1. Room temperature spin-layer locking of exciton-polariton nonlinearities
- Author
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Zhao, Jiaxin, Fieramosca, Antonio, Dini, Kevin, Shang, Qiuyu, Bao, Ruiqi, Luo, Yuan, Shen, Kaijun, Zhao, Yang, Su, Rui, Perez, Jesus Zuniga, Gao, Weibo, Ardizzone, Vincenzo, Sanvitto, Daniele, Xiong, Qihua, and Liew, Timothy C. H.
- Subjects
Physics - Optics - Abstract
Recent advancements in transition metal dichalcogenides (TMDs) have unveiled exceptional optical and electronic characteristics, opened up new opportunities, and provided a unique platform for exploring light-matter interactions under the strong coupling regime. The exploitation of exciton-polaritons, with their peculiar hybrid light-matter properties, for the development of spintronic customizable devices that enhance both the information capacity and functionality at ambient temperatures is often suggested as a promising route. However, although TMD polaritons have shown promising potential, the microscopic mechanisms leading to nonlinearities in TMD polaritons are complex and their spin-anisotropy, a crucial requirement for many proposed polaritonic devices, has been missing. Here, we demonstrate the absence of spin-anisotropic interaction in a monolayer WS2 microcavity (at room temperature) and show how spin-dependent interactions can be controlled and spin anisotropy recovered by engineering double WS2 layer structures with varied interlayer spacing. We attribute this phenomenon to a distinctive feature in exciton-polariton physics: layer-dependent polariton-phonon coupling. We use theoretical calculations of the phonon electrostatic potentials finding a drastically different coupling strength for single and double monolayer samples and discuss qualitatively how this explains the observed spin-anisotropic response. This is further consistent with experiments on multi WS2 layer samples and the identification of a critical separation distance, above which an effective single monolayer spin-anisotropic response is recovered, both in experiment and theory. Our work lays the groundwork for the development of spin-optronic polaritonic devices at room temperature.
- Published
- 2024