Librilight to its corresponding texts. The same as Librilight, Libriheavy also has three training subsets small, medium, large of the sizes 500h, 5000h, 50000h respectively. We also extract the dev and test evaluation sets from the aligned audios and guarantee there is no overlapping speakers and books in training sets. Baseline systems are built on the popular CTC-Attention and transducer models. Additionally, we open-source our dataset creatation pipeline which can also be used to other audio alignment tasks., Comment: Submitted to ICASSP 2024

Prompts are crucial to large language models as they provide context information such as topic or logical relationships. Inspired by this, we propose PromptASR, a framework that integrates prompts in end-to-end automatic speech recognition (E2E ASR) systems to achieve contextualized ASR with controllable style of transcriptions. Specifically, a dedicated text encoder encodes the text prompts and the encodings are injected into the speech encoder by cross-attending the features from two modalities. When using the ground truth text from preceding utterances as content prompt, the proposed system achieves 21.9% and 6.8% relative word error rate reductions on a book reading dataset and an in-house dataset compared to a baseline ASR system. The system can also take word-level biasing lists as prompt to improve recognition accuracy on rare words. An additional style prompt can be given to the text encoder and guide the ASR system to output different styles of transcriptions. The code is available at icefall., Comment: Proc. ICASSP 2024

Neural Transducer and connectionist temporal classification (CTC) are popular end-to-end automatic speech recognition systems. Due to their frame-synchronous design, blank symbols are introduced to address the length mismatch between acoustic frames and output tokens, which might bring redundant computation. Previous studies managed to accelerate the training and inference of neural Transducers by discarding frames based on the blank symbols predicted by a co-trained CTC. However, there is no guarantee that the co-trained CTC can maximize the ratio of blank symbols. This paper proposes two novel regularization methods to explicitly encourage more blanks by constraining the self-loop of non-blank symbols in the CTC. It is interesting to find that the frame reduction ratio of the neural Transducer can approach the theoretical boundary. Experiments on LibriSpeech corpus show that our proposed method accelerates the inference of neural Transducer by 4 times without sacrificing performance. Our work is open-sourced and publicly available https://github.com/k2-fsa/icefall., Comment: Accepted in INTERSPEECH 2023

Connectionist Temporal Classification (CTC) suffers from the latency problem when applied to streaming models. We argue that in CTC lattice, the alignments that can access more future context are preferred during training, thereby leading to higher symbol delay. In this work we propose the delay-penalized CTC which is augmented with latency penalty regularization. We devise a flexible and efficient implementation based on the differentiable Finite State Transducer (FST). Specifically, by attaching a binary attribute to CTC topology, we can locate the frames that firstly emit non-blank tokens on the resulting CTC lattice, and add the frame offsets to the log-probabilities. Experimental results demonstrate the effectiveness of our proposed delay-penalized CTC, which is able to balance the delay-accuracy trade-off. Furthermore, combining the delay-penalized transducer enables the CTC model to achieve better performance and lower latency. Our work is open-sourced and publicly available https://github.com/k2-fsa/k2., Comment: Accepted in INTERSPEECH 2023

Knowledge distillation(KD) is a common approach to improve model performance in automatic speech recognition (ASR), where a student model is trained to imitate the output behaviour of a teacher model. However, traditional KD methods suffer from teacher label storage issue, especially when the training corpora are large. Although on-the-fly teacher label generation tackles this issue, the training speed is significantly slower as the teacher model has to be evaluated every batch. In this paper, we reformulate the generation of teacher label as a codec problem. We propose a novel Multi-codebook Vector Quantization (MVQ) approach that compresses teacher embeddings to codebook indexes (CI). Based on this, a KD training framework (MVQ-KD) is proposed where a student model predicts the CI generated from the embeddings of a self-supervised pre-trained teacher model. Experiments on the LibriSpeech clean-100 hour show that MVQ-KD framework achieves comparable performance as traditional KD methods (l1, l2), while requiring 256 times less storage. When the full LibriSpeech dataset is used, MVQ-KD framework results in 13.8% and 8.2% relative word error rate reductions (WERRs) for non -streaming transducer on test-clean and test-other and 4.0% and 4.9% for streaming transducer. The implementation of this work is already released as a part of the open-source project icefall., Comment: Submitted to ICASSP 2022

In streaming automatic speech recognition (ASR), it is desirable to reduce latency as much as possible while having minimum impact on recognition accuracy. Although a few existing methods are able to achieve this goal, they are difficult to implement due to their dependency on external alignments. In this paper, we propose a simple way to penalize symbol delay in transducer model, so that we can balance the trade-off between symbol delay and accuracy for streaming models without external alignments. Specifically, our method adds a small constant times (T/2 - t), where T is the number of frames and t is the current frame, to all the non-blank log-probabilities (after normalization) that are fed into the two dimensional transducer recursion. For both streaming Conformer models and unidirectional long short-term memory (LSTM) models, experimental results show that it can significantly reduce the symbol delay with an acceptable performance degradation. Our method achieves similar delay-accuracy trade-off to the previously published FastEmit, but we believe our method is preferable because it has a better justification: it is equivalent to penalizing the average symbol delay. Our work is open-sourced and publicly available (https://github.com/k2-fsa/k2)., Comment: Submitted to 2023 IEEE International Conference on Acoustics, Speech and Signal Processing

The transducer architecture is becoming increasingly popular in the field of speech recognition, because it is naturally streaming as well as high in accuracy. One of the drawbacks of transducer is that it is difficult to decode in a fast and parallel way due to an unconstrained number of symbols that can be emitted per time step. In this work, we introduce a constrained version of transducer loss to learn strictly monotonic alignments between the sequences; we also improve the standard greedy search and beam search algorithms by limiting the number of symbols that can be emitted per time step in transducer decoding, making it more efficient to decode in parallel with batches. Furthermore, we propose an finite state automaton-based (FSA) parallel beam search algorithm that can run with graphs on GPU efficiently. The experiment results show that we achieve slight word error rate (WER) improvement as well as significant speedup in decoding. Our work is open-sourced and publicly available\footnote{https://github.com/k2-fsa/icefall}., Comment: Submitted to 2023 IEEE International Conference on Acoustics, Speech and Signal Processing

The RNN-Transducer (RNN-T) framework for speech recognition has been growing in popularity, particularly for deployed real-time ASR systems, because it combines high accuracy with naturally streaming recognition. One of the drawbacks of RNN-T is that its loss function is relatively slow to compute, and can use a lot of memory. Excessive GPU memory usage can make it impractical to use RNN-T loss in cases where the vocabulary size is large: for example, for Chinese character-based ASR. We introduce a method for faster and more memory-efficient RNN-T loss computation. We first obtain pruning bounds for the RNN-T recursion using a simple joiner network that is linear in the encoder and decoder embeddings; we can evaluate this without using much memory. We then use those pruning bounds to evaluate the full, non-linear joiner network.